{"id":242629,"date":"2022-10-10T07:16:58","date_gmt":"2022-10-09T23:16:58","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=242629"},"modified":"2022-10-09T15:17:37","modified_gmt":"2022-10-09T07:17:37","slug":"%e5%85%b3%e4%ba%8e%e6%b0%b4%ef%bc%8c%e4%bb%96%e4%bb%ac%e7%9a%84%e7%a0%94%e7%a9%b6%e5%8f%91%e8%a1%a8%e5%9c%a8nature%e4%b8%8a%ef%bc%81","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=242629","title":{"rendered":"\u5173\u4e8e\u6c34\uff0c\u4ed6\u4eec\u7684\u7814\u7a76\u53d1\u8868\u5728Nature\u4e0a\uff01"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

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\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

2022\u5e749\u670814\u65e5\uff0c\u82f1\u56fd\u5251\u6865\u5927\u5b66<\/strong>Angelos Michaelides<\/strong>\u6559\u6388\u56e2\u961f<\/strong>\u7ed3\u5408\u4e86\u4e00\u7cfb\u5217\u8ba1\u7b97\u65b9\u6cd5\uff0c\u5b9e\u73b0\u4e86\u5bf9\u7c7b\u77f3\u58a8\u70ef\u901a\u9053\u5185\u5355\u5c42\u6c34\u7684\u7b2c\u4e00\u6027\u539f\u7406\u7814\u7a76\u3002\u7814\u7a76\u8868\u660e\uff0c\u5355\u5c42\u6c34\u8868\u73b0\u51fa\u60ca\u4eba\u7684\u4e30\u5bcc\u591a\u6837\u7684\u76f8\u884c\u4e3a\uff0c\u5bf9\u6e29\u5ea6\u548c\u4f5c\u7528\u5728\u7eb3\u7c73\u901a\u9053\u5185\u7684\u8303\u5fb7\u534e\u538b\u529b\u9ad8\u5ea6\u654f\u611f\u3002\u9664\u4e86\u7194\u5316\u6e29\u5ea6\u968f\u538b\u529b\u975e\u5355\u8c03\u53d8\u5316\u8d85\u8fc7400 K\u7684\u591a\u4e2a\u5206\u5b50\u76f8\u4e4b\u5916\uff0c\u7814\u7a76\u4eba\u5458\u8fd8\u9884\u6d4b\u4e86\u516d\u8fb9\u5f62\u76f8\uff0c\u8fd9\u662f\u4e00\u79cd\u4ecb\u4e8e\u56fa\u4f53\u548c\u6db2\u4f53\u4e4b\u95f4\u7684\u4e2d\u95f4\u76f8\uff0c\u4ee5\u53ca\u5177\u6709\u8d85\u8fc7\u7535\u6c60\u6750\u6599\u7684\u9ad8\u7535\u5bfc\u7387\u7684\u8d85\u79bb\u5b50\u76f8\u3002\u8fd9\u4e9b\u7814\u7a76\u8868\u660e\u7eb3\u7c73\u9650\u5236\u53ef\u80fd\u662f\u5728\u5bb9\u6613\u63a5\u8fd1\u7684\u6761\u4ef6\u4e0b\u5b9e\u73b0\u8d85\u7535\u5b50\u884c\u4e3a\u7684\u4e00\u6761\u6709\u5e0c\u671b\u7684\u9014\u5f84\u3002\u8be5\u8bba\u6587\u4ee5\u9898\u4e3a\u201cThe first-principles phase diagram of monolayer nanoconfined water\u201d<\/strong>\u53d1\u8868\u5728\u77e5\u540d\u671f\u520aNature<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/p>\n

1\u3001\u5728\u8303\u5fb7\u534e\u538b\u529b\u4ecb\u4e8e0.5-2.0 GPa\u4e4b\u95f4\u7684\u77f3\u58a8\u70ef\u5c42\u7ea6\u675f\u7684\u6761\u4ef6\u4e0b\uff0c\u5355\u5c42\u6c34\u5448\u73b0\u51fa\u65e2\u975e\u56fa\u4f53\u4e5f\u975e\u6db2\u4f53\u7684\u76f8\u2014\u516d\u8fb9\u5f62\u76f8\u3002<\/p>\n

2\u3001\u57284 GPa\u548c400k\u4ee5\u4e0a\uff0c\u8d85\u8fc710%\u7684\u6c34\u5206\u5b50\u5728100ps\u5185\u5728\u5355\u5c42\u6c34\u4e2d\u89e3\u79bb\uff0c\u5355\u5206\u5b50\u5c42\u6c34\u76f8\u7684\u7535\u5bfc\u7387\u9ad8\u4e8e0.1 S cm-1<\/sup>\uff08\u8d85\u79bb\u5b50\u76f8\u9608\u503c\uff09\u3002<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u56fe<\/strong>1<\/strong>\u5355\u5c42\u7eb3\u7c73\u627f\u538b\u6c34\u7684\u76f8\u56fe<\/strong> \u00a9 2022 Springer Nature<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\uff08a-g\uff09\u4f7f\u7528\u5177\u6709\u7b2c\u4e00\u6027\u539f\u7406\u51c6\u786e\u6027\u7684MLP\u8ba1\u7b97\u7684\u5355\u5c42\u6c34\u7684\u538b\u529b-\u6e29\u5ea6\u76f8\u56fe\u3002<\/p>\n

\u56fe<\/strong>2<\/strong>\u4e2d\u7b49\u538b\u529b\u4e0b\u5355\u5c42\u6c34\u7684\u516d\u8fb9\u5f62\u76f8<\/strong> \u00a9 2022 Springer Nature<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a-b\uff09\u4e0d\u540c\u6e29\u5ea6\u4e0b\u6c27\u539f\u5b50\u7684\u6a2a\u5411\u5206\u5e03\u51fd\u6570g(r)\u4e0e\u52bf\u80fdU\u548c\u6269\u6563\u7cfb\u6570D\u57280.5 GPa\u65f6\u968f\u6e29\u5ea6\u7684\u51fd\u6570\u5173\u7cfb\uff0c\u8868\u660e\u53d1\u751f\u4e00\u7ea7\u76f8\u53d8\u3002<\/p>\n

\uff08c-d\uff09\u4e0d\u540c\u6e29\u5ea6\u4e0b\u6c27\u539f\u5b50\u7684\u6a2a\u5411\u5206\u5e03\u51fd\u6570g(r)\u4e0e\u52bf\u80fd(\u9ed1\u8272)\u548c\u6269\u6563\u7cfb\u6570\u57281.0 GPa\u65f6\u968f\u6e29\u5ea6\u7684\u51fd\u6570\u5173\u7cfb\uff0c\u8868\u660e\u4e00\u9636\u76f8\u8f6c\u53d8\u4e3a\u516d\u8fb9\u5f62\u76f8\uff0c\u8fde\u7eed\u76f8\u8f6c\u53d8\u4e3a\u6db2\u76f8\u3002<\/p>\n

\uff08e\uff09\u7b2c\u4e00\u6c34\u5408\u58f3\u4e2d\u7684\u6c27\u539f\u5b50\uff08\u7ea2\u8272\uff09\u548c\u952e\u5408\u6c22\u539f\u5b50\uff08\u9ed1\u8272\uff09\u76f8\u5bf9\u4e8e\u6c27\u539f\u5b50\u5728300-600 K\u30011\u2009GPa\u7684\u6e29\u5ea6\u4f9d\u8d56\u7a7a\u95f4\u5206\u5e03\u2009\u3002<\/p>\n

\uff08f\uff09\u6e29\u5ea6\u4f9d\u8d56\u6027\u7684\u7ed3\u6784\u56e0\u5b50\uff0c\u8868\u660e\u5728400 K\u65f6\u516d\u8fb9\u5f62\u76f8\u4e2d\u5931\u53bb\u4e86\u5e73\u52a8\u987a\u5e8f\uff0c\u4ee5\u53ca\u57281.0 GPa\u3001600 K\u65f6\u6db2\u4f53\u4e2d\u7684\u5b9a\u5411\u987a\u5e8f\u635f\u5931\u3002<\/p>\n

\u56fe<\/strong>3<\/strong>\u9ad8\u538b\u4e0b\u7684\u8d85\u79bb\u5b50\u884c\u4e3a<\/strong> \u00a9 2022 Springer Nature<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u5728100ps\u5185\uff0c\u4e0d\u540c\u538b\u529b\u4e0b\u5355\u5206\u5b50\u5c42\uff08\u5706\u5708\uff09\u548c\u51b0\u5757\uff08\u865a\u7ebf\uff09\u4e2d\u6e38\u79bbOH\u952e\u7684\u767e\u5206\u6bd4\u7684\u6e29\u5ea6\u4f9d\u8d56\u6027\u3002<\/p>\n

\uff08b\uff09\u5355\u5c42\u6c34\u57284 GPa\u5904\u7684\u6e29\u5ea6\u4f9d\u8d56\u6027\u79bb\u5b50\u7535\u5bfc\u7387\u3002<\/p>\n

\uff08c\uff09\u76f8\u5bf9\u4e8e\u4efb\u610f\u9009\u62e9\u7684\u6c27\u539f\u5b50\u7684\u6c27\u539f\u5b50\u7684\u7a7a\u95f4\u5206\u5e03\uff08\u7ea2\u8272\uff09\uff0c\u4ee5\u53ca\u5728600 K\u548c4 GPa\u5904\u5355\u4e2a\u6c22\u539f\u5b50\uff08\u9ed1\u8272\uff09\u7684\u8f68\u8ff9\uff0c\u8868\u660e\u8d28\u5b50\u8f6c\u79fb\u5f88\u5bb9\u6613\u3002<\/p>\n

\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

\u7efc\u8ff0\u6240\u8ff0\uff0c\u7814\u7a76\u4eba\u5458\u4ee5\u7b2c\u4e00\u6027\u539f\u7406\u7cbe\u786e\u5730\u9884\u6d4b\u4e86\u5355\u5c42\u627f\u538b\u6c34\u7684\u538b\u529b\u2014\u6e29\u5ea6\u76f8\u56fe\uff0c\u4ece\u4f4e\u6e29\u548c\u538b\u529b\u4e00\u76f4\u5230\u6c34\u7684\u89e3\u79bb\u72b6\u6001\u3002\u901a\u8fc7\u6e29\u5ea6\u2014\u538b\u529b\u76f8\u56fe\u5bf9\u7eb3\u7c73\u627f\u538b\u6c34\u7684\u590d\u6742\u884c\u4e3a\u8fdb\u884c\u4e86\u5168\u9762\u7684\u63cf\u8ff0\uff0c\u4e3a\u672a\u6765\u7684\u5b9e\u9a8c\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\uff0c\u5e76\u4e3a\u7eb3\u7c73\u6280\u672f\u80cc\u666f\u4e0b\u7684\u5408\u7406\u6750\u6599\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u4e00\u4e2a\u8d77\u70b9\u3002\u7b26\u5408KTHNY\u7406\u8bba\u7684\u4e24\u6b65\u7194\u5316\u673a\u5236\u548c\u516d\u8fb9\u5f62\u76f8\u7684\u5b58\u5728\u63d0\u4f9b\u4e86\u65b0\u7684\u7269\u7406\u89c1\u89e3\uff0c\u8bf4\u660e\u6c34\u5728\u7eb3\u7c73\u5c3a\u5ea6\u4e0a\u7684\u7194\u5316\u4e0d\u4e00\u5b9a\u662f\u4e00\u9636\u7684\uff0c\u8fd9\u53ef\u80fd\u5bf9\u7eb3\u7c73\u7cfb\u7edf\u7684\u70ed\u5de5\u7a0b\u6709\u76f4\u63a5\u7684\u5f71\u54cd\u3002\u7eb3\u7c73\u7ea6\u675f\u6761\u4ef6\u4e0b\u6c34\u89e3\u79bb\u589e\u5f3a\u7684\u8bc1\u636e\u4e3a\u5408\u7406\u89e3\u91ca\u7eb3\u7c73\u7ea6\u675f\u6c34\u7684\u53cd\u5e38\u6027\u8d28\u63d0\u4f9b\u4e86\u57fa\u7840\uff0c\u4f8b\u5982\uff0ch-BN2<\/sup>\u4e2d\u6c34\u6d41\u7684\u4f4e\u6ed1\u79fb\u53ef\u4ee5\u7406\u89e3\u4e3a\u7eb3\u7c73\u7ea6\u675f\u6c34\u4e2dO-H\u89e3\u79bb\u503e\u5411\u589e\u5f3a\u7684\u57fa\u7840\u3002\u6b64\u5916\uff0c\u8d85\u79bb\u5b50\u7eb3\u7c73\u627f\u538b\u6c34\u7684\u9ad8\u5bfc\u7535\u6027\u53ef\u7528\u4e8e\u6c34\u6eb6\u6db2\u7535\u89e3\u8d28\u7684\u5f00\u53d1\u3002\u672c\u7814\u7a76\u8868\u660e\uff0c\u7eb3\u7c73\u9650\u5236\u53ef\u80fd\u662f\u5728\u5bb9\u6613\u63a5\u8fd1\u7684\u6761\u4ef6\u4e0b\u68c0\u67e5\u8d85\u79bb\u5b50\u6750\u6599\u7684\u4e00\u6761\u9014\u5f84\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aThe first-principles phase diagram of monolayer nanoconfined water <\/a>( Naure <\/em>2022<\/strong>, 609<\/em>, 512-516)<\/p>\n","protected":false},"excerpt":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011 \u5bf9\u4e8e\u6c34\u7684\u5404\u79cd\u7279\u6027\uff0c\u6211\u4eec\u5df2\u7ecf\u4e86\u82e5\u6307\u638c\u3002\u7136\u800c\u5bf9\u7eb3\u7c73\u7ea7\u7a7a\u8154\u4e2d\u7684\u6c34\u5374\u6bd4\u8f83\u964c\u751f\uff0c\u8fd9\u4e9b\u6c34\u5bf9\u4e8e\u5730\u8d28\u5b66\u4ee5\u53ca\u751f\u7269\u5b66\u4e2d\u7684\u65e5\u5e38\u73b0\u8c61\u81f3\u5173\u91cd\u8981\u3002\u7eb3\u7c73\u5c3a\u5ea6\u6c34\u7684\u6027\u8d28\u53ef\u4ee5\u4e0e\u65e5\u5e38\u6c34…<\/p>\n","protected":false},"author":35234,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[2],"tags":[],"class_list":["post-242629","post","type-post","status-publish","format-standard","hentry","category-keji"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/242629"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/35234"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=242629"}],"version-history":[{"count":2,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/242629\/revisions"}],"predecessor-version":[{"id":243110,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/242629\/revisions\/243110"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=242629"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=242629"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=242629"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}