{"id":235514,"date":"2022-04-05T06:03:23","date_gmt":"2022-04-04T22:03:23","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=235514"},"modified":"2022-04-04T19:20:24","modified_gmt":"2022-04-04T11:20:24","slug":"%e6%b8%a4%e6%b5%b7%e5%a4%a7%e5%ad%a6%e8%94%a1%e5%85%8b%e8%bf%aa-%e9%83%8e%e7%ac%91%e7%9f%b3j-electrochem-soc%ef%bc%9amoo2%e5%90%8c%e6%97%b6%e8%b0%83%e6%8e%a7tio2%e5%b8%a6%e9%9a%99%e5%82%ac%e5%8c%96","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=235514","title":{"rendered":"\u6e24\u6d77\u5927\u5b66\u8521\u514b\u8fea&\u90ce\u7b11\u77f3J. Electrochem. Soc\uff1aMoO2\u540c\u65f6\u8c03\u63a7TiO2\u5e26\u9699\u50ac\u5316\u6d3b\u6027\u4ee5\u5b9e\u73b0LiPSs\u7684\u9ad8\u6548\u8f6c\u5316"},"content":{"rendered":"

\u4e00\u3001\u3010\u7814\u7a76\u80cc\u666f\u3011<\/strong><\/p>\n

\u8fd1\u51e0\u5341\u5e74\u6765\uff0c\u968f\u7740\u7535\u52a8\u6c7d\u8f66\u7684\u5feb\u901f\u53d1\u5c55\uff0c\u5bf9\u7535\u6c60\u50a8\u80fd\u7cfb\u7edf\u6280\u672f\u7684\u9700\u6c42\u8d8a\u6765\u8d8a\u9ad8\u3002\u9502\u786b\u7535\u6c60\u7531\u4e8e\u9ad8\u7684\u7406\u8bba\u6bd4\u5bb9\u91cf\u548c\u80fd\u91cf\u5bc6\u5ea6\uff0c\u5728\u4f17\u591a\u50a8\u80fd\u7cfb\u7edf\u4e2d\u8131\u9896\u800c\u51fa\u3002\u7136\u800c\uff0c\u591a\u786b\u5316\u9502\uff08LiPSs\uff09\u7684\u7a7f\u68ad\u6548\u5e94\u662f\u5bfc\u81f4\u9502\u786b\u7535\u6c60\u5bb9\u91cf\u8870\u51cf\u5feb\u548c\u786b\u5229\u7528\u7387\u4f4e\u7684\u4e3b\u8981\u539f\u56e0\u4e4b\u4e00\uff0c\u963b\u788d\u4e86\u5176\u5546\u4e1a\u5316\u5e94\u7528\u3002\u8bbe\u8ba1\u786b\u6b63\u6781\u6750\u6599\u53ef\u4ee5\u6548\u5730\u7269\u7406\/\u5316\u5b66\u5438\u9644LiPSs\uff0c\u5176\u4e2d\uff0c\u78b3\u57fa\u6750\u6599\u7531\u4e8e\u6bd4\u8868\u9762\u79ef\u5927\u3001\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\u4e30\u5bcc\u3001\u5b54\u9699\u5206\u5e03\u5e7f\u6cdb\u3001\u529b\u5b66\u6027\u80fd\u4f18\u5f02\uff0c\u5728\u6291\u5236\u7a7f\u68ad\u6548\u5e94\u65b9\u9762\u53d1\u6325\u7740\u91cd\u8981\u4f5c\u7528\u3002\u7136\u800c\uff0c\u78b3\u6750\u6599\u5185\u90e8\u78b3\u539f\u5b50SP2<\/sup>\u548cSP3<\/sup>\u6742\u5316\u5f62\u6210\u7684\u975e\u6781\u6027\u5171\u4ef7\u952e\u53ea\u80fd\u5b9e\u73b0\u4e0e\u6781\u6027LiPSs\u7684\u7269\u7406\u5438\u9644\uff0c\u4e0d\u8db3\u4ee5\u5b8c\u5168\u6291\u5236\u5f3a\u7a7f\u68ad\u6548\u5e94\u7684\u95ee\u9898\u3002\u56e0\u6b64\uff0c\u57fa\u4e8e\u91d1\u5c5e\u5316\u5408\u7269\u901a\u8fc7\u5316\u5b66\u76f8\u4e92\u4f5c\u7528\u4e0eLiPSs\u7ed3\u5408\uff0c\u6210\u4e3a\u63d0\u9ad8LiPSs\u8f6c\u5316\u7387\u7684\u4e00\u79cd\u6709\u6548\u7b56\u7565\u3002<\/p>\n

\u4e8c\u3001\u3010\u6587\u7ae0\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6e24\u6d77\u5927\u5b66<\/b><\/strong>\u5316\u5b66\u4e0e\u6750\u6599\u5de5\u7a0b\u5b66\u9662\u7855\u58eb\u7814\u7a76\u751f\u738b\u5766\u4e3a\u7b2c\u4e00\u4f5c\u8005\uff0c<\/b><\/strong>\u8521\u514b\u8fea<\/b><\/strong>\u6559\u6388\u548c\u90ce\u7b11\u77f3\u526f\u6559\u6388\u4e3a\u901a\u8baf\u4f5c\u8005<\/b><\/strong>\u63d0\u51fa\u4ee5\u4ea4\u7ec7CNT\u4e3a\u57fa\u5e95\uff0c\u901a\u8fc7\u5d4c\u5165\u7684MoO2<\/sub>\u540c\u65f6\u8c03\u8282TiO2<\/sub>\u5e26\u9699\u548c\u50ac\u5316\u6d3b\u6027\u4ee5\u5b9e\u73b0\u5bf9LiPSs\u7684\u9ad8\u6548\u5438\u9644\uff08CMT\uff09\uff0c\u5e76\u5bf9\u5176\u50ac\u5316\u8f6c\u5316\u673a\u7406\u8fdb\u884c\u4e86\u7814\u7a76\u3002\u5176\u4e2d\u4e00\u6b65\u6c34\u70ed\u6cd5\u5bf9\u751f\u957f\u5728\u4ea4\u7ec7\u591a\u5b54\u5bfc\u7535\u9aa8\u67b6\u7684TiO2<\/sub>\u8fdb\u884c\u5c3a\u5bf8\u7684\u8c03\u8282\uff0c\u4f7f\u5176\u66b4\u9732\u51fa\u4e30\u5bcc\u7684\u50ac\u5316\u6d3b\u6027\u4f4d\u70b9\uff0c\u7ed3\u5408\u5e7f\u6cdb\u5206\u5e03\u7684\u5b54\u9699\uff0c\u8fdb\u4e00\u6b65\u4fc3\u8fdb\u4e86\u7535\u89e3\u8d28\u7684\u6e17\u900f\u548c\u7535\u8377\u8f6c\u79fb\u3002\u57fa\u4e8e\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0cMo\u7684\u5f15\u5165\u53ef\u4ee5\u8c03\u63a7Ti\u7684\u7535\u5b50\u6001\uff0c\u5e76\u51cf\u5c0fTiO2<\/sub>\u7684\u5e26\u9699\uff0c\u4f7f\u5176\u8868\u73b0\u51fa\u5bf9Li2<\/sub>S6<\/sub>\u9ad8\u7684\u5438\u9644\u80fd\u529b\u3002\u6b64\u5916\uff0c\u57fa\u4e8e\u7535\u5316\u5b66\u4ea4\u6d41\u963b\u6297\u56fe\u8c31\u8fdb\u884c\u7b49\u6548\u7535\u8def\u5efa\u6a21\u53ef\u77e5\u7535\u6781\u5177\u6709\u4f4e\u7684\u7535\u5316\u5b66\u8f6c\u79fb\u7535\u963b\uff0868.39 \u03a9\uff09\u4ee5\u53ca\u9ad8\u7684\u9502\u79bb\u5b50\u6269\u6563\u901f\u7387\uff089.65 \u00d7 10-13<\/sup>\u00a0cm2<\/sup>\u00b7s-1<\/sup>\uff09\u3002\u6b64\u5916\u7535\u6781\u8fd8\u8868\u73b0\u51fa\u4ece\u957f\u94feLiPSs\u5230Li2<\/sub>S\u7684\u9ad8\u8f6c\u5316\u6548\u7387\u3001\u4f4e\u7684\u5bb9\u91cf\u8870\u51cf\u548c\u51fa\u8272\u7684\u5faa\u73af\u6027\u80fd\u3002\u76f8\u5173\u8bba\u6587\u4ee5\u9898\u4e3a\u201cSimultaneously regulating the band gap and catalytic activity of TiO2<\/sub>\u00a0via embedded MoO2<\/sub>\u00a0based on interlaced CNT carrier for Li-S battery to achieve efficient adsorption\u201d\u53d1\u8868\u5728\u7535\u5316\u5b66\u9886\u57df\u77e5\u540d\u56fd\u9645\u671f\u520aJournal of The Electrochemical Society\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001C<\/b><\/strong>MT<\/b><\/strong>\u786b\u57fa\u4f53\u6750\u6599\u7684\u5236\u5907\u6d41\u7a0b\u793a\u610f\u56fe<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\u56fe\u4e8c\u3001\u7ed3\u6784\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a) 0.1CMT\u30010.2CMT\u30010.4CMT\u7684XRD\u56fe<\/p>\n

(b) TiO2<\/sub>\u3001MoO2<\/sub>\/TiO2<\/sub>\u7684UV\u2013vis\u5149\u8c31\u56fe<\/p>\n

(c) 0.1CMT\u30010.2CMT\u30010.4CMT\u7684Raman\u5149\u8c31\u56fe<\/p>\n

(d) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u7684Raman\u5149\u8c31\u56fe<\/p>\n

\u56fe\u4e09\u3001\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u53ca\u50ac\u5316\u8f6c\u5316\u673a\u7406\u7814\u7a76<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a) L2<\/sub>S6<\/sub>\u57280.2CMT\u4e0a\u7684\u5206\u5b50\u6a21\u578b\u53ca\u5438\u9644\u80fd\u529b<\/p>\n

(b) LiPSs\u7684\u50ac\u5316\u8f6c\u5316\u673a\u7406\u5206\u6790<\/p>\n

\u56fe\u56db\u3001\u5f62\u8c8c\u8868\u5f81<\/b><\/strong><\/p>\n

\"\"<\/p>\n

(a-c)\u00a00.1CMT\u30010.2CMT\u30010.4CMT\u7684SEM\u56fe<\/p>\n

(a1<\/sub>-c1<\/sub>) 0.1CMT\u30010.2CMT\u30010.4CMT\u8d1f\u8f7d\u786b\u540e\u7684SEM\u56fe<\/p>\n

(d) 0.2CMT\u7684EDS\u56fe<\/p>\n

\u56fe\u4e94\u3001\u6781\u5316\u6027\u8d28\u7814\u7a76<\/b><\/strong><\/p>\n

 <\/p>\n

(a)\u00a00.1CMT\/\"\" S\u30010.2CMT\/S\u30010.4CMT\/S\u7684CV\u6d4b\u8bd5\u66f2\u7ebf<\/p>\n

(b) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u7684EIS\u66f2\u7ebf\uff08\u5185\u90e8\u4e3a\u7b49\u6548\u7535\u8def\u56fe\uff09<\/p>\n

(c) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u7535\u6781Z\u2032\u4e0e\u03c9-1\/2<\/sup>\u7684\u5173\u7cfb<\/p>\n

\u56fe\u516d\u3001\u7535\u5316\u5b66\u6027\u80fd\u6d4b\u8bd5<\/b><\/strong><\/p>\n

\"\"<\/p>\n

\"\"<\/p>\n

(a-c)\u00a00.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u57280.1\u00a0C\u30010.2\u00a0C\u30010.5\u00a0C\u7535\u6d41\u5bc6\u5ea6\u4e0b\u9996\u6b21\u5145\u653e\u7535\u66f2\u7ebf<\/p>\n

(d) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u7684Qlow<\/sub>\/Qhigh<\/sub>\u6bd4\u503c\u67f1\u72b6\u56fe<\/p>\n

(e) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u5faa\u73af\u6027\u80fd\u56fe<\/p>\n

(f) 0.1CMT\/S\u30010.2CMT\/S\u30010.4CMT\/S\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af130\u6b21\u540e\uff0c\u7ee7\u7eed\u57280.2 C\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5faa\u73af200\u6b21\u7684\u5faa\u73af\u6027\u80fd<\/p>\n

\u56db\u3001\u3010\u7ed3\u8bba\u3011<\/strong><\/p>\n

\u672c\u7814\u7a76\u63d0\u51fa\u4e86\u4e00\u79cd\u57fa\u4e8e\u4ea4\u7ec7\u6001CNT\u4e3a\u8f7d\u4f53\uff0c\u901a\u8fc7\u5d4c\u5165MoO2<\/sub>\u540c\u65f6\u8c03\u8282TiO2<\/sub>\u5e26\u9699\u548c\u50ac\u5316\u6d3b\u6027\u7684\u7b56\u7565\uff0c\u7528\u4e8e\u9ad8\u6027\u80fd\u9502\u786b\u7535\u6c60\u3002\u5176\u590d\u5408\u786b\u57fa\u4f53\u53ef\u6709\u6548\u50a8\u5b58LiPSs\uff0c\u5e76\u663e\u793a\u51fa\u9ad8\u7684\u5438\u9644-\u8f6c\u5316\u80fd\u529b\u3002\u540c\u65f6\u7531\u4e8eMoO2<\/sub>\u7684\u5d4c\u5165\u6539\u53d8\u4e86Ti\u7684\u4ef7\u7535\u5b50\u5206\u5e03\uff0c\u4f7f\u5176\u7981\u5e26\u5bbd\u5ea6\u51cf\u5c0f\uff0c\u7535\u5bfc\u7387\u589e\u5f3a\uff0c\u4f7f\u5176\u7535\u6781\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u7535\u5316\u5b66\u6027\u80fd\u3002<\/p>\n

\u4e94\u3001\u3010\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u738b\u5766<\/b><\/strong>\uff0c\u6e24\u6d77\u5927\u5b662019\u7ea7\u5206\u6790\u5316\u5b66\u4e13\u4e1a\u7855\u58eb\u7814\u7a76\u751f\u3002\u4e3b\u8981\u81f4\u529b\u4e8e\u9ad8\u6bd4\u80fd\u9502\u786b\u7535\u6c60\u4f53\u7cfb\u590d\u5408\u7535\u6781\u7684\u8bbe\u8ba1\u3001\u754c\u9762\u8c03\u63a7\u53ca\u7535\u5316\u5b66\u6027\u80fd\u7814\u7a76\u3002\u81ea\u5165\u5b66\u4ee5\u6765\u8363\u83b7\u56fd\u5bb6\u5956\u5b66\u91d1\u3001\u4e00\u7b49\u5b66\u4e1a\u5956\u5b66\u91d1\u7b49\u5956\u9879\uff0c\u8363\u83b7\u8fbd\u5b81\u7701\u4f18\u79c0\u6bd5\u4e1a\u751f\u3001\u6e24\u6d77\u5927\u5b66\u5b66\u672f\u4e4b\u661f\u3001\u6e24\u6d77\u5927\u5b66\u4f18\u79c0\u7814\u7a76\u751f\u7b49\u8363\u8a89\u79f0\u53f7\u3002\u5728Electrochim. Acta\uff0cJ. Electrochem. Soc\uff0cJ. Alloys Compd\uff0cInt. J.Energy Res\u7b49\u53d1\u8868SCI\u8bba\u65875\u7bc7\u3002\u7533\u8bf7\u53d1\u660e\u4e13\u52296\u9879\uff0c\u5176\u4e2d\u5df2\u6388\u67432\u9879\uff0c\u5305\u62ec1\u9879\u6fb3\u5927\u5229\u4e9a\u4e13\u5229\u3002\u4e3b\u6301\u6e24\u6d77\u5927\u5b66\u7814\u7a76\u751f\u521b\u65b0\u57fa\u91d1\u9879\u76ee1\u9879\uff0c\u53c2\u4e0e\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9762\u4e0a\u9879\u76ee1\u9879\u53ca\u7701\u90e8\u7ea7\u9879\u76ee2\u9879\u3002<\/p>\n

\u90ce\u7b11\u77f3<\/b><\/strong>\uff0c\u535a\u58eb\uff0c\u526f\u6559\u6388\uff0c\u7855\u58eb\u751f\u5bfc\u5e08\uff0c2015\u5e747\u6708\u6bd5\u4e1a\u4e8e\u54c8\u5c14\u6ee8\u5de5\u4e1a\u5927\u5b66\u5316\u5b66\u5de5\u7a0b\u4e0e\u6280\u672f\u4e13\u4e1a\u5e76\u83b7\u5de5\u5b66\u535a\u58eb\u5b66\u4f4d\u3002\u76ee\u524d\u5728\u6e24\u6d77\u5927\u5b66\u5316\u5b66\u4e0e\u6750\u6599\u5de5\u7a0b\u5b66\u9662\u4efb\u6559\uff0c\u52a0\u5165\u5148\u8fdb\u5316\u5b66\u7535\u6e90\u7814\u7a76\u6240\u4ece\u4e8b\u9502\u786b\u7535\u6c60\u3001\u94c5\u9178\u7535\u6c60\u3001\u9502\u79bb\u5b50\u7535\u6c60\u3001\u9502\u7a7a\u6c14\u7535\u6c60\u4ee5\u53ca\u8d85\u7ea7\u7535\u5bb9\u5668\u7b49\u9886\u57df\u7814\u7a76\u3002\u8fd1\u5e74\u6765\uff0c\u4e3b\u6301\u6216\u53c2\u4e0e\u56fd\u5bb6\u53ca\u7701\u90e8\u7ea7\u4ee5\u4e0a\u9879\u76ee10\u4f59\u9879\u3002\u5148\u540e\u5728Journal of Power Sources\uff0cElectrochimica Acta<\/em>\u7b49\u671f\u520a\u53d1\u8868\u5b66\u672f\u8bba\u658730\u4f59\u7bc7\u3002\u7533\u8bf7\u6216\u6388\u6743\u56fd\u5bb6\u53d1\u660e\u4e13\u522920\u4f59\u9879\uff0c\u5e76\u83b7\u8fbd\u5b81\u7701\u81ea\u7136\u79d1\u5b66\u5b66\u672f\u6210\u679c\u5956\u4e09\u7b49\u59561\u9879\uff0c\u9526\u5dde\u5e02\u81ea\u7136\u79d1\u5b66\u5b66\u672f\u6210\u679c\u5956\u4e00\u7b49\u59561\u9879\uff0c\u51fa\u7248\u5b66\u672f\u4e13\u84572\u90e8\u3002<\/p>\n

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\u516d\u3001\u3010\u6587\u7ae0\u4fe1\u606f\u3011<\/strong><\/p>\n

T Wang, SB Zhang, XS Lang *, L Li, CG Yao, KD Cai *, Simultaneously regulating the band gap and catalytic activity of TiO2<\/sub>\u00a0via embedded MoO2<\/sub>\u00a0based on interlaced CNT carrier for Li-S battery to achieve efficient adsorption, Journal of The Electrochemical Society<\/i><\/em>, 2022<\/b><\/strong>, 169:030512.<\/p>\n

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