{"id":230517,"date":"2021-12-06T06:30:57","date_gmt":"2021-12-05T22:30:57","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=230517"},"modified":"2021-12-05T20:07:19","modified_gmt":"2021-12-05T12:07:19","slug":"%e5%8c%97%e4%ba%ac%e7%a7%91%e6%8a%80%e5%a4%a7%e5%ad%a6sci-total-environ-fecoo-go%e6%94%b9%e6%80%a7%e9%98%b4%e6%9e%81%e5%be%ae%e7%94%9f%e7%89%a9%e7%87%83%e6%96%99%e7%94%b5%e6%b1%a0%e5%8d%8f%e5%90%8c","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=230517","title":{"rendered":"\u5317\u4eac\u79d1\u6280\u5927\u5b66Sci. Total Environ.: FeCoO\/GO\u6539\u6027\u9634\u6781\u5fae\u751f\u7269\u71c3\u6599\u7535\u6c60\u534f\u540c\u589e\u5f3a\u6c27\u8fd8\u539f\u53cd\u5e94\u548c\u571f\u9709\u7d20\u77ff\u5316"},"content":{"rendered":"<p>\u6297\u751f\u7d20\u88ab\u5e7f\u6cdb\u5e94\u7528\u4e8e\u4eba\u7c7b\u533b\u7597\u548c\u5bb6\u755c\u517b\u6b96\u9886\u57df\uff0c\u4ee5\u9884\u9632\u548c\u6cbb\u7597\u75be\u75c5\u3002\u4f46\u5176\u751f\u7269\u6bd2\u6027\u548c\u6297\u6027\u57fa\u56e0\u4f20\u64ad\u5bf9\u73af\u5883\u548c\u751f\u6001\u7cfb\u7edf\u9020\u6210\u5de8\u5927\u5a01\u80c1\u3002\u571f\u9709\u7d20\uff08OTC\uff09\u4f5c\u4e3a\u755c\u79bd\u517b\u6b96\u4e2d\u4e3b\u8981\u4f7f\u7528\u7684\u6297\u751f\u7d20\u4e4b\u4e00\uff0c\u9ad8\u8fbe75%\u901a\u8fc7\u4ee3\u8c22\u6392\u6cc4\u91ca\u653e\u5230\u73af\u5883\u4e2d\u3002\u7136\u800c\uff0c\u7531\u4e8e\u7ed3\u6784\u7a33\u5b9a\u4e14\u6297\u83cc\u6027\u80fd\uff0c\u4f20\u7edf\u5e9f\u6c34\u5904\u7406\u4e2dOTC\u53bb\u9664\u6548\u7387\u8f83\u4f4e\u3002\u9ad8\u7ea7\u6c27\u5316\u5de5\u827a(AOPs)\u5229\u7528\u0387OH\u6709\u6548\u53bb\u9664\u96be\u964d\u89e3\u7269\u8d28\uff0c\u5bf9\u5176\u5177\u6709\u8f83\u9ad8\u7684\u6c27\u5316\u901f\u7387\u548c\u77ff\u5316\u901f\u7387\uff0c\u5728\u6c34\u5904\u7406\u9886\u57df\u5177\u6709\u5e7f\u6cdb\u5e94\u7528\u3002\u4f20\u7edf\u7684Fenton\u6c27\u5316\u5de5\u827a\u9700\u8981\u5927\u91cf\u7684\u94c1\u6ce5\u548cH<sub>2<\/sub>O<sub>2<\/sub>\uff0c\u5177\u6709\u6210\u672c\u9ad8\u548c\u4e8c\u6b21\u6c61\u67d3\u95ee\u9898\u3002\u7535\u82ac\u987f\u53ef\u539f\u4f4d\u751f\u6210H<sub>2<\/sub>O<sub>2<\/sub>\u4ee5\u53caFe<sup>2+<\/sup>\u5728\u7535\u6781\u8868\u9762\u8f6c\u5316\uff0c\u4f46H<sub>2<\/sub>O<sub>2<\/sub>\u4ea7\u751f\u901f\u7387\u6162\u4ee5\u53ca\u9700\u8981\u5916\u90e8\u7535\u6e90\u4ecd\u662f\u9700\u8981\u9762\u4e34\u7684\u96be\u9898\u3002<\/p>\n<p>\u5fae\u751f\u7269\u71c3\u6599\u7535\u6c60(MFC)\u5229\u7528\u5fae\u751f\u7269\u5206\u89e3\u6709\u673a\u7269\u8f6c\u5316\u4e3a\u7535\u80fd\uff0c\u5177\u6709\u89e3\u51b3\u73af\u5883\u6c61\u67d3\u548c\u80fd\u6e90\u77ed\u7f3a\u53cc\u91cd\u96be\u9898\u7684\u4f18\u52bf\u3002\u5176\u4e2d\uff0c\u7a7a\u6c14\u9634\u6781MFC\u53ef\u4ee5\u901a\u8fc7\u6c27\u8fd8\u539f\u53cd\u5e94(ORR)\u4ea7\u751fH<sub>2<\/sub>O<sub>2<\/sub>\uff0c\u4fc3\u8fdb\u6c61\u67d3\u7269\u7684\u6c27\u5316\u548c\u77ff\u5316\u3002\u5e76\u4e14\u9633\u6781\u7684\u7535\u5b50\u548c\u8d28\u5b50\u8f6c\u79fb\u5230\u9634\u6781\u5f62\u6210\u5b8c\u6574\u56de\u8def\uff0c\u89e3\u51b3\u5916\u90e8\u7535\u6e90\u95ee\u9898\u3002\u7136\u800c\uff0c\u4f20\u7edf\u7684Pt\/C\u50ac\u5316\u5242\u6210\u672c\u9ad8\u3001\u751f\u6210H<sub>2<\/sub>O<sub>2<\/sub>\u901f\u7387\u4f4e\uff0c\u6781\u5927\u5730\u9650\u5236\u4e86\u5176\u5e94\u7528\u3002\u56e0\u6b64\uff0c\u50ac\u5316\u6d3b\u6027\u9ad8\u3001\u7a33\u5b9a\u6027\u9ad8\u3001\u5236\u5907\u7b80\u5355\u7684\u8fc7\u6e21\u91d1\u5c5e\u6c27\u5316\u7269\u4f5c\u4e3aORR\u7684\u50ac\u5316\u5242\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\u3002<\/p>\n<p>\u5317\u4eac\u79d1\u6280\u5927\u5b66\u7855\u58eb\u751f\u90d1\u7433\u59d7\u91c7\u7528\u6c34\u70ed\u6cd5\u5236\u5907\u4e86FeCoO\/GO\u590d\u5408\u50ac\u5316\u5242\u6539\u6027\u78b3\u6be1(CF)\u9634\u6781\u3002FeCoO\/GO\u6539\u6027\u540e\u7684\u9634\u6781\u5185\u963b\u663e\u8457\u964d\u4f4e\uff0c\u6c27\u50ac\u5316\u8fd8\u539f\u6027\u80fd\u63d0\u9ad8\u3002\u6b64\u5916\uff0cOTC\u7684\u964d\u89e3\u6548\u7387\u548c\u77ff\u5316\u7387\u4e5f\u5f97\u5230\u4e86\u63d0\u9ad8\u3002<\/p>\n<p>\u7531\u4e8e\u9ad8\u6e29\u9ad8\u538b\u53cd\u5e94\uff0cFe\u548cCo\u7684\u6c27\u5316\u7269\u7eb3\u7c73\u9897\u7c92\u4e0e\u6c27\u5316\u77f3\u58a8\u70ef\u7ed3\u5408\u7d27\u5bc6\u3002\u6c27\u5316\u77f3\u58a8\u70ef\u8584\u7247\u4f5c\u4e3a\u91d1\u5c5e\u6c27\u5316\u7269\u7eb3\u7c73\u9897\u7c92\u7684\u652f\u67b6\u53ef\u4ee5\u9632\u6b62\u7eb3\u7c73\u9897\u7c92\u7684\u805a\u96c6\uff0c\u5e76\u63d0\u4f9b\u66f4\u591a\u7684\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u3002\u6709\u5229\u4e8e\u6539\u5584\u5bf9\u6c27\u7684\u5438\u9644\u548c\u50ac\u5316\u8f6c\u5316\uff0c\u4ece\u800c\u964d\u4f4e\u4e86MFC\u4e2d\u53ef\u89c2\u7684\u529f\u7387\u8f93\u51fa\u6240\u9700\u7684\u6eb6\u89e3\u6c27\u9700\u6c42\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-230523\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/1-2.png\" alt=\"\" width=\"600\" height=\"412\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/1-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/1-2-300x206.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe1 (A-B)\u4f4e\u500d\u7387\u548c\u9ad8\u500d\u7387\u4e0bFeCoO\/GO\u7684\u5fae\u89c2\u5f62\u8c8c;(C-G) FeCoO\/GO\u7684EDS\u548c\u5143\u7d20\u6620\u5c04\u56fe<\/p>\n<p>FeCoO\/GO\u6539\u6027\u9634\u6781MFC\u7684\u6700\u5927\u529f\u7387\u5bc6\u5ea6\u4e3a461.2 mW\/m<sup>2<\/sup>\uff0c\u662fCF\u9634\u6781\u76844.5\u500d (102.5 mW\/m<sup>2<\/sup>)\u3002\u6781\u5316\u66f2\u7ebf\u7684\u7ebf\u6027\u90e8\u5206\u53ef\u4ee5\u53cd\u6620\u5185\u963b\uff0cFeCoO\/GO \u5177\u6709\u6700\u5c0f\u7684\u5185\u963b\uff08220.5 m\u03a9 m<sup>2<\/sup>\uff09\uff0c\u800c M-CF \u4e3a 355.8 m\u03a9 m<sup>2<\/sup>\u3002FeCoO\/GO\u50ac\u5316\u5242\u8f83\u9ad8\u7684\u7535\u5b50\u4f20\u9012\u6548\u7387\u53ef\u964d\u4f4e\u7535\u963b\u3002\u5728\u4e0d\u540c\u7cfb\u7edf\u4e2d\u9633\u6781\u7535\u4f4d\u7684\u53d8\u5316\u76f8\u4f3c\uff0c\u800c\u5728 FeCoO\/GO \u6539\u6027 MFC \u4e2d\u53d1\u73b0\u660e\u663e\u66f4\u9ad8\u7684\u9634\u6781\u7535\u4f4d\uff0c\u8868\u660e\u4ea7\u7535\u6027\u80fd\u663e\u7740\u63d0\u9ad8\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-230524\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/2-2.png\" alt=\"\" width=\"600\" height=\"231\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/2-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/2-2-300x116.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe2 MFC\u7684\u4ea7\u7535\u6027\u80fd:(A)\u529f\u7387\u5bc6\u5ea6\u548c\u6781\u5316\u66f2\u7ebf;(B)\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u9633\u6781\u548c\u9634\u6781\u7535\u4f4d\u7684\u53d8\u5316<\/p>\n<p>\u4f4e\u66dd\u6c14\u901f\u7387\u4e0b\u7684\u9ad8ORR\u901f\u7387\u540c\u65f6\u63d0\u9ad8\u4e86\u4ea7\u7535\u6548\u7387\u548cOTC\u964d\u89e3\u6548\u7387\uff0c\u800c\u9ad8\u66dd\u6c14\u901f\u7387\u540c\u65f6\u964d\u4f4e\u4e86\u4ea7\u7535\u91cf\u548cOTC\u964d\u89e3\u7387\uff0c\u8bf4\u660e\u8fdb\u4e00\u6b65\u63d0\u9ad8\u66dd\u6c14\u901f\u7387\u4f1a\u5f71\u54cd\u6c27\u5728\u7535\u6781\u8868\u9762\u7684\u5438\u9644\u548c\u53cd\u5e94\uff0c\u5bfc\u81f4\u8f93\u51fa\u7535\u538b\u964d\u4f4e\u3002\u6b64\u5916\uff0cORR\u6548\u7387\u7684\u63d0\u9ad8\u6709\u5229\u4e8eH<sub>2<\/sub>O<sub>2<\/sub>\u7684\u4ea7\u751f\uff0c\u6700\u7ec8\u4fc3\u8fdbFenton\u53cd\u5e94\u964d\u89e3OTC\u3002\u5f53\u66dd\u6c14\u901f\u7387\u4e3a100mL\/min\u65f6\uff0cM-CF\u7684\u964d\u89e3\u6548\u7387\u6700\u9ad8\u8fbe\u523060.57%\u3002M-FeCoO\/GO\u5728\u66dd\u6c14\u901f\u7387\u4e3a50 mL\/min\u65f6OTC\u964d\u89e3\u6548\u7387\u6700\u9ad8(80.34%)\uff0c\u662fM-CF\u76841.33\u500d\u3002M-FeCoO\/GO\u53ef\u4ee5\u5728\u4f4e\u6d41\u901f\u4e0b\u83b7\u5f97\u9ad8\u964d\u89e3\u7387\u7684OTC\uff0c\u5728\u957f\u671f\u5904\u7406\u8fc7\u7a0b\u4e2d\u5177\u6709\u6210\u672c\u6548\u76ca\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-230525\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/3-2.png\" alt=\"\" width=\"600\" height=\"461\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/3-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/3-2-300x231.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe3 (A-B)CF\u9634\u6781\u548cFeCoO\/GO\u9634\u6781\u5728\u7535\u89e3\u6db2\u4e2d\u542b\u670920 mg\/L OTC\u65f6\uff0c\u4e0d\u540c\u66dd\u6c14\u91cf\u4e0b\u7684\u8f93\u51fa\u7535\u538b;(C-D)CF\u9634\u6781\u548cFeCoO\/GO\u9634\u6781\u5728\u4e0d\u540c\u66dd\u6c14\u91cf\u4e0b\u5bf920 mg\/LOTC\u7684\u964d\u89e3\u6548\u7387<\/p>\n<p>\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u5355\u91d1\u5c5e\u7684\u6027\u80fd\u4e0d\u5982\u53cc\u91d1\u5c5e\u3002\u8fd9\u662f\u7531\u4e8eFe<sup>3+<\/sup>\u4e0eCo<sup>2+<\/sup>\u76f8\u4e92\u8f6c\u5316\uff0c\u6700\u5927\u9650\u5ea6\u5730\u5229\u7528H<sub>2<\/sub>O<sub>2<\/sub>\uff0c\u4fc3\u8fdb\u82ac\u987f\u53cd\u5e94\u7684\u8fdb\u884c\u5f62\u6210\u7f9f\u57fa\u81ea\u7531\u57fa\u4ee5\u53caOTC\u77ff\u5316\uff0c\u8868\u73b0\u51fa\u826f\u597d\u7684\u534f\u540c\u6548\u5e94\u3002\u53cc\u91d1\u5c5e\u6d3b\u6027\u4f4d\u70b9\u7684\u589e\u52a0\u523a\u6fc0\u4e86\u00b7OH\u7684\u751f\u6210\uff0c\u51cf\u5c11\u4e86\u81ea\u7531\u57fa\u7684\u8fc1\u79fb\u8ddd\u79bb\uff0c\u663e\u8457\u52a0\u901f\u4e86OTC\u7684\u7ed3\u6784\u7834\u574f\u3002OTC\u5728M-FeCoO\/GO\u4e2d\u88ab\u00b7OH\u6c27\u5316\uff0c\u540c\u65f6\u907f\u514d\u4e86H<sub>2<\/sub>O<sub>2<\/sub>\u5bf9FeCoO\/GO\u7684\u8150\u8680\u548c\u6bd2\u5bb3\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-230526\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/4-2.png\" alt=\"\" width=\"437\" height=\"362\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/4-2.png 437w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/4-2-300x249.png 300w\" sizes=\"(max-width: 437px) 100vw, 437px\" \/><\/p>\n<p>\u56fe4 \u4e0d\u540c\u50ac\u5316\u5242\u5bf9OTC\u7684\u964d\u89e3\u6027\u80fd(OTC\u6d53\u5ea6\u4e3a20 mg\/L\uff0c\u66dd\u6c14\u901f\u7387\u4e3a50 mL\/min)<\/p>\n<p>UPLC-QTOF-MS\u8bc1\u5b9e\uff0c\u7532\u57fa\u3001\u7f9f\u57fa\u548c\u7fb0\u57fa\u9010\u6e10\u88ab\u00b7OH\u7834\u574f\u5e76\u4eceOTC\u5206\u5b50\u4e2d\u5206\u79bb\u51fa\u6765\u3002\u964d\u89e3\u4e3b\u8981\u662f\u7531\u4e8e\u7a7a\u6c14\u9634\u6781\u4e2dORR\u548cFenton\u53cd\u5e94\u4ea7\u751f\u7684\u00b7OH\u7684\u6c27\u5316\u4f5c\u7528\u3002\u6839\u636e\u57fa\u56e2\u8d21\u732e\u7406\u8bba\uff0c\u82ef\u73af\u4e0a\u7684\u4f4d\u70b9\u4f1a\u88ab\u00b7OH\u653b\u51fb\u800c\u53d1\u751f\u7532\u57fa\u5316\u548c\u7f9f\u57fa\u5316\u3002\u8131\u6c34\u53cd\u5e94\u5f62\u6210\u4e0d\u9971\u548c\u78b3\u78b3\u53cc\u952e\u3002\u6700\u7ec8\uff0c\u4e2d\u95f4\u4f53\u88ab\u8f6c\u79fb\u5230\u5c0f\u5206\u5b50\u4e2d\uff0c\u5b9e\u73b0\u77ff\u5316\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-230527\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/5-2.png\" alt=\"\" width=\"600\" height=\"375\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/5-2.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2021\/12\/5-2-300x188.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u56fe5 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Zheng<sup>1<\/sup>, Xiaoqiu Lin<sup>1<\/sup>, Yuanfeng Liu, Huiyu Li, Yaxin Sun, Congju Li*. Synergistically enhanced oxygen reduction reaction and oxytetracycline mineralization by FeCoO\/GO modified cathode in microbial fuel cell, <strong><em>Science of the Total Environment, DOI: https:\/\/doi.org\/10.1016\/j.scitotenv.2021.151873.<\/em><\/strong><\/p>\n<p>\u672c\u6587\u7531\u4f5c\u8005\u6295\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u6297\u751f\u7d20\u88ab\u5e7f\u6cdb\u5e94\u7528\u4e8e\u4eba\u7c7b\u533b\u7597\u548c\u5bb6\u755c\u517b\u6b96\u9886\u57df\uff0c\u4ee5\u9884\u9632\u548c\u6cbb\u7597\u75be\u75c5\u3002\u4f46\u5176\u751f\u7269\u6bd2\u6027\u548c\u6297\u6027\u57fa\u56e0\u4f20\u64ad\u5bf9\u73af\u5883\u548c\u751f\u6001\u7cfb\u7edf\u9020\u6210\u5de8\u5927\u5a01\u80c1\u3002\u571f\u9709\u7d20\uff08OTC\uff09\u4f5c\u4e3a\u755c\u79bd\u517b\u6b96\u4e2d\u4e3b\u8981\u4f7f\u7528\u7684\u6297\u751f&#8230;<\/p>\n","protected":false},"author":11454,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-230517","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/230517"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/11454"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=230517"}],"version-history":[{"count":4,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/230517\/revisions"}],"predecessor-version":[{"id":230535,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/230517\/revisions\/230535"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=230517"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=230517"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=230517"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}