{"id":231312,"date":"2021-12-28T06:35:01","date_gmt":"2021-12-27T22:35:01","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=231312"},"modified":"2021-12-27T20:35:30","modified_gmt":"2021-12-27T12:35:30","slug":"%e4%b9%94%e4%b8%96%e7%92%8b-%e7%8e%8b%e6%b5%b7%e8%be%89nature-communications%ef%bc%9a%e7%a1%ab%e5%8c%96%e5%ad%a6%e6%8a%80%e6%9c%af%e6%8f%90%e9%ab%98%e7%94%b5%e6%b1%a0%e5%af%bf%e5%91%bd","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=231312","title":{"rendered":"\u4e54\u4e16\u748b\/\u738b\u6d77\u8f89Nature Communications\uff1a\u786b\u5316\u5b66\u6280\u672f\u63d0\u9ad8\u7535\u6c60\u5bff\u547d"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

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\"\"<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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a-c Mo5<\/sub>N6<\/sub>\u3001MoN\u548cMo2<\/sub>N\u7684HAADF-STEM\u56fe\u50cf\u3002\u63d2\u56fe\u4e3aMo\u6784\u578b\u793a\u610f\u56fe\uff0c\u5176\u4e2d\u7ea2\u8272\u3001\u84dd\u8272\u548c\u7eff\u8272\u7403\u4f53\u5206\u522b\u4ee3\u8868Mo5<\/sub>N6<\/sub>\u3001MoN\u548cMo2<\/sub>N\u4e2d\u7684Mo\u539f\u5b50\u3002<\/p>\n

d, e Mo5<\/sub>N6<\/sub>, MoN\u548cMo2<\/sub>N\u7684Mo 3d XPS\u548cMo L3, L2 edge NEXAFS\u5149\u8c31\u3002<\/p>\n

f Mo5<\/sub>N6<\/sub>(0 0 4)\u7684\u8ba1\u7b97\u6a21\u578b\u3002<\/p>\n

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\"\"<\/p>\n

a\u4e09\u79cd\u786b\u7535\u6781\u57281C\u4e0b\u7684\u5faa\u73af\u6027\u80fd\u548cCE\u3002<\/p>\n

b\u6bd4\u8f83\u6700\u8fd1\u62a5\u9053\u7684RT Na-S\u7ec6\u80de\u7684\u5468\u671f\u6570\u548c\u5bb9\u91cf\u4fdd\u6301\u7387\u4e0e\u76ee\u524d\u7684\u5de5\u4f5c\uff0c\u5176\u4e2d\u8f83\u6df1\u7684\u989c\u8272\u8868\u793a\u66f4\u5927\u7684\u7279\u5b9a\u7535\u6d41\u3002<\/p>\n

c S\/Mo5<\/sub>N6<\/sub>\u3001S\/MoN\u3001S\/Mo2<\/sub>N\u7684\u989d\u5b9a\u5bb9\u91cf\u3002<\/p>\n

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e\u94a0\u79bb\u5b50\u6269\u6563\u5728Mo5<\/sub>N6<\/sub>(0 0 4)\u3001MoN(0 0 2)\u548cMo2<\/sub>N(1 0 0)\u8868\u9762\u7684\u80fd\u91cf\u5206\u5e03\u3002<\/p>\n

\u56fe3. RT Na-S\u7535\u6c60\u4e2d\u786b\u8fd8\u539f\u53cd\u5e94\u7684\u603b\u4f53\u52a8\u529b\u5b66\u3002<\/p>\n

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a S\/C\u7535\u6781\u7684\u6d4b\u91cf\u548c\u62df\u5408\u66f2\u7ebf\u3002<\/p>\n

b\u5728\u4e0d\u540c\u7535\u538b\u4e0bS\/C\u7535\u6781\u7684\u6d3b\u5316\u80fd\u3002<\/p>\n

c S\/Mo5<\/sub>N6<\/sub> Rct\u7684Arrhenius\u56fe\u3002<\/p>\n

d\u4e09\u79cd\u786b\u7535\u6781\u5728\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u6d3b\u5316\u80fd\u3002<\/p>\n

\u56fe4. Na2S\u7535\u6c89\u79ef\u52a8\u529b\u5b66\u7814\u7a76\u3002<\/p>\n

\"\"<\/p>\n

a S\/Mo5<\/sub>N6<\/sub>\u7535\u6781\u7684\u6052\u6d41\u653e\u7535\u66f2\u7ebf\u548c\u76f8\u5e94\u7684\u540c\u6b65\u5c04\u7ebf\u884d\u5c04\u56fe\u3002<\/p>\n

b-d\u4e09\u79cd\u6750\u6599\u7535\u6c89\u79ef\u901f\u7387\u6d4b\u91cf\u7684\u6052\u7535\u4f4d\u653e\u7535\u66f2\u7ebf\u3002\u63d2\u56fe\u662f\u7535\u6c89\u79ef\u7684\u524d400\u79d2\u3002<\/p>\n

e-g\u4e09\u79cd\u9634\u6781\u6750\u6599\u7535\u6c89\u79ef\u8bd5\u9a8c\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u56fe5. Na2<\/sub>S\u7535\u6c89\u79ef\u7684\u8ba1\u7b97\u7814\u7a76\u3002<\/p>\n

\"\"<\/p>\n

a \u4e09\u4e2a\u8868\u9762\u4e0aNa2<\/sub>S2<\/sub>\u8f6c\u5316\u4e3aNaS *\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u56fe\u3002<\/p>\n

b\u8ba1\u7b97\u7684\u0394Gdiss-1<\/sub>\u6216\u0394GB<\/sub>\u503c\u4e0e\u4e09\u79cd\u6c2e\u5316\u94bc\u8868\u9762\u7535\u6c89\u79ef\u5bb9\u91cf\u4e4b\u95f4\u7684\u5173\u7cfb\u3002<\/p>\n

c Mo5<\/sub>N6<\/sub>\u8868\u9762NaS*\u5f62\u6210\u6b65\u9aa4\u7684\u539f\u5b50\u6784\u578b\u3002<\/p>\n

\u56fe6. \u94bc\u5728\u76f8\u5e94\u53cd\u5e94\u8fc7\u6e21\u6001\u4e0b\u7684\u7535\u5b50\u7ed3\u6784\u5206\u6790\u3002<\/p>\n

\"\"<\/p>\n

a-c Ex-situ NEXAFS\u7528\u4e8eS\/Mo5<\/sub>N6<\/sub>\u3001S\/MoN\u548cS\/Mo2<\/sub>N\u7684Mo L3<\/sub>-edge\u3002<\/p>\n

b-d\u4e09\u79cd\u9634\u6781\u6750\u6599\u4e0aNaS\u2217formation\u6b65\u9aa4\u7684\u8fc7\u6e21\u6001\u6784\u578b\u5206\u6790\u7535\u8377\u5dee\u5f02\u3002<\/p>\n

e \u5438\u9644\u4f4d\u70b9\u548c\u5438\u9644\u8d28\u8f68\u9053\u6742\u5316\u7684\u80fd\u7ea7\u56fe\u3002<\/p>\n

f\u5b9e\u7ebf\u8868\u793a\u56fe6b-d\u4e2d\u7ea2\u8272\u5706\u5708\u4e2dS\u7684DOS\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

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\u6587\u732e\u94fe\u63a5\uff1aA Mo5N6 electrocatalyst for efficient Na2S electrodeposition in room-temperature sodium-sulfur batteries<\/a>. 2021. Nature Communications, DOI: 10.1038\/s41467-021-27551-7.<\/p>\n

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