{"id":232194,"date":"2022-01-22T06:43:38","date_gmt":"2022-01-21T22:43:38","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=232194"},"modified":"2022-01-21T20:43:57","modified_gmt":"2022-01-21T12:43:57","slug":"nat-commun-%e5%a4%9a%e5%a3%b3%e5%b1%82%e9%87%91%e5%b1%9e%e6%9c%89%e6%9c%ba%e6%a1%86%e6%9e%b6%e5%af%b9%e9%85%b6%e8%bf%9b%e8%a1%8c%e5%88%86%e5%b1%82%e5%b0%81%e8%a3%85%e5%ae%9e%e7%8e%b0%e7%ba%a7","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=232194","title":{"rendered":"Nat. Commun. :\u591a\u58f3\u5c42\u91d1\u5c5e\u6709\u673a\u6846\u67b6\u5bf9\u9176\u8fdb\u884c\u5206\u5c42\u5c01\u88c5\u5b9e\u73b0\u7ea7\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94"},"content":{"rendered":"<p>\u3010\u5f15\u8a00\u3011<\/p>\n<p><strong>\u7ea7\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94<\/strong>\u5728\u751f\u7269\u4fe1\u53f7\u8f6c\u5bfc\u548c\u4ee3\u8c22\u9014\u5f84\u4e2d\u53d1\u6325\u91cd\u8981\u529f\u80fd\u3002\u5728\u751f\u7269\u7cfb\u7edf\u4e2d\uff0c\u590d\u6742\u7684\u751f\u7269\u50ac\u5316\u7ea7\u8054\u8fc7\u7a0b\u53d1\u751f\u5728\u4e0d\u540c\u7684\u7ec6\u80de\u819c\u5206\u79bb\u7684\u7ec6\u80de\u5668\u4e2d\uff0c\u4ee5\u9632\u6b62\u65e0\u6548\u7684\u4e32\u6270\u548c\u6545\u969c\uff0c\u4ece\u800c\u4ee5\u5353\u8d8a\u7684\u6548\u7387\u751f\u4ea7\u751f\u7269\u5236\u54c1\u3002\u6548\u4eff\u81ea\u7136\u7cfb\u7edf\u4e2d\u7684\u591a\u9176\u50ac\u5316\u7ea7\u8054\uff0c\u5e76\u4e14\u5b9e\u73b0\u5728\u5bc6\u95ed\u7ed3\u6784\u4e2d\u8fdb\u884c\u53cd\u5e94\uff0c\u5728\u65b0\u5174\u7684\u7cfb\u7edf\u5316\u5b66\u9886\u57df\u8d8a\u6765\u8d8a\u53d7\u5230\u5173\u6ce8\u3002MOFs\u5177\u6709\u53ef\u5b9a\u5236\u7684\u6676\u4f53\u548c\u5b54\u9053\u3001\u5927\u4e14\u53ef\u53ca\u7684\u6bd4\u8868\u9762\u79ef\u548c\u591a\u7528\u9014\u7684\u6846\u67b6\u7ec4\u6210\u7b49\u72ec\u7279\u4f18\u52bf\uff0c\u56e0\u6b64\u91d1\u5c5e-\u6709\u673a\u6846\u67b6(MOFs)\u652f\u67b6\u4e2d\u9176\u7684\u7a7a\u95f4\u7ec4\u7ec7\u4e3a\u8bbe\u8ba1\u591a\u9176\u50ac\u5316\u7ea7\u8054\u63d0\u4f9b\u4e86\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u65b9\u6cd5\u3002\u76ee\u524d\u51e0\u79cd\u81ea\u7ec4\u88c5\u7684MOF\u7ed3\u6784\u5df2\u88ab\u7528\u4e8e\u64cd\u4f5c\u751f\u7269\u50ac\u5316\u7ea7\u8054\u8fc7\u7a0b\u3002\u4f8b\u5982\uff0c\u7ec4\u88c5\u5728Pickering\u4e73\u6db2\u4e0a\u7684MOF\u80f6\u56ca\u548c\u4e92\u8865\u80bd\u8fde\u63a5\u7684MOF\u94fe\u53ef\u4ee5\u5f62\u6210\u4e0d\u540c\u7684\u7a7a\u95f4\u9694\u95f4\uff0c\u6765\u89e6\u53d1\u591a\u9176\u50ac\u5316\u7ea7\u8054\u53cd\u5e94\u3002\u8fd9\u4e9b\u7cfb\u7edf\u5206\u522b\u5c06\u4e0d\u540c\u7684\u9176\u56fa\u5b9a\u5728MOF\u80f6\u56ca\u6216\u9897\u7c92\u4e2d\u3002\u7136\u800c\uff0c\u7531\u4e8e\u4e2d\u95f4\u4ea7\u7269\u5728\u5404\u9694\u95f4\u4e4b\u95f4\u7684\u7f13\u6162\u8fd0\u8f93\uff0c\u50ac\u5316\u6548\u7387\u53d7\u5230\u4e86\u9650\u5236\u3002\u6b64\u5916\uff0c\u7531\u4e0d\u540c\u5927\u5c0f\u7684\u7a7a\u8154\u7ec4\u6210\u7684\u591a\u5c42\u7ed3\u6784\u7684MOFs\u4e5f\u53ef\u5e94\u7528\u4e8e\u4e00\u5bf9\u591a\u9176\u50ac\u5316\u7ea7\u8054\uff1b\u7136\u800c\uff0c\u8fd9\u4e9b\u7cfb\u7edf\u9700\u8981\u7b26\u5408\u4e25\u683c\u7684\u8bbe\u8ba1\u548c\u82db\u523b\u7684\u5408\u6210\u6761\u4ef6\u3002<\/p>\n<p>\u540c\u65f6\uff0c\u6784\u5efa\u80fd\u591f\u4f7f\u9176\u5728\u7eb3\u7c73\u53cd\u5e94\u5668\u4e2d\u7684\u5ba4\u72b6\u7a7a\u95f4\uff0c\u53ef\u4ee5\u4e3a\u9176\u76f8\u4e92\u4f5c\u7528\u7684\u8c03\u63a7\u548c\u9ad8\u6548\u7ea7\u8054\u7cfb\u7edf\u7684\u5f00\u53d1\u63d0\u4f9b\u91cd\u8981\u7684\u89c6\u89d2\u3002\u73b0\u6709\u7684\u6280\u672f\uff0c\u5982\u5085\u91cc\u53f6\u53d8\u6362\u7ea2\u5916\u5149\u8c31(FTIR)\u662f\u4e00\u79cd\u65e0\u635f\u3001\u65e0\u6807\u8bb0\u7684\u8868\u5f81\u6280\u672f\uff0c\u4f46\u53ea\u5c40\u9650\u4e8e\u5757\u72b6\u6837\u54c1\u68c0\u6d4b\u3002\u5171\u805a\u7126\u663e\u5fae\u955c\u662f\u4e00\u79cd\u7528\u4e8e\u68c0\u6d4b\u9650\u57df\u5728\u5355\u7a7a\u95f4\u5ba4MOFs\u5185\u7684\u9176\u7684\u6280\u672f\u3002\u7136\u800c\uff0c\u7531\u4e8e\u884d\u5c04\u6781\u9650\u7684\u9650\u5236\uff0c\u5176\u7a7a\u95f4\u5206\u8fa8\u7387\u65e0\u6cd5\u8fdb\u4e00\u6b65\u7814\u7a76\u7eb3\u7c73\u7ea7\u9176\u3002\u7eb3\u7c73\u7ea2\u5916\u5149\u8c31(nano-FTIR)\u662f\u4e00\u79cd\u72ec\u7279\u7684\u5149\u8c31\u6280\u672f\uff0c\u80fd\u591f\u4ee5~10 nm\u7684\u7a7a\u95f4\u5206\u8fa8\u7387\u63ed\u793a\u5c40\u90e8\u5316\u5b66\u6210\u5206\u3002nano-FTIR\u5149\u8c31\u662f\u57fa\u4e8e\u539f\u5b50\u529b\u663e\u5fae\u955c(AFM)\uff0c\u5176\u4e2d\u91d1\u5c5eAFM\u9488\u5c16\u88ab\u5bbd\u5e26\u7ea2\u5916\u8f90\u5c04\u7167\u5c04\u3002\u9488\u5c16\u53ef\u4ee5\u4f5c\u4e3a\u4e00\u4e2a\u5929\u7ebf\uff0c\u5c06\u5165\u5c04\u7ea2\u5916\u573a\u96c6\u4e2d\u5728\u9488\u5c16\u9876\u7aef\uff0c\u4ea7\u751f\u7531\u9488\u5c16\u534a\u5f84\u51b3\u5b9a\u7684\u7a7a\u95f4\u5206\u8fa8\u7387\u7684\u5c40\u57df\u7ea2\u5916\u5149\u8c31\u3002\u5728\u6b64\u57fa\u7840\u4e0a\uff0cnano-FTIR\u5149\u8c31\u80fd\u591f\u53ef\u9760\u5730\u63a2\u6d4b\u5e76\u4e14\u7ed8\u5236\u7eb3\u7c73\u7ea7\u5316\u5b66\u6210\u5206\uff0c\u5e76\u5df2\u5e94\u7528\u4e8e\u5355\u819c\u86cb\u767d\u3001\u591a\u7ec4\u5206\u805a\u5408\u7269\u5171\u6df7\u7269\u548c\u5171\u5b58\u7eb3\u7c73\u76f8\u7684\u7814\u7a76\uff0c\u4f46\u5c1a\u672a\u7528\u4e8e\u591a\u9176\u7684\u7814\u7a76\u3002<\/p>\n<p><strong>\u3010\u7814\u7a76\u8fdb\u5c55\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c\u534e\u4e1c\u5e08\u8303\u5927\u5b66\u674e\u4e3d\u7814\u7a76\u56e2\u961f\u5728<strong><em>Nat. Commun.<\/em><\/strong>\u4e0a\u53d1\u8868\u4e86\u4e00\u7bc7\u9898\u76ee\u4e3a\u201c<strong>Hierarchically encapsulating enzymes with multi-shelled metal-organic frameworks for tandem biocatalytic reactions<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u62a5\u4e86\u4e00\u79cd\u901a\u8fc7\u5916\u5ef6<strong>\u9010\u58f3\u5c42\u8fc7\u751f\u957f(shell-by-shell overgrowth)<\/strong>\u6280\u672f\u5236\u5907\u7684\u591a\u58f3\u5c42MOFs\u7528\u4e8e\u5c01\u88c5\u591a\u9176\uff0c\u8be5\u6280\u672f\u63d0\u9ad8\u4e86\u4e0d\u76f8\u5bb9\u4e32\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94\u7684\u50ac\u5316\u6548\u7387\u3002\u5229\u7528nano-FTIR\u5149\u8c31\uff0c\u5728\u7eb3\u7c73\u7ea7\u5206\u8fa8\u7387\u4e0b\uff0c\u7ed8\u5236\u4e86\u5355\u4e2a\u591a\u7a7a\u95f4\u5ba4MOF\u9897\u7c92\u4e2d\u591a\u9176\u7684\u7a7a\u95f4\u7ec4\u7ec7\u5f62\u6001\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u4e0e\u6eb6\u6db2\u4e2d\u5904\u4e8e\u81ea\u7531\u72b6\u6001\u7684\u9176\u76f8\u6bd4\uff0c\u7ea7\u8054\u5728\u591a\u58f3MOFs\u4e2d\u76f8\u5bb9\u548c\u4e0d\u76f8\u5bb9\u9176\u7684\u96c6\u5408\u4f53\u7684\u50ac\u5316\u6548\u7387\u63d0\u9ad8\u4e86~ 5.8 &#8211; 13.5\u500d\u3002\u66f4\u4e3a\u91cd\u8981\u7684\u662f\uff0c\u591a\u58f3MOFs\u53ef\u4ee5\u4f5c\u4e3a\u4e00\u4e2a\u591a\u7a7a\u95f4\u5206\u9694\u7684\u7eb3\u7c73\u53cd\u5e94\u5668\uff0c\u5141\u8bb8\u5728\u4e00\u4e2aMOF\u7eb3\u7c73\u9897\u7c92\u4e2d\u7269\u7406\u5730\u5212\u5206\u591a\u4e2a\u9176\uff0c\u4ee5\u4fbf\u5728\u4e00\u9505\u53cd\u5e94\u4e2d\u5b9e\u73b0\u4e0d\u76f8\u5bb9\u7684\u4e32\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94\u3002\u6b64\u5916\uff0c\u591a\u58f3MOFs\u8fd8\u53ef\u4ee5\u5b9e\u73b0\u5bf9\u591a\u9176\u7684\u4f4d\u7f6e\u8c03\u63a7\uff0c\u8fd9\u4f7f\u5f97\u50ac\u5316\u6548\u7387\u7684\u8c03\u8282\u66f4\u4e3a\u4fbf\u6377\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u7b80\u4ecb\u3011<\/strong><\/p>\n<p style=\"text-align: center;\"><strong>\u56fe1 <\/strong><strong>\u591a\u58f3ZIF-8 MOFs<\/strong><strong>\u4e2dGOx-HRP<\/strong><strong>\u7ea7\u8054 \u00a0<span style=\"color: #999999;\">\u00a9 2022 The Authors<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-232195\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/1-13.jpg\" alt=\"\" width=\"968\" height=\"796\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/1-13.jpg 968w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/1-13-300x247.jpg 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/1-13-768x632.jpg 768w\" sizes=\"(max-width: 968px) 100vw, 968px\" \/><\/p>\n<ol style=\"list-style-type: lower-alpha;\">\n<li>\u4ee5\u591a\u58f3ZIF-8\u5c01\u88c5\u7684\u517c\u5bb9\u9176(GOx\u548cHRP)\u9a71\u52a8\u4e32\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94;<\/li>\n<li>\u5408\u6210\u540e\u7684GOx@ZIF-8@HRP@ZIF-8\u7684TEM\u50cf;<\/li>\n<li>\u7528CIF\u6587\u4ef6\u6a21\u62dfZIF-8\u7684XRD\u8c31\u56fe(\u9ed1\u8272)\uff0c\u5408\u6210ZIF-8\u7684XRD(\u84dd\u8272)\uff0cGOx@ZIF-8@HRP@ZIF-8(\u7ea2\u8272)\u7684XRD;<\/li>\n<li>\u5408\u6210\u7684ZIF-8@ZIF-8(\u9ed1\u8272)\u548cGOx@ZIF8@HRP@ZIF-8(\u7ea2\u8272)\u7684TGA\u66f2\u7ebf;<\/li>\n<li>\u7eb3\u7c73\u5c3a\u5ea6\u7684FTIR\u5206\u6790\u793a\u610f\u56fe;<\/li>\n<li>GOx@ZIF-8@HRP@ZIF-8\u7684AFM\u56fe;<\/li>\n<li>GOx@ZIF-8@HRP@ZIF-8\u7684\u7ea2\u5916\u5149\u8c31\uff1b<\/li>\n<li>nano-FTIR\u7ebf\u626b\u63cf\u5149\u8c31\u56fe\uff1b<\/li>\n<li>\u7c92\u5b50\u5185\u58f3(\u5185)\u548c\u5916\u5c42\u58f3(\u5916\u5c421\u548c\u5916\u5c422)\u7684\u4ee3\u8868\u6027nano-FTIR\u70b9\u5149\u8c31\uff1b<\/li>\n<li>\u5728\u5355\u4e2a\u7c92\u5b50\u7684\u5185\u58f31652 cm\u22121\u548c\u5916\u5c421663 cm\u22121\u5904\u8bb0\u5f55\u7684\u7ea2\u5916\u76f8\u4f4d\u56fe\u50cf\uff1b<\/li>\n<li>GOx@ZIF-8@HRP@ZIF-8, free GOx &amp; HRP, GOx@ZIF-8 &amp; HRP@ZIF-8, GOx\/HRP@ZIF-8\u7cfb\u7edf\u7684\u50ac\u5316\u6548\u7387<\/li>\n<\/ol>\n<p style=\"text-align: center;\"><strong>\u56fe2\u00a0<\/strong><strong>\u591a\u58f3\u4e2d\u7a7aZIF-8 MOFs<\/strong><strong>\u4e2d\u7684Pro-ADH\/NAD+<\/strong><strong>\u7ea7\u8054 \u00a0<span style=\"color: #999999;\">\u00a9 2022 The Authors<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-232196\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/2-12.jpg\" alt=\"\" width=\"970\" height=\"854\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/2-12.jpg 970w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/2-12-300x264.jpg 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/2-12-768x676.jpg 768w\" sizes=\"(max-width: 970px) 100vw, 970px\" \/><\/p>\n<ol style=\"list-style-type: lower-alpha;\">\n<li>\u4e0d\u76f8\u5bb9\u9176\u548c\u8f85\u56e0\u5b50(Pro\u548cADH\/NAD+)\u9a71\u52a8\u591a\u58f3\u578b\u4e2d\u7a7aZIF-8\u4e32\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94\uff1b<\/li>\n<li>Pro@ZIF-8@ADH\/NAD+@ysZIF-8\u7684TEM\u56fe\uff1b<\/li>\n<li>Pro@ZIF-8@ADH\/NAD+@ysZIF-8\u7684EDX-mapping\uff1b<\/li>\n<\/ol>\n<p>d-g. Pro@ZIF-8@ADH\/NAD+@ysZIF-8\u7684nano-FTIR\u5206\u6790\uff1b<\/p>\n<p>h.\u5728\u5355\u4e2a\u7c92\u5b50\u7684\u5185\u58f31666 cm<sup>\u22121<\/sup>\u548c\u5916\u58f31658 cm<sup>\u22121<\/sup>\u5904\u7ea2\u5916\u76f8\u4f4d\u56fe\u50cf\uff1b<\/p>\n<p>i. Pro@ZIF-8@ADH\/NAD+ @ysZIF-8\u3001\u81ea\u7531Pro\u548cADH\/NAD+\u3001Pro\/ADH\/NAD+@ysZIF-8\u3001Pro@ZIF-8\u548cADH\/NAD+@ ysZIF-8\u4ee5\u53caPro@ZIF-8@ADH\/NAD+@ZIF-8\u4f53\u7cfb\u7684\u50ac\u5316\u6548\u7387\uff1b<\/p>\n<p>j. \u4e0d\u540c\u523b\u8680\u65f6\u95f4\u4e3a0\u5929\u30011\u5929\u30013\u5929\u30017\u5929\u7684Pro@ZIF-8@ADH\/NAD+@ZIF-67@ZIF-8\u7684ADH\u53d1\u5c04\u5149\u8c31<\/p>\n<p style=\"text-align: center;\"><strong>\u56fe3 <\/strong><strong>\u591a\u9176\u7ea7\u8054\u7684\u4f4d\u7f6e\u63a7\u5236 \u00a0<span style=\"color: #999999;\">\u00a9 2022 The Authors<\/span><\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-232197\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/3-13.jpg\" alt=\"\" width=\"818\" height=\"1022\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/3-13.jpg 818w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/3-13-240x300.jpg 240w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2022\/01\/3-13-768x960.jpg 768w\" sizes=\"(max-width: 818px) 100vw, 818px\" \/><\/p>\n<ol style=\"list-style-type: lower-alpha;\">\n<li>\u9176\u95f4\u8ddd\u79bb\u7684\u53ef\u63a7\u8c03\u6574<\/li>\n<\/ol>\n<p>\u00a0 \u00a0 \u00a0 b-c. GOx@ZIF-8x (x = 1\u20133) \u548c Pro@ZIF-8x (x = 1\u20133)\u7684TEM\uff1b<\/p>\n<ol style=\"list-style-type: lower-alpha;\">\n<li>GOx-FITC@ZIF-8x@HRP-RhB@ZIF-8\u7684\u5171\u805a\u7126\u663e\u5fae\u955c\u56fe\u50cf:(i)\u4eae\u573a\uff0c(ii)\u5728488 nm\u6fc0\u53d1\u548c\u76d1\u6d4b\u8367\u5149\u6807\u8bb0\u7684GOx\u5728520 nm\u7684\u8367\u5149;(iii)\u5728543 nm\u6fc0\u53d1\uff0c\u5e76\u76d1\u6d4bRHB\u6807\u8bb0\u7684HRP\u5728620 nm\u7684\u8367\u5149;(iv)\u5408\u5e76\u7684\u56fe\u50cf\uff1b<\/li>\n<li>ProRhB@ZIF-8x@ADH-FITC\/NAD+-coumarin@ysZIF-8\u7684\u5171\u805a\u7126\u663e\u5fae\u955c\u56fe\u50cf:(i)\u4eae\u573a\uff0c(ii)\u5728543 nm\u6fc0\u53d1\uff0c\u76d1\u6d4brhb\u6807\u8bb0Pro\u5728620 nm\u7684\u8367\u5149;(iii)\u5728488 nm\u5904\u6fc0\u53d1\uff0c\u5e76\u5728520 nm\u5904\u76d1\u6d4b\u8367\u5149\u6807\u8bb0ADH\u7684\u8367\u5149;(iv) 405 nm\u6fc0\u53d1\uff0c\u5e76\u76d1\u6d4b\u9999\u8c46\u7d20\u6807\u8bb0\u7684NAD+\u5728480 nm\u5904\u7684\u8367\u5149;(v)\u5408\u5e76\u7684\u56fe\u50cf\uff1b<\/li>\n<li>\u9176\u95f4\u8ddd\u79bb\u5bf9GOx-HRP\u548cg Pro-ADH\/NAD+\u7ea7\u8054\u6d3b\u6027\u7684\u5f71\u54cd\uff1b<\/li>\n<li>\u9176\u4f4d\u7f6e\u5bf9 GOx-HRP\u548ci Pro-ADH\/NAD+\u7ea7\u8054\u6d3b\u6027\u7684\u5f71\u54cd\uff1b<\/li>\n<\/ol>\n<p>j-k. GOx@ZIF-8@HRP@ZIF-8\u548cPro@ZIF-8@ADH\/NAD+@ysZIF-8\u7684\u50ac\u5316\u518d\u5faa\u73af\u80fd\u529b<\/p>\n<p>&nbsp;<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>\u603b\u4e4b\uff0c\u7814\u7a76\u8005\u8bc1\u660e\u4e86\u591a\u58f3MOFs\u53ef\u4ee5\u4f5c\u4e3a\u5206\u7ea7\u652f\u67b6\uff0c\u5728\u7eb3\u7c73\u5c3a\u5ea6\u4e0a\u7a7a\u95f4\u7ec4\u7ec7\u9176\uff0c\u4ee5\u63d0\u9ad8\u50ac\u5316\u6548\u7387\u3002\u4e0e\u5176\u4ed6\u7b56\u7565\u76f8\u6bd4\uff0c\u4f7f\u7528\u591a\u58f3MOF\u652f\u67b6\u8bbe\u8ba1\u591a\u9176\u50ac\u5316\u7ea7\u8054\u5177\u6709\u4ee5\u4e0b\u663e\u8457\u7279\u70b9:<\/p>\n<p>(1)\u591a\u5b54MOF\u652f\u67b6\u4e3a\u7a7a\u95f4\u53d7\u9650\u7684\u9176\u6d3b\u6027\u4f4d\u70b9\u4e4b\u95f4\u7684\u4f20\u8d28\u63d0\u4f9b\u4e86\u6307\u5b9a\u7684\u6269\u6563\u8def\u5f84\uff0c\u4fc3\u8fdb\u4e86\u4e32\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94\u7684\u9ad8\u6548\u8fd0\u884c;<\/p>\n<p>(ii)\u5728<strong>\u9010\u58f3\u5c42\u8fc7\u751f\u957f(shell-by-shell overgrowth)<\/strong>\u8fc7\u7a0b\u4e2d\uff0c\u4e0d\u76f8\u5bb9\u7684\u9176\u53ef\u4ee5\u72ec\u7acb\u52a0\u8f7d\u5728\u591a\u58f3MOFs\u7684\u4e0d\u540c\u533a\u57df\u4e2d;<\/p>\n<p>(iii)\u901a\u8fc7\u8c03\u6574\u5916\u5ef6\u8fc7\u751f\u957f\u7684\u5468\u671f\uff0c\u53ef\u4ee5\u4f7f\u591a\u9176\u5728\u7a7a\u95f4\u4e0a\u9650\u5236\u5728\u4e0d\u540c\u7684\u9176\u95f4\u8ddd\u79bb\uff1b\u901a\u8fc7\u8c03\u6574\u5c01\u88c5\u5e8f\u5217\uff0c\u53ef\u4ee5\u4f7f\u591a\u9176\u5728\u7a7a\u95f4\u4e0a\u9650\u5236\u5728\u4e0d\u540c\u4f4d\u70b9\uff1b\u56e0\u6b64\uff0c\u4e32\u8054\u751f\u7269\u50ac\u5316\u6548\u7387\u53ef\u4ee5\u5f88\u5bb9\u6613\u5730\u8c03\u8282\u3002\u603b\u7684\u6765\u8bf4\uff0c\u8fd9\u4e9b\u7279\u6027\u6709\u671b\u4f7f\u591a\u58f3\u5c42MOFs\u6210\u4e3a\u5728\u751f\u7269\u6280\u672f\u548c\u6cbb\u7597\u4e2d\u591a\u9176\u50ac\u5316\u7ea7\u8054\u53cd\u5e94\u7684\u6f5c\u5728\u7eb3\u7c73\u8f7d\u4f53\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5<\/strong>\uff1a<a href=\"https:\/\/doi.org\/10.1038\/s41467-022-27983-9\">Hierarchically encapsulating enzymes with multi-shelled metal-organic frameworks for<\/a><\/p>\n<p><a href=\"https:\/\/doi.org\/10.1038\/s41467-022-27983-9\">tandem biocatalytic reactions<\/a>. 2022, <em>Nat. Commun.<\/em> Doi: 10.1038\/s41467-022-27983-9.<\/p>\n<p>&nbsp;<\/p>\n<p>&nbsp;<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u3010\u5f15\u8a00\u3011 \u7ea7\u8054\u751f\u7269\u50ac\u5316\u53cd\u5e94\u5728\u751f\u7269\u4fe1\u53f7\u8f6c\u5bfc\u548c\u4ee3\u8c22\u9014\u5f84\u4e2d\u53d1\u6325\u91cd\u8981\u529f\u80fd\u3002\u5728\u751f\u7269\u7cfb\u7edf\u4e2d\uff0c\u590d\u6742\u7684\u751f\u7269\u50ac\u5316\u7ea7\u8054\u8fc7\u7a0b\u53d1\u751f\u5728\u4e0d\u540c\u7684\u7ec6\u80de\u819c\u5206\u79bb\u7684\u7ec6\u80de\u5668\u4e2d\uff0c\u4ee5\u9632\u6b62\u65e0\u6548\u7684\u4e32\u6270\u548c\u6545\u969c\uff0c&#8230;<\/p>\n","protected":false},"author":2114,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215,2],"tags":[],"class_list":["post-232194","post","type-post","status-publish","format-standard","hentry","category-jiedu","category-keji"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/232194"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/2114"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=232194"}],"version-history":[{"count":6,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/232194\/revisions"}],"predecessor-version":[{"id":232234,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/232194\/revisions\/232234"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=232194"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=232194"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=232194"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}