{"id":249552,"date":"2023-04-21T06:23:10","date_gmt":"2023-04-20T22:23:10","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=249552"},"modified":"2023-04-20T10:43:27","modified_gmt":"2023-04-20T02:43:27","slug":"adv-funct-mater-%ef%bc%9a%e8%87%b4%e5%af%86%e9%93%82-%e9%95%8d%e6%b0%a7%e5%8c%96%e7%89%a9%e5%bc%82%e8%b4%a8%e7%95%8c%e9%9d%a2%e5%ae%9e%e7%8e%b0%e5%ae%89%e5%9f%b9%e7%ba%a7%e9%ab%98%e6%95%88%e7%a8%b3","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=249552","title":{"rendered":"Adv. Funct. Mater.\uff1a\u81f4\u5bc6\u94c2\/\u954d\u6c27\u5316\u7269\u5f02\u8d28\u754c\u9762\u5b9e\u73b0\u5b89\u57f9\u7ea7\u9ad8\u6548\u7a33\u5b9a\u6790\u6c22"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u6c34\u78b1\u7535\u89e3\u6cd5\u5728\u5de5\u4e1a\u89c4\u6a21\u5236\u6c22\u65b9\u9762\u5177\u6709\u5f88\u5927\u7684\u524d\u666f\u3002\u76ee\u524d\u94c2\uff08Pt\uff09\u4ecd\u7136\u662f\u78b1\u6027\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u7684\u57fa\u51c6\u7535\u50ac\u5316\u5242\uff0c\u4f46\u7531\u4e8e\u7f3a\u4e4f\u80fd\u591f\u5728\u5b89\u57f9\u7ea7\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5de5\u4f5c\u7684\u7cbe\u5fc3\u8bbe\u8ba1\u7684\u8010\u7528Pt\u57fa\u6750\u6599\uff0c\u5176\u5de5\u4e1a\u89c4\u6a21\u7684\u6c22\u6c14\u751f\u4ea7\u53d7\u5230\u4e25\u91cd\u963b\u788d\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u9ad8\u7535\u6d41\u5bc6\u5ea6\u8010\u53d7\u6027\u7684HER\u7535\u50ac\u5316\u5242\u662f\u5de5\u4e1a\u89c4\u6a21\u78b1\u7535\u89e3\u5236\u6c22\u6240\u201c\u5fc5\u987b\u5b8c\u6210\u201d\u7684\u4efb\u52a1\uff1b\u7136\u800c\uff0c\u7531\u4e8e\u6d89\u53ca\u521d\u59cb\u6c34\u89e3\u79bb\u7684Volmer\u8fc7\u7a0b\uff08H2<\/sub>O H* + OH*\uff09\u548c\u968f\u540e\u7684OH*\u8131\u9644\u8fc7\u7a0b\uff08OH*+ e–<\/sup> OH–<\/sup>\uff09\u5177\u6709\u7f13\u6162\u7684\u52a8\u529b\u5b66\uff0c\u56e0\u6b64\u4f7f\u5f97\u4e0a\u8ff0\u4efb\u52a1\u7684\u5b9e\u73b0\u5145\u6ee1\u6311\u6218\u3002<\/p>\n

\u00a0<\/strong>\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u57fa\u4e8e\u6ce1\u6cab\u954d\uff08NF\uff09\u8868\u9762\u7684\u539f\u59cb\u6c27\u5316\u5c42\u548c\u51f8\u8d77\u7ed3\u6784\uff0c\u6fb3\u95e8\u5927\u5b66<\/strong>Kwun Nam Hui<\/strong>\u6559\u6388\u3001\u6e6f\u5b50\u5eb7\u6559\u6388\u8054\u5408\u5357\u4eac\u5de5\u4e1a\u5927\u5b66\u90b5\u5b97\u5e73\u6559\u6388\u3001\u82f1\u56fd\u4e1c\u82f1\u5409\u5229\u5927\u5b66<\/strong>Kwan San Hui<\/strong>\u6559\u6388<\/strong>\u7b49\u4eba\u5f00\u53d1\u4e86\u4e00\u79cd\u7531\u81f4\u5bc6Pt NPs\u56fa\u5b9a\u7684\u5bcc\u542b\u6c27\u7a7a\u4f4d\u7684NiOx<\/sub>\u5f02\u8d28\u7ed3\uff08Pt\/NiOx<\/sub>-OV<\/sub>\uff09\u7ec4\u6210\u7684\u4e09\u7ef4\u51c6\u5e73\u884c\u7ed3\u6784\u4f5c\u4e3a\u78b1\u6027HER\u50ac\u5316\u5242\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u7ed3\u5408\u8868\u660e\uff0c\u5c06Pt NPs\u951a\u5b9a\u5728NiOx<\/sub>-OV<\/sub>\u4e0a\u4f1a\u5bfc\u81f4\u6001\u5bc6\u5ea6\uff08DOS\uff09\u5206\u5e03\u6539\u53d8\u7684\u5bcc\u7535\u5b50Pt\u7269\u79cd\uff0c\u8fd9\u53ef\u4ee5\u6709\u6548\u5730\u4f18\u5316d\u5e26\u4e2d\u5fc3\u548c\u53cd\u5e94\u4e2d\u95f4\u4f53\u7684\u5438\u9644\uff0c\u5e76\u589e\u5f3a\u6c34\u7684\u89e3\u79bb\u80fd\u529b\u3002\u6240\u5236\u5907\u7684\u50ac\u5316\u5242\u8868\u73b0\u51fa\u5353\u8d8a\u7684HER\u6027\u80fd\uff0c\u572810 mA cm-2<\/sup>\u4e0b\u5177\u670919.4 mV\u7684\u4f4e\u8fc7\u7535\u4f4d\uff0c\u8d28\u91cf\u6d3b\u6027\u6bd420%Pt\/C\u9ad816.3\u500d\uff0c\u57281 A cm-2<\/sup>\u4e2d\u5177\u6709\u8d85\u8fc7100 h\u7684\u957f\u671f\u8010\u4e45\u6027\u3002\u6b64\u5916\uff0c\u4e0eNiFe\u5c42\u72b6\u53cc\u6c22\u6c27\u5316\u7269\u76f8\u7ed3\u5408\u7684\u7ec4\u88c5\u5f0f\u78b1\u6027\u7535\u89e3\u69fd\u53ea\u9700\u89811.776 V\u7684\u6781\u4f4e\u7535\u538b\u5c31\u80fd\u8fbe\u52301 A cm-2<\/sup>\uff0c\u5e76\u4e14\u53ef\u4ee5\u7a33\u5b9a\u8fd0\u884c400\u5c0f\u65f6\u4ee5\u4e0a\uff0c\u8fd9\u662f\u6781\u5c11\u5b9e\u73b0\u7684\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cDense Platinum\/Nickel Oxide Heterointerfaces with Abundant Oxygen Vacancies Enable Ampere-Level Current Density Ultrastable Hydrogen Evolution in Alkaline<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u77e5\u540d\u671f\u520aAdv. Funct. Mater.<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

\u5f00\u53d1\u4e86\u4e00\u79cd\u78b1\u6027HER\u50ac\u5316\u5242\uff0c\u572810 mA cm-2<\/sup>\u4e0b\u5177\u670919.4 mV\u7684\u4f4e\u8fc7\u7535\u4f4d\uff0c\u8d28\u91cf\u6d3b\u6027\u6bd420%Pt\/C\u9ad816.3\u500d\uff0c\u57281 A cm-2<\/sup>\u4e2d\u5177\u6709\u8d85\u8fc7100 h\u7684\u957f\u671f\u8010\u4e45\u6027\uff0c\u7ec4\u88c5\u7684R-NFPt||NiFe-LDH\u53cc\u7535\u6781\u7535\u89e3\u69fd\u53ea\u9700\u89811.776 V\u7684\u6781\u4f4e\u7535\u538b\u5373\u53ef\u8fbe\u52301 A cm-2<\/sup>\uff0c\u5e76\u5177\u6709\u8d85\u8fc7400\u5c0f\u65f6\u7684\u8d85\u957f\u7a33\u5b9a\u6027\u3002<\/p>\n

\u00a0<\/strong>\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\u56fe<\/strong>1\u00a0 R-NF-Pt<\/strong>\u7684\u5408\u6210\u56fe\u793a\u53ca\u5fae\u89c2\u5f62\u8c8c<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a\uff09R-NF-Pt\u7684\u5408\u6210\u8fc7\u7a0b\u793a\u610f\u56fe\u4ee5\u53ca\u4e0d\u540c\u5408\u6210\u9636\u6bb5\u7684\u76f8\u5e94SEM\u56fe\u50cf\u3002<\/p>\n

\uff08b-d\uff09\u672a\u5904\u7406\u7684\u548cNaBH4<\/sub>\u5904\u7406\u7684NF\u8868\u9762\u4ee5\u53caR-NF-Pt\u7684AFM\u56fe\u50cf\u3002<\/p>\n

\uff08e-g\uff09\u4e0d\u540c\u653e\u5927\u500d\u6570\u4e0bR-NF-Pt\u7684SEM\u56fe\u50cf\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>2 \u00a0R-NF-Pt<\/strong>\u7684\u5fae\u89c2\u7ed3\u6784\u5206\u6790<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a-e\uff09R-NF-Pt\u7684\u6a2a\u622a\u9762TEM\u56fe\u50cf\u3001\u6a2a\u622a\u9762HRTEM\u56fe\u50cf\u3001HAADF-STEM\u56fe\u50cf\u4ee5\u53ca\u7684\u76f8\u5e94EDX\u5143\u7d20\u6620\u5c04\u56fe\u50cf\u3002<\/p>\n

\uff08f-i\uff09R-NF-Pt\u7684TEM\u56fe\u50cf\u3001HRTEM\u56fe\u50cf\u548cHAADF-STEM\u56fe\u50cf\uff0c\u4ee5\u53ca\u4ece\u8868\u9762\u8d85\u58f0\u5265\u79bb\u7684\u6837\u54c1\u7684\u76f8\u5e94EDX\u5143\u7d20\u6620\u5c04\u56fe\u50cf\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>3 \u00a0<\/strong>\u50ac\u5316\u5242\u8868\u9762\u7684\u7535\u5b50\u7ed3\u6784\u548c\u5316\u5b66\u72b6\u6001<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a-b\uff09NF\u3001R-NF\u548cR-NF-Pt\u7684\u9ad8\u5206\u8fa8\u7387Ni 2p3\/2<\/sub>\u548cO 1s XPS\u5149\u8c31\u3002<\/p>\n

\uff08c\uff09\u4e0d\u540c\u50ac\u5316\u5242\u4e2d\u7684OV<\/sub>\u6bd4\u4f8b\u3002<\/p>\n

\uff08d\uff09Pt\/C\u548cR-NF-Pt\u7684\u9ad8\u5206\u8fa8\u7387Pt 4f XPS\u5149\u8c31\u3002<\/p>\n

\uff08e\uff09R-NF-Pt\u7684\u5dee\u5f02\u7535\u8377\u5bc6\u5ea6\u5206\u6790\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4 \u00a0<\/strong>\u7535\u5b50\u6784\u578b\u5bf9\u78b1\u6027<\/strong>HER<\/strong>\u8fc7\u7a0b\u7684\u5f71\u54cd<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a\uff09\u8ba1\u7b97\u7684H2<\/sub>O\u548cOH\u5728Pt\uff08111\uff09\u548cPt\/NiOx<\/sub>-OV<\/sub>\u4e0a\u7684\u5438\u9644\u80fd\u3002<\/p>\n

\uff08b\uff09\u8ba1\u7b97\u7684Pt\u56e2\u7c07\u548cPt\/NiOx<\/sub>-OV<\/sub>\u5f02\u8d28\u7ed3\u4e0aPt\u4f4d\u70b9\u7684\u603b\u6001\u5bc6\u5ea6\uff08TDOS\uff09\u3002<\/p>\n

\uff08c\uff09\u91d1\u5c5e\u548c\u975e\u91d1\u5c5e\u5143\u7d20\u8f68\u9053\u53d8\u5316\u793a\u610f\u56fe\u3002<\/p>\n

\uff08d\uff09\u5728Pt\u548cPt\/NiOx<\/sub>-OV<\/sub>\u4e0aHER\u7684\u5409\u5e03\u65af\u81ea\u7531\u80fd\u56fe\u3002<\/p>\n

\uff08e\uff09\u5438\u9644\u5728Pt\u548cPt\/NiOx<\/sub>-OV<\/sub>\u4e0a\u7684*H2O\u3001*OH-H\u3001*OH\u548cH*\u7684\u51e0\u4f55\u6784\u578b\u3002<\/p>\n

\uff08f\uff09\u8ba1\u7b97\u7684NiOx<\/sub>-OV<\/sub>\u548cPt\/NiOx<\/sub>-OV<\/sub>\u7684\u90e8\u5206\u6001\u5bc6\u5ea6\uff08PDOS\uff09\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>5 \u00a0<\/strong>\u50ac\u5316\u5242\u7684\u7535\u50ac\u5316<\/strong>HER<\/strong>\u6027\u80fd\u8bc4\u4f30<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a\uff09R-NF-Pt\u3001NF-Pt\u3001Pt-NPs\u3001NF\u548cPt\/C\u50ac\u5316\u5242\u7684HER\u6781\u5316\u66f2\u7ebf\u3002<\/p>\n

\uff08b\uff09\u4ece\uff08a\uff09\u4e2d\u7684\u6781\u5316\u66f2\u7ebf\u83b7\u5f97\u7684\u5854\u83f2\u5c14\u56fe\u3002<\/p>\n

\uff08c\uff09R-NF-Pt\u548c20%Pt\/C\u572810 mA cm-2<\/sup>\u4e0b\u7684\u8fc7\u7535\u4f4d\u548c-70 mV\u4e0b\u7684\u8d28\u91cf\u6d3b\u5ea6\u4e0eRHE\u7684\u5bf9\u6bd4\u3002<\/p>\n

\uff08d\uff09R-NF-Pt\u4e0e\u5176\u4ed6\u62a5\u9053\u7684Pt\/Ni\u57fa\u78b1\u6027HER\u7535\u50ac\u5316\u5242\u572810 mA cm-2<\/sup>\u4e0b\u7684\u8fc7\u7535\u4f4d\u548c\u8d28\u91cf\u6d3b\u6027\u7684\u5bf9\u6bd4\u3002<\/p>\n

\uff08e\uff09R-NF-Pt\u3001NF-Pt\u3001Pt-NPs\u3001NF\u548cPt\/C\u7684\u53cc\u5c42\u7535\u5bb9\uff08Cdl\uff09\u56fe\u3002<\/p>\n

\uff08f\uff09R-NF-Pt\u3001NF-Pt\u3001Pt-NPs\u3001NF\u548cPt\/C\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31\uff08EIS\uff09\u3002<\/p>\n

\uff08g\uff09\u57285000\u300120000\u548c50000\u6b21CV\u5faa\u73af\u524d\u540e\uff0cR-NF-Pt\u548cPt\/C\u572810 mA cm-2<\/sup>\u4e0b\u7684\u6781\u5316\u66f2\u7ebf\u548c\u76f8\u5e94\u7684\u8fc7\u7535\u4f4d\u53d8\u5316\u3002<\/p>\n

\uff08h\uff09R-NF-Pt\u548cPt\/C\u572810\u548c1000 mA cm-2<\/sup>\u7684\u6052\u5b9a\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u8ba1\u65f6\u7535\u4f4d\u5206\u6790\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>6 \u00a0<\/strong>\u6c34\u5206\u89e3\u7684\u7535\u50ac\u5316\u6027\u80fd<\/strong> \u00a9 Wiley-VCH GmbH<\/strong><\/p>\n

\uff08a\uff09\u78b1\u6027\u6c34\u5206\u89e3\u8fc7\u7a0b\u7684\u6574\u4f53\u56fe\u793a\u3002<\/p>\n

\uff08b\uff09R-NF-Pt||NiFe-LDH\u548c\u5546\u7528Pt\/C||RuO2<\/sub>\u7528\u4e8e\u6c34\u5206\u89e3\u7684\u6781\u5316\u66f2\u7ebf\u3002<\/p>\n

\uff08c\uff09\u4e0e\u62a5\u9053\u7684\u9ad8\u6027\u80fd\u8d35\u91d1\u5c5e\u57fa\u50ac\u5316\u5242\u572810\u3001500\u548c1000 mA cm-2<\/sup>\u4e0b\u7684\u6c34\u5206\u89e3\u6d3b\u6027\u5bf9\u6bd4\u3002<\/p>\n

\uff08d\uff09R-NF-Pt||NiFe-LDH\u548c\u5546\u7528Pt\/C||RuO2<\/sub>\u5728\u4e0d\u540c\u7535\u538b\u4e0b\u7684\u8d28\u91cf\u6d3b\u6027\u5bf9\u6bd4\u3002<\/p>\n

\uff08e\uff09R-NF-Pt||NiFe-LDH\u548c\u5546\u7528Pt\/C||RuO2<\/sub>\u57281000 mA cm-2<\/sup>\u4e0b\u7684\u8ba1\u65f6\u7535\u4f4d\u5206\u6790\u3002<\/p>\n

\uff08f\uff09R-NF-Pt||NiFe-LDH\u6392\u6c34\u6cd5\u6536\u96c6\u7684H2<\/sub>\u548cO2<\/sub>\u7684\u91cf\u968f\u65f6\u95f4\u7684\u53d8\u5316\u3002<\/p>\n

\u00a0<\/strong>\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

\u7efc\u4e0a\uff0c\u7814\u7a76\u4eba\u5458\u5f00\u53d1\u4e86\u4e00\u79cd\u7b80\u5355\u3001\u7eff\u8272\u7684\u65b9\u6cd5\u6765\u5236\u5907\u4e09\u7ef4\u51c6\u5e73\u884cR-NF-Pt\u7535\u50ac\u5316\u5242\uff0c\u7528\u4e8e\u7a33\u5b9a\u7684\u5927\u7535\u6d41\u5236\u6c22\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u7814\u7a76\u8868\u660e\uff0c\u5c06Pt NPs\u951a\u5b9a\u5728NiOx<\/sub>-OV<\/sub>\u4e0a\u4f1a\u5bfc\u81f4DOS\u5206\u5e03\u6539\u53d8\u7684\u5bcc\u7535\u5b50Pt\u7269\u79cd\uff0c\u53ef\u4ee5\u6709\u6548\u5730\u4f18\u5316d\u5e26\u4e2d\u5fc3\u548c\u53cd\u5e94\u4e2d\u95f4\u4f53\u7684\u5438\u9644\uff0c\u589e\u5f3a\u6c34\u7684\u89e3\u79bb\u80fd\u529b\u3002\u56e0\u6b64\uff0cR-NF-Pt\u50ac\u5316\u5242\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u78b1\u6027HER\u6d3b\u6027\uff0c\u572810 mA cm-2<\/sup>\u65f6\u5177\u670919.4 mV\u7684\u4f4e\u8fc7\u7535\u4f4d\uff0c\u8d28\u91cf\u6d3b\u6027\u6bd420%Pt\/C\u9ad816.3\u500d\uff0c\u57281000 mA cm-2<\/sup>\u4e2d\u5177\u6709\u826f\u597d\u7684\u957f\u671f\u8010\u4e45\u6027\u3002\u8fdb\u4e00\u6b65\u7814\u7a76\u8868\u660e\uff0c\u7ec4\u88c5\u7684R-NFPt||NiFe-LDH\u53cc\u7535\u6781\u7535\u89e3\u69fd\u53ea\u9700\u89811.418\u548c1.776 V\u7684\u6781\u4f4e\u7535\u538b\u5373\u53ef\u5206\u522b\u8fbe\u523010\u548c1000 mA cm-2<\/sup>\uff0c\u5e76\u57281000 mA cm-2<\/sup>\u4e0b\u63d0\u4f9b\u8d85\u8fc7400\u5c0f\u65f6\u7684\u8d85\u957f\u7a33\u5b9a\u6027\uff0c\u8fd9\u662f\u4ee5\u524d\u5f88\u5c11\u5b9e\u73b0\u7684\u3002\u672c\u7814\u7a76\u4e3a\u8bbe\u8ba1\u9ad8\u6548\u50ac\u5316\u5e94\u7528\u7684\u9ad8\u6027\u80fd\u5355\u7247\u7535\u6781\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u65b9\u6cd5\u3002<\/p>\n

\u539f\u6587\u8be6\u60c5<\/strong>\uff1aDense Platinum\/Nickel Oxide Heterointerfaces with Abundant Oxygen Vacancies Enable Ampere-Level Current Density Ultrastable Hydrogen Evolution in Alkaline<\/a> (Adv. Funct. Mater.<\/em> 2023<\/strong>, 33, 2211273)<\/p>\n

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