{"id":251271,"date":"2023-06-10T06:28:44","date_gmt":"2023-06-09T22:28:44","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=251271"},"modified":"2023-06-09T19:28:55","modified_gmt":"2023-06-09T11:28:55","slug":"%e6%9c%80%e6%96%b0nature-energy-%e7%8b%ac%e7%ab%8b%e4%ba%ba%e9%80%a0%e5%8f%b6%e7%89%87%e4%ba%a7%e5%a4%9a%e7%a2%b3%e9%86%87%e6%b6%b2%e4%bd%93%e7%87%83%e6%96%99","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=251271","title":{"rendered":"\u6700\u65b0Nature Energy: \u72ec\u7acb\u4eba\u9020\u53f6\u7247\u4ea7\u591a\u78b3\u9187\u6db2\u4f53\u71c3\u6599"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/span><\/p>\n

\u00a0 <\/strong>\u00a0\u5c06\u6e29\u5ba4\u6c14\u4f53\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u4e3a\u71c3\u6599\u7684\u65b9\u6cd5\u901a\u5e38\u662f\u901a\u8fc7\u4e00\u79cd\u88ab\u79f0\u4e3a\u201c\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u201d\u7684\u751f\u7269\u542f\u53d1\u8fc7\u7a0b\u6765\u5b9e\u73b0\u7684\uff0c\u5728\u8fd9\u79cd\u8fc7\u7a0b\u4e2d\uff0c\u592a\u9633\u80fd\u4ee5\u5316\u5b66\u80fd\u7684\u5f62\u5f0f\u50a8\u5b58\u5728\u4ea7\u54c1\u4e2d\u3002\u9ad8\u80fd\u91cf\u5bc6\u5ea6\u7684\u542b\u6c27\u5316\u5408\u7269\uff0c\u5982\u591a\u78b3\u9187\uff0c\u662f\u7279\u522b\u6709\u5438\u5f15\u529b\u7684\u4ea7\u54c1\uff0c\u56e0\u4e3a\u5b83\u4eec\u6613\u4e8e\u50a8\u5b58\u3001\u8fd0\u8f93\u548c\u53ef\u76f4\u63a5\u7528\u4f5c\u6db2\u4f53\u71c3\u6599\u3002\u76ee\u524d\u5f88\u591a\u7814\u7a76\u96c6\u4e2d\u5728\u63a2\u7d22\u5c06\u4e8c\u6c27\u5316\u78b3\u7535\u5316\u5b66\u8f6c\u5316\u4e3a\u591a\u78b3\u9187\uff0c\u800c\u5728\u4eba\u5de5\u53f6\u7247\u4e0a\u76f4\u63a5\u5229\u7528\u592a\u9633\u80fd\u5c06\u542b\u6c34\u4e8c\u6c27\u5316\u78b3\u8f6c\u53d8\u6210\u591a\u78b3\u9187\u7684\u65b9\u6cd5\u56e0\u5176\u73af\u4fdd\u4e5f\u5f00\u59cb\u5907\u53d7\u5173\u6ce8\u3002\u76ee\u524d\u8fd9\u9879\u7814\u7a76\u5c1a\u672a\u88ab\u8bc1\u660e\u662f\u80fd\u591f\u53ef\u6301\u7eed\u5730\u751f\u4ea7\u591a\u78b3\u6db2\u4f53\u71c3\u6599\u7684\u65b9\u6cd5\u3002\u56e0\u6b64\uff0c\u5408\u7406\u8bbe\u8ba1\u548c\u5f00\u53d1\u4eba\u9020\u6811\u53f6\u5b9e\u73b0\u53ef\u6301\u7eed\u201c\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u201d\u662f\u76ee\u524d\u5149\u50ac\u5316\u9886\u57df\u6700\u6d3b\u8dc3\u7684\u7814\u7a76\u4e4b\u4e00\u3002<\/p>\n

 <\/p>\n

\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/span><\/p>\n

\u00a0 <\/strong>\u00a0\u8fd1\u65e5\uff0c\u5251\u6865\u5927\u5b66Erwin Reisner\u6559\u6388\u7b49\u4eba\u5c06\u6c27\u5316\u7269\u884d\u751f\u7684Cu94<\/sub>Pd6<\/sub>\u7535\u50ac\u5316\u5242\u4e0e\u9499\u949b\u77ff-BiVO4<\/sub>\u4e32\u8054\u5149\u5438\u6536\u5242\u76f8\u7ed3\u5408\u6765\u7ec4\u88c5\u6210\u4eba\u9020\u6811\u53f6\uff0c\u8be5\u4eba\u9020\u6811\u53f6\u88c5\u7f6e\u53ef\u5b9e\u73b0\u9ad8\u6548\u591a\u78b3\u9187\u751f\u4ea7\u3002\u76f8\u5173\u7684\u7814\u7a76\u6210\u679c\u4ee5\u201cSolar-driven liquid multi-carbon fuel production using a standalone perovskite\u2013BiVO4<\/sub> artificial leaf<\/strong> <\/em>\u201d\u4e3a\u9898\u53d1\u8868\u5728Nature Energy<\/em><\/strong>\u4e0a\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/span><\/p>\n

1\u3001\u4f5c\u8005\u63d0\u51fa<\/strong>\u4e00\u79cd\u72ec\u7acb\u7684\u4eba\u9020\u6811\u53f6\u88c5\u7f6e\uff0c\u8be5\u88c5\u7f6e\u7531\u6d3b\u5316\u7684<\/strong>Cu94<\/sub>Pd6<\/sub><\/strong>\u53cc\u91d1\u5c5e\u50ac\u5316\u5242\u4e0e\u65e0\u504f\u538b\u9499\u949b\u77ff<\/strong>–<\/strong>BiVO4<\/sub><\/strong>\u4e32\u8054\u88c5\u7f6e\u8fde\u63a5\uff0c\u53ef\u5728<\/strong>1<\/strong>\u6b21\u9633\u5149\u7167\u5c04\u4e0b\u76f4\u63a5\u4ece<\/strong>CO2<\/sub><\/strong>\u6c34\u6eb6\u6db2\u548c\u6c34\u4e2d\u751f\u4ea7\u591a\u78b3\uff08<\/strong>C\u00a02,3<\/sub><\/strong>\uff09<\/strong>\u4ea7\u7269\u3002<\/strong><\/p>\n

2<\/strong>\u3001<\/strong>\u6709\u7ebf<\/strong>Cu94<\/sub>Pd6<\/sub><\/strong>|<\/strong>\u9499\u949b\u77ff<\/strong>–<\/strong>BiVO4<\/sub><\/strong>\u4e32\u8054\u8bbe\u5907\u5bf9\u591a\u78b3\u9187\uff08\u7ea6<\/strong>1:1 <\/strong>\u4e59\u9187\u548c\u6b63\u4e19\u9187\uff09\u5b9e\u73b0<\/strong>~7.5%<\/strong> \u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff0c\u800c\u65e0\u7ebf\u72ec\u7acb\u8bbe\u5907\u5728<\/strong>1.5 G<\/strong>\u548c<\/strong>~40 \u00b5mol h\u22121<\/sup>g\u00a0Cu94Pd6\u00a0<\/sub>\u22121<\/sup><\/strong>\u7684\u901f\u7387\u8f90\u5c04\u4e0b\u72ec\u7acb\u8fd0\u884c<\/strong> 20 <\/strong>\u5c0f\u65f6\u540e\u4ea7\u751f<\/strong>~1 \u00b5mol cm-2<\/sup><\/strong>\u9187\u3002<\/strong><\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/span><\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>1<\/strong> \u53cc\u91d1\u5c5e\u50ac\u5316\u5242\u7684\u4eba\u9020\u6811\u53f6\u6982\u89c8\u548c\u7269\u7406\u7279\u6027\u3002\u00a92023 Springer Nature<\/p>\n

\"\"<\/p>\n

\u56fe2<\/strong> \u00a0\u6d3b\u5316\u7684Cux<\/sub>Pdy<\/sub>\u50ac\u5316\u5242\u7684\u7535\u5316\u5b66\u5206\u6790\u3002\u00a92023 Springer Nature<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>3<\/strong> \u5728\u4f4e\u8fc7\u7535\u52bf\u4e0b\u6d3b\u5316\u7684Cu94<\/sub>Pd6<\/sub>\u50ac\u5316\u5242\u4e0a\u591a\u78b3\u751f\u4ea7\u7684\u673a\u7406\u5206\u6790\u3002\u00a92023 Springer Nature<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4<\/strong>\u4f7f\u7528\u6709\u7ebf\u4e32\u8054BiVO4<\/sub>\u00a0\u2013 \u9499\u949b\u77ffCu94<\/sub>Pd6<\/sub>\u8bbe\u5907\u548c\u65e0\u7ebf\u72ec\u7acb\u4eba\u9020\u53f6\u7684\u65e0\u8f85\u52a9\u591a\u78b3\u9187\u751f\u4ea7\u3002\u00a92023 Springer Nature<\/p>\n

\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/span><\/p>\n

\u00a0 \u7efc\u4e0a\u6240\u8ff0\u3002\u4f5c\u8005\u901a\u8fc7\u6d3b\u5316\u7684Cu94<\/sub>Pd6<\/sub>\u53cc\u91d1\u5c5e\u50ac\u5316\u5242\u4e0e\u65e0\u504f\u538b\u9499\u949b\u77ff-BiVO4<\/sub>\u4e32\u8054\u88c5\u7f6e\u8fde\u63a5\u63d0\u51fa\u4e00\u79cd\u72ec\u7acb\u7684\u4eba\u9020\u6811\u53f6\u88c5\u7f6e\u5b9e\u73b0\u9ad8\u6548\u7684\u592a\u9633\u80fd\u5236\u591a\u78b3\u9187\u7b56\u7565\u3002\u76f8\u5206\u79bb\u7684Cu94<\/sub>Pd6<\/sub>\u53cc\u91d1\u5c5e\u6750\u6599\u5728\u4f4e\u8fc7\u7535\u4f4d\u4e0b\u5bf9\u591a\u78b3\u751f\u6210\u5177\u6709\u7535\u50ac\u5316\u6d3b\u6027\u3002DFT \u8ba1\u7b97\u8868\u660e\uff0cCu \u57fa\u56e2\u4e2dPd\u7684\u5b58\u5728\u6539\u5584\u4e86*CO\u5438\u9644\u548c\u7a33\u5b9a\u6027\uff0c\u800c\u539f\u4f4d\u62c9\u66fc\u7814\u7a76\u663e\u793a\u5373\u4f7f\u57280 V\uff08\u76f8\u5bf9\u4e8e RHE\uff09\u65f6\u4e5f\u6709\u5f3a*CO \u5438\u9644\u5cf0\uff0c\u8868\u660e\u6d3b\u5316\u50ac\u5316\u5242\u9002\u7528\u4e8e\u591a\u78b3\u9187\u5728\u975e\u5e38\u4f4e\u7684\u8fc7\u7535\u4f4d\u4e0b\u751f\u4ea7\u3002\u56e0\u6b64\uff0c\u8fd9\u9879\u7814\u7a76\u5f00\u53d1\u7684\u65b0\u578b\u4eba\u9020\u6811\u53f6\u7cfb\u7edf\u6210\u529f\u5730\u5b9e\u73b0\u4e86\u5728\u4eba\u9020\u6811\u53f6\u4e0a\u5c06CO2<\/sub>\u76f4\u63a5\u8f6c\u5316\u4e3a\u591a\u78b3\u6db2\u4f53\u71c3\u6599\u3002\u5e76\u4e14\u8fd9\u9879\u7814\u7a76\u4e5f\u4fc3\u4f7f\u6211\u4eec\u52a0\u5feb\u4e86\u5229\u7528\u592a\u9633\u5149\u751f\u4ea7\u5177\u6709\u9644\u52a0\u503c\u7684\u590d\u6742\u4ea7\u54c1\u7684\u8fdb\u7a0b\u3002<\/strong><\/p>\n

\u00a0<\/strong><\/p>\n

\u539f\u6587\u8be6\u60c5\uff1a<\/strong> https:\/\/doi.org\/10.1038\/s41560-023-01262-3<\/p>\n

\u672c\u6587\u7531K . L\u64b0\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011 \u00a0 \u00a0\u5c06\u6e29\u5ba4\u6c14\u4f53\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u4e3a\u71c3\u6599\u7684\u65b9\u6cd5\u901a\u5e38\u662f\u901a\u8fc7\u4e00\u79cd\u88ab\u79f0\u4e3a\u201c\u4eba\u5de5\u5149\u5408\u4f5c\u7528\u201d\u7684\u751f\u7269\u542f\u53d1\u8fc7\u7a0b\u6765\u5b9e\u73b0\u7684\uff0c\u5728\u8fd9\u79cd\u8fc7\u7a0b\u4e2d\uff0c\u592a\u9633\u80fd\u4ee5\u5316\u5b66\u80fd\u7684\u5f62\u5f0f\u50a8\u5b58\u5728\u4ea7\u54c1\u4e2d…<\/p>\n","protected":false},"author":48789,"featured_media":251272,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[5063],"class_list":["post-251271","post","type-post","status-publish","format-standard","has-post-thumbnail","hentry","category-jiedu","tag-5063"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/251271"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/48789"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=251271"}],"version-history":[{"count":2,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/251271\/revisions"}],"predecessor-version":[{"id":251920,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/251271\/revisions\/251920"}],"wp:featuredmedia":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/media\/251272"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=251271"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=251271"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=251271"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}