{"id":236582,"date":"2022-05-07T06:56:26","date_gmt":"2022-05-06T22:56:26","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=236582"},"modified":"2022-05-06T17:01:26","modified_gmt":"2022-05-06T09:01:26","slug":"%e8%83%a1%e5%96%9c%e4%b9%90-nature-catalysis%ef%bc%9afe%e9%ab%98%e8%be%be90%ef%bc%81%e5%bc%ba%e9%85%b8%e6%80%a7%e4%bb%8b%e8%b4%a8%e4%b8%ad%e7%94%b5%e8%bf%98%e5%8e%9fco2","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=236582","title":{"rendered":"\u80e1\u559c\u4e50 Nature Catalysis\uff1aFE\u9ad8\u8fbe90%\uff01\u5f3a\u9178\u6027\u4ecb\u8d28\u4e2d\u7535\u8fd8\u539fCO2"},"content":{"rendered":"

\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u7535\u5316\u5b66\u8fd8\u539fCO2<\/sub>\u4ee5\u751f\u4ea7\u5316\u5b66\u54c1\u548c\u71c3\u6599\u662f\u4e00\u79cd\u6f5c\u5728\u7684\u53ef\u518d\u751f\u80fd\u6e90\u50a8\u5b58\u548cCO2<\/sub>\u5faa\u73af\u5229\u7528\u89e3\u51b3\u65b9\u6848\u3002\u7531\u4e8e\u5728\u9178\u6027\u6c34\u6eb6\u6db2\u4e2d\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u5360\u4e3b\u5bfc\u5730\u4f4d\uff0c\u56e0\u6b64CO2<\/sub>\u7535\u8fd8\u539f\u5728\u78b1\u6027\u6216\u8fd1\u4e2d\u6027\u4ecb\u8d28\u4e2d\u8fdb\u884c\u7684\u3002\u7136\u800c\uff0c\u8fd9\u4e9b\u53cd\u5e94\u4ecb\u8d28\u9020\u6210\u4e86\u9ad8\u6548\u3001\u7a33\u6001CO2<\/sub>\u7535\u89e3\u7684\u5173\u952e\u969c\u788d\u4e4b\u4e00\uff1aCO2<\/sub>\u4e0e\u6c22\u6c27\u6839\uff08OH–<\/sup>\uff09\u5bb9\u6613\u53cd\u5e94\u5f62\u6210\u78b3\u9178\u76d0\uff08CO3<\/sub>2-<\/sup>\uff09\u3002\u5728\u78b1\u6027\u4ecb\u8d28\u4e2d\uff0c\u4ece\u78b3\u9178\u76d0\u6c34\u6eb6\u6db2\u4e2d\u518d\u751fCO2<\/sub>\u548c2OH–<\/sup>\u9700\u8981\u80fd\u91cf\uff0c\u5e76\u5bfc\u81f4CO2<\/sub>\u7535\u8fd8\u539f\u7684\u80fd\u91cf\u6548\u7387\u4f4e\u751a\u81f3\u4e3a\u8d1f\u3002\u5728\u8fd1\u4e2d\u6027\u4ecb\u8d28\u4e2d\uff0c\u867d\u7136\u53ef\u4ee5\u8fdb\u884c\u7a33\u6001CO2<\/sub>\u7535\u89e3\uff0c\u4f46\u662fCO2<\/sub>\u4ecd\u4f1a\u88abCO2<\/sub>\u7535\u8fd8\u539f\u7535\u5316\u5b66\u4ea7\u751f\u7684OH–<\/sup>\u9634\u79bb\u5b50\u6d88\u8017\u3002\u6b64\u5916\uff0c\u5728\u8fd1\u4e2d\u6027\u4ecb\u8d28\u4e2d\uff0c\u6eb6\u6db2\u7684\u9ad8\u7535\u963b\u548c\u8f83\u9ad8\u7684\u6790\u6c27\u53cd\u5e94\uff08OER\uff09\u8fc7\u7535\u4f4d\u5bfc\u81f4\u7535\u6c60\u7535\u538b\u9ad8\u548c\u80fd\u91cf\u6548\u7387\u4f4e\u3002\u5728\u5f3a\u9178\u6027\u4ecb\u8d28\u4e2d\uff0cOER\u7684\u7535\u963b\u548c\u8fc7\u7535\u4f4d\u8f83\u4f4e\uff0c\u7531\u4e8e\u78b3\u9178\u76d0\u4e0d\u4f1a\u7a7f\u8fc7\u4ecb\u8d28\u5230\u8fbe\u9633\u6781\uff0c\u56e0\u6b64\u53ef\u4ee5\u89e3\u51b3\u78b3\u9178\u76d0\u95ee\u9898\u3002\u5728\u9178\u6027\u4ecb\u8d28\u4e2d\u8fdb\u884c\u6709\u6548\u7684CO2<\/sub>\u7535\u8fd8\u539f\u8fd8\u5177\u6709\u6311\u6218\u6027\uff0c\u56e0\u4e3aHER\u6bd4CO2<\/sub>\u8fd8\u539f\u66f4\u5bb9\u6613\u3002\u6839\u636e\u5df2\u62a5\u9053\u6210\u679c\u53d1\u73b0\uff0c\u78b1\u91d1\u5c5e\u9633\u79bb\u5b50\u5bf9\u4e8eCO2<\/sub>\u8fd8\u539f\u81f3\u5173\u91cd\u8981\uff0c\u4f46\u9633\u79bb\u5b50\u4fc3\u8fdb\u7684\u673a\u5236\u4ecd\u4e0d\u6e05\u695a\uff0c\u4ec5\u8bc1\u660e\u4e86\u78b1\u91d1\u5c5e\u9633\u79bb\u5b50\u5bf9\u4e8e\u7a33\u5b9aCO2<\/sub>\u7269\u79cd\u5fc5\u4e0d\u53ef\u5c11\u3002\u56e0\u6b64\uff0c\u76ee\u524d\u5c1a\u4e0d\u6e05\u695a\u78b1\u6027\u9633\u79bb\u5b50\u5982\u4f55\u6291\u5236\u9178\u6027\u4ecb\u8d28\u4e2d\u4e3b\u8981\u7684HER\u3002
\n \"\"
\n \u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u745e\u58eb\u6d1b\u6851\u8054\u90a6\u7406\u5de5\u5b66\u9662\u80e1\u559c\u4e50\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u7b49\u4eba<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u901a\u8fc7\u5229\u7528\u78b1\u6027\u9633\u79bb\u5b50\u6291\u5236\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u7684\u65b9\u6cd5\uff0c\u5728\u5f3a\u9178\u6027\u4ecb\u8d28\uff08pH=1.0\uff09\u4e2d\u5c55\u793a\u4e86\u9ad8\u6548\u7684CO2<\/sub>\u7535\u8fd8\u539f\uff0c\u5176\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u9ad8\u8fbe90%\u3002\u5728\u6587\u4e2d\uff0c\u4f5c\u8005\u5c06\u8fd9\u79cd\u65b9\u6cd5\u5e94\u7528\u4e8e\u4e09\u7c7b\u5177\u6709\u4ee3\u8868\u6027\u7684\u50ac\u5316\u5242\uff0c\u5373\u78b3\u8d1f\u8f7d\u7684SnO2<\/sub>\u3001Au\u548cCu\u7eb3\u7c73\u9897\u7c92\uff08SnO2<\/sub>\/C\u3001Au\/C\u548cCu\/C\uff09\uff0c\u5b83\u4eec\u53ef\u7528\u4e8e\u4ea7\u751f\u7532\u9178\u3001CO\u548c\u78b3\u6c22\u5316\u5408\u7269\uff0c\u5206\u522b\u4f5c\u4e3aCO2<\/sub>\u7535\u8fd8\u539f\u7684\u4e3b\u8981\u4ea7\u7269\uff0c\u5176\u4e2d\u751f\u6210\u7532\u9178\u548cCO\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u9ad8\u8fbe90%\u3002\u901a\u8fc7\u6a21\u62df\u548c\u5206\u6790\u8868\u660e\uff0c\u9634\u6781\u53cc\u5c42\u4e2d\u7684\u78b1\u91d1\u5c5e\u9633\u79bb\u5b50\u6709\u6548\u5730\u5c4f\u853d\u4e86\u6269\u6563\u5c42\u4e2d\u7684\u7535\u573a\uff0c\u6291\u5236\u4e86\u6c34\u5408\u6c22\u79bb\u5b50\u5411\u9634\u6781\u7684\u8fc1\u79fb\uff0c\u4ece\u800c\u964d\u4f4e\u4e86\u5916\u4ea5\u59c6\u970d\u5179\u5e73\u9762\uff08outer Helmholtz plane, OHP\uff09\u4e2d\u6c34\u5408\u6c22\u79bb\u5b50\u7684\u6d53\u5ea6\uff0c\u8fdb\u800c\u6709\u6548\u7684\u6291\u5236\u4e86HER\u3002\u540c\u65f6\uff0c\u9633\u79bb\u5b50\u589e\u5f3a\u4e86Stern\u5c42\u7684\u7535\u573a\uff0c\u5e76\u7a33\u5b9a\u4e86CO2<\/sub>\u8fd8\u539f\u8fc7\u7a0b\u4e2d\u7684\u5173\u952e\u4e2d\u95f4\u4f53\uff0c\u4ee5\u4fc3\u8fdbCO2\u8fd8\u539f\u3002\u8be5\u5de5\u4f5c\u4e0d\u4ec5\u8bc1\u660e\u4e86\u5229\u7528\u78b1\u6027\u9633\u79bb\u5b50\u6291\u5236HER\u4ee5\u4fc3\u8fdbCO2<\/sub>\u8fd8\u539f\u7b56\u7565\u5bf9\u4e8e\u5404\u79cd\u50ac\u5316\u5242\u548c\u9633\u79bb\u5b50\u5177\u6709\u901a\u7528\u6027\uff0c\u800c\u4e14\u63ed\u793a\u4e86\u9633\u79bb\u5b50\u8bf1\u5bfc\u7684\u7535\u573a\u8c03\u5236\u662f\u9633\u79bb\u5b50\u6548\u5e94\u7684\u4fc3\u8fdb\u673a\u5236\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201cModulating electric field distribution by alkali cations for CO2<\/sub> electroreduction in strongly acidic medium\u201d<\/strong>\u53d1\u5e03\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Catalysis<\/em>\u4e0a\u3002<\/p>\n

\u672c\u6587\u6240\u6709\u56fe\u6765\u6e90\u4e8e\u00a9 2022 Springer Nature Limited\u3002
\n \"\"
\n \u3010\u6838\u5fc3\u521b\u65b0\u3011<\/strong><\/p>\n

1\u3001\u4f5c\u8005\u63d0\u51fa\u4e86\u5229\u7528\u78b1\u91d1\u5c5e\u9633\u79bb\u5b50\u6765\u8c03\u5236\u7535\u573a\uff0c\u4ee5\u6291\u5236HER\uff0c\u4ece\u800c\u53ef\u5728\u9178\u6027\u4ecb\u8d28\u4e2d\u8fdb\u884c\u6709\u6548\u7684CO2<\/sub>\u7535\u8fd8\u539f\uff0c\u514b\u670d\u78b3\u9178\u76d0\u95ee\u9898\u3002<\/p>\n

2\u3001\u5229\u7528SnO2<\/sub>\/C\u3001Au\/C\u50ac\u5316\u5242\u8fdb\u884cCO2<\/sub>\u7535\u8fd8\u539f\u751f\u6210\u7532\u9178\u548cCO\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u9ad8\u8fbe90%\u3002<\/p>\n

\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u56fe\u4e00\u3001\u5728\u542b\u6709K+<\/sup>\u79bb\u5b50\u7684\u9178\u6027\u6eb6\u6db2\u4e2dCO2<\/sub>\u8fd8\u539f\u7684\u6027\u80fd<\/strong>
\n \"\"\uff08a\uff09SnO2<\/sub>\/C\u57280.1\u2009M HOTf\u4e0eN2<\/sub>\u548cCO2<\/sub>\u30010.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\u4e0eN2<\/sub>\u548cCO2<\/sub>\u7684CV\u66f2\u7ebf\uff0c\u4ee5\u53caVulcan XC-72R\u57280.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\u4e0eCO2<\/sub>\u7684CV\u66f2\u7ebf\uff1b<\/p>\n

\uff08b-c\uff09SnO2\/C\u50ac\u5316\u52420.1\u2009M H2<\/sub>SO4<\/sub>\u2009+\u20090.4\u2009M K2<\/sub>SO4<\/sub>\u4e2d\u4e0d\u540c\u8fd8\u539f\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u548c\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\uff1b<\/p>\n

\uff08d-e\uff09Au\/C\u50ac\u5316\u52420.1\u2009M H2<\/sub>SO4<\/sub>\u2009+\u20090.4\u2009M K2<\/sub>SO4<\/sub>\u4e2d\u4e0d\u540c\u8fd8\u539f\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u548c\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\uff1b<\/p>\n

\uff08f-g\uff09Cu\/C\u50ac\u5316\u52420.1\u2009M H2<\/sub>SO4<\/sub>\u2009+\u20090.4\u2009M K2<\/sub>SO4<\/sub>\u4e2d\u4e0d\u540c\u8fd8\u539f\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff08FE\uff09\u548c\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u3002<\/p>\n

\u56fe\u4e8c\u3001\u6bd4\u8f83\u9178\u6027\u3001\u8fd1\u4e2d\u6027\u548c\u78b1\u6027\u4ecb\u8d28\u4e2dCO2<\/sub>\u7535\u8fd8\u539f<\/strong>
\n \"\"\uff08a\uff09Au\/C\u548cIrO2<\/sub>\u5206\u522b\u4f5c\u4e3a\u9634\u6781\u548c\u9633\u6781\u50ac\u5316\u5242\u7684\u53cc\u7535\u6781\u6d41\u901a\u6c60\u7684\u7535\u6c60\u7535\u538b\uff1b<\/p>\n

\uff08b\uff09\u7535\u89e3\u524d\u540e\uff0c\u7535\u89e3\u8d28\u6eb6\u6db2\u7684pH\u503c\u3002<\/p>\n

\u56fe\u4e09\u3001\u4f30\u7b97\u53ef\u6301\u7eedCO2<\/sub>\u7535\u8fd8\u539f\u7684\u80fd\u8017<\/strong>
\n \"\"\uff08a-b\uff09\u5047\u5b9a\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u4e3a200\u2009mA\u2009cm-2<\/sup>\uff0c\u751f\u4ea71\u2009 mol CO\u548c\u4e59\u70ef\u6240\u9700\u7684\u80fd\u91cf\u6d88\u8017\u3002<\/p>\n

\u56fe\u56db\u3001\u9633\u79bb\u5b50\u5bf9HER\u548cCO2<\/sub>\u8fd8\u539f\u7684\u5f71\u54cd<\/strong>
\n \"\"\uff08a\uff09N2<\/sub>\u9971\u548c\u6eb6\u6db2\u4e2dAu RDE\u7684LSV\u66f2\u7ebf\uff1a0.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\u30010.4\u2009M KOTf\u30010.1\u2009M HOTf\u548c0.5\u2009M HOTf\uff1b<\/p>\n

\uff08b-c\uff09\u57280.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\uff08Li\u3001Na\u3001K\u548cCs\uff09\u4e2d\uff0c\u5728-1.34 V vs. RHE\u65f6\u7532\u9178\u3001CO\u548cH2<\/sub>\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u548c\u5c40\u90e8\u7535\u6d41\u5bc6\u5ea6\u3002<\/p>\n

\u56fe\u4e94\u3001\u9633\u79bb\u5b50\u5bf9\u7535\u573a\u5206\u5e03\u7684\u5f71\u54cd<\/strong>
\n \"\"\uff08a-b\uff09\u6a21\u62df\u5256\u9762\u548cOHP\u8ddd\u79bb\u5185\u7684\u7535\u573a\u5f3a\u5ea6\u5206\u5e03\u5256\u9762\uff1b<\/p>\n

\uff08c-d\uff09HOTf\u2009+\u2009MOTf\u548cHOTf\u4ecb\u8d28\u4e2d\u9634\u6781\u9644\u8fd1\u7684\u53cc\u5c42\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe\u516d\u3001\u6a21\u62df\u5c40\u90e8pH\u6548\u5e94<\/strong>
\n \"\"\uff08a\uff090.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\u548c0.1\u2009M HOTf\u5728-0.70\u2009V vs. PZC\u4e2d\u8ddd\u79bbOHP\u7684pH\u66f2\u7ebf\uff1b\u76f8\u5e94\u7684\u9634\u6781\u7535\u6d41\u5bc6\u5ea6\u5206\u522b\u4e3a90\u548c524\u2009mA\u2009cm-2<\/sup>\uff1b<\/p>\n

\uff08b\uff090.1\u2009M HOTf\u2009+\u20090.4\u2009M KOTf\u548c0.1\u2009M HOTf\u4e2d\u7684pH\u66f2\u7ebf\uff0c\u9634\u6781\u7535\u6d41\u5bc6\u5ea6\u5747\u4e3a221\u2009mA\u2009cm-2<\/sup>\u3002<\/p>\n

\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u4f5c\u8005\u5229\u7528\u78b1\u91d1\u5c5e\u9633\u79bb\u5b50\u6291\u5236\u6c34\u5408\u6c22\u79bb\u5b50\u8fd8\u539f\uff0c\u4ee5\u4fc3\u8fdbCO2<\/sub>\u8fd8\u539f\uff0c\u5c55\u793a\u4e86\u5f3a\u9178\u6027\u4ecb\u8d28\u4e2d\u6709\u6548\u7684CO2<\/sub>\u7535\u8fd8\u539f\u3002\u4f5c\u8005\u8bc1\u660e\u4e86\u8fd9\u79cd\u65b9\u6cd5\u9002\u7528\u4e8e\u5404\u79cd\u50ac\u5316\u5242\u548c\u9633\u79bb\u5b50\uff0c\u5e76\u63ed\u793a\u4e86\u9633\u79bb\u5b50\u8bf1\u5bfc\u7684\u7535\u573a\u8c03\u5236\u662f\u9633\u79bb\u5b50\u6548\u5e94\u7684\u8d77\u56e0\u3002\u8be5\u7814\u7a76\u4e3a\u907f\u514dCO2<\/sub>\u7535\u8fd8\u539f\u8fc7\u7a0b\u4e2d\u7684\u78b3\u9178\u76d0\u95ee\u9898\u63d0\u4f9b\u4e86\u4e00\u79cd\u6709\u524d\u666f\u7684\u7b56\u7565\uff0c\u800cCO2<\/sub>\u7535\u8fd8\u539f\u662f\u4f4e\u6e29CO2<\/sub>\u7535\u89e3\u7684\u4e3b\u8981\u969c\u788d\u4e4b\u4e00\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aModulating electric field distribution by alkali cations for CO2<\/sub> electroreduction in strongly acidic medium<\/strong>. Nature Catalysis<\/em>, 2022<\/strong>, DOI: 10.1038\/s41929-022-00761-y.<\/p>\n

\u672c\u6587\u7531CQR\u7f16\u8bd1\u3002<\/p>\n

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