{"id":246430,"date":"2023-01-28T06:10:00","date_gmt":"2023-01-27T22:10:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=246430"},"modified":"2023-01-27T15:19:02","modified_gmt":"2023-01-27T07:19:02","slug":"%e8%a5%bf%e6%b9%96%e5%a4%a7%e5%ad%a6%e5%b7%a5%e5%ad%a6%e9%99%a2%e7%8e%8b%e8%95%be%e3%80%81%e6%96%87%e7%87%8e%e5%8b%87%e5%9b%a2%e9%98%9fcell-reports-physical-science-%e5%a4%a9%e7%84%b6%e9%ab%98","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=246430","title":{"rendered":"\u897f\u6e56\u5927\u5b66\u5de5\u5b66\u9662\u738b\u857e\u3001\u6587\u71ce\u52c7\u56e2\u961fCell Reports Physical Science: \u5929\u7136\u9ad8\u5206\u5b50\u6fc0\u5149\u8bf1\u5bfc\u77f3\u58a8\u7a00\u5236\u5907\u53ca\u5e94\u7528"},"content":{"rendered":"<p><strong>\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p>\u968f\u7740\u6211\u56fd\u5de5\u4e1a\u5316\u8fdb\u7a0b\u7684\u52a0\u5feb\uff0c\u73af\u5883\u95ee\u9898\u4e5f\u65e5\u76ca\u4e25\u5cfb\uff0c\u7279\u522b\u662f\u6e29\u5ba4\u6c14\u4f53\u7684\u8fc7\u5ea6\u6392\u653e\u548c\u6e05\u6d01\u6c34\u8d44\u6e90\u7684\u77ed\u7f3a\u3002\u4e00\u65b9\u9762\uff0cCO<sub>2<\/sub>\u4f5c\u4e3a\u4e3b\u8981\u6e29\u5ba4\u6c14\u4f53\uff0c\u5176\u6392\u653e\u91cf\u968f\u7740\u5de5\u4e1a\u548c\u519c\u4e1a\u6d3b\u52a8\u7684\u589e\u52a0\u5feb\u901f\u589e\u957f\u3002\u5176\u4e2d\uff0c\u7535\u5316\u5b66\u8fd8\u539f\u65b9\u6cd5\u662f\u5176\u4e2d\u4e00\u79cd\u9ad8\u6548\u73af\u4fdd\u7684\u65b9\u6cd5\u53ef\u5c06\u6392\u653e\u7684CO<sub>2<\/sub>\u8f6c\u5316\u4e3a\u591a\u79cd\u9ad8\u9644\u52a0\u503c\u7684\u5316\u5b66\u54c1\u539f\u6599\u3002\u53e6\u4e00\u65b9\u9762\uff0c\u77ff\u7269\u5f00\u91c7\u548c\u5316\u5de5\u751f\u4ea7\u5e9f\u6c34\u4e2d\u7684\u91cd\u91d1\u5c5e\u79bb\u5b50\u548c\u6709\u673a\u5fae\u6c61\u67d3\u7269\u5bf9\u751f\u6001\u7cfb\u7edf\u548c\u4eba\u7c7b\u5065\u5eb7\u4e5f\u6784\u6210\u4e86\u4e25\u91cd\u7684\u5a01\u80c1\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246432\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-7.jpg\" alt=\"\" width=\"600\" height=\"387\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-7.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/1-7-300x194.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>\u00a0Figure 1. Schematic drawing of upcycling of post-consumer waste to M-LIG catalysts for producing green chemicals and clean water<\/p>\n<p><strong>\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u897f\u6e56\u5927\u5b66\u738b\u857e\u3001\u6587\u71ce\u52c7\u56e2\u961f<\/strong>\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8e\u6fc0\u5149\u8bf1\u5bfc\u6280\u672f\u8f6c\u5316\u542b\u91cd\u91d1\u5c5e\u58f3\u805a\u7cd6\u4e3a\u91d1\u5c5e\u63ba\u6742\u77f3\u58a8\u7a00\u7684\u901a\u7528\u6027\u5347\u7ea7\u5faa\u73af\u7b56\u7565\u3002\u4f8b\u5982\uff0c\u94dc\u63ba\u6742\u77f3\u58a8\u70ef\u53ef\u4f5c\u4e3a\u50ac\u5316\u5242\u88ab\u5e94\u7528\u4e8eCO<sub>2<\/sub>\u7535\u5316\u5b66\u8fd8\u539f\u548c\u6709\u673a\u5fae\u6c61\u67d3\u7269\u964d\u89e3\uff0c\u4ee5\u4fbf\u63d0\u4f9b\u4e00\u79cd\u53ef\u6301\u7eed\u7684\u6218\u7565\u6765\u6709\u6548\u3001\u534f\u540c\u5730\u89e3\u51b3\u6e29\u5ba4\u6c14\u4f53\u8fc7\u91cf\u6392\u653e\u548c\u6c34\u6c61\u67d3\u7684\u95ee\u9898\uff08Figure 1\uff09\u3002\u7814\u7a76\u6210\u679c\u4ee5\u201cSustainable upcycling of post-consumer waste to metal-graphene catalysts for green chemicals and clean water\u201d\u4e3a\u9898\u53d1\u8868\u5728Cell\u51fa\u7248\u793e\u65d7\u4e0b\u65b0\u664b\u9ad8\u6c34\u5e73\u671f\u520a \u300aCell Reports Physical Science\u300b\uff0c\u897f\u6e56\u5927\u5b66\u738b\u857e\u8bfe\u9898\u7ec4\u535a\u58eb\u7814\u7a76\u751f\u5218\u949f\u7426\u3001\u6587\u71ce\u52c7\u8bfe\u9898\u7ec4\u80e1\u5c0f\u677e\u535a\u58eb\u4e3a\u672c\u6587\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\uff0c\u897f\u6e56\u5927\u5b66\u5de5\u5b66\u9662\u6587\u71ce\u52c7\u3001\u738b\u857e\u7814\u7a76\u5458\u4e3a\u672c\u6587\u5171\u540c\u901a\u8baf\u4f5c\u8005\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246433\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-7.jpg\" alt=\"\" width=\"561\" height=\"203\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-7.jpg 561w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/2-7-300x109.jpg 300w\" sizes=\"(max-width: 561px) 100vw, 561px\" \/><\/p>\n<p><strong>\u00a0\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p>\u58f3\u805a\u7cd6 (Chitosan) \u4f5c\u4e3a\u4e00\u79cd\u4ece\u8783\u87f9\u7b49\u6d77\u4ea7\u54c1\u7684\u5de5\u4e1a\u5e9f\u7269\u4e2d\u63d0\u53d6\u7684\u5929\u7136\u9ad8\u5206\u5b50\uff0c\u5df2\u88ab\u5e7f\u6cdb\u7528\u4e8e\u5e9f\u6c34\u4e2d\u91cd\u91d1\u5c5e\u79bb\u5b50\u7684\u5438\u9644\u3002\u4f46\u4f7f\u7528\u540e\u6750\u6599\u542b\u6709\u7684\u91cd\u91d1\u5c5e\u79bb\u5b50\u9700\u8981\u88ab\u91cd\u65b0\u89e3\u5438\u6216\u76f4\u63a5\u8fde\u540c\u6750\u6599\u4f5c\u4e3a\u5371\u9669\u5e9f\u7269\u5904\u7406\u3002\u7814\u7a76\u56e2\u961f\u5c06\u87af\u5408\u4e86\u4e0d\u540c\u91d1\u5c5e\u79bb\u5b50\uff08Cu<sup>2+<\/sup>\u3001Pd<sup>2+<\/sup>\u3001 Cd<sup>2+<\/sup>\u3001Mn<sup>2+<\/sup>\u3001Zn<sup>2+<\/sup>\u3001Ni<sup>2+<\/sup>\u3001Ag<sup>+<\/sup> \u548c Cr<sup>6+<\/sup>\uff09\u7684\u58f3\u805a\u7cd6\u8584\u819c\u901a\u8fc7\u6fc0\u5149\u6253\u5370\uff0c\u5728\u7a7a\u6c14\u73af\u5883\u4e0b\u76f4\u63a5\u78b3\u5316\u4e3a\u91d1\u5c5e\u63ba\u6742\u7684\u77f3\u58a8\u70ef\uff08Metal-doped laser-induced graphene, M-LIG, Figure 2\uff09\u3002\u540c\u65f6\uff0c\u901a\u8fc7\u6539\u53d8\u91d1\u5c5e\u542b\u91cf\u548c\u6fc0\u5149\u53c2\u6570\u83b7\u5f97\u5177\u6709\u4e0d\u540c\u91d1\u5c5e\u4ef7\u6001\u3001\u6c2e\u5143\u7d20\u4f4d\u70b9\u548c\u7ed3\u6784\u7684\u77f3\u58a8\u7a00\u6750\u6599\u3002\u5728\u6fc0\u5149\u6761\u4ef6\u4e0b\uff0c\u4e0d\u540c\u4e8e\u5929\u7136\u9ad8\u5206\u5b50\u88ab\u76f4\u63a5\u5206\u89e3\u4e3a\u6c14\u6001\u5206\u5b50CO<sub>2<\/sub>\uff0c\u87af\u5408\u7684\u91d1\u5c5e\u79bb\u5b50\u80fd\u591f\u63d0\u9ad8\u58f3\u805a\u7cd6\u8584\u819c\u7684\u70ed\u7a33\u5b9a\u6027\uff0c\u964d\u4f4e\u8584\u819c\u7684\u8868\u9762\u6e29\u5ea6\u3002\u540c\u65f6\uff0c\u91d1\u5c5e\u79bb\u5b50\u5728\u6fc0\u5149\u6253\u5370\u8fc7\u7a0b\u4e2d\u88ab\u8fd8\u539f\u4e3a\u91d1\u5c5e\u5355\u8d28\uff0c\u5e76\u50ac\u5316\u78b3\u539f\u5b50\u91cd\u6392\u751f\u6210\u77f3\u58a8\u70ef\u7ed3\u6784\u3002\u6b64\u5916\uff0c\u58f3\u805a\u7cd6\u5206\u5b50\u62e5\u6709\u5927\u91cf\u81ea\u7531\u6c28\u57fa\uff0c\u80fd\u591f\u5728\u77f3\u58a8\u70ef\u7ed3\u6784\u4e2d\u5f62\u6210\u4e0d\u540c\u7684\u6c2e\u5143\u7d20\u4f4d\u70b9\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246434\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-6.jpg\" alt=\"\" width=\"600\" height=\"868\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-6.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/3-6-207x300.jpg 207w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>Figure 2. Fabrication of M-LIG based on metal-chelated chitosan film<\/p>\n<p>\u7814\u7a76\u56e2\u961f\u4ee5\u94dc\u63ba\u6742\u77f3\u58a8\u70ef\uff08Cu-LIG\uff09\u4f5c\u4e3a\u50ac\u5316\u5242\uff0c\u8fdb\u884c\u4e86CO<sub>2<\/sub>\u7535\u8fd8\u539f\u6d4b\u8bd5\uff08Figure 3\uff09\u3002\u4ee5\u6d41\u52a8\u6c60\u53cd\u5e94\u4e2d\uff0c\u542b\u78b3\u4ea7\u7269\u7684\u603b\u6cd5\u62c9\u7b2c\u6548\u7387\uff08Faraday efficiency, FE\uff09\u8d85\u8fc780%\uff0c\u5176\u4e2d\u4e59\u70ef\u4f5c\u4e3a\u4e3b\u8981C<sub>2<\/sub>\u4ea7\u7269\uff0cFE\u7ea6\u4e3a25%\u3002\u901a\u8fc7DFT\u8ba1\u7b97\uff0c\u6211\u4eec\u9884\u6d4b\u5728CO<sub>2<\/sub>\u7535\u8fd8\u539f\u8fc7\u7a0b\u4e2d\uff0c\u5171\u540c\u5b58\u5728\u7684Cu<sup>+<\/sup> \u548c Cu<sup>0<\/sup>\u4fc3\u8fdb\u4e86C-C\u5076\u8054\u8fc7\u7a0b\uff0c\u6709\u5229\u4e8eC<sub>2<\/sub>\u4ea7\u7269\u7684\u751f\u6210\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246435\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-6.jpg\" alt=\"\" width=\"600\" height=\"874\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-6.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/4-6-206x300.jpg 206w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>Figure 3. CO<sub>2<\/sub>ER based on Cu-LIG catalysts<\/p>\n<p>\u540c\u65f6\uff0c\u7814\u7a76\u56e2\u961f\u4ee5Cu-LIG\u8584\u819c\u4f5c\u4e3a\u7c7b\u82ac\u987f\u53cd\u5e94\u50ac\u5316\u5242\uff0c\u964d\u89e3\u6c61\u6c34\u4e2d\u516d\u79cd\u5e38\u89c1\u7684\u6709\u673a\u5fae\u6c61\u67d3\u7269\uff08Figure 4\uff09\u3002\u7814\u7a76\u7ed3\u679c\u8868\u660e\uff0c\u66f4\u5bb9\u6613\u88ab\u56de\u6536\u548c\u5faa\u73af\u4f7f\u7528\u7684Cu-LIG\u8584\u819c\u53ef\u4ee5\u9ad8\u6548\u7684\u50ac\u5316\u8fc7\u6c27\u5316\u6c22\u4ea7\u751f\u7f9f\u57fa\u81ea\u7531\u57fa\u964d\u89e3\u6c61\u67d3\u7269\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246436\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-5.jpg\" alt=\"\" width=\"600\" height=\"452\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-5.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/5-5-300x226.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>Figure 4. Organic micropollutants degradation based on Cu-LIG<\/p>\n<p>\u6700\u540e\uff0c\u7814\u7a76\u56e2\u961f\u5bf9\u6574\u4e2a\u7b56\u7565\u8fdb\u884c\u4e86\u7cfb\u7edf\u7684\u751f\u547d\u5468\u671f\u8bc4\u4ef7\uff08Figure 5\uff09\u3002\u5229\u7528\u5316\u5de5\u8fc7\u7a0b\u6a21\u62df\u624b\u6bb5Aspen Plus, \u5c06CO<sub>2<\/sub>\u7535\u8fd8\u539f\u3001\u53cd\u5e94\u5668\u8bbe\u8ba1\u3001\u4e0b\u6e38\u4ea7\u7269\u7684\u8fdb\u4e00\u6b65\u8f6c\u5316\u548c\u5206\u79bb\u8fdb\u884c\u6574\u5408\u4e0e\u4f18\u5316\u3002\u7ed3\u679c\u663e\u793a\u5728\u672a\u6765\u7684\u4f4e\u78b3\u60c5\u666f\u4e0b\uff0c\u5229\u7528\u542b\u5e9f\u6c34\u91cd\u91d1\u5c5e\u7684\u58f3\u805a\u7cd6\u57fa\u77f3\u58a8\u70ef\u6750\u6599\u4f5c\u4e3a\u50ac\u5316\u5242\u5c06CO<sub>2<\/sub>\u7535\u8fd8\u539f\u4e3aC<sub>2<\/sub>\u4ea7\u7269\u53ef\u5b9e\u73b0\u663e\u8457\u7684\u78b3\u51cf\u6392\u6548\u76ca\u3002\u00a0\u00a0<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-246437\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-3.jpg\" alt=\"\" width=\"600\" height=\"354\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-3.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/01\/6-3-300x177.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p>Figure 5. LCA of applications of Cu-LIG catalyst<\/p>\n<p>\u5728\u8fd9\u9879\u5de5\u4f5c\u4e2d\uff0c\u7814\u7a76\u56e2\u961f\u63d0\u51fa\u4e86\u4e00\u79cd\u901a\u7528\u7684\u5347\u7ea7\u56de\u6536\u7b56\u7565\uff0c\u4ee5\u5e94\u5bf9\u7531\u591a\u79cd\u5e9f\u5f03\u7269\uff08\u56fa\u5e9f\u3001\u5e9f\u6c14\u3001\u5e9f\u6c34\uff09\u5f15\u8d77\u7684\u73af\u5883\u6311\u6218\u53ca\u95ee\u9898\u3002\u901a\u8fc7\u4e00\u6b65\u6cd5\u6fc0\u5149\u8bf1\u5bfc\u78b3\u5316\uff0c\u6211\u4eec\u5c06\u542b\u6709\u5e9f\u6c34\u91cd\u91d1\u5c5e\u79bb\u5b50\u7684\u58f3\u805a\u7cd6\u6210\u529f\u8f6c\u5316\u4e3a M-LIG\uff0c\u5e76\u5e94\u7528\u4e8eCO<sub>2<\/sub>\u7535\u5316\u5b66\u8fd8\u539f\u751f\u4ea7C2\u4ea7\u7269\u548c\u9ad8\u7ea7\u6c27\u5316\u5904\u7406\u6c61\u6c34\u4e2d\u7684\u6709\u673a\u5fae\u6c61\u67d3\u7269\u3002<strong>\u603b\u7684\u6765\u8bf4\uff0c\u7814\u7a76\u56e2\u961f\u63d0\u51fa\u7684\u6218\u7565\u53ef\u4ee5\u4e3a\u5b9e\u73b0\u4f4e\u78b3\u3001\u53ef\u6301\u7eed\u7684\u672a\u6765\u63d0\u4f9b\u4e00\u79cd\u534f\u540c\u89e3\u51b3\u65b9\u6848\u3002<\/strong>\u8be5\u9879\u76ee\u5f97\u5230\u897f\u6e56\u5927\u5b66\u4ea4\u53c9\u521d\u521b\u4e2d\u5fc3\uff08MRIC\uff09\u652f\u6301\u3002<\/p>\n<p>\u539f\u6587\u94fe\u63a5:<\/p>\n<p><a href=\"https:\/\/doi.org\/10.1016\/j.xcrp.2023.101256\">https:\/\/doi.org\/10.1016\/j.xcrp.2023.101256<\/a><\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u3010\u5bfc\u8bfb\u3011 \u968f\u7740\u6211\u56fd\u5de5\u4e1a\u5316\u8fdb\u7a0b\u7684\u52a0\u5feb\uff0c\u73af\u5883\u95ee\u9898\u4e5f\u65e5\u76ca\u4e25\u5cfb\uff0c\u7279\u522b\u662f\u6e29\u5ba4\u6c14\u4f53\u7684\u8fc7\u5ea6\u6392\u653e\u548c\u6e05\u6d01\u6c34\u8d44\u6e90\u7684\u77ed\u7f3a\u3002\u4e00\u65b9\u9762\uff0cCO2\u4f5c\u4e3a\u4e3b\u8981\u6e29\u5ba4\u6c14\u4f53\uff0c\u5176\u6392\u653e\u91cf\u968f\u7740\u5de5\u4e1a\u548c\u519c\u4e1a\u6d3b\u52a8\u7684&#8230;<\/p>\n","protected":false},"author":2,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-246430","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/246430"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=246430"}],"version-history":[{"count":1,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/246430\/revisions"}],"predecessor-version":[{"id":246438,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/246430\/revisions\/246438"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=246430"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=246430"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=246430"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}