{"id":233139,"date":"2022-02-15T06:30:35","date_gmt":"2022-02-14T22:30:35","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=233139"},"modified":"2022-02-14T19:30:45","modified_gmt":"2022-02-14T11:30:45","slug":"%e6%b2%b3%e5%8c%97%e5%a4%a7%e5%ad%a6nat-commun-%e5%bc%82%e8%b4%a8%e5%85%89%e7%83%ad%e6%9d%90%e6%96%99%e5%ae%9e%e7%8e%b0%e5%a4%a7%e8%a7%84%e6%a8%a1%e5%ae%a4%e5%a4%96%e5%85%89%e7%83%ad%e5%88%b6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=233139","title":{"rendered":"\u6cb3\u5317\u5927\u5b66Nat. Commun.: \u5f02\u8d28\u5149\u70ed\u6750\u6599\u5b9e\u73b0\u5927\u89c4\u6a21\u5ba4\u5916\u5149\u70ed\u5236\u6c22"},"content":{"rendered":"

\u3010\u5f15\u8a00<\/strong>\u3011<\/p>\n

\u5149\u70ed\u50ac\u5316\uff0c\u80fd\u591f\u5c06\u592a\u9633\u5149\u8f6c\u6362\u4e3a\u70ed\u80fd\u9a71\u52a8\u50ac\u5316\u53cd\u5e94\uff0c\u6210\u4e3a\u7814\u7a76\u70ed\u70b9\u3002\u5149\u70ed\u6750\u6599\u662f\u5149\u70ed\u50ac\u5316\u7684\u5173\u952e\uff0c\u4f46\u9762\u4e34\u5ba4\u5916\u592a\u9633\u5149\u8f90\u7167\u6e29\u5ea6\u8f83\u4f4e\u7684\u6311\u6218\u3002\u9ad8\u6548\u5438\u5149\u4e0e\u4f4e\u70ed\u5bfc\u8026\u5408\u662f\u73b0\u6709\u62a5\u9053\u4e2d\u63d0\u9ad8\u5149\u70ed\u6750\u6599\u8f90\u7167\u6e29\u5ea6\u7684\u4e3b\u8981\u7b56\u7565\uff0c\u5982ZIFs\u4e0e\u77f3\u58a8\u70ef\u8026\u5408\u6750\u6599\uff08\u5177\u670998%\u9ad8\u5149\u70ed\u8f6c\u5316\u6548\u7387\uff0c0.2 W mK-1<\/sup>\u7684\u4f4e\u70ed\u5bfc\uff09\u5728\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u6e29\u5ea6\u4e3a120 \u2103\uff0c\u4f46\u8fd9\u4e00\u6e29\u5ea6\u4ecd\u7136\u96be\u4ee5\u9a71\u52a8\u5927\u591a\u6570\u50ac\u5316\u53cd\u5e94\u3002\u4e9f\u9700\u65b0\u7b56\u7565\u6765\u63d0\u9ad8\u5149\u70ed\u6750\u6599\u7684\u8f90\u7167\u6e29\u5ea6\u3002<\/p>\n

\u53e6\u4e00\u65b9\u9762\uff0c\u6c22\u6c14\u662f\u672a\u6765\u793e\u4f1a\u7684\u57fa\u7840\u80fd\u6e90\u4e4b\u4e00\uff0c\u4ee5\u7532\u9187\u4e3a\u6c22\u6c14\u8f7d\u4f53\u80fd\u89e3\u51b3\u6c22\u6c14\u5b58\u50a8\u5bc6\u5ea6\u4f4e\u3001\u9ad8\u538b\u3001\u6cc4\u9732\u7b49\u95ee\u9898\u3002\u7532\u9187\u91cd\u6574\u5236\u6c22\u53cd\u5e94\u9700\u8981\u6d88\u8017\u5927\u91cf\u80fd\u6e90\uff0c\u5236\u7ea6\u4e86\u7532\u9187-\u6c22\u6c14\u80fd\u6e90\u7cfb\u7edf\u7684\u53d1\u5c55\u3002\u5229\u7528\u592a\u9633\u5149\u9a71\u52a8\u7532\u9187\u91cd\u6574\u53cd\u5e94\u6709\u6f5c\u529b\u89e3\u51b3\u5176\u80fd\u6e90\u6d88\u8017\u95ee\u9898\u3002\u4f46\u662f\uff0c\u76ee\u524d\u62a5\u9053\u7684\u5149\u9a71\u52a8\u7532\u9187\u91cd\u6574\u4ea7\u6c22\u7cfb\u7edf\u7684\u6700\u9ad8\u6548\u7387\u7ea6\u4e3a46 mmol g-1<\/sup> h-1<\/sup>\uff0c\u8fdc\u4e0d\u80fd\u6ee1\u8db3\u5de5\u4e1a\u9700\u6c42\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u8fd1\u65e5\uff0c\u6cb3\u5317\u5927\u5b66\u674e\u4e9a\u5149\u7814\u7a76\u5458\u3001\u738b\u6dd1\u82b3\u6559\u6388\u4e0e\u5929\u6d25\u5927\u5b66\u7f57\u4fca\u6559\u6388\u5408\u4f5c<\/strong>\u901a\u8fc7\u5f02\u8d28\u7ed3\u6784\u7b56\u7565\u63d0\u9ad8\u5149\u70ed\u6750\u6599\u5728\u5149\u8f90\u7167\u4e0b\u7684\u6e29\u5ea6\u4f4e\u7684\u95ee\u9898\u5e76\u4e14\u5229\u7528\u5149\u70ed\u6750\u6599\u548c\u9ad8\u6548\u50ac\u5316\u5242\u7ed3\u5408\u5b9e\u73b020 m3<\/sup> \u91cf\u7ea7\u5ba4\u5916\u5149\u70ed\u4ea7\u6c22\u3002\u672c\u5de5\u4f5c\u4e3b\u8981\u5206\u4e3a\u4ee5\u4e0b\u4e09\u90e8\u5206\uff1a<\/p>\n

1.\u672c\u5de5\u4f5c\u5229\u7528\u7a84\u5e26\u9699\u5149\u70ed\u6750\u6599\u548c\u7ea2\u5916\u53cd\u5c04\u6750\u6599\u6784\u7b51\u5f02\u8d28\u7ed3\u6784\u7684\u7b56\u7565\u5b9e\u73b0\u4e86\u9ad8\u6548\u592a\u9633\u5149\u5438\u6536\u548c\u4f4e\u7ea2\u5916\u8f90\u5c04\u7684\u534f\u540c\uff0c\u663e\u8457\u63d0\u5347\u4e86\u5149\u70ed\u6750\u6599\u7684\u8f90\u7167\u6e29\u5ea6\u3002\u5e76\u4e14\u8be5\u5f02\u8d28\u7ed3\u6784\u7b56\u7565\u666e\u9002\u4e8e\u591a\u79cd\u5149\u70ed\u6750\u6599\uff0c\u80fd\u591f\u5c06Ti2<\/sub>O3<\/sub>\u3001Cu2<\/sub>Se\u548cCu2<\/sub>S\u7684\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u6e29\u5ea6\u63d0\u9ad8\u5230295 \u2103\u3001271 \u2103\u548c248 \u2103\u3002<\/p>\n

2.\u5f00\u53d1\u4e86PVP\u8f85\u52a9\u5171\u6c89\u6dc0\u6cd5\u53bb\u5b8f\u91cf\u5236\u5907CuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\uff0c\u8be5\u50ac\u5316\u5242\u5728260 \u2103\u7684\u7532\u9187\u91cd\u6574\u5236\u6c22\u901f\u7387\u8fbe\u52301.02 mmol g-1<\/sup> h-1<\/sup>,\u5e76\u5177\u6709\u5f88\u597d\u7684\u7a33\u5b9a\u6027\u3002<\/p>\n

3.\u4ee5Bi2<\/sub>Te3<\/sub>\/Cu\u4e3a\u57fa\u7840\u7684\u65b0\u578b\u5149\u70ed\u7cfb\u7edf\u5728\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u80fd\u591f\u5c06CuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\u52a0\u70ed\u81f3305 \u2103\uff0c\u7532\u9187\u91cd\u6574\u5236\u6c22\u901f\u7387\u8fbe\u5230310 mmol g-1<\/sup> h-1<\/sup>\uff0c\u592a\u9633\u80fd\u5230\u6c22\u80fd\u8f6c\u5316\u6548\u7387\u8fbe\u523030.1 %\uff0c\u89c4\u6a21\u5316\u5236\u6c22\u91cf\u9ad8\u8fbe23.27 m3<\/sup>\/\u5929\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb<\/strong>\u3011<\/p>\n

\u56fe<\/strong>1. <\/strong>\u6784\u7b51\u5f02\u8d28\u7ed3\u6784\u63d0\u9ad8<\/strong>Bi2<\/sub>Te3<\/sub><\/strong>\u8f90\u7167\u6e29\u5ea6<\/strong><\/p>\n

\"\"<\/p>\n

(a) Bi2<\/sub>Te3<\/sub>\u7684\u70ed\u8017\u6563\u793a\u610f\u56fe\uff0c\uff08b\uff09 Bi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784\u7684\u5236\u5907\u793a\u610f\u56fe\uff0c\uff08c-e\uff09 3 um, 100 nm, 15 nm Bi2<\/sub>Te3<\/sub>\u7684Bi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784SEM\u548cTEM\u56fe\uff0c\uff08f-h\uff09 3 um, 100 nm, 15 nm Bi2<\/sub>Te3<\/sub>\u7684Bi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784\u7ea2\u5916\u6210\u50cf\u56fe\uff08\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\uff09\u3002<\/p>\n

\u56fe<\/strong>2. <\/strong>\u539a\u5ea6\u5f71\u54cd\u548c\u5f02\u8d28\u7ed3\u6784\u666e\u9002\u6027<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-c\uff09 3 um, 100 nm, 15 nm Bi2<\/sub>Te3<\/sub>\u7684Bi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784\u5149\u5438\u6536\u8c31\uff0c\uff08d-f\uff09 3 um, 100 nm, 15 nm Bi2<\/sub>Te3<\/sub>\u7684Bi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784\u7ea2\u5916\u8f90\u5c04\u56fe\uff08\u5e95\u6e29\u4e3a93 \u2103\uff09\uff0c\uff08g-i\uff09 \u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u7684Ti2<\/sub>O3<\/sub>\/Cu, Cu2<\/sub>Se\/Cu, Cu2<\/sub>S\/Cu\u5f02\u8d28\u7ed3\u6784\u7ea2\u5916\u8f90\u5c04\u56fe\u3002<\/p>\n

\u56fe<\/strong>3. Bi2<\/sub>Te3<\/sub>\/Cu<\/strong>\u5149\u70ed\u7cfb\u7edf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09 Bi2<\/sub>Te3<\/sub>\/Cu\u57fa\u5149\u70ed\u7cfb\u7edf\u7684\u5149\u70ed\u7532\u9187\u91cd\u6574\u5236\u6c22\u793a\u610f\u56fe\uff0c\uff08b\uff09 Bi2<\/sub>Te3<\/sub>\/Cu\u57fa\u5149\u70ed\u7cfb\u7edf\u5b9e\u7269\u56fe\uff0c\uff08c\uff09 \u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u7684Bi2<\/sub>Te3<\/sub>\/Cu\u57fa\u5149\u70ed\u7cfb\u7edf\u7ea2\u5916\u622a\u9762\u56fe\uff0c\uff08d\uff09 \u4e0d\u540c\u5149\u7167\u4e0bBi2<\/sub>Te3<\/sub>\/Cu\u57fa\u5149\u70ed\u7cfb\u7edf\u4e2d\u50ac\u5316\u5242\u6e29\u5ea6\u3002<\/p>\n

\u56fe<\/strong>4. CuZnAl<\/strong>\u4e8c\u7ef4\u50ac\u5316\u5242\u7684\u5236\u5907\u548c\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

(a) CuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\u7684\u5236\u5907\u793a\u610f\u56fe\uff0cCuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\u7684\uff08b\uff09 TEM\u56fe\uff0c\uff08c\uff09 \u5143\u7d20\u5206\u5e03\u56fe\uff0c\uff08d\uff09 HRTEM\u56fe\uff0c\uff08e\uff09 AFM\u56fe\uff0c\uff08f\uff09N2<\/sub>\u5438\u9644-\u8131\u9644\u66f2\u7ebf\uff0c(g) CuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\u548c\u5de5\u4e1aCuZnAl\u50ac\u5316\u5242\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684\u7532\u9187\u91cd\u6574\u5236\u6c22\u6027\u80fd\u56fe\u3002<\/p>\n

\u56fe<\/strong>5. Bi2<\/sub>Te3<\/sub>\/Cu<\/strong>\u57fa<\/strong>\u5149\u70ed\u7cfb\u7edf\u4e2d<\/strong>CuZnAl<\/strong>\u4e8c\u7ef4\u50ac\u5316\u5242\u7684\u5149\u70ed\u7532\u9187\u91cd\u6574\u5236\u6c22\u6027\u80fd<\/strong><\/p>\n

\"\"<\/p>\n

(a) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u7684\u7532\u9187\u91cd\u6574\u5236\u6c22\u6027\u80fd\u56fe\uff0c(b) \u4e0e\u5176\u5b83\u6587\u732e\u7684\u6027\u80fd\u5bf9\u6bd4\u56fe\uff0c(c) \u4e0d\u540c\u5149\u7167\u6761\u4ef6\u4e0b\u7684\u592a\u9633\u80fd\u5230\u6c22\u80fd\u8f6c\u5316\u6548\u7387\u56fe\uff0c(d) \u5ba4\u5916\u5149\u70ed\u7532\u9187\u91cd\u6574\u5236\u6c22\u7cfb\u7edf\u5b9e\u7269\u56fe\uff0c(e) \u6d4b\u8bd5\u671f\u95f4\u7684\u592a\u9633\u5149\u5bc6\u5ea6\uff0c(f) \u81ea\u7136\u5149\u7167\u6761\u4ef6\u4e0b\u4ea7\u6c22\u901f\u7387\u968f\u65f6\u95f4\u53d8\u5316\u56fe\u3002<\/p>\n

\u3010\u5c0f\u7ed3<\/strong>\u3011<\/p>\n

\u9488\u5bf9\u4f20\u7edf\u5149\u70ed\u6750\u6599\u81ea\u7136\u592a\u9633\u5149\u8f90\u7167\u6e29\u5ea6\u8f83\u4f4e\u7684\u74f6\u9888\uff0c\u63d0\u51fa\u8026\u5408\u7a84\u5e26\u9699\u5149\u70ed\u6750\u6599\u548c\u7ea2\u5916\u53cd\u5c04\u6750\u6599\u6784\u7b51\u5f02\u8d28\u7ed3\u6784\u3002\u5f53Bi2<\/sub>Te3<\/sub>\u539a\u5ea6\u4e3a100 nm\u65f6\uff0cBi2<\/sub>Te3<\/sub>\/Cu\u5f02\u8d28\u7ed3\u6784\u5728\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u53ef\u4ee5\u5c06Bi2<\/sub>Te3<\/sub>\u52a0\u70ed\u81f3317 \u2103\u3002\u5c06CuZnAl\u4e8c\u7ef4\u50ac\u5316\u5242\u548cBi2<\/sub>Te3<\/sub>\/Cu\u57fa\u5149\u70ed\u7cfb\u7edf\u8026\u5408\uff0c\u6807\u51c6\u592a\u9633\u5149\u8f90\u7167\u4e0b\u7684\u50ac\u5316\u5242\u6e29\u5ea6\u8fbe\u5230305 \u2103\uff0c\u7532\u9187\u91cd\u6574\u5236\u6c22\u901f\u7387\u8fbe\u5230310 mmol g-1 <\/sup>h-1<\/sup>\uff0c\u592a\u9633\u80fd\u5230\u6c22\u80fd\u8f6c\u5316\u6548\u7387\u8fbe\u523030.1 %\uff0c\u89c4\u6a21\u5316\u5236\u6c22\u91cf\u9ad8\u8fbe23.27 m3<\/sup>\/\u5929\uff0c\u5b9e\u73b0\u4e86\u65e0\u4eba\u5de5\u80fd\u6e90\u6d88\u8017\u4e0b\u7684\u9ad8\u6548\u5149\u9a71\u52a8\u5236\u6c22\u3002<\/p>\n

\u3010\u6587\u7ae0\u4fe1\u606f<\/strong>\u3011<\/p>\n

General heterostructure strategy of photothermal materials for scalable solar-heating hydrogen production without the consumption of artificial energy Nat. Commun.<\/em> 2022, 13:776. https:\/\/doi.org\/10.1038\/s41467-022-28364-y<\/p>\n

\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong>\u3011<\/p>\n

\u674e\u4e9a\u5149<\/strong>\uff0c\u6cb3\u5317\u5927\u5b66\u7814\u7a76\u5458\uff08\u6821\u8058\u6559\u6388\uff09\uff0c\u5764\u8206\u9752\u5e74\u5b66\u8005\u30022015\u5e74\u535a\u58eb\u6bd5\u4e1a\u4e8e\u6d59\u6c5f\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\uff0c\u5176\u540e\u8fdb\u5165\u6cb3\u5317\u5927\u5b66\u5de5\u4f5c\uff0c\u73b0\u4e3a\u5149\u9a71\u52a8\u50ac\u5316\u7814\u7a76\u7ec4\u8bfe\u9898\u7ec4\u957f\u3002\u8fd1\u5e74\u6765\u4e3b\u8981\u4ece\u4e8b\u5149\u9a71\u52a8\u50ac\u5316\u7684\u7814\u7a76\u3002\u4e3b\u6301\u6216\u53c2\u4e0e\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\u3001\u6cb3\u5317\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u4f18\u79c0\u9752\u5e74\u57fa\u91d1\u9879\u76ee\u3001\u6cb3\u5317\u7701\u6559\u80b2\u5385\u9752\u5e74\u62d4\u5c16\u9879\u76ee\u7b49\u591a\u9879\u79d1\u7814\u9879\u76ee\uff0c\u4ee5\u7b2c\u4e00\u6216\u901a\u8baf\u4f5c\u8005\u5728Nat. Commun.\u3001Nano Energy\u3001Adv. Science\u3001Appl. Catal. B.\u3001Green Chem.\u3001Small\u3001J. Mater. Chem. A.\u7b49\u5b66\u672f\u671f\u520a\u4e0a\u53d1\u8868\u8bba\u658750\u4f59\u7bc7\uff1b\u83b7\u6388\u6743\u56fd\u5bb6\u53d1\u660e\u4e13\u52297\u9879\u3002<\/p>\n

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