{"id":242882,"date":"2022-10-14T07:53:03","date_gmt":"2022-10-13T23:53:03","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=242882"},"modified":"2022-10-13T16:53:11","modified_gmt":"2022-10-13T08:53:11","slug":"%e8%a7%a3%e5%86%b3%e5%8d%95%e5%8e%9f%e5%ad%90%e5%82%ac%e5%8c%96%e5%89%82%e5%b7%a5%e4%b8%9a%e5%8c%96%e5%88%b6%e5%a4%87%e9%9a%be%e9%a2%98%ef%bc%9fnat-commun%ef%bc%9a%e9%87%87%e7%94%a8%e5%89%8d%e4%bd%93","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=242882","title":{"rendered":"\u89e3\u51b3\u5355\u539f\u5b50\u50ac\u5316\u5242\u5de5\u4e1a\u5316\u5236\u5907\u96be\u9898\uff1fNat. Commun\uff1a\u91c7\u7528\u524d\u4f53\u96fe\u5316\u7b56\u7565\u5efa\u7acb\u5355\u539f\u5b50\u50ac\u5316\u5242\u5e93\u548c\u751f\u4ea7\u7ebf"},"content":{"rendered":"

\u89e3\u51b3\u5355\u539f\u5b50\u50ac\u5316\u5242\u5de5\u4e1a\u5316\u5236\u5907\u96be\u9898\uff1f<\/strong>Nat. Commun<\/em><\/strong>\uff1a\u91c7\u7528\u524d\u4f53\u96fe\u5316\u7b56\u7565\u5efa\u7acb\u5355\u539f\u5b50\u50ac\u5316\u5242\u5e93\u548c\u751f\u4ea7\u7ebf<\/strong><\/p>\n

lwb<\/strong><\/p>\n

01<\/strong>\u3001\u5bfc\u8bfb<\/strong><\/p>\n

\u5355\u539f\u5b50\u50ac\u5316\u5242\uff08SAC\uff09\u662f\u4e00\u7c7b\u5f88\u6709\u524d\u9014\u7684\u6750\u6599\uff0c\u5b83\u7ed3\u5408\u4e86\u5747\u76f8\u50ac\u5316\u5242\u548c\u975e\u5747\u76f8\u50ac\u5316\u5242\u7684\u4f18\u70b9\uff0c\u5728\u5b9e\u9645\u5e94\u7528\u4e2d\u663e\u793a\u51fa\u4f18\u5f02\u7684\u50ac\u5316\u6027\u80fd\uff0c\u5305\u62ec\u9ad8\u4ef7\u503c\u5316\u5b66\u54c1\u751f\u4ea7\u3001\u80fd\u91cf\u8f6c\u6362\u548c\u6d88\u9664\u6c61\u67d3\u3002\u7136\u800c\uff0c\u4eba\u4eec\u666e\u904d\u8ba4\u4e3aSACs\u4ecd\u6709\u8bb8\u591a\u672a\u77e5\u4e4b\u5904\u6709\u5f85\u63a2\u7d22\uff0c\u5305\u62ec\u53d1\u73b0\u72ec\u7279\u7684\u50ac\u5316\u6027\u80fd\uff0c\u7406\u89e3\u7ed3\u6784-\u6027\u80fd\u5173\u7cfb\u4ee5\u53ca\u5b9e\u73b0\u5de5\u4e1a\u5e94\u7528\u3002\u8fdb\u4e00\u6b65\u7814\u7a76SACs\u7684\u5148\u51b3\u6761\u4ef6\u662f\u5f00\u53d1\u7075\u6d3b\u548c\u53ef\u6269\u5c55\u7684\u5236\u5907\u65b9\u6cd5\uff0c\u4f46\u8fd9\u4ecd\u7136\u662f\u4e00\u4e2a\u5de8\u5927\u7684\u6311\u6218\u3002\u9996\u5148\uff0c\u5236\u5b9a\u4e00\u79cd\u901a\u7528\u7684\u8def\u7ebf\u6765\u5236\u9020\u5177\u6709\u4e0d\u540c\u91d1\u5c5e\u4f4d\u70b9\u548c\u8f7d\u4f53\u7684\u5404\u79cdSACs\u662f\u975e\u5e38\u56f0\u96be\u7684\uff0c\u56e0\u4e3a\u5b83\u4eec\u5177\u6709\u660e\u663e\u4e0d\u540c\u7684\u7269\u7406\/\u5316\u5b66\u6027\u8d28\uff0c\u5305\u62ec\u4f46\u4e0d\u9650\u4e8e\u91d1\u5c5e\u524d\u9a71\u4f53\u7684\u6eb6\u89e3\u5ea6\u3001\u70ed\u7a33\u5b9a\u6027\uff0c\u4ee5\u53ca\u8868\u9762\u914d\u4f4d\u73af\u5883\u548c\u8f7d\u4f53\u7684\u4eb2\u758f\u6c34\u6027\u7b49\u3002\u5176\u6b21\u662f\u89c4\u6a21\u5316\u6548\u5e94\u4e25\u91cd\u963b\u788dSACs\u7684\u6279\u91cf\u751f\u4ea7\u3002\u91c7\u7528\u5e38\u7528\u7684\u6e7f\u5316\u5b66\u65b9\u6cd5\u5bf9\u91d1\u5c5e\u79cd\u7c7b\u7684\u805a\u96c6\u72b6\u6001\u6709\u663e\u8457\u5f71\u54cd\u3002\u5c3d\u7ba1\u8fd9\u4e9b\u6761\u4ef6\u5728\u5b9e\u9a8c\u5ba4\u89c4\u6a21\u4e0a\u53ef\u4ee5\u5f88\u597d\u5730\u63a7\u5236\uff0c\u4f46\u5728\u5de5\u5382\u89c4\u6a21\u4e0a\u51e0\u4e4e\u4e0d\u53ef\u80fd\u5b9e\u73b0\uff0c\u56e0\u4e3a\u4e0d\u53ef\u907f\u514d\u7684\u4f20\u8d28\u548c\u4f20\u70ed\u4e0d\u5747\u5300\uff0c\u4f1a\u5bfc\u81f4\u5c40\u90e8\u6d53\u5ea6\u8fc7\u9ad8\uff0c\u4ece\u800c\u4ea7\u751f\u4e0d\u5e0c\u671b\u7684\u91d1\u5c5e\u79cd\u7c7b\u805a\u96c6\uff0c\u4e00\u79cd\u89e3\u51b3\u65b9\u6cd5\u662f\u91c7\u7528\u8fde\u7eed\u7684\u5236\u5907\u65b9\u6cd5(\u968f\u65f6\u95f4\u589e\u52a0\u4ea7\u91cf)\u6765\u4ee3\u66ff\u76ee\u524d\u7684\u6279\u91cf\u5236\u5907\u65b9\u6cd5\uff0c\u4f46\u76f8\u5173\u62a5\u9053\u975e\u5e38\u5c11\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u4e00\u79cd\u901a\u7528\u3001\u8fde\u7eed\u548c\u76f4\u63a5\u7684\u65b9\u6cd5\u6765\u5236\u9020SACs\u662f\u79d1\u5b66\u548c\u6280\u672f\u4e0a\u7684\u5f53\u52a1\u4e4b\u6025\u3002<\/p>\n

02<\/strong>\u3001\u6210\u679c\u63a0\u5f71<\/strong><\/p>\n

\u5728\u6b64\uff0c\u4e2d\u5c71\u5927\u5b66\u7eaa\u7ea2\u5175\u6559\u6388\u56e2\u961f\u8054\u5408\u5317\u4eac\u5927\u5b66\u9a6c\u4e01\u6559\u6388\u56e2\u961f\u62a5\u9053\u4e86\u4e00\u79cd\u7528\u4e8e\u5408\u6210SACs\u53ca\u5176\u884d\u751f\u7269\u7684\u524d\u4f53\u96fe\u5316\u7b56\u7565\uff0c\u6574\u4e2a\u5236\u5907\u8fc7\u7a0b\u53ea\u5305\u62ec\u4e24\u4e2a\u6b65\u9aa4\uff1a\u7b2c\u4e00\u6b65\uff0c\u524d\u4f53\u7684\u7a00\u6eb6\u6db2\u88ab\u539f\u5b50\u5316\u5e76\u55b7\u5230\u652f\u67b6\u4e0a\uff1b\u7b2c\u4e8c\u6b65\uff0c\u5bf9\u4e0a\u8ff0\u6837\u54c1\u8fdb\u884c\u70ed\u5904\u7406\u5206\u89e3\u524d\u9a71\u4f53\uff0c\u5f97\u5230\u76f8\u5e94\u7684SACs\uff1b\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8be5\u65b9\u6cd5\u9002\u7528\u4e8e\u6210\u529f\u5408\u6210\u4e00\u7cfb\u5217\u50ac\u5316\u5242\uff0c\u53ef\u4ee5\u4e3a\u5404\u79cd\u4e0d\u540c\u7684\u91d1\u5c5e\u652f\u6491\u7ec4\u5408\u5efa\u7acbSACs\u5e93\uff0c\u5305\u62ec19\u4e2a\u5177\u6709\u4e0d\u540c\u91d1\u5c5e\u4f4d\u70b9\u548c\u8f7d\u4f53\u7684SACs\u548c3\u79cdSACs\u884d\u751f\u7269\uff08\u5355\u539f\u5b50\u5408\u91d1\uff0c\u53cc\u539f\u5b50\u50ac\u5316\u5242\u548c\u53cc\u91d1\u5c5eSACs\uff09\u3002\u6b64\u5916\uff0c\u8be5\u5408\u6210\u8def\u7ebf\u53ef\u4ee5\u901a\u8fc7\u81ea\u5236\u76841\u516c\u65a4\/\u5929\u7684\u751f\u4ea7\u7ebf\u8fdb\u884c\u653e\u5927\uff0c\u5e76\u4e14\u5728Suzuki-Miyaura\u4ea4\u53c9\u8026\u5408\u8fc7\u7a0b\u4e2d\u5177\u6709\u76f8\u540c\u7684\u8868\u5f81\u7ed3\u679c\u548c\u50ac\u5316\u6027\u80fd\uff0c\u8fd9\u8bc1\u660e\u4e86\u8be5\u5de5\u4e1a\u5408\u6210\u8fc7\u7a0b\u5177\u6709\u826f\u597d\u7684\u50ac\u5316\u5242\u5747\u5300\u6027\u63a7\u5236\u3002\u8be5\u7b56\u7565\u4e3aSACs\u7684\u8fdb\u4e00\u6b65\u7814\u7a76\u5960\u5b9a\u4e86\u57fa\u7840\uff0c\u5e76\u53ef\u80fd\u52a0\u5febSACs\u4ece\u57fa\u7840\u7814\u7a76\u5411\u5de5\u4e1a\u5e94\u7528\u7684\u8f6c\u53d8\u3002<\/p>\n

\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cBuilding up libraries and production line for single atom catalysts with precursor-atomization strategy<\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Communications<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

03<\/strong>\u3001\u6838\u5fc3\u521b\u65b0\u70b9<\/strong><\/p>\n

1\u3001\u524d\u4f53\u96fe\u5316\u7b56\u7565\u9002\u7528\u4e8e\u6210\u529f\u5408\u6210\u4e00\u7cfb\u5217\u50ac\u5316\u5242\uff0c\u53ef\u4ee5\u4e3a\u5404\u79cd\u4e0d\u540c\u7684\u91d1\u5c5e\u652f\u6491\u7ec4\u5408\u5efa\u7acbSACs\u5e93\uff0c\u5305\u62ec19\u4e2a\u5177\u6709\u4e0d\u540c\u91d1\u5c5e\u4f4d\u70b9\u548c\u8f7d\u4f53\u7684SACs\u548c3\u79cdSACs\u884d\u751f\u7269\u3002<\/p>\n

2\u3001\u524d\u4f53\u96fe\u5316\u7b56\u7565\u5728SACs\u7684\u6279\u91cf\u751f\u4ea7\u4e2d\u5177\u6709\u5f88\u5927\u7684\u6f5c\u529b\uff0cPd1<\/sub>\/FeOx<\/sub>\u5728\u81ea\u5236\u7684\u751f\u4ea7\u7ebf\u4e0a\u751f\u4ea7\u529b\u53ef\u4ee5\u8fbe\u52301\u516c\u65a4\/\u5929\u3002<\/p>\n

04<\/strong>\u3001\u6570\u636e\u6982\u89c8<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>1 Pd1<\/sub>\/FeOx<\/sub><\/strong>\u7684\u5236\u5907\u53ca\u7ed3\u6784\u8868\u5f81<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

\uff08a\uff09\u524d\u9a71\u4f53\u96fe\u5316\u7b56\u7565\u5236\u5907Pd1<\/sub>\/FeOx<\/sub>\u7684\u65b9\u6848\uff1b<\/p>\n

\uff08b\uff09Pd1<\/sub>\/FeOx<\/sub>\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09Pd1<\/sub>\/FeOx<\/sub>\u7684\u5143\u7d20\u6620\u5c04\uff1b<\/p>\n

\uff08d\uff09Pd1<\/sub>\/FeOx<\/sub>\u7684AC HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff09Pd1<\/sub>\/FeOx<\/sub>\uff0c\u672a\u7145\u70e7Pd1<\/sub>\/FeOx<\/sub>\uff0cPdO\u548cPd\u7b94\u7684Pd K-edge EXAFS\u7684k3<\/sup>-\u52a0\u6743FT\u8c31\uff1b<\/p>\n

\uff08f\uff09Pd K-edge EXAFS\u7528\u4e8ePd1<\/sub>\/FeOx<\/sub>\uff0cPdO\u548cPd\u7b94\uff1b<\/p>\n

\uff08g\uff09\u672a\u7145\u70e7Pd1<\/sub>\/FeOx<\/sub>\u7684AC HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>2 <\/strong>\u524d\u4f53\u96fe\u5316\u7b56\u7565\u7684\u666e\u904d\u6027<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>3 SACs<\/strong>\u884d\u751f\u7269\u7684\u5236\u5907\u4e0e\u7ed3\u6784\u8868\u5f81<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

\uff08a-d\uff09 Pd1<\/sub>\/Cu\u7684AC HAADF-STEM\u56fe\u50cf\u3001\u5143\u7d20\u6620\u5c04\u3001FT-EXAFS\u548cXANES Pd k-edge\uff1b<\/p>\n

\uff08e-h\uff09 AC HAADF-STEM\u56fe\u50cf\uff0c\u5728\u6807\u8bb0\u4e3a1-3\u7684\u533a\u57df\u83b7\u5f97\u7684\u5f3a\u5ea6\u5206\u5e03\uff0cFT-EXAFS\uff0cPd2<\/sub>\/FeOx<\/sub>\u7684Pd K-edge XANES\u5149\u8c31\uff1b<\/p>\n

\uff08i-l\uff09 Pd1<\/sub>-Pt1<\/sub>\/FeOx<\/sub>\u7684AC HAADF-STEM\u56fe\u50cf\u3001\u5143\u7d20\u6620\u5c04\u548cPd K-edge FT-EXAFS\u5149\u8c31\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe5<\/strong>\u00a0<\/strong>\u57fa\u4e8e\u524d\u9a71\u4f53\u96fe\u5316\u7b56\u7565\u7684\u751f\u4ea7\u7ebf<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

\uff08a\uff09 \u57fa\u4e8e\u524d\u4f53\u96fe\u5316\u7b56\u7565\u7684\u751f\u4ea7\u7ebf\u65b9\u6848\uff1b<\/p>\n

\uff08b-e\uff09 Pd1<\/sub>\/FeOx<\/sub>-1,2,3,4\u7684AC HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09 Pd1<\/sub>\/FeOx<\/sub>-1\u548c4\u3001PdO\u548cPd\u7b94\u7684Pd K-edge XANES\u7684k3<\/sup>-\u52a0\u6743FT\u5149\u8c31\uff1b<\/p>\n

\uff08g\uff09 Pd1<\/sub>\/FeOx<\/sub>-1,4\u3001PdO\u548cPd\u7b94K-edge XANES\u7684WT\uff1b<\/p>\n

\uff08h\uff09 Pd1<\/sub>\/FeOx<\/sub>-1\u548c4\u3001PdO\u548cPd\u7b94\u7684Pd K-edge XANES\uff1b<\/p>\n

\uff08i\uff09 Pd1<\/sub>\/FeOx<\/sub>-1,2,3,4\u7684Pd 3d\u7684XPS\u6a21\u5f0f\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe6<\/strong>\u00a0Pd1<\/sub>\/FeOx<\/sub><\/strong>\u5728<\/strong>Suzuki\u2013Miyaura<\/strong>\u4ea4\u53c9\u5076\u8054\u53cd\u5e94\u4e2d\u7684\u50ac\u5316\u6027\u80fd<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

\uff08a,b\uff09 Suzuki\u2013Miyaura\u4ea4\u53c9\u5076\u8054\u5206\u522b\u753119\u79cdSACs\u548c\u4e0d\u540c\u7684\u5546\u7528\u94af\u50ac\u5316\u5242\u50ac\u5316\uff1b<\/p>\n

\uff08c\uff09 Pd1<\/sub>\/FeOx<\/sub>-1\u7684\u56de\u6536\u5b9e\u9a8c\uff1b<\/p>\n

\uff08d\uff09 Pd1<\/sub>\/FeOx<\/sub>-1,2,3,4\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u7684\u50ac\u5316\u6027\u80fd\uff1b<\/p>\n

\uff08e\uff09 \u4e0d\u540c\u78b1\u91d1\u5c5ePd1<\/sub>\/FeOx<\/sub>-1,2,3,4\u7684\u50ac\u5316\u6027\u80fd\uff1b<\/p>\n

\uff08f\uff09 Pd1<\/sub>\/FeOx<\/sub>-1,2,3,4\u5bf9\u5f62\u6210\u4e0d\u540c\u4ea7\u7269\u7684\u50ac\u5316\u6027\u80fd\uff1b<\/p>\n

\"\"<\/p>\n

\u56fe7<\/strong>\u00a0Pd1<\/sub>\/FeOx<\/sub>-1<\/strong>\u50ac\u5316\u82b3\u57fa\u6eb4\u548c\u82b3\u57fa\u787c\u9178\u7684<\/strong>Suzuki\u2013Miyaura<\/strong>\u4ea4\u53c9\u5076\u8054<\/strong> \u00a9 2022 The Author(s)<\/strong><\/p>\n

05<\/strong>\u3001\u6210\u679c\u542f\u793a<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u5de5\u4f5c\u5f00\u53d1\u4e86\u4e00\u79cd\u591a\u529f\u80fd\u524d\u4f53\u96fe\u5316\u7b56\u7565\uff0c\u53ef\u4ee5\u7cbe\u786e\u64cd\u4f5c\u548c\u6392\u5217\u539f\u5b50\uff0c\u4ece\u800c\u83b7\u5f97SACs\u5e93\uff08\u5305\u62ec19\u4e2aSACs\u4ee5\u53caSAAs\u3001DACs\u548c\u53cc\u91d1\u5c5eSACs\uff09\uff0c\u57fa\u672c\u6db5\u76d6\u4e86\u76ee\u524d\u5e7f\u6cdb\u5173\u6ce8\u7684SACs\u50ac\u5316\u5242\u7ed3\u6784\u3002\u6b64\u5916\uff0c\u8be5\u5de5\u4f5c\u8fd8\u5efa\u7acb\u4e86\u5927\u89c4\u6a21\u5408\u6210SACs\u7684\u751f\u4ea7\u7ebf\uff0c\u751f\u4ea7\u80fd\u529b\u53ef\u63d0\u9ad8\u52301\u516c\u65a4\/\u5929\u4ee5\u4e0a\u3002Pd1<\/sub>\/FeOx<\/sub>\u5728Suzuki-Miyaura\u4ea4\u53c9\u5076\u8054\u53cd\u5e94\u4e2d\u5177\u6709\u76f8\u540c\u7684\u50ac\u5316\u5242\u7ed3\u6784\u548c\u50ac\u5316\u6027\u80fd\uff0c\u5373\u4fbf\u751f\u4ea7\u7684\u6279\u6b21\u4e0d\u540c\uff0c\u5747\u8868\u73b0\u51fa\u663e\u8457\u7684\u91cd\u590d\u6027\uff0c\u56e0\u6b64\u8be5\u5de5\u4f5c\u5177\u6709\u5927\u89c4\u6a21\u5408\u6210SACs\u7684\u5de8\u5927\u6f5c\u529b\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Building up libraries and production line for single atom catalysts with precursor-atomization strategy<\/strong>\uff0c<\/strong>2022<\/strong>\uff0c<\/strong>https:\/\/doi.org\/10.1038\/s41467-022-33442-2<\/strong>\uff09<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"

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