{"id":236659,"date":"2022-05-06T06:08:01","date_gmt":"2022-05-05T22:08:01","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=236659"},"modified":"2022-05-05T14:16:43","modified_gmt":"2022-05-05T06:16:43","slug":"%e6%b2%b3%e5%8d%97%e5%a4%a7%e5%ad%a6%e9%ab%98%e8%b7%83%e5%b2%b3%e5%89%af%e6%95%99%e6%8e%88%e6%9c%80%e6%96%b0solar-rrl-%e7%9c%9f%e7%a9%ba%e8%be%85%e5%8a%a9%e4%bd%8e%e6%b8%a9%e7%94%9f%e9%95%bf%e7%ad%96","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=236659","title":{"rendered":"\u6cb3\u5357\u5927\u5b66\u9ad8\u8dc3\u5cb3\u526f\u6559\u6388\u6700\u65b0Solar RRL: \u771f\u7a7a\u8f85\u52a9\u4f4e\u6e29\u751f\u957f\u7b56\u7565\u5236\u5907\u9ad8\u6548\u7a33\u5b9a\u7684\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60"},"content":{"rendered":"

\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6cb3\u5357\u5927\u5b66\u5149\u4f0f\u6750\u6599\u7701\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u9ad8\u8dc3\u5cb3\u526f\u6559\u6388\uff0c\u5cb3\u6839\u7530\u526f\u6559\u6388\uff0c\u9f50\u9f50\u54c8\u5c14\u5927\u5b66\u8463\u56fd\u534e\u526f\u6559\u6388\u4e0e\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u6d82\u7528\u5e7f\u526f\u6559\u6388\u5408\u4f5c\u63d0\u51fa\u91c7\u7528\u52a8\u6001\u771f\u7a7a\u8f85\u52a9<\/b><\/strong>\u4f4e\u6e29\u751f\u957f\u7b56\u7565<\/b><\/strong>\u5236\u5907\u9ad8\u8d28\u91cfCsPbIB<\/b><\/strong>2<\/b><\/sub><\/strong>\u8584\u819c\uff0c\u5e76\u5e94\u7528\u4e8e\u6784\u7b51\u9ad8\u6027\u80fd\u5168\u65e0\u673a\u9499\u949b\u77ff\u7535\u6c60<\/b><\/strong>\uff0c\u8be5\u5de5\u4f5c\u4ee5“<\/b><\/strong>\u00a0Efficient and Stable All-Inorganic CsPbIBr<\/b><\/strong>2<\/b><\/sub><\/strong>\u00a0Perovskite Solar Cells Enabled by Dynamic Vacuum-Assisted Low-Temperature Engineering”<\/b><\/strong>\u4e3a\u9898\uff0c\u53d1\u8868\u5728\u671f\u520aSolar RRL<\/b><\/strong>,\u94fe\u63a5\uff1a<\/p>\n

https:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/solr.202100839<\/u><\/a>\u3002<\/p>\n

\u6709\u673a\u65e0\u673a\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u4f5c\u4e3a\u65b0\u4e00\u4ee3\u53ef\u518d\u751f\u80fd\u6e90\u6280\u672f\uff0c\u56e0\u5176\u4f18\u826f\u7684\u5438\u6536\u7cfb\u6570\u3001\u4f4e\u6fc0\u5b50\u7ed3\u5408\u80fd\u548c\u6613\u4e8e\u6eb6\u6db2\u6280\u672f\u5236\u5907\u7b49\u4f18\u70b9\u800c\u5907\u53d7\u5173\u6ce8\u3002\u7ecf\u8fc7\u7814\u7a76\u4eba\u5458\u7684\u4e0d\u65ad\u52aa\u529b\uff0c\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u5728\u77ed\u77ed\u51e0\u5e74\u5185\u5149\u7535\u8f6c\u6362\u6548\u7387\u4ece3.8%\u8fc5\u901f\u63d0\u5347\u81f325.7%\uff0c\u751a\u81f3\u53ef\u4ee5\u4e0e\u5546\u7528\u7845\u592a\u9633\u80fd\u7535\u6c60\u76f8\u5ab2\u7f8e\u3002\u7136\u800c\uff0c\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u6d3b\u6027\u5c42\u542b\u6709\u673a\u79bb\u5b50\uff08CH3<\/sub>NH3<\/sub>+<\/sup>, CH3<\/sub>(NH2<\/sub>)2<\/sub>+<\/sup>\uff09\u5bf9\u6c34\u6c27\u8f83\u4e3a\u654f\u611f\u3001\u4e0d\u7a33\u5b9a\u4e14\u6613\u6325\u53d1\uff0c\u5bf9\u5176\u5927\u89c4\u6a21\u5546\u4e1a\u5316\u4ea7\u751f\u4e0d\u5229\u5f71\u54cd\u3002\u6700\u8fd1\uff0c\u91c7\u7528\u65e0\u673aCs+<\/sup>\u53d6\u4ee3\u6742\u5316\u9499\u949b\u77ff\u4e2d\u6709\u673a\u9633\u79bb\u5b50\u6784\u7b51\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u6210\u4e3a\u89e3\u51b3\u6742\u5316\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7a33\u5b9a\u6027\u6b20\u4f73\u7684\u6709\u6548\u9014\u5f84\u3002\u5728\u4f17\u591a\u5168\u65e0\u673a\u9499\u949b\u77ff\u6750\u6599\u4e2d\uff0cCsPbIBr2<\/sub>\u56e0\u5176\u5408\u9002\u7684\u5e26\u9699\u548c\u51fa\u8272\u76f8\u7a33\u5b9a\u6027\u95f4\u7684\u8c03\u8c10\u800c\u5907\u53d7\u5173\u6ce8\u3002\u7136\u800c\uff0c\u4f20\u7edf\u65b9\u6cd5\u5236\u5907\u7684CsPbIBr2<\/sub>\u8584\u819c\u5f80\u5f80\u7ed3\u6676\u8fc7\u5feb\u5bfc\u81f4\u5f62\u8c8c\u4e0d\u53ef\u63a7\uff0c\u8584\u819c\u8d28\u91cf\u5dee\uff0c\u6613\u5f62\u6210\u9488\u5b54\u4ea7\u751f\u6f0f\u7535\u800c\u9650\u5236\u5176\u5668\u4ef6\u6027\u80fd\u3002<\/p>\n

\u9274\u4e8e\u4e0a\u8ff0\u7814\u7a76\u73b0\u72b6\uff0c\u6cb3\u5357\u5927\u5b66\u9ad8\u8dc3\u5cb3\u526f\u6559\u6388\u4e0e\u7855\u58eb\u751f\u9ec4\u519b\u610f\u63d0\u51fa\u4e86\u4e00\u79cd\u52a8\u6001\u7684\u771f\u7a7a\u8f85\u52a9\u4f4e\u6e29\u751f\u957f\u7b56\u7565\uff08VAST\uff09\u7528\u6765\u5236\u5907\u9ad8\u6548\u3001\u7a33\u5b9a\u7684\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u3002\u56e2\u961f\u6307\u51fa\u901a\u8fc7\u8c03\u63a7\u8584\u819c\u9000\u706b\u65f6\u7684\u771f\u7a7a\u5ea6\u548c\u9000\u706b\u6e29\u5ea6\u53ef\u6709\u6548\u63a7\u5236CsPbIBr2<\/sub>\u8584\u819c\u7684\u5f62\u8c8c\u548c\u7ed3\u6676\u8d28\u91cf\u3002\u7ecf\u8fc7\u591a\u65b9\u4f4d\u4f18\u5316\uff0c\u901a\u8fc7VAST\u7b56\u7565\u53ef\u4ee5\u5b9e\u73b0\u65e0\u9488\u5b54\u3001\u9ad8\u7ed3\u6676\u5ea6CsPbIBr2<\/sub>\u8584\u819c\u5236\u5907\uff0c\u8fdb\u800c\u5b9e\u73b0\u4e86\u7535\u8377\u63d0\u53d6\u548c\u7f3a\u9677\u6001\u5bc6\u5ea6\u5f31\u5316\u7684\u53cc\u91cd\u529f\u6548\u3002\u7279\u522b\u7684\u662f\uff0c\u57fa\u4e8eVAST\u7b56\u7565\u5236\u5907\u7684\u5668\u4ef6\u6548\u7387\u7531\u7a7a\u767d\u76849.00%\u53ef\u63d0\u5347\u81f311.01%\uff0c\u5176\u4e2d\u66f4\u662f\u5c55\u73b0\u51fa75.31%\u7684\u9ad8\u586b\u5145\u56e0\u5b50\uff0c\u4e5f\u662fCsPbIBr2<\/sub>\u9499\u949b\u77ff\u7535\u6c60\u4e2d\u62a5\u9053\u7684\u6700\u9ad8\u503c\u3002\u6b64\u5916\uff0c\u4f18\u5316\u5668\u4ef6\u7684\u70ed\u7a33\u5b9a\u6027\u548c\u7a7a\u6c14\u7a33\u5b9a\u6027\u5747\u5f97\u5230\u8fdb\u4e00\u6b65\u63d0\u9ad8\u3002\u8be5\u5de5\u4f5c\u8868\u660eVAST\u7b56\u7565\u4e3a\u5236\u5907\u9ad8\u6548\u7a33\u5b9a\u5168\u65e0\u673a\u9499\u949b\u77ff\u7535\u6c60\u63d0\u4f9b\u4e86\u65b0\u7684\u8def\u5f84\u3002<\/p>\n

\u3010\u56fe\u6587\u89e3\u8bfb\u3011<\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

Scheme1.<\/strong>\u00a0<\/strong>The schematic illustration of the dynamic vacuum-assisted low-temperature engineering for preparing VALT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0film.<\/strong><\/p>\n

\"\"<\/b><\/strong><\/p>\n

Figure 1. a,d) SEM, b,e) AFM, and c,f ) KPFM images of HT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0film<\/strong>, <\/strong>(a<\/strong>–<\/strong>c)<\/strong>\u00a0<\/strong>and<\/strong>\u00a0<\/strong>VALT-CsPbIBr<\/strong>2<\/sub><\/strong>film<\/strong>\u00a0<\/strong>(d<\/strong>–<\/strong>f),<\/strong>\u00a0<\/strong>respectively.<\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

Figure 2. a) XRD patterns; b) energy level diagram of functional layers in PSCs of this work; c) steady PL spectra with quartz glasses as substrate; d) TRPL<\/strong>\u00a0<\/strong>spectra with quartz glasses as substrate; e,f ) time dependence of absorption spectra in the ambient environment (25<\/strong>\u2103<\/strong>, 40\u201350% relative humidity),<\/strong>\u00a0<\/strong>where two samples correspond to HT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0and VALT-CsPbIBr<\/strong>2<\/sub><\/strong>, respectively.<\/strong>\"\"<\/b><\/strong><\/p>\n

Figure 3. a) Schematic illustration and b) cross-sectional SEM image of VALT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0PSCs; c) J<\/strong>–<\/strong>V curves measured from the reverse direction, d) EQE<\/strong>\u00a0<\/strong>spectra coupled with J<\/strong>int<\/sub><\/strong>, e) steady-state output of PCE at the maximum power point, and f ) statistical histogram of PCE from 20 individual HT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0<\/sub><\/strong>PSCs and VALT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0PSCs, respectively.<\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

Figure 4. a) TPC, b) P<\/strong>light<\/sub><\/strong>\u00a0depended on J<\/strong>SC<\/sub><\/strong>, c) TPV, d) P<\/strong>light<\/sub><\/strong>\u00a0depended on V<\/strong>OC<\/sub><\/strong>, e) SCLC results of single-carrier devices with the structure of ITO\/ZnO\/CsPbIBr<\/strong>2<\/sub><\/strong>\/PCBM\/Ag, and f ) Mott<\/strong>–<\/strong>Schottky curves of PSCs based on HT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0and VALT-CsPbIBr<\/strong>2<\/sub><\/strong>,<\/strong>\u00a0<\/strong>respectively.<\/strong><\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

Figure 5. Time-dependent variations of normalized PCE of the unencapsulation HT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0PSCs and VALT-CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0PSCs a) storing in the ambient<\/strong>\u00a0<\/strong>environment (25<\/strong>–<\/strong>28<\/strong>\u2103<\/strong>, 50% relative humidity) and b) continuously heated at 80 <\/strong>\u2103<\/strong>\u00a0in the glovebox (H<\/strong>2<\/sub><\/strong>O < 1 ppm, O<\/strong>2<\/sub><\/strong>\u00a0< 1 ppm), respectively; photovoltaic parameters and fabrication parameters of CsPbIBr<\/strong>2<\/sub><\/strong>\u00a0PSCs via different methods, where c) plots of PCE against Voc, d) plots of FF against PCE,<\/strong>\u00a0<\/strong>e) plots of PCE against the temperature of ETL, and f ) plots of PCE against the temperature of the photoactive layer<\/strong><\/p>\n

\u6cb3\u5357\u5927\u5b66\u4e3a\u8bba\u6587\u7b2c\u4e00\u5b8c\u6210\u5355\u4f4d\uff0c\u7855\u58eb\u751f\u9ec4\u519b\u610f<\/b><\/strong>\u548c\u4f55\u76db\u534e<\/b><\/strong>\u4e3a\u7b2c\u4e00\u8bba\u6587\u5171\u540c\u4f5c\u8005\uff0c\u9ad8\u8dc3\u5cb3\u526f\u6559\u6388\u4e3a\u7b2c\u4e00\u901a\u8baf\u4f5c\u8005\uff0c\u6cb3\u5357\u5927\u5b66\u5cb3\u6839\u7530\u526f\u6559\u6388\u548c\u9f50\u9f50\u54c8\u5c14\u5927\u5b66\u8463\u56fd\u534e<\/b><\/strong>\u526f\u6559\u6388<\/b><\/strong>\u4e3a\u8bba\u6587\u5171\u540c\u901a\u8baf\u4f5c\u8005\u3002\u6b64\u5916<\/b><\/strong>\uff0c\u8be5\u5de5\u4f5c\u53d7\u5230\u897f\u5317\u5de5\u4e1a\u5927\u5b66\u6d82\u7528\u5e7f\u526f\u6559\u6388\u7684<\/b><\/strong>\u5927\u529b<\/b><\/strong>\u6307\u5bfc<\/b><\/strong>\u4e0e\u652f\u6301\u3002<\/b><\/strong>\u7814\u7a76\u5de5\u4f5c\u53d7\u5230\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\u3001\u56fd\u5bb6\u535a\u58eb\u540e\u9762\u4e0a\u57fa\u91d1\u9879\u76ee\u3001\u6cb3\u5357\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u7b49\u8d44\u52a9\u3002<\/p>\n

\u3010\u5ef6\u4f38\u9605\u8bfb\u3011<\/b><\/strong><\/p>\n

\u9ad8\u8dc3\u5cb3<\/strong><\/p>\n

\u6cb3\u5357\u5927\u5b66\u5149\u4f0f\u6750\u6599\u7701\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u7814\u7a76\u5458\uff0c\u7855\u58eb\u751f\u5bfc\u5e08\uff0c\u6bd5\u4e1a\u4e8e\u54c8\u5c14\u6ee8\u5de5\u4e1a\u5927\u5b66\uff0c\u5e08\u4ece\u5f20\u52c7\u7814\u7a76\u5458\/\u6768\u7389\u6797\u6559\u6388\uff0c\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u6709\u673a\u592a\u9633\u80fd\u7535\u6c60\u3001\u5168\u65e0\u673a\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u3001\u67d3\u6599\u654f\u534e\u592a\u9633\u80fd\u7535\u6c60\u3002\u76ee\u524d\u4ee5\u7b2c\u4e00\u6216\u901a\u8baf\u4f5c\u8005\u5728Nano Energy\uff0cSmall\uff0cJournal of Materials Chemistry A\uff0cJournal of Materials Chemistry C\uff0cSolar RRL\uff0cMacromolecules\u7b49\u56fd\u9645SCI\u671f\u520a\u53d1\u8868\u8bba\u658715\u7bc7\u3002<\/p>\n

\u5cb3\u6839\u7530<\/strong><\/p>\n

\u6cb3\u5357\u5927\u5b66\u5149\u4f0f\u6750\u6599\u7701\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u7814\u7a76\u5458\uff0c\u7855\u58eb\u751f\u5bfc\u5e08\uff0c\u6bd5\u4e1a\u4e8e\u534e\u4fa8\u5927\u5b66\uff0c\u5e08\u4ece\u5434\u5b63\u6000\u6559\u6388\uff0c\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u67d3\u6599\u654f\u534e\u592a\u9633\u80fd\u7535\u6c60\u3001\u8d85\u7ea7\u7535\u5bb9\u5668\u3002\u76ee\u524d\u4ee5\u7b2c\u4e00\u6216\u901a\u8baf\u4f5c\u8005\u5728Nano Energy,\u00a0Journal of Materials Chemistry A,\u00a0Journal of Physical Chemistry C, Electrochimica Acta\u7b49\u56fd\u9645SCI\u671f\u520a\u53d1\u8868\u8bba\u658740\u4f59\u7bc7\u3002<\/p>\n

\u8463\u56fd\u534e<\/strong><\/p>\n

\u9f50\u9f50\u54c8\u5c14\u5927\u5b66\u526f\u6559\u6388\uff0c\u7855\u58eb\u751f\u5bfc\u5e08\uff0c\u6bd5\u4e1a\u4e8e\u54c8\u5c14\u6ee8\u5de5\u4e1a\u5927\u5b66\uff0c\u5e08\u4ece\u6768\u7389\u6797\u6559\u6388\uff0c\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u65e0\u673a\u7eb3\u7c73\u6750\u6599\u5236\u5907\u53ca\u5149\u7535\u50ac\u5316\uff0c\u8584\u819c\u592a\u9633\u80fd\u7535\u6c60\u7684\u6027\u80fd\u4f18\u5316\uff0c\u751f\u7269\u8d28\u6750\u6599\u5e94\u7528\u529f\u80fd\u6027\u8f6c\u5316\u3002\u76ee\u524d\u5728Adv.Energy Mater., ACS Appl. Mater. Interfaces, Chemsuschem, Electrochemica Acta, Applied surface science\u7b49\u56fd\u9645SCI\u671f\u520a\u53d1\u8868\u8bba\u658720\u4f59\u7bc7\u3002<\/p>\n

\u6d82\u7528\u5e7f<\/strong><\/p>\n

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