{"id":253157,"date":"2023-07-31T06:03:29","date_gmt":"2023-07-30T22:03:29","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=253157"},"modified":"2023-07-30T21:03:41","modified_gmt":"2023-07-30T13:03:41","slug":"%e9%87%8d%e5%ba%86%e5%a4%a7%e5%ad%a6nat-catal-%ef%bc%9a%e6%83%b3%e8%a6%81%e6%8f%90%e9%ab%98pt%e5%9c%a8mea%e4%b8%ad%e7%9a%84%e5%82%ac%e5%8c%96%e6%80%a7%e8%83%bd%ef%bc%8c%e8%af%95%e8%af%95%e5%8a%a0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=253157","title":{"rendered":"\u91cd\u5e86\u5927\u5b66Nat. Catal.\uff1a\u60f3\u8981\u63d0\u9ad8Pt\u5728MEA\u4e2d\u7684\u50ac\u5316\u6027\u80fd\uff0c\u8bd5\u8bd5\u52a0\u70b9\u73af\u5df1\u9187"},"content":{"rendered":"<p><strong>\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p>\u94c2\u57fa\u7eb3\u7c73\u6750\u6599\u88ab\u8ba4\u4e3a\u662f\u8d28\u5b50\u4ea4\u6362\u819c\u71c3\u6599\u7535\u6c60\uff08PEMFC\uff09\u6700\u6709\u6548\u7684\u50ac\u5316\u5242\u7136\u800c\u5176\u9ad8\u6602\u7684\u6210\u672c\u963b\u788d\u4e86PEMFC\u7684\u5e7f\u6cdb\u5e94\u7528\u3002\u5728\u65cb\u8f6c\u5706\u76d8\u7535\u6781\uff08RDE\uff09\u4e2d\uff0c\u6240\u6709\u57fa\u4e8e\u94c2\u7684\u7eb3\u7c73\u9897\u7c92\u90fd\u6d78\u6ce1\u5728\u6db2\u4f53\u7535\u89e3\u8d28\u4e2d\uff0c\u53ef\u4ee5\u901a\u8fc7\u6c34\u5408\u8d28\u5b50\u548c\u7535\u89e3\u8d28\u4f20\u8f93\u7684\u6eb6\u89e3\u6c27\u4e0e\u6eb6\u6db2\u5b8c\u5168\u63a5\u89e6\uff1b\u5bf9\u4e8e\u819c\u7535\u6781\uff08MEA\uff09\uff0c\u8d28\u5b50\u8f93\u8fd0\u53d1\u751f\u5728\u8986\u76d6\u50ac\u5316\u5242\u8868\u9762\u7684\u5168\u6c1f\u78fa\u9178\uff08PFSA\uff09\u79bb\u805a\u4f53\u5c42\uff08\u4f8b\u5982Nafion\uff09\u4e0a\uff0c\u5e76\u4e14\u6c14\u4f53O<sub>2<\/sub>\u9010\u6e10\u6e17\u900f\u901a\u8fc7\u8986\u76d6\u7684\u79bb\u805a\u4f53\u5c42\uff08&lt;10 nm\u539a\uff09\u5230\u8fbePt\u8868\u9762\u3002\u78fa\u9178\u57fa\u56e2\u5728Pt\u8868\u9762\u7684\u5f3a\u70c8\u5438\u9644\u9650\u5236\u4e86Nafion\u79bb\u805a\u4f53\u7684\u4fa7\u94fe\u4eb2\u6c34\u4f5c\u7528\uff0c\u4ece\u800c\u964d\u4f4e\u4e86\u79bb\u805a\u4f53\u7684\u5fae\u76f8\u5206\u79bb\uff0c\u5bfc\u81f4\u8d28\u91cf\u4f20\u8f93\u963b\u529b\u8fdb\u4e00\u6b65\u589e\u52a0\u3002\u6b64\u5916\uff0c\u78fa\u9178\u76d0\u57fa\u56e2\u53ef\u4ee5\u4e25\u91cd\u6bd2\u5bb3\u94c2\u4f4d\u70b9\uff0c\u5e76\u663e\u7740\u964d\u4f4e\u94c2\u7684\u8d28\u91cf\u6d3b\u6027\u3002\u56e0\u6b64\uff0c\u6d88\u9664\u79bb\u805a\u4f53\u5c42\u5bf9\u94c2\u7684\u6709\u5bb3\u5f71\u54cd\uff0c\u4ee5\u5f7b\u5e95\u91ca\u653e\u94c2\u5728MEA\u4e2d\u7684\u6027\u80fd\u662f\u4e00\u4e2a\u5f88\u5927\u7684\u6311\u6218\u3002<\/p>\n<p><strong>\u00a0<\/strong><strong>\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n<p>\u57fa\u4e8e\u6b64\uff0c<strong>\u91cd\u5e86\u5927\u5b66\u9b4f\u5b50\u680b\u6559\u6388\u3001\u9648\u56db\u56fd\u526f\u6559\u6388\u548c\u4e2d\u77f3\u5316\u77f3\u6cb9\u5316\u5de5\u79d1\u5b66\u7814\u7a76\u9662\u90ed\u7433<\/strong>\u7b49\u62a5\u9053\u4e86\u4e00\u79cd\u4f7f\u7528\u73af\u5df1\u9187\u7684\u963b\u65ad\u7b56\u7565\uff0c\u4ee5\u7cbe\u786e\u5c01\u95edNafion\u7684\u78fa\u9178\u57fa\u56e2\u4ee5\u63d0\u9ad8Pt\u5728MEA\u4e2d\u7684\u50ac\u5316\u6027\u80fd\u3002\u7ed3\u679c\u663e\u793a\uff0c\u5728\u73af\u5df1\u9187\u50ac\u5316\u5242\u5c42\u4e2d\uff0cPt\u8868\u9762\u7684\u78fa\u9178\u57fa\u56e2\u8986\u76d6\u7387\u964d\u4f4e\u52307%\uff0c\u8fdc\u4f4e\u4e8e\u4ec5\u4f7f\u7528Nafion\u79bb\u805a\u4f53\u7684\u50ac\u5316\u5242\u5c42\uff0821%\uff09\u3002\u5728\u71c3\u6599\u7535\u6c60\u5b9e\u9a8c\u4e2d\uff0c\u4e0e\u5355\u72ec\u4f7f\u7528Nafion\u79bb\u805a\u4f53\u7684MEA\u76f8\u6bd4\uff0c\u7528\u73af\u5df1\u9187\u5236\u5907\u7684MEA\u5728\u52a8\u529b\u5b66\u6d3b\u6027\u8868\u73b0\u51fa\u660e\u663e\u7684\u6027\u80fd\u63d0\u9ad8\uff0c\u5e76\u4e14\u8868\u73b0\u51fa\u66f4\u597d\u7684\u8d28\u91cf\u4f20\u8f93\u6027\u80fd\u3002\u5728\u76f8\u5e94\u7684MEA\u4e2d\uff0cNafion\u79bb\u805a\u4f53\u4e2d\u7684\u73af\u5df1\u9187\u7ecf\u8fc7\u957f\u671f\u6052\u7535\u4f4d\u6d4b\u8bd5\u548c30000\u4e2a\u5faa\u73af\u540e\u663e\u793a\u51fa\u4f18\u5f02\u7684\u7a33\u5b9a\u6027\u3002\u672c\u7814\u7a76\u63d0\u51fa\u7684\u7b56\u7565\u4e3a\u8c03\u8282Pt\/\u79bb\u805a\u7269\u754c\u9762\u548c\u63d0\u9ad8Pt\u5728MEA\u4e2d\u7684\u50ac\u5316\u6d3b\u6027\u63d0\u4f9b\u4e86\u65b9\u5411\u3002\u7814\u7a76\u6210\u679c\u4ee5\u9898\u4e3a\u201c<strong>Blocking the Sulfonate Group in Nafion to Unlock Platinum\u2019s Activity in Membrane Electrode Assemblies<\/strong>\u201d\u53d1\u8868\u5728\u77e5\u540d\u671f\u520a<strong><em>Nature Catalysis<\/em><\/strong>\u4e0a\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-253158\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/0-5.png\" alt=\"\" width=\"600\" height=\"264\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/0-5.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/0-5-300x132.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n<p>\u5f00\u53d1\u4e86\u4e00\u79cd\u6709\u6548\u7684\u7b56\u7565\uff0c\u901a\u8fc7\u7528\u73af\u5df1\u9187\u7cbe\u786e\u963b\u65adNafion\u7684\u78fa\u9178\u57fa\u56e2\u6765\u63d0\u9ad8Pt\u5728MEA\u4e2d\u7684\u50ac\u5316\u6027\u80fd\uff0c\u5728\u71c3\u6599\u7535\u6c60\u5b9e\u9a8c\u4e2d\uff0c\u7528\u73af\u5df1\u9187\u5236\u5907\u7684MEA\u5728\u52a8\u529b\u5b66\u6d3b\u6027\u548c\u7a33\u5b9a\u6027\u8868\u73b0\u51fa\u660e\u663e\u7684\u6027\u80fd\u63d0\u9ad8\u3002<\/p>\n<p><strong>\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n<p><strong>\u00a0<img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-253159\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/1-12.png\" alt=\"\" width=\"600\" height=\"764\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/1-12.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/1-12-236x300.png 236w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/strong><\/p>\n<p><strong>\u56fe<\/strong><strong>1\u00a0 <\/strong><strong>\u73af\u5df1\u9187<\/strong><strong>-Nafion<\/strong><strong>\u7684\u7ed3\u6784\u8868\u5f81<\/strong><strong>\u00a9 2023 Springer Nature<\/strong><\/p>\n<p>\uff08a\uff09\u4f20\u7edf\u7684\u63a5\u89e6Pt\/\u79bb\u805a\u4f53\u754c\u9762\u548c\u9634\u6781\u50ac\u5316\u5242\u5c42\u7684\u975e\u63a5\u89e6Pt\/\u79bb\u805a\u4f53\u7a7a\u95f4\u793a\u610f\u56fe\u3002<\/p>\n<p>\uff08b\uff09\u73af\u5df1\u9187\u3001\u73af\u5df1\u9187-Nafion\u79bb\u805a\u7269\u548cNafion\u79bb\u805a\u4f53\u5728DMSO-<em>d<\/em><sub>6<\/sub>\u4e2d\u7684<sup>1<\/sup>H NMR\u3002<\/p>\n<p>\uff08c\uff09\u73af\u5df1\u9187\u3001\u5e72\u71e5\u73af\u5df1\u9187-Nafion-HP\u819c\u548cNafion-HP\u819c\u7684ATR-FTIR\u5149\u8c31\u3002<\/p>\n<p>\uff08d-e\uff09Nafion\u79bb\u805a\u7269-Pt\/C\u3001\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u548cJM-Pt\/C\u5728\u50ac\u5316\u5242\u5c42\u4e2d\u7684C 1<em>s<\/em>\u548cPt 4<em>f<\/em> XPS\u5149\u8c31\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-253160\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/2-11.png\" alt=\"\" width=\"600\" height=\"516\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/2-11.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/2-11-300x258.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u56fe<\/strong><strong>2\u00a0 <\/strong><strong>\u73af\u5df1\u9187\u63ba\u5165\u5bf9<\/strong><strong>Nafion<\/strong><strong>\u819c\u5fae\u76f8\u5206\u79bb\u548c\u8d28\u5b50\u7535\u5bfc\u7387\u7684\u5f71\u54cd<\/strong><strong> \u00a9 2023 Springer Nature<\/strong><\/p>\n<p>\uff08a-b\uff09\u5e72\u71e5\u7684Nafion HP\u819c\u548c\u5e72\u71e5\u7684\u73af\u5df1\u9187-Nafion HP\u819c\u76842D SAXS\u56fe\u8c31\u3002<\/p>\n<p>\uff08c\uff09\u901a\u8fc7\u5bf92D SAXS\u56fe\u8c31\u8fdb\u884c\u79ef\u5206\uff0c\u83b7\u5f97\u4e86\u5e72\u71e5\u7684Nafion HP\u819c\u548c\u5e72\u71e5\u7684\u73af\u5df1\u9187-Nafion HP\u819c\u7684\u76f8\u5e94SAXS\u5149\u8c31\u3002<\/p>\n<p>\uff08d\uff09\u5728\u4e0d\u540c\u6e29\u5ea6\uff0825\u2103\uff0c40\u2103\uff0c60\u2103\u548c80\u2103\uff09\u7684\u6c34\u4e2d\uff0c\u5229\u7528EIS\u8ba1\u7b97\u7684Nafion HP\u548c\u73af\u5df1\u9187-Nafion HP\u819c\u7684\u5e73\u9762\u5185\u8d28\u5b50\u7535\u5bfc\u7387\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-253161\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/3-11.png\" alt=\"\" width=\"600\" height=\"315\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/3-11.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/3-11-300x158.png 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u56fe<\/strong><strong>3\u00a0 <\/strong><strong>\u71c3\u6599\u7535\u6c60\u4e2d\u73af\u5df1\u9187<\/strong><strong>-Nafion<\/strong><strong>\u79bb\u805a\u7269<\/strong><strong>Pt\/C<\/strong><strong>\u9634\u6781\u7684\u7535\u5316\u5b66\u8bc4\u4ef7<\/strong><strong> \u00a9 2023 Springer Nature<\/strong><\/p>\n<p>\uff08a-b\uff09Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42\u7684CV\u66f2\u7ebf\u548cCO-stripping\u66f2\u7ebf\u3002<\/p>\n<p>\uff08c\uff09\u8ba1\u7b97ECSA\u503c\u3002<\/p>\n<p>\uff08d\uff09\u57280.4 V\u4e0b\u5206\u522b\u6d4b\u91cf\u4e86Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42\u7684\u5171\u4f4d\u79fb\u7535\u6d41\u5bc6\u5ea6-\u65f6\u95f4\u66f2\u7ebf\u3002<\/p>\n<p>\uff08e\uff09\u901a\u8fc70.4 V\u4e0bCO\u7f6e\u6362\u4ee5\u53ca\u8131\u9644\u6d4b\u91cf\u7684Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u4e2d\u78fa\u9178\u57fa\u8986\u76d6\u7387\u3002<\/p>\n<p>\uff08f\uff09\u57280.1 V\u4e0b\u6d4b\u91cf\u7684\u5171\u4f4d\u79fb\u7535\u6d41\u5bc6\u5ea6-\u65f6\u95f4\u66f2\u7ebf\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-253162\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/4-11.png\" alt=\"\" width=\"600\" height=\"650\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/4-11.png 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2023\/07\/4-11-277x300.png 277w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><strong>\u56fe<\/strong><strong>4\u00a0 <\/strong><strong>\u73af\u5df1\u9187\u63ba\u5165\u5bf9\u71c3\u6599\u7535\u6c60\u6027\u80fd\u7684\u5f71\u54cd<\/strong><strong> \u00a9 2023 Springer Nature<\/strong><\/p>\n<p>\uff08a\uff09Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42H<sub>2<\/sub>-O<sub>2<\/sub>\u71c3\u6599\u7535\u6c60\u7684\u6027\u80fd\u3002<\/p>\n<p>\uff08b\uff09\u5728H<sub>2<\/sub>-O<sub>2<\/sub>\u6761\u4ef6\u4e0b\u6d4b\u5b9a\u4e86Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42\u7684HFR\u6821\u6b63Tafel\u56fe\u3002<\/p>\n<p>\uff08c\uff09Nafion\u79bb\u805a\u4f53-Pt\/C\u548c\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42H<sub>2<\/sub>-\u7a7a\u6c14\u71c3\u6599\u7535\u6c60\u7684\u6027\u80fd\u3002<\/p>\n<p>\uff08d\uff09\u5728H<sub>2<\/sub>-\u7a7a\u6c14\u6761\u4ef6\u4e0b\uff0c\u8f93\u51fa\u7535\u6d41\u5bc6\u5ea6\u4e3a1 A cm<sup>-2<\/sup>\u65f6\u6d4b\u91cf\u7684\u539f\u4f4dEIS\u66f2\u7ebf\u3002<\/p>\n<p>\uff08e\uff09\u73af\u5df1\u9187-Nafion\u79bb\u805a\u4f53-Pt\/C\u50ac\u5316\u5242\u5c42\u57280.6 V H<sub>2<\/sub>-\u7a7a\u6c14\u71c3\u6599\u7535\u6c60\u4e2d\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5\u3002<\/p>\n<p><strong>\u00a0<\/strong><\/p>\n<p><strong>\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n<p>\u7814\u7a76\u4eba\u5458\u6210\u529f\u5730\u5f00\u53d1\u4e86\u4e00\u79cd\u6709\u6548\u7684\u7b56\u7565\uff0c\u901a\u8fc7\u7528\u73af\u5df1\u9187\u7cbe\u786e\u963b\u65adNafion\u7684\u78fa\u9178\u57fa\u56e2\u6765\u63d0\u9ad8Pt\u5728MEA\u4e2d\u7684\u50ac\u5316\u6027\u80fd\u3002<sup>1<\/sup>H NMR\u3001ATR-FTIR\u548cXPS\u5149\u8c31\u63ed\u793a\u4e86\u79bb\u805a\u7269\u4e2d\u73af\u5df1\u9187\u7684\u7f9f\u57fa\u4e0e\u78fa\u9178\u6839\u4e4b\u95f4\u7684\u5f3a\u914d\u4f4d\u76f8\u4e92\u4f5c\u7528\u3002\u540c\u6b65\u8f90\u5c04SAXS\u8bc1\u5b9e\uff0c\u4e0d\u540c\u6784\u8c61\u7684\u73af\u5df1\u9187\u663e\u8457\u589e\u5f3a\u4e86Nafion\u7684\u5fae\u76f8\u5206\u79bb\u3002\u73af\u5df1\u9187\u901a\u8fc7\u51cf\u5c11\u78fa\u9178\u6839\u5728Pt\u8868\u9762\u7684\u8986\u76d6\u7387\u548c\u6539\u5584\u79bb\u805a\u7269\u7684\u5206\u5e03\uff0c\u6709\u6548\u5730\u589e\u5f3a\u4e86\u52a8\u529b\u5b66\u6d3b\u6027\u548c\u8d28\u91cf\u4f20\u8f93\u3002<\/p>\n<p><strong>\u539f\u6587\u8be6\u60c5<\/strong>\uff1a<a href=\"https:\/\/www.nature.com\/articles\/s41929-023-00949-w\" target=\"_blank\" rel=\"noopener\">Blocking the Sulfonate Group in Nafion to Unlock Platinum\u2019s Activity in Membrane Electrode Assemblies<\/a> (<em>Nat Catal. <\/em><strong>2023<\/strong>, <em>6<\/em>, 392-401)<\/p>\n<p>\u672c\u6587\u7531\u8d5b\u6069\u65af\u4f9b\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u4e00\u3001\u3010\u5bfc\u8bfb\u3011 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