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\u56fe<\/b><\/strong>2<\/b><\/strong>\u00a0<\/b><\/strong>\u5178\u578b\u7684\u8d85\u9ad8\u5bc6\u5ea6SACs:\u00a0(A-E)\u77f3\u58a8\u70ef\u91cf\u5b50\u70b9AFCs (Ir1<\/sub>\/NC); (F-H)\u70ed\u89e3\u78b3\u57faAFCs (Fe1<\/sub>\/NSFC); (I-K) \u77f3\u58a8\u7094\u57faAFCs (Go1<\/sub>\/GDY)\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/b><\/strong><\/p>\n

\u76ee\u524d\uff0c\u5355\u539f\u5b50\u50ac\u5316\u5242\uff08SAC\uff09\u7684\u7814\u7a76\u70ed\u70b9\u65b9\u5411\u5305\u62ec\uff1a\u914d\u4f4d\u73af\u5883\uff08\u5305\u62ec\u7b2c\u4e00\u914d\u4f4d\u548c\u76f8\u90bb\u73af\u5883\uff09\u3001\u5206\u5b50\u5de5\u7a0b\uff08\u6d89\u53ca\u524d\u9a71\u4f53\u5206\u5b50\u8bbe\u8ba1\u548c\u5206\u5b50\u50ac\u5316\u5242\u63a5\u679d\uff09\u3001\u652f\u6491\u5de5\u7a0b\uff08\u4f8b\u5982\u7eb3\u7c73\u7ed3\u6784\u8bbe\u8ba1\u548c\u7f3a\u9677\u7ed3\u6784\u8c03\u63a7\uff0c\u70ed\u529b\u5b66\u7a33\u5b9a\u6027\uff08\u5982\u5236\u5907\u4e2d\u7684\u70ed\u539f\u5b50\u5316\u548c\u5e94\u7528\u4e2d\u7684\u7a33\u5b9a\u6027\uff09\u3001\u52a8\u6001\u50ac\u5316\u7ed3\u6784\uff08\u50ac\u5316\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u91d1\u5c5e\u539f\u5b50\u7684\u52a8\u6001\u53d8\u5316\u548c\u53ef\u5851\u6027\uff09\u3001\u5206\u6279\u5236\u5907\uff08\u5982\u514b\u7ea7\u548c\u5343\u514b\u7ea7\u5236\u5907\uff09\uff0c\u548c\u8d85\u9ad8\u542b\u91cf\uff08\u4e0d\u540c\u8f7d\u4f53\u4e0a\u7684\u6781\u9650\u8f7d\u8377\u548c\u91d1\u5c5e\u539f\u5b50\u7684\u4f4d\u7f6e\u5bc6\u5ea6\/\u8ddd\u79bb\u6548\u5e94\uff09\uff08\u8be6\u89c1\u56fe3\u5de6\uff09\u3002\u5f88\u660e\u663e\uff0c\u5982\u679c\u5bf9\u4e0a\u8ff0\u4e94\u70b9\u8fdb\u884c\u5145\u5206\u7814\u7a76\u548c\u4f18\u5316\uff0cSACs\u53ef\u4ee5\u8003\u8651\u7528\u4e8e\u5927\u89c4\u6a21\u751f\u4ea7\uff08\u5de5\u4e1a\u6761\u4ef6\u4e0b\u7684\u6279\u91cf\u5236\u5907\uff09\u548c\u5b9e\u9645\u5e94\u7528\u3002\u5bf9\u4e8e\u7279\u5b9a\u7684\u5de5\u4e1a\u5e94\u7528\uff08\u4f8b\u5982\uff0c\u9ad8\u5f3a\u5ea6\u50ac\u5316\u548c\u4f53\u79ef\u9650\u5236\u50ac\u5316\uff09\uff0c\u8d85\u9ad8\u542b\u91cf\u6216\u8d85\u9ad8\u5bc6\u5ea6SACs\uff0c\u5373\u539f\u5b50\u6ce1\u6cab\u50ac\u5316\u5242\uff08AFC<\/b><\/strong>s<\/b><\/strong>\uff09<\/b><\/strong>\uff0c\u5373\u5c06\u53d1\u6325\u5173\u952e\u4f5c\u7528\uff0c\u7531\u4e8e\u5176\u5927\u5927\u589e\u5f3a\u7684\u6574\u4f53\u50ac\u5316\u6d3b\u6027\u548c\u6700\u5c0f\u5316\u7684\u50ac\u5316\u5242\u5c42\u539a\u5ea6\uff0c\u5177\u6709\u4e0d\u53ef\u66ff\u4ee3\u7684\u5730\u4f4d\u3002AFCs\u7684\u7ed3\u6784\u529f\u80fd\u53ef\u4ee5\u4ece\u4ee5\u4e0b\u4e09\u4e2a\u65b9\u9762\u6765\u8bf4\u660e\uff1a\uff08i\uff09\u5bc6\u96c6\u4f4d\u6548\u5e94\uff0c\uff08ii\uff09\u534f\u540c\u6548\u5e94\uff0c\u4ee5\u53ca\uff08iii\uff09\u7acb\u4f53\u6548\u5e94\uff0c\u8fd9\u4e9b\u6548\u5e94\u4f7f\u5f97AFC\u5728\u7279\u5b9a\u7684\u5de5\u4e1a\u5e94\u7528\u9886\u57df\u4e2d\u4e0d\u53ef\u66ff\u4ee3\uff08\u8be6\u89c1\u56fe3\u53f3\uff09\u3002\u4f8b\u5982\uff0cAFCs\u53ef\u7528\u4e8e\u56fa\u5b9a\u8702\u7a9d\u53cd\u5e94\u5668\u4e2d\u6c7d\u8f66\u5c3e\u6c14\u7684\u5f3a\u5316\u50ac\u5316\u6c27\u5316\u6a21\u5757\uff0c\u5e76\u53ef\u7528\u4e8e\u4f53\u79ef\u56fa\u5b9a\u7535\u5316\u5b66\u88c5\u7f6e\u4e2d\u7684\u9ad8\u6548\u80fd\u91cf\u50ac\u5316\u96c6\u6210\uff0c\u6216\u8005\u901a\u8fc7\u81ea\u52a8\u5316\u5343\u514b\u7ea7\u522b\u5408\u6210AFCs\u5e76\u7528\u4e8e\u5e7f\u6cdb\u7684\u5de5\u4e1a\u50ac\u5316\uff08\u8be6\u89c1\u56fe4\uff09\u3002<\/p>\n

\"\"<\/p>\n

\u56fe3 <\/b><\/strong>SACs\u7684\u7814\u7a76\u70ed\u70b9\u53caAFCs\u7684\u7ed3\u6784\u529f\u80fd\u3002 \u00a0<\/p>\n

\"\"<\/p>\n

Fig. 4<\/b><\/strong>\u00a0\u6d78\u6e0d\u4e24\u6b65\u9000\u706b\u6cd5\u5236\u5907AFCs:\u00a0(A)\u7684\u5236\u5907\u8fc7\u7a0b, (B)\u4e0d\u540c\u91d1\u5c5e\u542b\u91cf\u67f1\u72b6\u56fe, (C) AC-STEM Pt1<\/sub>\/NC\u7684\u56fe\u50cf, (D) EXAFS\u56fe\u8c31, (E)\u624b\u52a8\u548c\u81ea\u52a8\u5408\u6210\u6bd4\u8f83\u56fe,\u00a0(F) \u5343\u514b\u7ea7\u522b\u4ea7\u54c1Ni1<\/sub>\/PCN\u7167\u7247\u53ca\u5176(G) EXAFS\u6bd4\u8f83\u56fe\u8c31\u3002 \u00a0<\/p>\n

\u76ee\u524d\uff0c\u9ad8\u5206\u6563\u9ad8\u8d1f\u8f7d\u7684SACs\u5728\u591a\u76f8\u50ac\u5316\u5e94\u7528\u4e2d\u7684\u76ee\u6807\u4ea7\u7269\u6216\u50ac\u5316\u5bf9\u8c61\u4e3b\u8981\u96c6\u4e2d\u5728\u4ee5\u4e0b\u51e0\u4e2a\u65b9\u9762\uff1a\uff081\uff09\u5316\u5b66\u71c3\u6599\uff1a\u6c22\u71c3\u6599\u3001\u78b3\u6c22\u5316\u5408\u7269\uff08\u5982\u7532\u70f7\u3001\u4e59\u9187\u7b49\uff09\u548c\u6c27\u5316\u7269\u71c3\u6599\uff08\u5982\u7532\u9178\u3001\u4e59\u9178\u7b49\uff09\uff1b\uff082\uff09 \u5316\u5de5\u539f\u6599\uff1a\u4e59\u70ef\u3001\u6c28\u3001\u4e00\u6c27\u5316\u78b3\u7b49\uff1b\uff083\uff09\u7cbe\u7ec6\u5316\u5b66\u54c1\uff1a\u836f\u7269\uff08\u5982\u6d3b\u6027\u836f\u7269\u6210\u5206\uff08API\uff09\uff09\u3001\u6740\u866b\u5242\u7b49\uff1b\uff084\uff09\u590d\u6742\u73af\u72b6\u6709\u673a\u5316\u5408\u7269\uff08COCs\uff09\uff1a\u82b3\u9999\u5316\u5408\u7269\u3001\u6742\u73af\u5316\u5408\u7269\u7b49\uff1b\uff085\uff09\u80fd\u91cf\u8f6c\u6362\u7535\u6c60\uff1a\u6c22\u6c27\u71c3\u6599\u7535\u6c60\u3001\u91d1\u5c5e\u7a7a\u6c14\u7535\u6c60\u7b49\uff1b\uff086\uff09\u751f\u7269\u5b66\u548c\u73af\u5883\uff1a\u7eb3\u7c73\u9176\u6297\u83cc\u548c\u8fc7\u786b\u9178\u76d0\u6d3b\u5316\uff08\u5982\u56fe5\u6240\u793a\uff09\u3002\u5f53\u5728\u6781\u9650\u91d1\u5c5e\u8d1f\u8f7d\u4e0b\u4e0d\u53d1\u751f\u539f\u5b50\u56e2\u805a\uff08100%\u539f\u5b50\u5229\u7528\u7387\uff09\u65f6\uff0c\u8d85\u9ad8\u5bc6\u5ea6SAC\uff08\u5373AFC<\/b><\/strong>s<\/b><\/strong>\uff09\u53ef\u4ee5\u5728\u591a\u79cd\u591a\u76f8\u50ac\u5316\u5e94\u7528\u4e2d\u63d0\u4f9b\u4f18\u5316\u7684\u50ac\u5316\u6027\u80fd\uff0c\u8fd9\u5bf9\u5de5\u4e1a\u50ac\u5316\u7684\u5b9e\u9645\u5e94\u7528\u5177\u6709\u91cd\u8981\u610f\u4e49\u3002\u672c\u6587\u5c06\u4ece\u70ed\u50ac\u5316<\/b><\/strong>\u3001\u5149\u50ac\u5316<\/b><\/strong>\u3001\u7535\u50ac\u5316<\/b><\/strong>\u548c\u5176\u4ed6\u50ac\u5316<\/b><\/strong>\u56db\u4e2a\u9886\u57df\u603b\u7ed3AFCs\u7684\u5e94\u7528\u8fdb\u5c55\u3002<\/p>\n

\"\" <\/p>\n

\u56fe5 <\/b><\/strong>AFCs\u5728\u591a\u76f8\u50ac\u5316\u4e2d\u7684\u5e94\u7528\u9886\u57df\u53ca\u76ee\u6807\u4ea7\u7269\u3002 \u00a0<\/p>\n

\uff081\uff09<\/b><\/strong>\u70ed\u50ac\u5316<\/b><\/strong>\uff1a<\/b><\/strong><\/p>\n

\u9ad8\u5ea6\u5206\u6563\u7684SAC\uff08\u5c24\u5176\u662f\u5177\u6709\u8d85\u9ad8\u539f\u5b50\u5bc6\u5ea6\u7684AFC<\/b><\/strong>s<\/b><\/strong>\uff09\u5df2\u88ab\u8bc1\u660e\u5728\u8bb8\u591a\u5316\u5b66\u5408\u6210\uff08\u5982\u5316\u5b66\u71c3\u6599\u3001\u5316\u5b66\u539f\u6599\u3001\u6d3b\u6027\u836f\u7269\u6210\u5206\u3001\u590d\u6742\u73af\u72b6\u6709\u673a\u5316\u5408\u7269\u7b49\uff09\u7684\u70ed\u50ac\u5316\u4e2d\u662f\u6709\u6548\u7684\uff0c\u7531\u4e8e\u5176\u7279\u6b8a\u7684\u201c\u7535\u5b50\/\u51e0\u4f55\u7ed3\u6784\u201d\u548c\u4e30\u5bcc\u7684\u201c\u5b64\u7acb\/\u534f\u540c\u6d3b\u6027\u4f4d\u70b9\u201d\u7684\u591a\u91cd\u4f18\u52bf\u3002\u672c\u7efc\u8ff0\u9009\u62e9\u4e86\u51e0\u79cd\u5178\u578b\u7684\u50ac\u5316\u53cd\u5e94\uff0c\u4ee5\u5c55\u793aAFC\u5728\u70ed\u50ac\u5316\u5e94\u7528\u4e2d\u7684\u4f18\u52bf\u548c\u8d21\u732e\uff0c\u5305\u62ec\u9009\u62e9\u6027\u52a0\u6c22\u53cd\u5e94\u3001\u50ac\u5316\u6c27\u5316\u53cd\u5e94<\/b><\/strong>\u3001\u4ea4\u53c9\u5076\u8054\u53cd\u5e94<\/b><\/strong>\u548c\u6c34\u7164\u6c14\u53d8\u6362<\/b><\/strong>\u53cd\u5e94<\/b><\/strong>\uff08WGS\uff09<\/b><\/strong>\u6216\u5176\u9006\u53cd\u5e94<\/b><\/strong>\uff08<\/b><\/strong>R<\/b><\/strong>WGS\uff09<\/b><\/strong>\uff08\u89c1\u56fe6\uff09\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe6<\/b><\/strong>\u57fa\u4e8e\u4e0d\u540cAFCs\u7684\u50ac\u5316WGS(\u6216RWGS)\u53cd\u5e94:(A-C) Pt1<\/sub>-Ptn<\/sub>\/\u03b1-MoC\u7528\u4e8eWGS\uff0c(D) Ir1<\/sub>\/FeOx<\/sub>\u7528\u4e8eWGS\uff0c(E-H) Pd1<\/sub>\/\u03b1-MoC\u7528\u4e8eRWGS\uff0c(I-O) Fe1<\/sub>\/MoS2<\/sub>\u7528\u4e8eRWGS\u3002 \u00a0<\/p>\n

\uff08<\/b><\/strong>2<\/b><\/strong>\uff09\u5149<\/b><\/strong>\u50ac\u5316<\/b><\/strong>\uff1a<\/b><\/strong><\/p>\n

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\u56fe7<\/b><\/strong>\u57fa\u4e8e\u4e0d\u540cAFCs\u7684\u5149\u50ac\u5316\u201c\u6c27\u5316\/\u5076\u8054\/\u73af\u52a0\u6210\u201d\u53cd\u5e94:\u00a0(A-D) Sb1<\/sub>\/g-C3<\/sub>N4<\/sub>\u7528\u4e8e\u5c06H2<\/sub>O\u6c27\u5316\u6210H2<\/sub>O2<\/sub>\uff0c(E-H) Cu1<\/sub>\/S-g-C3<\/sub>N4<\/sub>\u7528\u4e8e\u5c06HMF\u6c27\u5316\u6210DFF\uff0c(I-K) Co1<\/sub>\/NC\u7528\u4e8e\u5076\u8054\uff0c(L-N) Zn1<\/sub>\/NC\u7528\u4e8e\u73af\u52a0\u6210\u3002 \u00a0<\/p>\n

\uff08<\/b><\/strong>3<\/b><\/strong>\uff09\u7535<\/b><\/strong>\u50ac\u5316<\/b><\/strong>\uff1a<\/b><\/strong><\/p>\n

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\uff08<\/b><\/strong>4<\/b><\/strong>\uff09\u5176\u4ed6<\/b><\/strong>\u50ac\u5316<\/b><\/strong>\uff1a<\/b><\/strong><\/p>\n

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\"\"<\/p>\n

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\"\"<\/p>\n

\u56fe10<\/b><\/strong>\u57fa\u4e8eAFCs\u591a\u786b\u5316\u7269\u7684\u50ac\u5316\u8f6c\u6362:(A\u548cB) FeN2<\/sub>-NC,(C\u548cD) Fe-NSC,(E\u548cF) CoSA-N-C,(G\u548cH) CoN2<\/sub>,(I, J) Co-SAC\u3002<\/p>\n

\u3010<\/b><\/strong>\u7ed3\u8bba<\/b><\/strong>\u3011<\/b><\/strong><\/p>\n

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\u8bba\u6587\u4fe1\u606f\uff1aLi Z, Li B, Hu Y, Liao X, Yu H, Yu C. Emerging ultra-high-density single atom catalysts for versatile heterogeneous catalysis applications: redefinition, recent progress and challenges. Small Structures.2022<\/p>\n

\u8bba\u6587\u7f51\u5740\uff1ahttps:\/\/onlinelibrary.wiley.com\/doi\/full\/10.1002\/sstr.202200041<\/u><\/a>\u00a0\u00a0\u00a0<\/p>\n","protected":false},"excerpt":{"rendered":"

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