{"id":245999,"date":"2023-01-24T06:00:32","date_gmt":"2023-01-23T22:00:32","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=245999"},"modified":"2023-01-25T23:12:38","modified_gmt":"2023-01-25T15:12:38","slug":"%e3%80%90%e5%b7%b2%e5%ae%a1%e3%80%91jacs%ef%bc%9amn%e6%8e%ba%e6%9d%82%e9%92%99%e9%92%9b%e7%9f%bf%e7%ba%b3%e7%b1%b3%e7%89%87%e7%9a%84%e8%87%aa%e6%97%8b%e6%9e%81%e5%8c%96%e5%ae%9e%e7%8e%b0%e6%9b%b4","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=245999","title":{"rendered":"JACS\uff1aMn\u63ba\u6742\u9499\u949b\u77ff\u7eb3\u7c73\u7247\u7684\u81ea\u65cb\u6781\u5316\u5b9e\u73b0\u66f4\u9ad8\u6548\u5149\u50ac\u5316CO2\u8fd8\u539f\uff01"},"content":{"rendered":"<p><strong>\u4e00\u3001\u5bfc\u8bfb<\/strong><\/p>\n<p>\u8fd1\u5e74\u6765\u5229\u7528\u592a\u9633\u80fd\u9a71\u52a8\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u5c06\u4e8c\u6c27\u5316\u78b3\u53d8\u4e3a\u71c3\u6599\u548c\u5316\u5b66\u54c1\u7684\u7b56\u7565\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\uff0c\u56e0\u4e3a\u5b83\u540c\u65f6\u89e3\u51b3\u4e86\u5168\u7403\u53d8\u6696\u95ee\u9898\u548c\u53ef\u518d\u751f\u80fd\u6e90\u95ee\u9898\u3002\u7136\u800c\uff0c\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u8fc7\u7a0b\u6d89\u53ca\u7f13\u6162\u7684\u591a\u7535\u5b50\u53cd\u5e94\u52a8\u529b\u5b66\uff0c\u6240\u4ee5\u592a\u9633\u80fd\u9a71\u52a8\u7684CO<sub>2<\/sub>\u8fd8\u539f\u8f6c\u5316\u6548\u7387\u8fdc\u4e0d\u80fd\u6ee1\u8db3\u5b9e\u9645\u5e94\u7528\u8981\u6c42\u3002\u5364\u5316\u7269\u9499\u949b\u77ff\u534a\u5bfc\u4f53\u662f\u4e00\u79cd\u65b0\u5174\u7684\u53ef\u6eb6\u6db2\u52a0\u5de5\u7684\u5149\u7535\u6750\u6599\uff0c\u8868\u73b0\u51fa\u5149\u5b66\u5438\u6536\u7cfb\u6570\u5927\uff0c\u6210\u672c\u4f4e\uff0c\u5e26\u9699\u53ef\u8c03\u8c10\uff0c\u6269\u6563\u957f\u5ea6\u957f\u548c\u8f7d\u6d41\u5b50\u5bff\u547d\u957f\u7b49\u4f18\u5f02\u7684\u7269\u7406\u6027\u80fd\u3002\u7531\u4e8e\u5364\u5316\u7269\u9499\u949b\u77ff\u56fa\u6709\u7684\u7279\u6027\uff0c\u5728\u592a\u9633\u80fd\u9a71\u52a8\u7684CO<sub>2<\/sub>\u8fd8\u539f\u6216\u6790\u6c22\u5149\u50ac\u5316\u5e94\u7528\u4e2d\u6709\u5de8\u5927\u6f5c\u529b\u3002<\/p>\n<p>\u201c\u81ea\u65cb\u201d\u662f\u7535\u5b50\u7684\u672c\u5f81\u7279\u6027\uff0c\u662f\u53ef\u4ee5\u63d0\u9ad8\u7535\u50ac\u5316\u5242\u548c\u5149\u50ac\u5316\u5242\u6027\u80fd\u7684\u53e6\u4e00\u4e2a\u91cd\u8981\u7535\u5b50\u81ea\u7531\u5ea6\u3002\u81ea\u65cb\u9009\u62e9\u88ab\u8ba4\u4e3a\u662f\u4fc3\u8fdb\u7535\u50ac\u5316\u6790\u6c27\u53cd\u5e94(OER)\u7684\u4e00\u79cd\u53ef\u80fd\u65b9\u6cd5\uff0c\u8be5\u53cd\u5e94\u6d89\u53ca\u4ece\u5355\u7ebf\u6001\u7269\u8d28(OH\u2212\u6216H<sub>2<\/sub>O)\u5f62\u6210\u4e09\u7ebf\u6001O<sub>2<\/sub>\u7684\u8fc7\u7a0b\u3002\u56e0\u6b64\uff0c\u6d3b\u6027\u50ac\u5316\u5242\u8868\u9762\u7684\u81ea\u65cb\u6781\u5316\u6709\u5229\u4e8e\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u6c27\u539f\u5b50\u7684\u5e73\u884c\u81ea\u65cb\u6392\u5217\u3002\u64cd\u7eb5\u81ea\u65cb\u6781\u5316\u7535\u5b50\u4e5f\u53ef\u80fd\u662f\u589e\u5f3a\u6750\u6599\u5149\u50ac\u5316\u6d3b\u6027\u7684\u6709\u6548\u7b56\u7565\u3002\u901a\u8fc7\u63a7\u5236\u91d1\u5c5e\u6c27\u5316\u7269\u4e2d\u91d1\u5c5e\u6216\u6c27\u7a7a\u4f4d\u7684\u6d53\u5ea6\u4ea7\u751f\u81ea\u65cb\u6781\u5316\u7535\u5b50\u53ef\u4ee5\u663e\u8457\u589e\u5f3a\u5176\u5149\u50ac\u5316\u6d3b\u6027\u3002\u7136\u800c\uff0c\u5c3d\u7ba1\u4ea7\u751f\u7a7a\u4f4d\u662f\u589e\u5f3a\u81ea\u65cb\u6781\u5316\u7535\u5b50\u7684\u6709\u6548\u65b9\u6cd5\uff0c\u4f46\u6750\u6599\u5185\u7684\u80fd\u9631\u548c\u7f3a\u9677\u7684\u5f62\u6210\u53ef\u80fd\u540c\u65f6\u963b\u788d\u8f7d\u6d41\u5b50\u7684\u6269\u6563\u548c\u4f20\u8f93\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u5c06\u78c1\u6027\u5143\u7d20\u63ba\u6742\u5230\u534a\u5bfc\u4f53\u4e2d\u53ef\u80fd\u662f\u53e6\u4e00\u79cd\u5728\u5149\u50ac\u5316\u4e2d\u64cd\u7eb5\u81ea\u65cb\u6781\u5316\u7535\u5b50\u800c\u4e0d\u4f1a\u8fc7\u5ea6\u727a\u7272\u6750\u6599\u7ed3\u6676\u5ea6\u7684\u6709\u6548\u7b56\u7565\u3002<\/p>\n<p><strong>\u4e8c\u3001\u6210\u679c\u63a0\u5f71<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c\u53f0\u6e7e\u5927\u5b66\u9648\u4fca\u7ef4\u548c\u53f0\u6e7e\u5e08\u8303\u5927\u5b66Chia-Chun Chen\u56e2\u961f\u901a\u8fc7\u63a7\u5236\u5364\u5316\u7269\u9499\u949b\u77ff\u7eb3\u7c73\u7247(NPLs)CsPbBr<sub>3<\/sub>\u4e2d\u81ea\u65cb\u6781\u5316\u7535\u5b50\uff0c\u663e\u8457\u63d0\u9ad8\u4e86CO<sub>2<\/sub>\u8fd8\u539f\u8f6c\u5316\u6548\u7387\u3002<\/p>\n<p>\u8be5\u9879\u5de5\u4f5c\u4e2d\uff0c\u4ee5\u63a7\u5236CsPbBr<sub>3<\/sub>\u4e2d\u63ba\u6742\u9530\u9633\u79bb\u5b50(Mn<sup>2+<\/sup>)\u5e76\u65bd\u52a0\u5916\u90e8\u78c1\u573a\u6765\u5c55\u5f00\u5b9e\u9a8c\u3002\u7ed3\u679c\u8868\u660e\u4e0e\u539f\u59cbCsPbBr<sub>3<\/sub> NPLs\u76f8\u6bd4\uff0cMn\u63ba\u6742CsPbBr<sub>3<\/sub> (Mn-CsPbBr<sub>3<\/sub>) NPLs\u7531\u4e8e\u63ba\u6742\u540e\u4ea7\u751f\u4e86\u81ea\u65cb\u6781\u5316\u7535\u5b50\uff0c\u5b9e\u73b0\u4e86\u66f4\u51fa\u8272\u7684\u5149\u50ac\u5316CO<sub>2<\/sub>RR\u3002\u5e76\u4e14\u5916\u52a0\u78c1\u573a\u53ef\u4ee5\u663e\u8457\u63d0\u9ad8MnCsPbBr<sub>3<\/sub> NPLs\u7684\u5149\u50ac\u5316CO<sub>2<\/sub>RR\u3002\u5728300 mT\u7684\u6c38\u78c1\u4f53\u4e0b\uff0cMnCsPbBr<sub>3<\/sub> NPLs\u7684\u5149\u50ac\u5316CO<sub>2<\/sub>RR\u6027\u80fd\u63d0\u9ad8\u4e865.7\u500d\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246000\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-16.png\" alt=\"\" width=\"1237\" height=\"411\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-16.png 1237w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-16-300x100.png 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-16-768x255.png 768w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-16-1024x340.png 1024w\" sizes=\"(max-width: 1237px) 100vw, 1237px\" \/><\/p>\n<p>\u76f8\u5173\u7814\u7a76\u5de5\u4f5c\u4ee5\u201c<strong>Spin-Polarized Photocatalytic CO2 Reduction of Mn-Doped<\/strong><\/p>\n<p><strong>Perovskite Nanoplates<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520a<em>Journal of the American Chemical Society<\/em>\u4e0a\u3002<\/p>\n<p><strong>\u4e09\u3001\u6838\u5fc3\u521b\u65b0<\/strong><\/p>\n<p>\u7814\u7a76\u8005\u4eec\u8bc1\u660e\u4e86\u901a\u8fc7\u63a7\u5236\u5364\u5316\u7269\u9499\u949b\u77ffCsPbBr<sub>3<\/sub>\u7eb3\u7c73\u677f(NPL)\u7684\u81ea\u65cb\u6781\u5316\u7535\u5b50\u53ef\u4ee5\u663e\u8457\u63d0\u9ad8\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u8f6c\u5316\u6548\u7387\u3002\u901a\u8fc7\u78c1\u5706\u4e8c\u8272\u8c31\u3001\u8d85\u5feb\u77ac\u6001\u5438\u6536\u8c31\u548c\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u6a21\u62df\uff0c\u7cfb\u7edf\u5730\u7814\u7a76\u4e86\u5176\u673a\u7406\uff0cMn-CsPbBr<sub>3<\/sub> NPLs\u5149\u50ac\u5316CO<sub>2<\/sub>RR\u6548\u7387\u63d0\u9ad8\u7684\u539f\u56e0\u662f\u78c1\u6027\u63ba\u6742\u548c\u65bd\u52a0\u78c1\u573a\u589e\u52a0\u4e86\u81ea\u65cb\u6781\u5316\u8f7d\u6d41\u5b50\u7684\u6570\u91cf\uff0c\u4ece\u800c\u5ef6\u957f\u4e86\u8f7d\u6d41\u5b50\u5bff\u547d\u5e76\u6291\u5236\u4e86\u7535\u8377\u590d\u5408\u3002\u7ed3\u679c\u8868\u660e\uff0c\u64cd\u7eb5\u5149\u50ac\u5316\u534a\u5bfc\u4f53\u4e2d\u7684\u81ea\u65cb\u6781\u5316\u7535\u5b50\u662f\u4e00\u79cd\u63d0\u9ad8\u5149\u50ac\u5316CO<sub>2<\/sub>RR\u6548\u7387\u7684\u6709\u6548\u65b9\u6cd5\u3002<\/p>\n<p><strong>\u00a0<\/strong><\/p>\n<p><strong>\u56db\u3001\u6570\u636e\u6982\u89c8<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246001\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-16.png\" alt=\"\" width=\"607\" height=\"693\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-16.png 607w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-16-263x300.png 263w\" sizes=\"(max-width: 607px) 100vw, 607px\" \/><\/p>\n<p><strong>\u56fe1 CsPbBr<sub>3<\/sub> \u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5f62\u8c8c\u548c\u7ed3\u6784\u8868\u5f81\u3002 <\/strong>\u00a9 2022 American Chemical Society<\/p>\n<p>(a) \u5728 3D \u5168\u65e0\u673a\u9499\u949b\u77ffCsPbBr<sub>3<\/sub> \u4e2d\u63ba\u6742\u78c1\u6027 Mn<sup>2+ <\/sup>\u79bb\u5b50\u5f62\u6210\u7535\u5b50\u81ea\u65cb\u6781\u5316\u7684\u793a\u610f\u56fe\u3002(b) CsPbBr<sub>3<\/sub> \u548c (c) Mn-CsPbBr<sub>3 <\/sub>NPLs \u7684 TEM \u56fe\u50cf\u3002\u63d2\u56fe\u662f CsPbBr<sub>3<\/sub>\u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u7684HR-TEM \u56fe\u50cf\u3002(d) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684 HAADF-STEM \u548c EDS \u5143\u7d20mapping\uff08Mn\u3001Cs\u3001Pb \u548c Br\uff09\u56fe\u50cf\u3002(e) CsPbBr<sub>3<\/sub>\uff08\u84dd\u8272\uff09\u548c Mn-CsPbBr<sub>3<\/sub> NPLs\uff08\u7ea2\u8272\uff09\u7684 PXRD \u56fe\u6848\u3002(f) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684 Mn L<sub>3.2<\/sub>-edge XANES \u5149\u8c31\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246002\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-16.png\" alt=\"\" width=\"363\" height=\"668\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-16.png 363w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-16-163x300.png 163w\" sizes=\"(max-width: 363px) 100vw, 363px\" \/><\/p>\n<p><strong>\u56fe2 CsPbBr<sub>3<\/sub> \u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5149\u5b66\u6027\u8d28\u3001\u81ea\u65cb\u6781\u5316\u6027\u8d28\u548c\u5149\u50ac\u5316\u6027\u80fd\u3002 <\/strong>\u00a9 2022 American Chemical Society<\/p>\n<p>(a) CsPbBr<sub>3<\/sub>\u548c (b) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684UV\u2013vis\u5438\u6536\u5149\u8c31\u548c PL \u5149\u8c31\u3002(c) CsPbBr<sub>3<\/sub>\uff08\u84dd\u8272\uff09\u548c Mn-CsPbBr<sub>3<\/sub>\uff08\u7ea2\u8272\uff09NPLs \u7684 EPR \u5149\u8c31\u3002(d) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u81ea\u65cb\u6781\u5316 DOS\u3002\u63d2\u56fe\u662f Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5b9e\u7a7a\u95f4\u7535\u8377\u5206\u5e03\u3002(e) \u5728 AM 1.5 \u6a21\u62df\u592a\u9633\u8f90\u7167\u4e0b 6 \u5c0f\u65f6\u5185\uff0cCsPbBr<sub>3<\/sub> \u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u4e0a\u7684 CO \u548c CH4 \u4ea7\u7387\u3002(f) 6\u5c0f\u65f6\u540e\uff0cCsPbBr<sub>3<\/sub> \u548c Mn-CsPbBr<sub>3<\/sub>\u00a0 NPLs \u7684\u5149\u50ac\u5316 CO<sub>2<\/sub>RR\u4ea7\u7269\u4ea7\u7387\u3002(g) CsPbBr<sub>3<\/sub> \u548cMn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5f52\u4e00\u5316\u5149\u81f4\u77ac\u6001\u53cd\u5c04\u7387\u53d8\u5316 (\u0394R\/R)\u3002(h) \u7535\u5b50\u81ea\u65cb\u6781\u5316\u6291\u5236\u4e86 Mn-CsPbBr<sub>3<\/sub> NPLs \u8f7d\u6d41\u5b50\u590d\u5408\u7684\u793a\u610f\u56fe\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246003\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-15.png\" alt=\"\" width=\"453\" height=\"610\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-15.png 453w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-15-223x300.png 223w\" sizes=\"(max-width: 453px) 100vw, 453px\" \/><\/p>\n<p><strong>\u56fe3 CsPbBr<sub>3<\/sub> \u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\u60c5\u51b5\u4e0b\u7684\u5149\u50ac\u5316\u6027\u80fd\u3002 <\/strong>\u00a9 2022 American Chemical Society<\/p>\n<p>\u5728\u5149\u7167 6 \u5c0f\u65f6\u540e\uff0c\u5728\u4e0d\u540c\u7684\u5916\u90e8\u78c1\u573a\uff080 \u81f3300 mT\uff09\u4e0b\uff0c (a) CsPbBr<sub>3<\/sub> \u548c (b) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5149\u50ac\u5316 CO<sub>2<\/sub>RR\u4ea7\u7269\u4ea7\u7387\u3002\u5728\u5149\u7167\u5c04\u4e0b 6 \u5c0f\u65f6\u5185\uff0c\u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\uff080 \u548c 300 mT\uff09\u7684\u60c5\u51b5\u4e0b\uff0c(c) CsPbBr<sub>3<\/sub> \u548c(d) Mn-CsPbBr<sub>3<\/sub> NPLs\u7684 CO \u548c CH<sub>4<\/sub> \u6c14\u4f53\u4ea7\u7269\u4ea7\u7387\u3002(e) \u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\uff080 \u548c 300 mT\uff09\u7684\u60c5\u51b5\u4e0b\uff0cCsPbBr3\uff08\u4e0a\uff09\u548c Mn-CsPbBr<sub>3<\/sub>\uff08\u4e0b\uff09NPLs\u8fdb\u884c\u56db\u6b21 6 \u5c0f\u65f6\u5faa\u73af\u7684\u5149\u50ac\u5316\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002(f) Mn-CsPbBr<sub>3<\/sub> NPLs \u5728\u56db\u6b21\u5149\u50ac\u5316 CO<sub>2<\/sub>RR 6 \u5c0f\u65f6\u5faa\u73af\u524d\u540e\u7684 EPR \u5149\u8c31\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246004\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-13.png\" alt=\"\" width=\"702\" height=\"751\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-13.png 702w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-13-280x300.png 280w\" sizes=\"(max-width: 702px) 100vw, 702px\" \/><\/p>\n<p><strong>\u56fe4 \u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\u60c5\u51b5\u4e0b\uff0c CsPbBr<sub>3<\/sub>\u548c Mn-CsPbBr<sub>3<\/sub> NPLs \u7684MCD \u5149\u8c31\u548c\u8d85\u5feb\u8f7d\u6d41\u5b50\u52a8\u529b\u5b66\u3002 <\/strong>\u00a9 2022 American Chemical Society<\/p>\n<p>\u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\uff080 \u548c300 mT\uff09\u60c5\u51b5\u4e0b\uff0c(a) CsPbBr<sub>3<\/sub> \u548c (b) Mn-CsPbBr<sub>3<\/sub> NPLs \u7684 MCD \u5149\u8c31\u3002\u5728\u6709\u548c\u6ca1\u6709\u5916\u90e8\u78c1\u573a\uff080 \u548c 300 mT\uff09\u7684\u60c5\u51b5\u4e0b\uff0c(c) CsPbBr<sub>3<\/sub> \u548c (d) Mn-CsPbBr<sub>3<\/sub> NPLs\u7684\u5f52\u4e00\u5316\u5149\u81f4\u77ac\u6001\u53cd\u5c04\u7387\u53d8\u5316 (\u0394R\/R)\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-246005\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-5.png\" alt=\"\" width=\"1062\" height=\"416\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-5.png 1062w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-5-300x118.png 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-5-768x301.png 768w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-5-1024x401.png 1024w\" sizes=\"(max-width: 1062px) 100vw, 1062px\" \/><\/p>\n<p><strong>\u56fe5 \u673a\u7406\u793a\u610f\u56fe\u3002 <\/strong>\u00a9 2022 American Chemical Society<\/p>\n<p>\u5728 Mn-CsPbBr<sub>3<\/sub> NPLs \u4e2d\uff0c\u5728\u5916\u90e8\u78c1\u573a\u4e0b\uff0c\u7535\u5b50\u81ea\u65cb\u6781\u5316\u8bf1\u5bfc\u5b9e\u73b0\u66f4\u957f\u7684\u5149\u6fc0\u53d1\u8f7d\u6d41\u5b50\u5bff\u547d\u3002<\/p>\n<p><strong>\u4e94\u3001\u6210\u679c\u542f\u793a<\/strong><\/p>\n<p>\u8be5\u7814\u7a76\u901a\u8fc7\u5728\u5168\u65e0\u673a CsPbBr<sub>3<\/sub> \u9499\u949b\u77ff NPLs \u4e2d\u63ba\u6742\u78c1\u6027 Mn<sup>2+<\/sup> \u79bb\u5b50\uff0c\u8bbe\u8ba1\u5e76\u5408\u6210\u4e86\u81ea\u65cb\u6781\u5316\u5364\u5316\u7269\u9499\u949b\u77ff NPLs\u3002\u5728\u78c1\u6027\u5143\u7d20\u534f\u540c\u63ba\u6742\u548c\u5916\u52a0\u78c1\u573a\u5e2e\u52a9\u4e0b\uff0c\u4e0e\u539f\u59cb CsPbBr<sub>3 <\/sub>NPLs \u76f8\u6bd4\uff0c Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5149\u50ac\u5316 CO<sub>2<\/sub> \u8fd8\u539f\u6548\u7387\u5927\u5927\u63d0\u9ad8\u3002\u8fd9\u662f\u7531\u4e8e Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u81ea\u65cb\u6781\u5316\u589e\u5f3a\uff0c\u5e76\u663e\u8457\u6291\u5236\u4e86\u8f7d\u6d41\u5b50\u590d\u5408\u7387\u3002\u503c\u5f97\u6ce8\u610f\u7684\u662f\uff0c\u8fd9\u79cd\u663e\u8457\u63d0\u9ad8\u7684 Mn-CsPbBr<sub>3<\/sub> NPLs \u7684\u5149\u50ac\u5316 CO<sub>2<\/sub>\u8fd8\u539f\u6548\u7387\u53ef\u4ee5\u901a\u8fc7\u7b80\u5355\u5730\u5e94\u7528\u6c38\u78c1\u4f53\uff08\u65e0\u9700\u989d\u5916\u7684\u529f\u8017\uff09\u6765\u5b9e\u73b0\u3002\u5728\u592a\u9633\u80fd\u5230\u71c3\u6599\u8f6c\u6362\u7684\u672a\u6765\u5e94\u7528\u4e2d\uff0c\u8fd9\u662f\u4e00\u79cd\u6709\u524d\u9014\u4e14\u53ef\u884c\u7684\u65b9\u6cd5\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>\u539f\u6587\u94fe\u63a5\uff1ahttps:\/\/pubs.acs.org\/doi\/10.1021\/jacs.2c06060<\/p>\n<p>\u672c\u6587\u7531\u5f20\u7199\u7199\u4f9b\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u4e00\u3001\u5bfc\u8bfb \u8fd1\u5e74\u6765\u5229\u7528\u592a\u9633\u80fd\u9a71\u52a8\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u5c06\u4e8c\u6c27\u5316\u78b3\u53d8\u4e3a\u71c3\u6599\u548c\u5316\u5b66\u54c1\u7684\u7b56\u7565\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\uff0c\u56e0\u4e3a\u5b83\u540c\u65f6\u89e3\u51b3\u4e86\u5168\u7403\u53d8\u6696\u95ee\u9898\u548c\u53ef\u518d\u751f\u80fd\u6e90\u95ee\u9898\u3002\u7136\u800c\uff0c\u5149\u50ac\u5316CO2\u8fd8\u539f\u8fc7\u7a0b&#8230;<\/p>\n","protected":false},"author":39557,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-245999","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/245999"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/39557"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=245999"}],"version-history":[{"count":6,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/245999\/revisions"}],"predecessor-version":[{"id":246247,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/245999\/revisions\/246247"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=245999"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=245999"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=245999"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}