{"id":232621,"date":"2022-02-01T06:29:59","date_gmt":"2022-01-31T22:29:59","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=232621"},"modified":"2022-01-31T11:30:07","modified_gmt":"2022-01-31T03:30:07","slug":"%e5%8c%97%e4%ba%ac%e5%a4%a7%e5%ad%a6%e6%bd%98%e9%94%8b%e6%95%99%e6%8e%88%e5%9b%a2%e9%98%9f2021%e5%b9%b4%e5%9c%a8%e7%94%b5%e6%b1%a0%e9%a2%86%e5%9f%9f%e7%9a%84%e4%bb%a3%e8%a1%a8%e6%80%a7%e7%a0%94","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=232621","title":{"rendered":"\u5317\u4eac\u5927\u5b66\u6f58\u950b\u6559\u6388\u56e2\u961f2021\u5e74\u5728\u7535\u6c60\u9886\u57df\u7684\u4ee3\u8868\u6027\u7814\u7a76\u6210\u679c"},"content":{"rendered":"

\u6f58\u950b\u6559\u6388\uff0c\u5317\u4eac\u5927\u5b66\u8bb2\u5e2d\u6559\u6388\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\uff0c\u5317\u4eac\u5927\u5b66\u6df1\u5733\u7814\u7a76\u751f\u9662\u526f\u9662\u957f\u548c\u65b0\u6750\u6599\u5b66\u9662\u521b\u9662\u9662\u957f\u3002\u6f58\u950b\u6559\u6388\u4e8e1985\u5e74\u6bd5\u4e1a\u4e8e\u5317\u4eac\u5927\u5b66\u5316\u5b66\u7cfb\uff0c1988\u5e74\u5728\u4e2d\u79d1\u9662\u798f\u5efa\u7269\u6784\u6240\u83b7\u5f97\u7855\u58eb\u5b66\u4f4d\uff0c1994\u5e74\u5728\u82f1\u56fdStrathclyde\u5927\u5b66\u83b7\u5f97\u535a\u58eb\u5b66\u4f4d\uff0c\u5e76\u83b7\u5f97\u6700\u4f73\u535a\u58eb\u8bba\u6587\u5956\uff0c\u540c\u5e74\u5728\u745e\u58ebETH\u4ece\u4e8b\u535a\u58eb\u540e\u7814\u7a76\u3002\u4ed6\u957f\u671f\u81f4\u529b\u4e8e\u7ed3\u6784\u5316\u5b66\u548c\u6750\u6599\u57fa\u56e0\u7684\u63a2\u7d22\u3001\u7535\u6c60\u548c\u50ac\u5316\u6750\u6599\u7ed3\u6784\u4e0e\u6027\u80fd\u53ca\u5e94\u7528\u7814\u7a76\uff0c\u53d1\u8868\u4e86\u5305\u62ecNature\uff0cNature Energy\u3001Nature Nanotech\u3001Joule\u3001JACS \u7b49\u5185\u7684SCI\u4ee3\u8868\u6027\u8bba\u6587300\u4f59\u7bc7\u30022020\u5e74\u4efb\u300a\u7ed3\u6784\u5316\u5b66\u300b\u6742\u5fd7\u7684\u6267\u884c\u4e3b\u7f16\uff0c\u83b72021\u5e74\u83b7\u201c\u4e2d\u56fd\u7535\u5316\u5b66\u8d21\u732e\u5956\u201d\u30012018\u5e74\u7f8e\u56fd\u7535\u5316\u5b66\u5b66\u4f1a\u7535\u6c60\u79d1\u6280\u5956\u4e0e2016\u5e74\u56fd\u9645\u7535\u52a8\u8f66\u9502\u7535\u6c60\u534f\u4f1a\u6770\u51fa\u7814\u7a76\u5956\u3002\uff08\u4ee5\u4e0a\u5185\u5bb9\u53c2\u8003\u81ea\uff1a\u5317\u4eac\u5927\u5b66\u5b98\u7f51\uff09<\/p>\n

\u8fd1\u65e5\uff0c\u6211\u4eec\u68b3\u7406\u4e86\u6f58\u950b\u6559\u6388\u56e2\u961f2021\u5e74\u5728\u7535\u6c60\u9886\u57df\u53d1\u8868\u7684\u4e00\u4e9b\u91cd\u8981\u7684\u7814\u7a76\u6210\u679c\u3002<\/p>\n

Nat. Energy\uff1a\u7406\u89e3\u9502\u7535\u6c60\u4e2d\u94b4\u7684\u4f5c\u7528\u53ca\u5f00\u53d1\u65e0\u94b4\u9ad8\u954d\u6b63\u6781\u6750\u6599<\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/www.nature.com\/articles\/s41560-021-00776-y.<\/strong><\/p>\n

Nature Nanotechnology\uff1a\u94b4\u9178\u9502\u9ad8\u538b\u4e0d\u7a33\u5b9a\u6027\u7684\u7ed3\u6784\u6210\u56e0\u7814\u7a76<\/p>\n

\"\"<\/p>\n

\u5c42\u72b6\u94b4\u9178\u9502(LiCoO2<\/sub>, LCO)\u662f\u9502\u79bb\u5b50\u7535\u6c60\u4e2d\u6700\u6210\u529f\u7684\u5546\u4e1a\u5316\u6b63\u6781\u6750\u6599\u3002\u867d\u7136\u5176\u7406\u8bba\u5bb9\u91cf\u662f274 mAh g\u22121<\/sup>\uff0c\u5b9e\u9645\u5b89\u5168\u4f7f\u7528\u5bb9\u91cf\u662f\u57284.25V(\u76f8\u5bf9\u4e8eLi\/Li+<\/sup>)\u7ea6150 mAh g\u22121<\/sup>\uff0c\u56e0\u4e3a\u5f53\u7535\u538b\u5347\u9ad8\u540e\u5176\u8868\u73b0\u51fa\u663e\u8457\u7684\u7ed3\u6784\u4e0d\u7a33\u5b9a\u6027\u3002\u867d\u7136\u76ee\u524d\u4e00\u4e9b\u9ad8\u538bLCO (H-LCO)\u6750\u6599\u5df2\u88ab\u53d1\u73b0\u5e76\u5546\u4e1a\u5316\uff0c\u4f46\u5176\u7a33\u5b9a\u6027\u7684\u7ed3\u6784\u673a\u7406\u4ecd\u96be\u4ee5\u786e\u5b9a\u3002\u5728\u6b64\uff0c\u8be5\u56e2\u961f\u5229\u7528\u4e09\u7ef4\u8fde\u7eed\u65cb\u8f6c\u7535\u5b50\u884d\u5c04\u65b9\u6cd5\u8f85\u52a9\u9ad8\u5206\u8fa8\u7387\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\uff0c\u7814\u7a76\u4e86\u4e24\u79cd\u5546\u7528LCO\u6750\u6599:\u6b63\u5e384.25V \u7a33\u5b9aLCO (N-LCO)\u548c\u9ad8\u7535\u538b4.5V\u7a33\u5b9a\u7684H-LCO\u5728\u539f\u5b50\u6c34\u5e73\u4e0a\u7684\u7ed3\u6784\u5dee\u5f02\u3002\u8fd9\u4e9b\u5f3a\u6709\u529b\u7684\u5de5\u5177\u8868\u660e\uff0c\u94b4\u6c27\u5316\u7269\u5c42\u5c42\u662f\u5426\u5f2f\u66f2\uff08\u7279\u522b\u662f\u8868\u9762\u9644\u8fd1\u7684\u5f2f\u66f2\u66f2\u7387\uff09\u51b3\u5b9a\u4e86\u6750\u6599\u5728\u9ad8\u7535\u538b\u4e0b\u7684\u7ed3\u6784\u662f\u5426\u7a33\u5b9a\u6027\uff0c\u5e73\u6574\u7684\u94b4\u6c27\u5316\u7269\u5c42\u80fd\u63d0\u9ad8\u5728\u9ad8\u7535\u538b\u4e0b\u7684\u7535\u6c60\u7ed3\u6784\u548c\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u5728\u7406\u8bba\u8ba1\u7b97\u7684\u652f\u6301\u4e0b\uff0c\u8fd9\u79cd\u5bf9\u5c42\u72b6LCO\u6750\u6599\u7ed3\u6784\u6027\u80fd\u5173\u7cfb\u5728\u539f\u5b50\u5c3a\u5ea6\u7684\u7406\u89e3\u4e3a\u672a\u6765\u8bbe\u8ba1\u5728\u9ad8\u7535\u538b\u4e0b\u5177\u6709\u4f18\u5f02\u7ed3\u6784\u7a33\u5b9a\u6027\u7684\u65b0\u578b\u6b63\u6781\u6750\u6599\u63d0\u4f9b\u4e86\u6709\u7528\u7684\u6307\u5bfc\u3002\u8be5\u6210\u679c\u4ee5\u201cStructural origin of the high-voltage instability of lithium cobalt oxide<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nature Nanotechnology<\/strong>\u4e0a\u3002DOI<\/strong>\uff1a<\/strong>10.1038\/s41565-021-00855-x<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/www.nature.com\/articles\/s41565-021-00855-x<\/a>.<\/strong><\/p>\n

Nat. Commun\uff1a\u683e\u6676\u6676\u754c\u6539\u5584\u5c16\u6676\u77f3\u9530\u9178\u9502\u6b63\u6781\u6750\u6599\u7684\u9502\u79bb\u5b50\u6269\u6563\u548c\u5feb\u5145<\/p>\n

\"\"<\/p>\n

\u7535\u6781\u6750\u6599\u4e0a\u7684\u7f3a\u9677\u5de5\u7a0b\u88ab\u8ba4\u4e3a\u662f\u6539\u5584\u7535\u6c60\u7535\u5316\u5b66\u6027\u80fd\u7684\u6709\u6548\u9014\u5f84\uff0c\u8fd9\u662f\u56e0\u4e3a\u5404\u79cd\u4e0d\u540c\u5c3a\u5ea6\u7f3a\u9677\u7684\u5b58\u5728\u53ef\u80fd\u4f1a\u4fc3\u8fdb\u79bb\u5b50\u6269\u6563\u5e76\u63d0\u4f9b\u989d\u5916\u7684\u50a8\u9502\u4f4d\u70b9\u3002\u7136\u800c\uff0c\u5904\u7406\u7f3a\u9677\u5e76\u6df1\u5165\u4e86\u89e3\u5176\u5728\u7535\u6781\u6750\u6599\u4e2d\u7684\u4f5c\u7528\u4ecd\u7136\u5177\u6709\u6311\u6218\u6027\u3002\u8be5\u5de5\u4f5c\u901a\u8fc7\u8c03\u6574\u5408\u6210\u6761\u4ef6\uff0c\u6709\u610f\u5730\u5728\u5c16\u6676\u77f3\u9530\u9178\u9502\u6b63\u6781\u4e2d\u5f15\u5165\u5927\u91cf\u5b6a\u6676\u754c\u3002\u901a\u8fc7\u9ad8\u5206\u8fa8\u7387\u626b\u63cf\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u548c\u4e2d\u5b50\u884d\u5c04\uff0c\u9610\u660e\u4e86\u5b6a\u6676\u754c\u7f3a\u9677\u7684\u8be6\u7ec6\u7ed3\u6784\uff0c\u5b6a\u6676\u754c\u7f3a\u9677\u7684\u5f62\u6210\u5f52\u56e0\u4e8e\u5360\u636e\u5b6a\u6676\u754c\u5468\u56f4Mn\u4f4d\u7684\u805a\u96c6\u5927\u91cf\u7684\u9502\u539f\u5b50\u3002\u7ed3\u5408\u7535\u5316\u5b66\u5b9e\u9a8c\u548c\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\uff0c\u8bc1\u660e\u4e86\u5c16\u6676\u77f3\u9530\u9178\u9502\u6b63\u6781\u4e2d\u5b6a\u6676\u754c\u7684\u5b58\u5728\u80fd\u591f\u5b9e\u73b0\u9502\u79bb\u5b50\u7684\u5feb\u901f\u6269\u6563\uff0c\u4ece\u800c\u83b7\u5f97\u4f18\u5f02\u7684\u5feb\u5145\u6027\u80fd\uff0c\u5373\u57285 C\u548c10 C\u7684\u500d\u7387\u4e0b\uff0c\u5bb9\u91cf\u4fdd\u6301\u7387\u5206\u522b\u4e3a75%\u548c58%\u3002\u8fd9\u4e00\u53d1\u73b0\u8bc1\u660e\u4e86\u901a\u8fc7\u7f3a\u9677\u5de5\u7a0b\u5236\u9020\u5feb\u5145\u9634\u6781\u7684\u7b80\u5355\u6709\u6548\u7684\u65b9\u6cd5\u3002\u8be5\u6210\u679c\u4ee5\u201cTwin boundary defect engineering improves lithium-ion diffusion for fast-charging spinel cathode materials<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Nat. Commun<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1038\/s41467-021-23375-7<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/www.nature.com\/articles\/s41467-021-23375-7<\/a>.<\/strong><\/p>\n

Joule\uff1aLi2<\/sub>MnO3<\/sub>\u7684\u5faa\u73af\u673a\u7406: Li-CO2<\/sub>\u7535\u6c60\u5faa\u73af\u673a\u7406\u53ca\u6b63\u6781\u6750\u6599\u4e2d\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u7684\u5171\u6027<\/p>\n

\"\"<\/p>\n

Li2<\/sub>MnO3<\/sub>\u88ab\u8ba4\u4e3a\u662f\u9502\u7535\u6c60\u5bcc\u9502\u9530\u57fa\uff08xLi2<\/sub>MnO3<\/sub>\uff1ayNMC\uff09\u6b63\u6781\u6750\u6599\u4ee3\u8868\u6027\u7684\u5bcc\u9502\u5316\u5408\u7269\uff0c\u5bf9\u5176\u6c27\u7684\u6d3b\u6027\u6709\u4e00\u5b9a\u7684\u4e89\u8bae\u3002\u8be5\u5de5\u4f5c\u901a\u8fc7\u5bf9Li2<\/sub>MnO3<\/sub>\u57fa\u4f53\u548c\u8868\u9762Mn\u548cO\u72b6\u6001\u7684\u8bc4\u4ef7\uff0c\u9610\u8ff0\u4e86Mn(III\/IV)\u6c27\u5316\u8fd8\u539f\u4e3b\u5bfc\u4e86Li2<\/sub>MnO3<\/sub>\u7684\u53ef\u9006\u672c\u4f53\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\uff0c\u800c\u521d\u59cb\u7535\u8377\u5e73\u53f0\u662f\u7531\u6c27\u91ca\u653e\u548c\u78b3\u9178\u76d0\u5206\u89e3\u7684\u8868\u9762\u53cd\u5e94\u4ea7\u751f\u7684\u3002\u5728\u4efb\u4f55\u7535\u5316\u5b66\u9636\u6bb5\u90fd\u4e0d\u6d89\u53ca\u6676\u683c\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u3002\u78b3\u9178\u76d0\u7684\u5f62\u6210\u548c\u5206\u89e3\u8868\u660e\u4e86Li2<\/sub>MnO3<\/sub>\u8868\u9762\u7684\u50ac\u5316\u6027\u80fd\uff0c\u4ece\u800c\u6fc0\u53d1\u4e86Li2<\/sub>MnO3<\/sub>\u4f5c\u4e3a\u4f18\u826f\u7535\u50ac\u5316\u5242\u7684Li-CO2<\/sub>\/\u7a7a\u6c14\u7535\u6c60\u3002Li2<\/sub>MnO3<\/sub>\u4e2d\u6ca1\u6709\u6676\u683c\u6c27\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\uff0c\u8fd9\u5bf9\u5bcc\u9502\u5316\u5408\u7269\u4e2d\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u7684\u6765\u6e90\u63d0\u51fa\u4e86\u8d28\u7591\uff0c\u901a\u8fc7\u5149\u8c31\u6bd4\u8f83\u53d1\u73b0\uff0c\u5bcc\u9502\u5316\u5408\u7269\u4e0e\u4f20\u7edf\u6750\u6599\u4e2d\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u5177\u6709\u76f8\u540c\u7684\u6027\u8d28\u3002\u8fd9\u4e9b\u53d1\u73b0\u4e3a\u7406\u89e3\u548c\u63a7\u5236\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u9634\u6781\u6c27\u6d3b\u6027\u53ca\u7535\u5316\u5b66\u754c\u9762\u50ac\u5316\u53cd\u5e94\u63d0\u4f9b\u4e86\u6307\u5bfc\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cCycling mechanism of Li2<\/sub>MnO3<\/sub>: Li\u2013CO2<\/sub> batteries and commonality on oxygen redox in cathode materials<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Joule<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1016\/j.joule.2021.02.004<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/www.sciencedirect.com\/science\/article\/pii\/S2542435121000817?via%3Dihub.<\/strong><\/p>\n

ACS Energy Lett\uff1aLi2<\/sub>MO3<\/sub> (M= Mn, Ru, Ir)\u4e2d\u4e0d\u540c\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u6d3b\u6027<\/p>\n

\"\"<\/p>\n

Li2<\/sub>MO3<\/sub> (M =\u8fc7\u6e21\u91d1\u5c5e)\u4f53\u7cfb\u662f\u5bcc\u9502\u6750\u6599\u7684\u6bcd\u4f53\u5316\u5408\u7269\uff0c\u88ab\u5e7f\u6cdb\u8ba4\u4e3a\u53ef\u4ee5\u4e3a\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7535\u6c60\u63d0\u4f9b\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u6027\u3002\u7136\u800c\uff0c\u6700\u8fd1\u7684\u7814\u7a76\u8868\u660e\uff0c\u5728\u4e09\u4e2a\u5177\u6709\u4ee3\u8868\u6027\u7684Li2<\/sub>MO3<\/sub> (M = Mn, Ru, Ir)\u5316\u5408\u7269\u4e2d\uff0cMn\u548cIr\u4f53\u7cfb\u4e2d\u6ca1\u6709\u53d1\u751f\u53ef\u9006\u7684\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u3002\u8fd9\u9879\u5de5\u4f5c\u901a\u8fc7\u5148\u8fdb\u7684\u5149\u8c31\u6280\u672f\u5bf9Li2<\/sub>RuO3<\/sub>\u4e2d\u7684\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u8fdb\u884c\u4e86\u91cd\u65b0\u8bc4\u4ef7\uff0c\u7ed3\u679c\u8868\u660e\uff0c\u948c\u6c27\u5316\u8fd8\u539f\u548c\u9ad8\u5ea6\u53ef\u9006\u7684O\u6c27\u5316\u8fd8\u539f\u6027(\u521d\u59cb\u5faa\u73af\u53ef\u9006\u602796%\uff0c10\u6b21\u5faa\u73af\u540e\u4fdd\u755980%\uff0c50\u6b21\u5faa\u73af\u540e\u4fdd\u755977%)\u3002\u8fd9\u4e0eLi2<\/sub>MnO3<\/sub>\u548cLi2<\/sub>IrO3<\/sub>\u4f53\u7cfb\u5f62\u6210\u4e86\u9c9c\u660e\u5bf9\u6bd4\uff0c\u5f97\u51fa\u4e86Li2<\/sub>MO3<\/sub>\u4f53\u7cfb\u5728\u5145\u7535\u8fc7\u7a0b\u4e2d\u7684\u4e09\u79cd\u4e0d\u540c\u6c27\u7684\u884c\u4e3a: (i)Li2<\/sub>MnO3<\/sub>\u4e2d\u53ea\u6709\u4e0d\u53ef\u9006\u6c27\u7684\u6c27\u5316; (ii)\u53ef\u9006\u7684Ru\u548cO\u5728Li2<\/sub>RuO3<\/sub>\u4e2d\u7684\u6c27\u5316\u8fd8\u539f; (iii)Li2<\/sub>IrO3<\/sub>\u4e2d\u4ec5\u5b58\u5728\u9633\u79bb\u5b50\u6c27\u5316\u8fd8\u539f\u3002\u8fd9\u9879\u5de5\u4f5c\u8868\u660e\u4e86\u8fc7\u6e21\u91d1\u5c5e\u53ca\u5176\u4e0e\u6c27\u7684\u8026\u5408\u5728\u7ef4\u6301\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7535\u6c60\u7684\u53ef\u9006\u6c27\u7684\u6c27\u5316\u8fd8\u539f\u6d3b\u6027\u65b9\u9762\u7684\u5173\u952e\u4f5c\u7528\u3002\u8be5\u9879\u7814\u7a76\u6210\u679c\u4ee5\u201cDistinct Oxygen Redox Activities in Li2<\/sub>MO3<\/sub> (M= Mn, Ru, Ir)<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728ACS Energy Lett<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1021\/acsenergylett.1c01101<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/pubs.acs.org\/doi\/10.1021\/acsenergylett.1c01101.<\/strong><\/p>\n

Adv. Energy Mater\uff1a\u57fa\u4e8e\u4f5c\u8005\u6d88\u6b67\u7684\u6750\u6599\u77e5\u8bc6\u56fe\u8c31\u6784\u5efa\u4e0e\u5e94\u7528\u2014\u2014\u518d\u8bbaLiFePO4<\/sub>\u7684\u53d1\u73b0\u4e0e\u5e94\u7528\u8fc7\u7a0b<\/p>\n

\"\"<\/p>\n

\u7531\u4e8e\u8fd1\u5e74\u6765\u8ba1\u7b97\u673a\u6280\u672f\u7684\u521b\u65b0\uff0c\u6750\u6599\u4fe1\u606f\u5b66\u8fd9\u4e00\u65b0\u5174\u9886\u57df\u5df2\u7ecf\u6210\u4e3a\u6750\u6599\u79d1\u5b66\u7814\u7a76\u8303\u5f0f\u9769\u547d\u7684\u50ac\u5316\u5242\u3002\u77e5\u8bc6\u56fe\u80fd\u591f\u4ece\u6d77\u91cf\u7684\u79d1\u7814\u8bba\u6587\u4e2d\u96c6\u4e2d\u83b7\u53d6\u79d1\u5b66\u77e5\u8bc6\uff0c\u5b9e\u73b0\u5b9e\u4f53\u95f4\u5173\u7cfb\u7684\u81ea\u52a8\u8bc6\u522b\uff0c\u4e3a\u77e5\u8bc6\u7ba1\u7406\u63d0\u4f9b\u652f\u6301\u3002\u5728\u672c\u7814\u7a76\u4e2d\uff0c\u4f5c\u8005\u6784\u5efa\u4e86\u4e00\u4e2a\u6750\u6599\u77e5\u8bc6\u56fe\u8c31MatKG\uff0c\u5b83\u5728\u6750\u6599\u79d1\u5b66\u9886\u57df\u7684\u4e3b\u4f53\u548c\u5ba2\u4f53\u4e4b\u95f4\u5efa\u7acb\u4e86\u72ec\u7279\u7684\u5bf9\u5e94\u5173\u7cfb\u3002\u89e3\u51b3\u6750\u6599\u77e5\u8bc6\u56fe\u8c31\u4e2d\u5173\u952e\u79d1\u5b66\u95ee\u9898–\u6d88\u9664\u4f5c\u8005\u7684\u6b67\u4e49\uff08\u4f5c\u8005\u6d88\u6b67\uff09\u4ee5\u53ca\u89e3\u51b3\u4e86\u57fa\u4e8e\u673a\u5668\u5b66\u4e60\u548c\u5339\u914d\u4f9d\u8d56\u7b97\u6cd5\u7684\u91cd\u590d\u6570\u636e\u5220\u9664\u6a21\u578b\u3002\u4ee5\u57fa\u4e8e\u9502\u7535\u6c60\u7684\u8bfa\u5956\u83b7\u5f97\u8005Goodenough\u5148\u751f\u6240\u53d1\u73b0\u7684LiFePO4<\/sub>\u6b63\u6781\u6750\u6599\uff0c\u8fd0\u7528MatKG\u8ddf\u8e2aLiFePO4<\/sub>\u7814\u7a76\u8fc7\u7a0b\uff0c\u81ea\u52a8\u8bb0\u5f55\u5230\u76ee\u524d\u4e3a\u6b62\u6240\u53d6\u5f97\u7684\u91cc\u7a0b\u7891\u53ca\u9884\u6d4b\u5176\u7814\u7a76\u8d8b\u52bf\u3002\u4f5c\u8005\u76f8\u4fe1MatKG\u53ef\u4ee5\u4f5c\u4e3a\u4e00\u4e2a\u591a\u529f\u80fd\u7684\u7814\u7a76\u5e73\u53f0\uff0c\u6574\u5408\u548c\u63d0\u70bc\u6750\u6599\u7684\u5404\u4e2a\u5b50\u9886\u57df\u548c\u4ea4\u53c9\u9886\u57df\u7684\u79d1\u5b66\u77e5\u8bc6\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cConstruction and Application of Materials Knowledge Graph Based on Author Disambiguation: Revisiting the Evolution of LiFePO4<\/sub><\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Adv. Energy Mater<\/strong>\u7684\u671f\u520a\u4e0a\u3002DOI:<\/strong> 10.1002\/aenm.202003580<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/aenm.202003580.<\/strong><\/p>\n

Angew\uff1a\u57fa\u4e8eGrotthuss\u8d28\u5b50\u534f\u540c\u4f20\u8f93\u63d0\u9ad8\u6c34\u7cfb\u7535\u6c60\u7684\u80fd\u91cf\u5bc6\u5ea6<\/p>\n

\"\"<\/p>\n

\u968f\u7740\u53ef\u5145\u7535\u6c34\u7cfb\u7535\u6c60\u7684\u53d1\u5c55\uff0c\u8d28\u5b50\u5728\u6b63\u6781\u6750\u6599\u4e2d\u7684\u4f20\u8f93\u673a\u7406\u5f15\u8d77\u4e86\u4eba\u4eec\u7684\u5e7f\u6cdb\u5173\u6ce8\u3002\u5728\u6b64\uff0c\u8be5\u5de5\u4f5c\u9996\u6b21\u62a5\u9053\u4e86\u03b1-MnO2<\/sub>\u4e2d\u5177\u6709\u5bbd[2 \u00d7 2]\u96a7\u9053\u7684Grotthuss\u8d28\u5b50\u534f\u540c\u4f20\u8f93\u673a\u5236\u3002\u4ee5\u03b1-MnO2<\/sub>\u4e2dNi (\u7ea65 at.%)\u53d6\u4ee3\u63ba\u6742\u4f7f\u7535\u6781\u7684\u80fd\u91cf\u5bc6\u5ea6\u63d0\u9ad825%\u4e3a\u4f8b\uff0c\u63ed\u793a\u4e86\u6676\u683c\u56db\u65b9\u6b63\u4ea4(TO)\u7578\u53d8\u4e0e\u8d28\u5b50\u5728\u96a7\u9053\u4e2d\u7684\u6269\u6563\u52a8\u529b\u5b66\u4e4b\u95f4\u7684\u5bc6\u5207\u8054\u7cfb\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u7ed3\u679c\u8868\u660e\uff0cNi\u63ba\u6742\u52a0\u5267\u4e86\u653e\u7535\u8fc7\u7a0b\u4e2dTO\u7684\u626d\u66f2\uff0c\u4ece\u800c\u4fc3\u8fdb\u4e86\u03b1-MnO2<\/sub>\u4f53\u4e2d\u6c22\u952e\u7684\u5f62\u6210\u3002\u8d28\u5b50\u4f20\u8f93\u7684\u5b64\u7acb\u76f4\u63a5\u8df3\u8dc3\u6a21\u5f0f\u8f6c\u53d8\u4e3a\u4e00\u79cd\u7b80\u5355\u7684\u534f\u540c\u6a21\u5f0f\uff0c\u5373\u901a\u8fc7Grotthuss\u8d28\u5b50\u534f\u540c\u4f20\u8f93\u673a\u5236\uff0c\u5728\u8d28\u5b50\u9635\u5217\u4e2d\u5f62\u6210O-H\u952e\u5e76\u4f34\u968f\u88c2\u89e3\u3002\u8be5\u5de5\u4f5c\u4e3a\u7406\u89e3MnO2<\/sub>\u4e2d\u7684\u8d28\u5b50\u4f20\u8f93\u63d0\u4f9b\u4e86\u91cd\u8981\u7684\u89c1\u89e3\uff0c\u5e76\u53ef\u4f5c\u4e3a\u53ef\u5145\u7535\u6c34\u7cfb\u7535\u6c60\u9634\u6781\u6750\u6599\u7ec4\u6210\u8bbe\u8ba1\u7684\u6a21\u578b\u3002\u8be5\u7814\u7a76\u6210\u679c\u4ee5\u201cBoosting the Energy Density of Aqueous Batteries via Facile Grotthuss Proton Transport<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u8457\u540d\u671f\u520aAngew. Chem. Int. Ed.<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1002\/anie.202011588.<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/anie.202011588.<\/strong><\/p>\n

Adv. Funct. Mater\uff1a\u5148\u8fdb\u7535\u6c60\u7535\u5b50\u80fd\u91cf\u635f\u5931\u8c31\u7814\u7a76<\/p>\n

\"\"<\/p>\n

\u7535\u5b50\u80fd\u91cf\u635f\u5931\u8c31(EELS)\u662f\u5316\u5b66\u6210\u5206\u5206\u6790\u7684\u6709\u529b\u5de5\u5177\uff0c\u53ef\u4ee5\u63ed\u793a\u5404\u79cd\u6750\u6599\u539f\u5b50\u7ea7\u7535\u5b50\u6001\u7684\u4e30\u5bcc\u4fe1\u606f\uff0c\u5305\u62ec\u5143\u7d20\u7c7b\u578b\u53ca\u5176\u4ef7\u6001\u548c\u6d53\u5ea6\u5206\u5e03\uff0c\u4ee5\u53ca\u4e0e\u7ed3\u6784\u76f8\u5173\u7684\u539f\u5b50\u5f84\u5411\u5206\u5e03\u3002\u5f97\u76ca\u4e8e\u5176\u72ec\u7279\u7684\u6027\u80fd\u548c\u6700\u65b0\u5f00\u53d1\u7684\u5148\u8fdb\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c(TEM)\u914d\u7f6e(\u5373\u539f\u4f4d\u504f\u7f6e\u3001\u539f\u4f4d\u52a0\u70ed\u3001\u4f4e\u6e29TEM\u7b49)\uff0cEELS\u4fc3\u8fdb\u4e86\u7535\u6c60\u5728\u5404\u4e2a\u65b9\u9762\u7684\u7814\u7a76\u3002\u672c\u6587\u7b80\u8981\u7efc\u8ff0\u4e86EELS\u5de5\u4f5c\u539f\u7406\u4ee5\u53ca\u5728\u7535\u6c60\u6750\u6599\u7814\u7a76\u4e2d\u7684\u6700\u65b0\u8fdb\u5c55\uff0c\u5e76\u5bf9\u7535\u6c60\u8868\u5f81\u6280\u672f\u7684\u53d1\u5c55\u53ca\u5176\u5728\u7535\u6c60\u7814\u7a76\u4e2d\u7684\u5e94\u7528\u8fdb\u884c\u4e86\u5c55\u671b\u3002\u8be5\u7efc\u8ff0\u4ee5\u201cAdvanced Electron Energy Loss Spectroscopy for Battery Studies<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u6750\u6599\u9886\u57df\u8457\u540d\u671f\u520aAdv. Funct. Mater<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1002\/adfm.202107190.<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/epdf\/10.1002\/adfm.202107190.<\/strong><\/p>\n

Chem. Soc. Rev\uff08\u8bfe\u7a0b\u7c7b\u8bc4\u8ff0\uff09\uff1a\u4ece\u672c\u4f53\u5230\u754c\u9762: \u5229\u7528\u7535\u5316\u5b66\u77f3\u82f1\u6676\u4f53\u5fae\u5929\u5e73\u7814\u7a76\u7535\u6c60\u7684\u7535\u5316\u5b66\u73b0\u8c61\u53ca\u673a\u7406<\/p>\n

\"\"<\/p>\n

\u4e86\u89e3\u7535\u6c60\uff08\u5982\u9502\u79bb\u5b50\u7535\u6c60\u3001\u94a0\u79bb\u5b50\u7535\u6c60\u3001\u9502\u6c27\u7535\u6c60\u7b49\uff09\u5728\u8fd0\u884c\u8fc7\u7a0b\u4e2d\u7684\u672c\u4f53\u548c\u754c\u9762\u884c\u4e3a\uff0c\u5bf9\u4e8e\u6301\u7eed\u6539\u8fdb\u7535\u6c60\u6027\u80fd\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u7535\u5316\u5b66\u77f3\u82f1\u6676\u4f53\u5fae\u5929\u5e73\uff08EQCM\uff09\u662f\u5b9e\u73b0\u8fd9\u4e00\u76ee\u6807\u7684\u6709\u529b\u5de5\u5177\uff0c\u56e0\u4e3a\u5b83\u53ef\u4ee5\u539f\u4f4d\u7814\u7a76\u5404\u79cd\u73b0\u8c61\uff0c\u5305\u62ec\u7535\u6781\u5185\u7684\u79bb\u5b50\u5d4c\u5165\/\u8131\u51fa\u3001\u7535\u89e3\u8d28\u4e2d\u7684\u56fa\u4f53\u6210\u6838\u3001\u76f8\u95f4\u5f62\u6210\/\u6f14\u5316\u548c\u56fa\u6db2\u754c\u9762\u914d\u4f4d\u3002\u56e0\u6b64\uff0cEQCM\u5206\u6790\u6709\u52a9\u4e8e\u7834\u8bd1\u6574\u4f53\u548c\u754c\u9762\u7684\u6f5c\u5728\u673a\u5236\u3002\u672c\u6587\u5c06\u4ecb\u7ecd\u901a\u8fc7EQCM\u6280\u672f\u5b9e\u73b0\u7684\u7535\u6c60\u529b\u5b66\u7814\u7a76\u7684\u6700\u65b0\u7814\u7a76\u8fdb\u5c55\u3002\u9996\u5148\u8ba8\u8bba\u4e86EQCM\u7684\u57fa\u672c\u539f\u7406\u548c\u72ec\u7279\u6027\u80fd\uff0c\u5e76\u4e0e\u5176\u4ed6\u6280\u672f\u8fdb\u884c\u4e86\u6bd4\u8f83\uff0c\u7136\u540e\u4ecb\u7ecd\u4e86EQCM\u4e0e\u5176\u4ed6\u539f\u4f4d\u6280\u672f\u7684\u7ed3\u5408\u3002\u6b64\u5916\uff0c\u8be5\u6587\u7ae0\u8fd8\u7efc\u8ff0\u4e86\u8fd1\u5e74\u6765\u5229\u7528EQCM\u6280\u672f\u63ed\u793a\u5404\u79cd\u7535\u6c60\u73b0\u8c61\u548c\u673a\u7406\u7684\u7814\u7a76\u3002\u6700\u540e\u5c55\u671b\u4e86EQCM\u5728\u7535\u6c60\u7814\u7a76\u4e2d\u7684\u5e94\u7528\u524d\u666f\u3002\u8be5\u9879\u7814\u7a76\u6210\u679c\u4ee5\u201cFrom bulk to interface: electrochemical phenomena and mechanism studies in batteries via electrochemical quartz crystal microbalance<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Chem Soc Rev<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1039\/d1cs00629k<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/pubs.rsc.org\/en\/content\/articlelanding\/2021\/CS\/D1CS00629K.<\/strong><\/p>\n

Adv. Energy Mater\uff1aCo\u548cNi\u5728\u5bcc\u9530\u5c42\u72b6\u6b63\u6781\u4e2d\u7684\u4f5c\u7528<\/p>\n

\"\"<\/p>\n

\u6700\u8fd1\uff0c\u4eba\u4eec\u8feb\u5207\u9700\u8981\u51cf\u5c11\u5bf9\u6602\u8d35\u7684\u94b4\u548c\u954d\u5143\u7d20\u7684\u4f9d\u8d56\uff0c\u8fd9\u4f7f\u5f97\u5bcc\u9502\u9530\u7684\u5c42\u72b6\u6c27\u5316\u7269\u4f5c\u4e3a\u53ef\u5145\u7535\u9502\u79bb\u5b50\u7535\u6c60\u7684\u6f5c\u5728\u6b63\u6781\u6750\u6599\u3002\u5c3d\u7ba1\u79d1\u7814\u5de5\u4f5c\u8005\u5bf9\u9ad8\u954d\u6b63\u6781\u6750\u6599\u4e2d\u7684\u94b4\u548c\u954d\u673a\u7406\u8fdb\u884c\u4e86\u8be6\u7ec6\u7684\u7814\u7a76\uff0c\u4f46\u5bf9\u4e8e\u94b4\u548c\u954d\u53d6\u4ee3\u5bf9\u5bcc\u9530\u5c42\u72b6\u9634\u6781\u7684\u7ed3\u6784\u548c\u7535\u5316\u5b66\u6027\u80fd\u7684\u5f71\u54cd\u4ecd\u7136\u7f3a\u4e4f\u57fa\u672c\u7684\u4e86\u89e3\u3002\u5728\u8fd9\u91cc\uff0c\u8be5\u5de5\u4f5c\u8bbe\u8ba1\u4e86\u94b4\u53d6\u4ee3\u3001\u94b4\u548c\u954d\u5171\u53d6\u4ee3\u4ee5\u53ca\u954d\u53d6\u4ee3\u7684\u5bcc\u9502\u9530\u5c42\u72b6Li2<\/sub>MnO3<\/sub>.Li\uff08Mn,Ni,Co\uff09O2<\/sub>\uff0c\u4ee5\u63a2\u7d22\u94b4\u548c\u954d\u7684\u4f5c\u7528\u3002\u8fd9\u4e9b\u7ed3\u679c\u8868\u660e\uff0c\u7531\u4e8e\u6676\u683c\u6c27\u7684\u4e0d\u7a33\u5b9a\u6027\u589e\u52a0\uff0c\u5c24\u5176\u662f\u5728\u9ad8\u7535\u4f4d\u4e0b\uff0cCo4+<\/sup>\u5bf9\u5bcc\u9502\u9530\u6b63\u6781\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\u5177\u6709\u7834\u574f\u6027\uff0c\u4ece\u800c\u5bfc\u81f4\u5faa\u73af\u7a33\u5b9a\u6027\u5dee\uff0cNi\u53d6\u4ee3Co\u5f15\u5165\u4e86Li\/Ni\u6df7\u5408\u63d0\u9ad8\u4e86\u6676\u683c\u6c27\u7a33\u5b9a\u6027\uff0c\u6291\u5236\u4e86\u76f8\u504f\u6790\u548c\u4e0d\u53ef\u9006\u76f8\u53d8\uff0c\u4ece\u800c\u5927\u5927\u63d0\u9ad8\u4e86\u5faa\u73af\u7a33\u5b9a\u6027\u3002\u8fd9\u4e9b\u53d1\u73b0\u8865\u5145\u4e86\u94b4\u3001\u954d\u548c\u9530\u57fa\u5c42\u72b6\u6c27\u5316\u7269\u9634\u6781\u7684\u5143\u7d20\u5316\u5b66\uff0c\u5e76\u6709\u52a9\u4e8e\u5f00\u53d1\u7528\u4e8e\u672a\u6765\u53ef\u5145\u7535\u9502\u79bb\u5b50\u7535\u6c60\u7684\u65e0\u94b4\u5bcc\u9530\u5c42\u72b6\u9634\u6781\u6750\u6599\u3002\u8be5\u9879\u7814\u7a76\u6210\u679c\u4ee5\u201cRevealing Roles of Co and Ni in Mn-Rich Layered Cathodes<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Adv. Energy Mater<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1002\/aenm.202102646<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/aenm.202102646.<\/strong><\/p>\n

Adv. Funct. Mater\uff1aPIM-1\u4f5c\u4e3a\u4e00\u4e2a\u591a\u529f\u80fd\u6846\u67b6\u5b9e\u73b0\u9ad8\u6027\u80fd\u56fa\u6001\u9502\u786b\u7535\u6c60<\/p>\n

\"\"<\/p>\n

\u805a(\u73af\u6c27\u4e59\u70ef)(PEO)\u662f\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u56fa\u6001\u9502\u786b\u7535\u6c60\u7684\u7535\u89e3\u8d28\u6750\u6599\uff0c\u4f46\u5176\u672c\u5f81\u79bb\u5b50\u7535\u5bfc\u7387\u4f4e\u3001\u529b\u5b66\u6027\u80fd\u5dee\u3001\u65e0\u6cd5\u963b\u788d\u591a\u786b\u5316\u7269\u7a7f\u68ad\u6548\u5e94\u7b49\u9650\u5236\u4e86\u5176\u5e94\u7528\u3002\u672c\u6587\u5408\u6210\u4e86\u4e00\u79cd\u56fa\u6709\u5fae\u5b54\u805a\u5408\u7269(PIM)\uff0c\u5e76\u5c06\u5176\u4f5c\u4e3a\u6709\u673a\u9aa8\u67b6\uff0c\u901a\u8fc7\u5f62\u6210\u590d\u5408\u7535\u89e3\u8d28(PEO-PIM)\u6765\u5168\u9762\u63d0\u9ad8PEO\u7684\u6027\u80fd\u3002PIM-1\u7684\u72ec\u7279\u7ed3\u6784\u4e0d\u4ec5\u63d0\u9ad8\u4e86PEO\u7535\u89e3\u8d28\u7684\u673a\u68b0\u5f3a\u5ea6\u548c\u786c\u5ea6\uff0c\u589e\u52a0\u4e86\u5bf9\u91d1\u5c5e\u9502\u8d1f\u6781\u7684\u7a33\u5b9a\u6027\uff0c\u8fd8\u901a\u8fc7\u964d\u4f4e\u7ed3\u6676\u5ea6\u589e\u52a0\u4e86\u5176\u79bb\u5b50\u7535\u5bfc\u7387\u3002\u6b64\u5916\uff0c\u7814\u7a76\u8868\u660e\uff0cPIM-1\u53ef\u4ee5\u6709\u6548\u5730\u6355\u83b7\u591a\u786b\u5316\u7269\uff0c\u4ee5\u51cf\u7f13\u6709\u5bb3\u7684\u591a\u786b\u5316\u7269\u7684\u7a7f\u68ad\u6548\u5e94\uff0c\u8fd9\u662f\u7531\u4e8e\u4eb2\u7535\u76841,4-\u4e8c\u6c30\u57fa\u5b98\u80fd\u56e2\u4e0e\u591a\u786b\u5316\u7269\u5177\u6709\u66f4\u9ad8\u7684\u7ed3\u5408\u80fd\u3002\u5f97\u76ca\u4e8e\u8fd9\u4e9b\u7279\u6027\uff0cPEO-PIM\u590d\u5408\u7535\u89e3\u8d28\u7684\u4f7f\u7528\u5927\u5927\u63d0\u9ad8\u4e86\u56fa\u6001\u9502\u786b\u7535\u6c60\u7684\u500d\u7387\u6027\u80fd\u3001\u957f\u5468\u671f\u7a33\u5b9a\u6027\u548c\u4f18\u826f\u7684\u5b89\u5168\u6027\u80fd\u3002\u8be5\u65b9\u6cd5\u4e3a\u56fa\u6001\u805a\u5408\u7269\u7535\u89e3\u8d28\u7684\u4f18\u5316\u63d0\u4f9b\u4e86\u4e00\u4e2a\u65b0\u7684\u65b9\u5411\u3002\u8be5\u9879\u7814\u7a76\u6210\u679c\u4ee5\u201cPIM-1 as a Multifunctional Framework to Enable High-Performance Solid-State Lithium\u2013Sulfur Batteries<\/strong>\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728Adv. Funct. Mater<\/strong>\u4e0a\u3002DOI:<\/strong> 10.1002\/adfm.202104830<\/strong>\u3002<\/strong><\/p>\n

\u539f\u6587\u94fe\u63a5\uff1a<\/strong>https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/adfm.202104830.<\/strong><\/p>\n

Nano Energy\uff1a\u8c03\u8282Zn2+<\/sup>\u914d\u4f4d\u73af\u5883\u6291\u5236\u9ad8\u6027\u80fd\u950c\u79bb\u5b50\u7535\u6c60\u679d\u6676\u5f62\u6210<\/p>\n

\"\"<\/p>\n

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\u539f\u6587\u94fe\u63a5\uff1a<\/strong><\/p>\n

https:\/\/www.sciencedirect.com\/science\/article\/abs\/pii\/S2211285520310533?via%3Dihub.<\/strong><\/p>\n

\u672c\u6587\u7531\u79d1\u7814\u767e\u6653\u751f\u4f9b\u7a3f\uff0c\u7ecf\u8fc7\u6f58\u950b\u6559\u6388\u56e2\u961f\u6821\u6b63\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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