{"id":251020,"date":"2023-05-18T08:24:48","date_gmt":"2023-05-18T00:24:48","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=251020"},"modified":"2023-05-18T08:24:48","modified_gmt":"2023-05-18T00:24:48","slug":"%e6%9d%8e%e4%ba%9a%e6%a0%8b%e9%99%a2%e5%a3%ab%e5%9b%a2%e9%98%9f%e6%9c%80%e6%96%b0nature%ef%bc%9a%e6%b0%af%e7%a2%b1%e5%b7%a5%e8%89%ba%e7%9a%84%e6%96%b0%e7%aa%81%e7%a0%b4","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=251020","title":{"rendered":"\u674e\u4e9a\u680b\u9662\u58eb\u56e2\u961f\u6700\u65b0Nature\uff1a\u6c2f\u78b1\u5de5\u827a\u7684\u65b0\u7a81\u7834"},"content":{"rendered":"

\u4e00\u3001<\/strong> \u3010\u5bfc\u8bfb\u3011<\/strong>\u00a0 <\/strong><\/p>\n

\u6c2f\u78b1\u6cd5\u6d41\u7a0b\u81ea19\u4e16\u7eaa\u4ee5\u6765\u4e00\u76f4\u5728\u8fd0\u884c\uff0c\u901a\u8fc7\u5bf9\u6c2f\u5316\u94a0\u6eb6\u6db2\u8fdb\u884c\u7535\u89e3\uff0c\u751f\u6210\u6c2f\u548c\u6c22\u6c27\u5316\u94a0\uff0c\u8fd9\u4e24\u79cd\u7269\u8d28\u90fd\u5bf9\u5316\u5b66\u5236\u9020\u4e1a\u975e\u5e38\u91cd\u8981\u3002\u7531\u4e8e\u8be5\u8fc7\u7a0b\u7684\u80fd\u91cf\u6d88\u8017\u975e\u5e38\u5927\uff0c\u5168\u7403\u751f\u4ea7\u7684\u7535\u529b4%\uff08\u7ea6150TWh\uff09\u7528\u4e8e\u6c2f\u78b1\u5de5\u4e1a\uff0c\u56e0\u6b64\u5373\u4f7f\u662f\u5c0f\u5e45\u5ea6\u7684\u6548\u7387\u63d0\u5347\u4e5f\u80fd\u5e26\u6765\u5927\u91cf\u7684\u6210\u672c\u548c\u80fd\u6e90\u8282\u7701\u3002\u5728\u6b64\u65b9\u9762\u7684\u7279\u522b\u5173\u6ce8\u70b9\u662f\u8981\u89e3\u51b3\u82db\u523b\u7684\u6790\u6c2f\u53cd\u5e94\u95ee\u9898\u3002\u867d\u7136\u5df2\u7ecf\u6709\u4e00\u4e9b\u65b0\u7684\u6790\u6c2f\u53cd\u5e94\u50ac\u5316\u5242\u62a5\u9053\uff0c\u4f46\u5b83\u4eec\u4ecd\u7136\u4e3b\u8981\u7531\u8d35\u91d1\u5c5e\u7ec4\u6210\u3002<\/p>\n

\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u6e05\u534e\u5927\u5b66\u674e\u4e9a\u680b\u9662\u58eb\u548c\u738b\u5b9a\u80dc\u526f\u6559\u6388\u56e2\u961f<\/strong>\u53d1\u73b0\u4e00\u79cd\u542b\u6709\u9170\u80fa\u57fa\u56e2\u7684\u6709\u673a\u5206\u5b50\uff08\u547d\u540d\u4e3aRCON-H\uff09\u80fd\u591f\u4ea7\u751f\u6c2f\uff0c\u800c\u52a0\u5165\u4e8c\u6c27\u5316\u78b3\u4f1a\u4ea7\u751f\u4e2d\u95f4\u4f53NCOOH\uff0c\u4ece\u800c\u6307\u6570\u589e\u5f3a\u50ac\u5316\u6548\u7387\u3002\u53cd\u5e94\u540e\uff0c\u57fa\u4e8e\u7269\u7406\u6027\u8d28\u53ef\u4ee5\u8f7b\u677e\u5c06CO2<\/sub>\u4e0eCl2<\/sub>\u5206\u79bb\u8fdb\u884c\u56de\u6536\u548c\u91cd\u590d\u4f7f\u7528\u3002\u6b64\u5916\uff0c\u867d\u7136CO2<\/sub>\u53ef\u4ee5\u901a\u8fc7\u5206\u79bb\u9633\u6781\u548c\u9634\u6781\u533a\u57df\u7684\u819c\uff0c\u7136\u800c\u7531\u4e8e\u901f\u7387\u8fc7\u4f4e\u4ee5\u81f3\u4e8e\u5bf9\u9634\u6781\u8fc7\u7a0b\u6ca1\u6709\u663e\u8457\u7684\u5f71\u54cd\u3002<\/p>\n

\u76f8\u5173\u7814\u7a76\u6587\u7ae0\u4ee5\u201cCO2<\/sub>-mediated organocatalytic chlorine evolution under industrial conditions<\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u00a0<\/strong>\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

    \n
  1. \u672c\u6587\u4f7f\u7528\u4e86\u4e00\u79cd\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u5b9e\u73b0\u4e86\u5b9e\u73b0\u6790\u6c2f\u53cd\u5e94\u3002<\/li>\n
  2. \u5728\u6709CO2<\/sub>\u5b58\u5728\u7684\u60c5\u51b5\u4e0b\uff0c\u5b83\u5728\u53ea\u670989 mV\u7684\u8fc7\u7535\u4f4d\u4e0b\u5b9e\u73b0\u4e8610 kA\/m2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u548c6%\u7684\u9009\u62e9\u6027\u3002<\/li>\n<\/ol>\n

    \u00a0<\/strong><\/p>\n

    \u00a0<\/strong>\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

    \u00a0\"\"<\/strong><\/p>\n

    \u56fe<\/strong>1<\/strong>\u6c2f\u5236\u5907\u7684\u793a\u610f\u56fe\u3002<\/strong>a<\/strong>\u3001\u672c\u7814\u7a76\u4e2d\u63a2\u8ba8\u7684\u6c2f\u78b1\u6cd5\u8fc7\u7a0b\u4e2d\u7684\u53cd\u5e94\u7269\u548c\u4ea7\u7269\u5f62\u6210\u3002\u5982\u56fe\u6240\u793a\uff0c\u8981\u91cd\u70b9\u5173\u6ce8\u9633\u6781\u5904\u9ad8\u6548\u4ea7\u751f<\/strong>Cl2<\/sub><\/strong>\u3002<\/strong>b<\/strong>\u3001\u53d1\u5c55\u7528\u4e8e\u7535\u5316\u5b66\u6c2f\u6c14\u6f14\u5316\u7684\u9633\u6781\u6750\u6599\u6982\u8ff0\u3002<\/strong>c<\/strong>\u3001\u6709\u673a\u50ac\u5316\u5242\u4e0a\u7684\u6c2f\u6c14\u6f14\u5316\uff0c\u7531<\/strong>CO2<\/sub><\/strong>\u4ecb\u5bfc\uff1b\u4f7f\u7528<\/strong>operando<\/strong>\u89c2\u6d4b\u548c\u7406\u8bba\u8ba1\u7b97\u63a2\u8ba8\u4e86\u673a\u7406\u7684\u7ec6\u8282\u3002<\/strong>SET<\/strong>\uff0c\u5355\u7535\u5b50\u8f6c\u79fb\u3002<\/strong>\u00a9 2023 Springer Nature<\/strong><\/p>\n

    \u00a0\"\"<\/strong><\/p>\n

    \u56fe<\/strong>2<\/strong> CER<\/strong>\u7684\u7535\u5316\u5b66\u8868\u5f81\u3002<\/strong>a<\/strong>\u3001\u5728<\/strong>90<\/strong>\u2103\u4e0b\uff0c<\/strong>NCOOH<\/strong>\u3001\u5e26\u6709<\/strong>iR<\/strong>\u6821\u6b63\u7684<\/strong>NCOOH<\/strong>\u3001<\/strong>RCON-H<\/strong>\u548c\u5e26\u6709<\/strong>iR<\/strong>\u6821\u6b63\u7684<\/strong>DSA<\/strong>\u7684\u6781\u5316\u66f2\u7ebf\u3002\u5728<\/strong>CO2<\/sub><\/strong>\u5b58\u5728\u4e0b\uff0c\u6709\u673a\u50ac\u5316\u5242\u7684\u6d3b\u6027\u5927\u5927\u589e\u52a0\u3002<\/strong>b<\/strong>\u3001<\/strong>NCOOH<\/strong>\u548c<\/strong>DSA<\/strong>\u7684\u8d28\u91cf\u6d3b\u6027\u3002<\/strong>c<\/strong>\u3001\u6bcf\u5428<\/strong>NaOH<\/strong>\u7684\u7528\u7535\u91cf\uff0c\u57fa\u4e8e\u5728\u4e00\u4e2a\u6c27\u5316\u6781\u5316\u9634\u6781\uff08<\/strong>ODC<\/strong>\uff09\u7cfb\u7edf\u4e0b\u8fdb\u884c\u7684\u5de5\u4e1a\u6761\u4ef6\u4e0b\u7684\u5b9e\u9a8c\u5916\u63a8\u3002\u6570\u636e\u662f\u81f3\u5c11\u56db\u4e2a\u72ec\u7acb\u5b9e\u9a8c\u7684\u5e73\u5747\u503c\u00b1\u6807\u51c6\u5dee\u3002<\/strong>d<\/strong>\u3001\u5728<\/strong>1.6 V<\/strong>\u65f6<\/strong>NCOOH<\/strong>\u3001<\/strong>RCON-H<\/strong>\u548c<\/strong>DSA<\/strong>\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31\u3002<\/strong>e<\/strong>\u3001<\/strong>NCOOH<\/strong>\u4f7f\u7528\u4e0d\u540c\u9891\u7387\u6d4b\u91cf\u7684\u7535\u5316\u5b66\u963b\u6297\u8c31\uff0c\u5728<\/strong>1.0<\/strong>\u81f3<\/strong>1.8 V vs. NHE<\/strong>\u7684\u7535\u4f4d\u8303\u56f4\u5185\u3002\u9891\u7387\u8303\u56f4\u4e3a<\/strong>1 Hz<\/strong>\u81f3<\/strong>10 Hz<\/strong>\uff08\u5373\uff0c<\/strong>1 Hz<\/strong>\u3001<\/strong>3 Hz<\/strong>\u3001<\/strong>5 Hz<\/strong>\u3001<\/strong>8 Hz<\/strong>\u548c<\/strong>10 Hz<\/strong>\uff09\u3002<\/strong>f<\/strong>\u3001<\/strong>NCOOH<\/strong>\u5bf9<\/strong>Cl2<\/sub><\/strong>\u548c<\/strong>O2<\/sub><\/strong>\u7684\u9009\u62e9\u6027\u3002\u6570\u636e\u662f\u81f3\u5c11\u4e09\u4e2a\u72ec\u7acb\u5b9e\u9a8c\u7684\u5e73\u5747\u503c\u00b1\u6807\u51c6\u5dee\u3002<\/strong>g<\/strong>\u3001\u5728\u6052\u5b9a\u7535\u6d41\u548c\u6052\u5b9a\u7535\u538b\u6761\u4ef6\u4e0b\u6d4b\u8bd5<\/strong>NCOOH<\/strong>\u7684\u7a33\u5b9a\u6027\u3002<\/strong>h<\/strong>\u3001\u96f7\u8fbe\u56fe\u603b\u7ed3\u4e86<\/strong>NCOOH<\/strong>\u7684\u50ac\u5316\u6027\u8d28\u3002\u5b9e\u9a8c<\/strong>a-f<\/strong>\u5728<\/strong>5 M NaCl<\/strong>\uff08<\/strong>pH=2<\/strong>\uff09\u4e2d\u4ee5<\/strong>10mV\/s<\/strong>\u7684\u626b\u63cf\u901f\u7387\u8fdb\u884c\u3002<\/strong>\u00a9 2023 Springer Nature<\/strong><\/p>\n

    \u00a0\"\"<\/strong><\/p>\n

    \u56fe<\/strong>3<\/strong>\u63a2\u7a76<\/strong>CER<\/strong>\u673a\u5236\u3002<\/strong>a<\/strong>\u3001<\/strong>b<\/strong>\u3001<\/strong>NCOOH<\/strong>\u7684\u539f\u4f4d<\/strong>ATR-SEIRAS<\/strong>\u3002<\/strong>c<\/strong>\u3001<\/strong>1a<\/strong>\u5728\u5747\u76f8\u7535\u5316\u5b66\u6d4b\u8bd5\u4e2d\u7684\u5faa\u73af\u4f0f\u5b89\u66f2\u7ebf\u3002\u7eff\u8272\u9634\u5f71\u533a\u57df\u6307\u7684\u662f\u6c27\u5316\u8fd8\u539f\u5cf0\u533a\u57df\uff0c\u7bad\u5934\u8868\u660e\u81ea\u7531\u57fa\u5f62\u6210\u7684\u6c27\u5316\u8fd8\u539f\u7535\u4f4d\u968f\u7740<\/strong>CO2<\/sub><\/strong>\u7684\u51cf\u5c11\u800c\u964d\u4f4e\u3002<\/strong>d<\/strong>\u3001\u5728<\/strong>CO2<\/sub><\/strong>\u5b58\u5728\u4e0b\u7684<\/strong>1.6 V CER 3<\/strong>\u5c0f\u65f6\u8fc7\u7a0b\u4e2d\uff0c<\/strong>1a<\/strong>\u7684\u539f\u4f4d\u65f6\u95f4\u5206\u8fa8<\/strong>ATR-SEIRAS<\/strong>\uff0c\u4ee5\u76d1\u6d4b\u4e2d\u95f4\u4f53\u7684\u5f62\u6210\u3002\u539f\u4f4d<\/strong>ATR-SEIRAS<\/strong>\u5206\u6790\u5728<\/strong>5 M NaCl<\/strong>\uff08<\/strong>pH=2<\/strong>\uff09\u4e2d\u8fdb\u884c\u3002\u5728<\/strong>c<\/strong>\u4e2d\uff0c<\/strong>1a<\/strong>\u6eb6\u89e3\u5728<\/strong>10 ml <\/strong>\u7532\u9187\u4e2d\uff08\u52a0\u5165<\/strong>0.1 mol\/l LiClO4<\/sub><\/strong>\u548c<\/strong>1 ml H2<\/sub>O<\/strong>\uff09\uff0c\u4ee5\u8fbe\u5230<\/strong>40 mmol\/l<\/strong>\u7684\u6d53\u5ea6\uff0c\u5e76\u52a0\u5165<\/strong>10 mM <\/strong>\u56db\u4e01\u57fa\u94f5\u76d0\u3002\u5728\u5145\u6ee1\u6c14\u4f53<\/strong>15<\/strong>\u5206\u949f\u4ee5\u4e0a\uff08<\/strong>200 sccm<\/strong>\uff09\u540e\u8fdb\u884c<\/strong>CO2<\/sub><\/strong>\u6d4b\u8bd5\uff0c\u7136\u540e\u4ee5<\/strong>100 mV\/s<\/strong>\u7684\u626b\u63cf\u901f\u7387\u5feb\u901f\u8fdb\u884c\u5faa\u73af\u4f0f\u5b89\u6d4b\u8bd5\u3002<\/strong>\u00a9 2023 Springer Nature<\/strong><\/p>\n

    \u00a0\"\"<\/strong><\/p>\n

    \u56fe<\/strong>4 CER<\/strong>\u6709\u673a\u50ac\u5316\u5242\u7684\u7ed3\u6784<\/strong>–<\/strong>\u6d3b\u6027\u76f8\u5173\u6027\u3002<\/strong>a<\/strong>\uff0c<\/strong>1a-Int-5-p<\/strong>\u7684\u9759\u7535\u52bf\u3002\u7ea2\u8272\u548c\u84dd\u8272\u533a\u57df\u8868\u793a\u76f8\u5bf9\u4e8e\u7b49\u503c\u9762\u503c\u4e3a<\/strong>0.03 e Bohr-3<\/strong>\u7684\u6b63\u7535\u9759\u7535\u52bf\u548c\u8d1f\u7535\u9759\u7535\u52bf\u503c\u3002\u5728\u53e0\u52a0\u7684\u5206\u5b50\u7ed3\u6784\u4e2d\uff0c\u78b3\u3001\u6c22\u3001\u6c27\u3001\u6c2e\u548c\u6c1f\u5206\u522b\u7528\u7070\u8272\u3001\u6d45\u7c89\u8272\u3001\u7ea2\u8272\u3001\u7d2b\u8272\u548c\u6df1\u7c89\u8272\u8868\u793a\u3002<\/strong>b<\/strong>\uff0c\u6295\u5f71\u5728<\/strong>x-y<\/strong>\u5e73\u9762\u4e0a\u7684<\/strong>1a-Int-5-p<\/strong>\u7684\u7535\u5b50\u5c40\u90e8\u5316\u51fd\u6570\u3002\u5728\u53e0\u52a0\u7684\u5206\u5b50\u7ed3\u6784\u4e2d\uff0c\u78b3\u3001\u6c22\u3001\u6c27\u3001\u6c2e\u548c\u6c1f\u5206\u522b\u7528\u68d5\u8272\u3001\u7c89\u8272\u3001\u7ea2\u8272\u3001\u84dd\u8272\u548c\u7d2b\u8272\u8868\u793a\u3002<\/strong>c<\/strong>\uff0c<\/strong>1a-Int-5-p<\/strong>\u7684\u7535\u5b50\u5bc6\u5ea6\u7684\u62c9\u666e\u62c9\u65af\u53d8\u6362\uff0c\u663e\u793a\u4e3a\u5728<\/strong>b<\/strong>\u4e2d\u6295\u5f71\u7684\u7b49\u9ad8\u7ebf\u3002\u84dd\u8272\u7b49\u9ad8\u7ebf\u8868\u793a\u76f8\u5bf9\u8f83\u9ad8\u7684\u62c9\u666e\u62c9\u65af\u7535\u5b50\u5bc6\u5ea6\u503c\u8d85\u8fc7<\/strong>1<\/strong>\uff0c\u56e0\u4e3a\u5b83\u4eec\u4ee3\u8868\u4e0e\u952e\u5408\u6210\u5206\u6709\u5173\u7684\u5c40\u90e8\u5316\u7535\u5b50\u3002\u5916\u90e8\u7684\u7ea2\u8272\u7b49\u9ad8\u7ebf\u5927\u591a\u4e0e\u4ef7\u7535\u5b50\u4e0d\u952e\u5408\uff0c\u53ef\u80fd\u8d1f\u8d23\u53cd\u5e94\u3002\u84dd\u8272\u7bad\u5934\u6307\u5411\u5176\u4e2d\u4e00\u4e2a\u6c2e\u539f\u5b50\uff0c\u7a81\u51fa\u663e\u793a\u4e0e\u5f62\u6210\u952e\u7684\u7535\u5b50\u533a\u57df\u76f8\u90bb\u7684\u7ea2\u8272\u7b49\u9ad8\u7ebf\u5b58\u5728\u4e0d\u8fde\u7eed\u6027\u3002\u4e0d\u8fde\u7eed\u6027\u8868\u660e\uff0c\u867d\u7136\u7535\u5b50\u4ecd\u7136\u5b58\u5728\uff0c\u4f46\u7535\u5b50\u5bc6\u5ea6\u5728\u6cbf\u7740\u7bad\u5934\u65b9\u5411\u7684\u8fd9\u4e2a\u4f4d\u7f6e\u5feb\u901f\u4e0b\u964d\uff0c\u4ece\u800c\u4fc3\u8fdb\u4e86\u4eb2\u6838\u8bd5\u5242\u5982<\/strong>Cl–<\/sup><\/strong>\u7684\u8fdb\u653b\u3002\u8bf7\u6ce8\u610f\uff0c<\/strong>x<\/strong>\u8f74\u4e5f\u9002\u7528\u4e8e<\/strong>b<\/strong>\u3002<\/strong>d<\/strong>\uff0c\u53bb\u9664\u6216\u66f4\u6539\u5b98\u80fd\u56e2\u4ee5\u63a2\u7d22\u9170\u80fa\u6216\u4e9a\u80fa\uff08<\/strong>-NH<\/strong>\uff09\u5b98\u80fd\u56e2\u7684\u7535\u50ac\u5316\u4f5c\u7528\u7684\u6709\u673a\u50ac\u5316\u5242\u53d8\u4f53\u3002<\/strong>e<\/strong>\uff0c<\/strong>d<\/strong>\u4e2d\u663e\u793a\u7684\u6709\u673a\u50ac\u5316\u5242\u7684<\/strong>CER<\/strong>\u6027\u80fd\uff0c\u4ee5\u5b83\u4eec\u5728<\/strong>10 mA\/cm2<\/sup><\/strong>\u548c<\/strong>1.6 V<\/strong>\u5904\u7684\u8d85\u7535\u52bf\u548c\u7535\u8377\u4f20\u9012\u7535\u963b\uff08<\/strong>Rct<\/sub><\/strong>\uff09\u8868\u793a\u3002<\/strong>\u00a9 2023 Springer Nature<\/strong><\/p>\n

     <\/p>\n

    \u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

    \u672c\u6587\u8868\u660e\uff0c\u5177\u6709\u9170\u80fa\u5b98\u80fd\u56e2\u7684\u6709\u673a\u50ac\u5316\u5242\u53ef\u4fc3\u8fdb\u6c2f\u79bb\u5b50\u7535\u5316\u5b66\u6c27\u5316\u53cd\u5e94\uff1b\u5728CO2<\/sub>\u5b58\u5728\u7684\u60c5\u51b5\u4e0b\uff0c\u5176\u572889 mV\u7684\u8fc7\u7535\u4f4d\u4e0b\u5b9e\u73b0\u4e8610 kA\/m2<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u548c99.6%\u7684\u9009\u62e9\u6027\u3002\u4f5c\u8005\u53d1\u73b0\uff0cCO2<\/sub>\u53ef\u9006\u5730\u4e0e\u9170\u80fa\u6c2e\u5f62\u6210\u7ed3\u5408\u7269\uff0c\u4fc3\u8fdb\u4e86\u751f\u6210\u5173\u952e\u7684\u81ea\u7531\u57fa\u7269\u79cd\uff0c\u8fd9\u5728\u6c2f\u79bb\u5b50\u7535\u6c60\u548c\u6709\u673a\u5408\u6210\u7b49\u9886\u57df\u4e5f\u53ef\u80fd\u5177\u6709\u5b9e\u7528\u4ef7\u503c\u3002\u5c3d\u7ba1\u6709\u673a\u50ac\u5316\u5242\u901a\u5e38\u4e0d\u88ab\u8ba4\u4e3a\u662f\u9002\u5408\u82db\u6c42\u7535\u5316\u5b66\u5e94\u7528\u7684\u6709\u524d\u9014\u7684\u50ac\u5316\u5242\uff0c\u4f46\u672c\u6587\u8bc1\u5b9e\u4e86\u5b83\u4eec\u66f4\u5e7f\u6cdb\u7684\u6f5c\u529b\uff0c\u4ee5\u53ca\u5728\u5f00\u53d1\u5de5\u4e1a\u76f8\u5173\u7684\u65b0\u5de5\u827a\u548c\u63a2\u7d22\u65b0\u7535\u5316\u5b66\u673a\u5236\u65b9\u9762\u6240\u63d0\u4f9b\u7684\u673a\u4f1a\u3002<\/p>\n

     <\/p>\n

    \u539f\u6587\u8be6\u60c5<\/strong>\uff1aYang, J., Li, WH., Tang, HT. et al. CO2-mediated organocatalytic chlorine evolution under industrial conditions. Nature 617, 519\u2013523 (2023). https:\/\/doi.org\/10.1038\/s41586-023-05886-z<\/p>\n

     <\/p>\n

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