{"id":234924,"date":"2022-03-24T06:48:03","date_gmt":"2022-03-23T22:48:03","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=234924"},"modified":"2022-03-23T11:52:23","modified_gmt":"2022-03-23T03:52:23","slug":"nature-energy%ef%bc%9a%e6%80%a7%e8%83%bd%e4%b8%80%e6%b5%81%ef%bc%81%e6%9c%89%e6%9c%ba%e9%ab%98%e6%95%88%e5%85%89%e5%82%ac%e5%8c%96%e5%89%82%e8%ae%be%e8%ae%a1%ef%bc%81","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=234924","title":{"rendered":"Nature Energy\uff1a\u6027\u80fd\u4e00\u6d41\uff01\u6709\u673a\u9ad8\u6548\u5149\u50ac\u5316\u5242\u8bbe\u8ba1\uff01"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

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\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/b><\/strong><\/p>\n

\u5728\u6b64\uff0c\u963f\u535c\u675c\u62c9\u56fd\u738b\u79d1\u6280\u5927\u5b66\uff08KAUST\uff09<\/strong>Iain McCulloch\u6559\u6388<\/strong>\u548cJan Kosco\uff0c\u82f1\u56fd\u5e1d\u56fd\u7406\u5de5\u5b66\u9662James R. Durrant\u6559\u6388<\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba<\/strong>\u5c55\u793a\u4e86\u6709\u673a\u534a\u5bfc\u4f53\u5f02\u8d28\u7ed3\u7eb3\u7c73\u9897\u7c92<\/span><\/strong>\u672c\u8d28\u4e0a\u53ef\u4ee5\u4ea7\u751f\u957f\u5bff\u547d\u7684\u53cd\u5e94\u7535\u8377\uff0c\u4f7f\u5b83\u4eec\u80fd\u591f\u6709\u6548\u5730\u9a71\u52a8\u6c22\u7684\u6790\u51fa\u3002\u672c\u6587\u4f18\u5316\u7684\u5f02\u8d28\u7ed3\u5149\u50ac\u5316\u5242\u5305\u542b\u4e0eY6\u6216PCBM\u7535\u5b50\u53d7\u4f53\u5339\u914d\u7684\u5171\u8f6d\u805a\u5408\u7269 PM6\uff0c\u5728400\u81f3900 nm\u548c400\u81f3700 nm\u5904\u5206\u522b\u5b9e\u73b01.0%\u81f35.0%\u548c8.7%\u81f32.6% \u7684\u5916\u90e8\u91cf\u5b50\u6548\u7387\u3002\u540c\u65f6\uff0c\u4f7f\u7528\u77ac\u6001\u548c\u539f\u4f4d\u5149\u8c31\uff0c\u53d1\u73b0\u5373\u4f7f\u5728\u6ca1\u6709\u7535\u5b50\/\u7a7a\u7a74\u6e05\u9664\u5242\u6216Pt\u7684\u60c5\u51b5\u4e0b\uff0c\u8fd9\u4e9b\u7eb3\u7c73\u9897\u7c92\u4e2d\u7684\u5f02\u8d28\u7ed3\u7ed3\u6784\u4e5f\u6781\u5927\u5730\u589e\u5f3a\u957f\u5bff\u547d\u7535\u8377\u7684\u4ea7\u751f\uff08\u6beb\u79d2\u5230\u79d2\u65f6\u95f4\u5c3a\u5ea6\uff09\u3002\u8fd9\u79cd\u957f\u5bff\u547d\u7684\u6d3b\u6027\u7535\u8377\u5728\u6c34\u5206\u89e3Z-\u65b9\u6848\u548c\u52a8\u529b\u5b66\u7f13\u6162\u548c\u6280\u672f\u4e0a\u7406\u60f3\u7684\u6c27\u5316\u53cd\u5e94\u65b9\u9762\u5177\u6709\u5e94\u7528\u6f5c\u529b\u3002<\/p>\n

\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cGeneration of long-lived charges in organic semiconductor heterojunction nanoparticles for efficient photocatalytic hydrogen evolution<\/i><\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Energy<\/i><\/em><\/strong>\u4e0a\u3002\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/b><\/strong><\/p>\n

\u221a \u5f00\u53d1\u4e86\u4e24\u4e2a\u542b\u6709\u4f9b\u4f53\/\u53d7\u4f53\uff08D\/A\uff09\u5f02\u8d28\u7ed3\u7684\u6709\u673aNP\u00a0HEPs<\/span><\/strong>\u3002NPs\u662f\u7531\u4f9b\u4f53\u805a\u5408\u7269PBDB-T-2F\uff08PM6,1\uff09\u4e0e\u7a84\u5e26\u9699\u975e\u5bcc\u52d2\u70ef\u53d7\u4f53BTP-4F\uff08Y6,2\uff09\u6216\u5bcc\u52d2\u70ef[6,6]-\u82ef\u57faC71\u4e01\u9178\u7532\u916f\uff08PCBM\uff0c3\uff09\u5339\u914d\u7684\u6df7\u5408\u7269\u5f62\u6210\u7684\uff1b<\/p>\n

\u221a \u4e24\u79cdNP\u5149\u50ac\u5316\u5242\u90fd\u662f\u8fc4\u4eca\u4e3a\u6b62\u62a5\u9053\u7684\u6700\u6709\u6548\u7684\u6709\u673a\u9ad8\u6548\u5149\u50ac\u5316\u5242<\/span><\/strong>\u4e4b\u4e00\uff1b<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/b><\/strong><\/p>\n

\u56fe<\/b><\/strong>\u4e00<\/b><\/strong>\u3001\u5316\u5b66\u7ed3\u6784\u548c\u80fd\u7ea7<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/b><\/strong><\/p>\n

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\uff08b\uff09\u771f\u7a7a\u4e0b\u8584\u819cPM6\u3001Y6\u548cPCBM\u7684UPS\u548cIPES\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff09UPS\u3001IPES\u6d4b\u91cf\u7684PM6\u3001Y6\u3001PCBM\u80fd\u7ea7\u56fe\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e8c\u3001\u6df7\u5408\u4f18\u5316 \u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff09\u5728PM6\uff1aY6\u6bd4\u503c\u8303\u56f4\u5185\u5f62\u6210\u7684PM6\uff1aY6\u7eb3\u7c73\u9897\u7c92\u7684H2<\/sub>\u6f14\u5316\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b<\/p>\n

\uff08b\uff09\u5728PM6\uff1aPCBM\u6bd4\u503c\u8303\u56f4\u5f62\u6210\u7684PM6\uff1aPCBM\u7eb3\u7c73\u9897\u7c92\u7684H2<\/sub>\u6f14\u5316\u968f\u65f6\u95f4\u7684\u53d8\u5316\uff1b<\/p>\n

\uff08c\uff09PM6\uff1aY6\u548cPM6\uff1aPCBM\u7eb3\u7c73\u9897\u7c92\u572816\u5c0f\u65f6\u5185\u7684\u5e73\u5747H2<\/sub>\u8fdb\u5316\u901f\u7387\u4e0e\u4f9b\u4f53\uff08PM6\uff09\u4e0e\u53d7\u4f53\uff08Y6\u6216PCBM\uff09\u5171\u6df7\u6bd4\u7684\u51fd\u6570\uff1b<\/p>\n

\uff08d\uff09PM6\uff1aY6\u548cPM6\uff1aPCBM\u7eb3\u7c73\u9897\u7c92\u5728\u4f18\u5316\u5171\u6df7\u6bd4\u4e0b\u7684\u7d2b\u5916-\u53ef\u89c1\u5438\u5149\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>\u4e09<\/b><\/strong>\u3001\u5916\u90e8\u91cf\u5b50\u6548\u7387\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/p>\n

\uff08a\uff09\u5177\u670910%Pt\u7684PM6:Y6 7:3 NPs\u5728400\u3001500\u3001560\u3001620\u3001650\u3001750\u3001800\u3001850\u548c900\u00b110nm\u7684EQE\u548c\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08b\uff09\u5177\u67095%\u00a0Pt\u7684PM6\uff1aPCBM2\uff1a8\u00a0NPs\u5728400\u3001470\u3001560\u3001620\u548c700\u00b110nm\u7684EQE\u548c\u5438\u6536\u5149\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>\u56db<\/b><\/strong>\u3001\u7eb3\u7c73<\/b><\/strong>\u9897\u7c92<\/b><\/strong>\u7684\u660e\u573a<\/b><\/strong>cryo-TEM<\/b><\/strong>\u56fe\u50cf\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/p>\n

\uff08a\uff0cb\uff09PM6:Y6 7:3NPs\u5728\u5149\u6c89\u79ef10wt%Pt\u548c20h\u00a0H2<\/sub>\u6f14\u5316\u524d\u540e\u7684\u56fe\u50cf\uff1b<\/p>\n

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\u56fe<\/b><\/strong>\u4e94<\/b><\/strong>\u3001\u7a33\u6001PL\u5149\u8c31\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/b><\/strong><\/p>\n

\uff08a\uff0cb\uff09\u4e0d\u540cPM6\uff1aPCBM\u7ec4\u6210\u6bd4\u4e0bPM6\uff1aPCBM\u00a0NPs\u7684\u7a33\u6001PL\u5149\u8c31\uff1b<\/p>\n

\uff08c\uff0cd\uff09\u4e0d\u540c\u7684PM6\uff1aY6\u7ec4\u6210\u6bd4\u4e0bPM6\uff1aY6\u00a0NPs\u7684\u7a33\u6001PL\u5149\u8c31\u3002<\/p>\n

\u56fe<\/b><\/strong>\u516d<\/b><\/strong>\u3001\u7eafPM6\u3001PM6:Y6 7:3\u548cPM6:PCBM 2:8\u7eb3\u7c73\u9897\u7c92\u5728\u6c34\u6027\u60ac\u6d6e\u6db2\u4e2d\u7684\u8d85\u5febTAS\u8868\u5f81\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/p>\n

\uff08a\uff09PM6 NPs\u5728550 nm\u6fc0\u53d1\u540e\u4e0d\u540c\u65f6\u95f4\u5ef6\u8fdf\u7684\u77ac\u6001\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

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\uff08c\uff0cd\uff09PM6:PCBM\u00a02:8\u548cPM6:Y6 7:3\u00a0NPs\u5728\u4e0d\u540c\u5ef6\u8fdf\u6761\u4ef6\u4e0b\u7684\u77ac\u6001\u5438\u6536\u5149\u8c31\uff1b<\/p>\n

\uff08e\uff09\u7eb3\u7c73\u9897\u7c92\u4e2d\u6fc0\u5b50\u8870\u53d8\u548c\u7535\u5b50\/\u80fd\u91cf\u8f6c\u79fb\u8fc7\u7a0b\u7684\u793a\u610f\u56fe\u00a0<\/p>\n

\u56fe<\/b><\/strong>\u4e03<\/b><\/strong>\u3001\u6dfb\u52a0\u548c\u4e0d\u6dfb\u52a0Pt\u548cAA\u7684NPs\u7684\u77ac\u6001\u5438\u6536\u8870\u51cf\u52a8\u529b\u5b66\u548cPIAS\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/p>\n

\uff08a\uff0cb\uff09\u5728\u6ca1\u6709Pt\u548cAA\uff08\u9ed1\u8272\uff09\u3001Pt\uff08\u84dd\u8272\uff09\u548cPt\u548cAA\uff08\u7ea2\u8272\uff09\u5b58\u5728\u7684\u60c5\u51b5\u4e0b\uff0cPM6:PCBM\u00a02:8\u548cPM6:Y6 7:3\u00a0NPs\u5728\u6c34\u4e2d\u7684\u77ac\u6001\u5438\u6536\u8870\u51cf\u52a8\u529b\u5b66\uff1b<\/p>\n

\uff08c\uff09\u5728\u6ca1\u6709Pt\u548cAA\u7684\u60c5\u51b5\u4e0b\uff0c\u5728700 nm\u5904\u63a2\u6d4bPM6\u3001PM6:PCBM\u00a02:8\u548cPM6:Y6 7:3\u00a0NPs\u60ac\u6d6e\u6db2\u7684PIAS\u52a8\u529b\u5b66\uff1b<\/p>\n

\uff08d\uff09\u57284\u79d2\u65f6\u95f4\u5ef6\u8fdf\u4e0b\u6d4b\u91cf\u7684\u76f8\u540cNPs\u60ac\u6d6e\u6db2\u7684PIAS\u5149\u8c31\u5bf9\u6bd4\uff1b<\/p>\n

\uff08e\uff0cf\uff09PM6:PCBM\u00a02:8\u548cPM6:Y6 7:3\u00a0NPs\u5728\u4e0d\u6dfb\u52a0\u548c\u6dfb\u52a0Pt\u6216AA\u57284s\u65f6\u7684\u6d4b\u7684PIAS\u5149\u8c31\u00a0<\/p>\n

\u56fe<\/b><\/strong>\u516b<\/b><\/strong>\u3001\u6027\u80fd<\/b><\/strong>\u5bf9\u6bd4\u00a0<\/b><\/strong> \u00a9 2022 Springer Nature<\/span>\"\"<\/p>\n

\uff08a\uff09H2<\/sub>\u6f14\u5316\u4e0e\u65f6\u95f4\u7684\u5173\u7cfb\uff1b<\/p>\n

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\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/b><\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u6587\u5f00\u53d1\u4e86\u7531PM6:Y6\u548cPM6:PCBM\u5171\u6df7\u7269\u7ec4\u6210\u7684\u6709\u673a\u534a\u5bfc\u4f53\u5236\u6c22\u5149\u50ac\u5316\u5242<\/strong>\u3002\u4f18\u5316\u540e\u7684PM6:Y6\u00a0NPs\u7684HER\u901f\u7387\u4e3a9.9\u00a0\u00b5mol\u00a0h–<\/sup>1<\/sup>cm–<\/sup>2<\/sup>\uff0843.9\u00a0mmol\u00a0h–<\/sup>1<\/sup>g–<\/sup>1<\/sup>\uff09\uff0c\u4e14\u5728\u2264400nm\u5230\u2265900nm\u4e4b\u95f4\u5177\u6709\u6d3b\u6027\u3002\u4f18\u5316\u540e\u7684PM6:PCBM\u00a0NPs\u5728400~620nm\u65f6\u7684EQEs\u901f\u7387\u4e3a8.7%~6.6%\uff0cHER\u901f\u7387\u4e3a16.7\u00a0\u00b5mol\u00a0h–<\/sup>1<\/sup>cm–<\/sup>2<\/sup>\uff0873.7 mmol\u00a0h–<\/sup>1<\/sup>g–<\/sup>1<\/sup>\uff09\u3002\u4f7f\u7528TAS\u548cPIAS\u7ec4\u5408\u7684\u5149\u7269\u7406\u8868\u5f81\u663e\u793a\uff0c\u5728NPs\u4e2dD\/A\u7684\u5f02\u8d28\u7ed3\uff0c\u5373\u4f7f\u5728\u6ca1\u6709\u6dfb\u52a0Pt\u6216AA\u7684\u60c5\u51b5\u4e0b\uff0c\u4e5f\u4f1a\u5bfc\u81f4\u660e\u663e\u957f\u5bff\u547d\u7684\u5149\u751f\u7535\u8377\u7684\u79ef\u7d2f\u3002\u8fd9\u4e9b\u7535\u8377\u5728Pt\u5171\u50ac\u5316\u5242\u548cAA\u4e2d\u88ab\u6709\u6548\u63d0\u53d6\uff0c\u8fd9\u8868\u660e\u5b83\u4eec\u589e\u5f3a\u7684NPs\u5149\u50ac\u5316\u6d3b\u6027\u3002\u4e0ePM6:Y6\u00a0NPs\u76f8\u6bd4\uff0cPM6:PCBM\u00a0NPs\u8868\u73b0\u51fa\u66f4\u5feb\u7684\u7535\u8377\u4ea7\u751f\u548c\u66f4\u957f\u7684\u7535\u8377\u79ef\u7d2f\uff0c\u540e\u8005\u7531\u4e8e\u5176\u66f4\u76f8\u5206\u79bb\u7684\u7eb3\u7c73\u5f62\u6001\u66f4\u6709\u6548\u5730\u963b\u788d\u7535\u8377\u91cd\u7ec4\u3002\u8fd9\u4e0e\u5b83\u4eec\u540cPM6:Y6\u00a0NPs\u76f8\u6bd4\u5177\u6709\u66f4\u9ad8\u7684EQEs\u662f\u4e00\u81f4\u7684\u3002\u8fd9\u4e9b\u7ed3\u679c\u8868\u660e\uff0c\u542b\u6709D\/A\u5f02\u8d28\u7ed3\u7684\u6709\u673a\u5149\u50ac\u5316\u5242\u53ef\u4ee5\u672c\u8d28\u4e0a\u89e3\u79bb\u6fc0\u5b50\u4ea7\u751f\u957f\u5bff\u547d\u7684\u6d3b\u6027\u7535\u8377\uff0c\u800c\u4e0d\u4f9d\u8d56\u4e8e\u727a\u7272\u8bd5\u5242\u5feb\u901f\u8fd8\u539f\u6fc0\u5b50\u6765\u9a71\u52a8\u7535\u8377\u5206\u79bb\u3002\u8fd9\u6807\u5fd7\u7740\u8bbe\u8ba1\u9ad8\u6548\u6709\u673a\u5149\u50ac\u5316\u5242\u8fc8\u51fa\u4e86\u91cd\u8981\u7684\u4e00\u6b65\uff0c\u8be5\u50ac\u5316\u5242\u53ef\u4ee5\u5728\u4e0d\u9700\u8981\u727a\u7272\u8bd5\u5242\u7684\u60c5\u51b5\u4e0b\u5de5\u4f5c\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a\u201c<\/strong>Generation of long-lived charges in organic semiconductor heterojunction nanoparticles for efficient photocatalytic hydrogen evolution<\/i><\/u><\/em><\/strong><\/a>\u201d<\/strong>\uff08<\/strong>Nature Energy<\/i><\/em><\/strong>\uff0c<\/b><\/strong>202<\/strong>2<\/strong>\uff0c<\/strong>10.1038\/s41560-022-00990-2<\/strong>\uff09<\/strong><\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4ebaCYM\u7f16\u8bd1\u4f9b\u7a3f\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n

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