{"id":254625,"date":"2023-09-28T06:44:38","date_gmt":"2023-09-27T22:44:38","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=254625"},"modified":"2023-09-28T16:31:52","modified_gmt":"2023-09-28T08:31:52","slug":"adv-mater-%e7%bb%bc%e8%bf%b0%ef%bc%9a%e5%a4%9a%e5%ad%94%e6%9d%90%e6%96%99%e7%94%a8%e4%ba%8e%e7%94%b5%e5%8c%96%e5%ad%a6-%e5%85%89%e5%8c%96%e5%ad%a6co2rr","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=254625","title":{"rendered":"Adv. Mater.\u7efc\u8ff0\uff1a\u591a\u5b54\u6750\u6599\u7528\u4e8e\u7535\u5316\u5b66\/\u5149\u5316\u5b66CO2RR"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u5168\u7403\u6c14\u6e29\u4e0a\u5347\u3001\u6d77\u6d0b\u9178\u5316\u548c\u6781\u7aef\u5929\u6c14\u4e8b\u4ef6\u9891\u53d1\u5747\u53ef\u5f52\u56e0\u4e8e\u5927\u6c14\u4e2dCO2<\/sub>\u6d53\u5ea6\u4e0a\u5347\u3002\u5229\u7528\u53ef\u6301\u7eed\u80fd\u6e90\uff0c\u901a\u8fc7\u591a\u7535\u5b50\u3001\u591a\u8d28\u5b50\u8f6c\u79fb\u53cd\u5e94\u8fc7\u7a0b\u50ac\u5316CO2<\/sub>\u51cf\u5c11\u5e76\u5c06\u8f6c\u5316\u4e3a\u589e\u503c\u4ea7\u54c1\u662f\u4e00\u79cd\u5f88\u6709\u524d\u9014\u7684\u7b56\u7565\u3002\u8fd9\u4e00\u76ee\u6807\u6fc0\u53d1\u4e86\u4f7f\u7528\u7535\u5316\u5b66\u548c\u5149\u5316\u5b66\u65b9\u6cd5\u8fdb\u884c\u9009\u62e9\u6027\u548c\u9ad8\u6548CO2<\/sub>\u8f6c\u5316\u7684\u50ac\u5316\u5242\u7684\u5f00\u53d1\u3002\u5728\u5404\u79cd\u50ac\u5316\u5242\u7cfb\u7edf\u4e2d\uff0c\u5177\u6709\u591a\u5b54\u6027\u76842D\u548c3D\u5e73\u53f0\u5177\u5907\u4e86\u78b3\u6355\u83b7\u548cCO2<\/sub>\u8f6c\u5316\u7ed3\u5408\u7684\u6f5c\u529b\uff0c\u8fd9\u5176\u4e2d\u5305\u62ec\u5171\u4ef7\u6709\u673a\u6846\u67b6\uff08COFs\uff09\u3001\u91d1\u5c5e-\u6709\u673a\u6846\u67b6\uff08MOFs\uff09\u3001\u591a\u5b54\u5206\u5b50\u7b3c\u548c\u5176\u4ed6\u6742\u5316\u5206\u5b50\u6750\u6599\uff0c\u8fd9\u4e9b\u6750\u6599\u65e8\u5728\u589e\u52a0\u6d3b\u6027\u4f4d\u70b9\u66b4\u9732\u3001\u7a33\u5b9a\u6027\u548c\u6c34\u76f8\u5bb9\u6027\uff0c\u540c\u65f6\u4fdd\u6301\u7cbe\u786e\u7684\u5206\u5b50\u53ef\u8c03\u6027\u3002<\/p>\n

\u00a0<\/strong>\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u52a0\u5dde\u5927\u5b66\u4f2f\u514b\u5229\u5206\u6821<\/strong>Christopher J. Chang<\/strong>\u6559\u6388<\/strong>\u7efc\u8ff0\u5c55\u793a\u4e86\u7528\u4e8eCO2<\/sub>\u8fd8\u539f\u53cd\u5e94\uff08CO2<\/sub>RR\uff09\u7684\u591a\u5b54\u50ac\u5316\u5242\uff0c\u8fd9\u4e9b\u50ac\u5316\u5242\u5c06\u660e\u786e\u5b9a\u4e49\u7684\u5206\u5b50\u5143\u7d20\u6574\u5408\u5230\u591a\u5b54\u6750\u6599\u7ed3\u6784\u4e2d\u3002\u7efc\u8ff0\u4e2d\u9009\u5b9a\u7684\u5b9e\u4f8b\u63d0\u4f9b\u4e86\u5bf9\u8fd9\u79cd\u603b\u4f53\u8bbe\u8ba1\u7b56\u7565\u7684\u4e0d\u540c\u65b9\u6cd5\u5982\u4f55\u589e\u5f3a\u5176\u7535\u50ac\u5316\u548c\/\u6216\u5149\u50ac\u5316CO2<\/sub>\u8fd8\u539f\u6d3b\u6027\u7684\u89c1\u89e3\u3002\u6700\u540e\uff0c\u4f5c\u8005\u8fd8\u5c55\u671b\u4e86\u672a\u6765\u8be5\u9886\u57df\u7684\u7814\u7a76\u65b9\u5411\uff0c\u4e3a\u540e\u7eed\u7814\u7a76\u6307\u660e\u4e86\u65b9\u5411\u3002\u8be5\u7efc\u8ff0\u4ee5\u9898\u4e3a\u201cPorosity as a Design Element for Developing Catalytic Molecular Materials for Electrochemical and Photochemical Carbon Dioxide Reduction<\/strong>\u201d\u53d1\u8868\u5728\u77e5\u540d\u671f\u520aAdv. Mater.<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/strong><\/p>\n

\u672c\u7814\u7a76\u7efc\u8ff0\u4e86\u7528\u4e8eCO2<\/sub>RR\u7684\u5404\u7c7b\u578b\u591a\u5b54\u50ac\u5316\u5242\uff0c\u7136\u540e\u5c55\u793a\u4e86\u4e0d\u540c\u65b9\u6cd5\u589e\u5f3a\u5176\u7535\u50ac\u5316\u548c\/\u6216\u5149\u50ac\u5316CO2<\/sub>\u8fd8\u539f\u6d3b\u6027\uff0c\u6700\u540e\u5c55\u671b\u4e86\u8be5\u9886\u57df\u7684\u7814\u7a76\u65b9\u5411\u3002<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\u56fe<\/strong>1\u00a0 <\/strong>\u7528\u4e8e<\/strong>CO2<\/sub>RR<\/strong>\u7684\u591a\u5b54\u5206\u5b50\u6750\u6599\u50ac\u5316\u5242\u8bbe\u8ba1<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\u7528\u4e8eCO2<\/sub>RR\u7684\u591a\u5b54\u5206\u5b50\u6750\u6599\u50ac\u5316\u5242\u7684\u6982\u5ff5\u8bbe\u8ba1\u793a\u610f\u56fe\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>2\u00a0 <\/strong>\u7528\u4e8e<\/strong>CO2<\/sub>RR<\/strong>\u7684\u4ee3\u8868\u6027<\/strong>COF<\/strong>\u50ac\u5316\u5242<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\uff08a\uff09COF-366\u3001COF-367\u548c\u5408\u6210\u7c7b\u4f3c\u7269\u7b49Co\u914d\u5408\u7269\u7684\u5316\u5b66\u7ed3\u6784\u3002<\/p>\n

\uff08b\uff09COF-366-Co\u3001COF-367-Co\u548cCo\uff08TAP\uff09\u7684\u7535\u5316\u5b66CO2<\/sub>RR\u6d3b\u6027\u7684Tafel\u56fe\u3002<\/p>\n

\uff08c\uff09\u5177\u6709-H\u3001-(OMe)2<\/sub>\u3001-F\u548c-(F)4<\/sub>\u53d6\u4ee3\u57fa\u7684COF-366-Co\u7684\u7535\u6d41\u5bc6\u5ea6\u5bf9\u6bd4\u3002<\/p>\n

\uff08d\uff09Co-iBFBim-COF-I\u2013<\/sup>\u7684\u6676\u4f53\u7ed3\u6784\u56fe\u793a\u3002<\/p>\n

\uff08e\uff09\u7531\u5429\u55ea\u8fde\u63a5\u915e\u83c1\u5f62\u6210\u7684COF\uff0cCoPc-PDQ-COF\u7684\u7ed3\u6784\u3002<\/p>\n

\uff08f-g\uff09CoPc-PI-COF-3\u7684\u5316\u5b66\u7ed3\u6784\u4ee5\u53caCoPc-PI COF\u76842D\u30013D\u548c\u65e0Co\u7c7b\u4f3c\u7269\u7684\u7535\u6d41\u5bc6\u5ea6\u5bf9\u6bd4\u56fe\u3002<\/p>\n

\uff08h\uff09Re-bpy-sp2c-COF\u7684\u5408\u6210\u8def\u7ebf\u3002<\/p>\n

 <\/p>\n

\u8868<\/strong>1. <\/strong>\u4ee3\u8868\u6027<\/strong>COF<\/strong>\u50ac\u5316\u5242\u7684<\/strong>CO2<\/sub>RR<\/strong>\u50ac\u5316\u6d3b\u6027<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\"\"<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>3\u00a0 <\/strong>\u7528\u4e8e<\/strong>CO2<\/sub>RR<\/strong>\u7684\u4ee3\u8868\u6027<\/strong>MOF<\/strong>\u50ac\u5316\u5242<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\uff08a\uff09Cu-\u535f\u5549MOFs\u7684\u5355\u5c42\u548c\u53cc\u5c42\u793a\u610f\u56fe\u3002<\/p>\n

\uff08b-c\uff09\u4e24\u79cd\u50ac\u5316\u5242\u7ec4\u5408\u7269\u4e4b\u95f4\u7684\u5149\u4f9d\u8d56\u6027\u4e59\u9187\u751f\u6210\u548c\u5149\u4f9d\u8d56\u6027C2<\/sub>\/C1<\/sub>\u9009\u62e9\u6027\u7684\u5bf9\u6bd4\u3002<\/p>\n

\uff08d\uff09\u7535\u5b50\u4ece\u7535\u6781\u901a\u8fc7Co-PMOF\u4f20\u8f93\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\uff08e\uff09\u9996\u6b21\u62a5\u9053\u7684ZIF-8\u7684\u6676\u4f53\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/p>\n

\uff08f\uff09\u7531\u4e0d\u540c\u7684Zn\u8d77\u59cb\u6750\u6599\u5408\u6210\u7684ZIF-8\u7684\u7535\u5316\u5b66CO2<\/sub>RR\u7684\u7535\u6d41\u5bc6\u5ea6\u56fe\u3002<\/p>\n

\uff08g\uff09\u63ba\u6742\u7684\u83f2\u54af\u5549\u914d\u4f53\uff08ZIF-A-LD\/CB\uff09\u76f8\u5bf9\u4e8e\u65e0\u63ba\u6742\uff08ZIF-8\/CB\uff09\u7684\u7535\u5316\u5b66CO2<\/sub>RR\u7684\u7535\u6d41\u5bc6\u5ea6\u56fe\u3002<\/p>\n

 <\/p>\n

\u8868<\/strong>2. <\/strong>\u4ee3\u8868\u6027<\/strong>MOF<\/strong>\u50ac\u5316\u5242\u7684<\/strong>CO2<\/sub>RR<\/strong>\u50ac\u5316\u6d3b\u6027<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\"\"<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4\u00a0 <\/strong>\u7528\u4e8e\u9ad8\u6d3b\u6027<\/strong>CO2<\/sub>RR<\/strong>\u7684\u591a\u5b54\u5206\u5b50\u7b3c\u7ed3\u6784<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\uff08a\uff09\u4e0e\u7535\u6781\u4e0a\u7684\u591a\u5b54\u8d85\u5206\u5b50Fe-PB\u76f8\u6bd4\uff0c\u5e73\u9762Fe-TPP\u535f\u5549\u91c7\u7528\u7684\u7279\u5b9a\u53d6\u5411\uff0c\u5176\u4e2d3D\u7ed3\u6784\u4fc3\u8fdb\u4e86\u8d28\u91cf\u4f20\u8f93\u3002<\/p>\n

\uff08b\uff09\u4ec5\u901a\u8fc7\u5b54\u9699\u7387\uff08Fe-PB\uff09\u6216\u5b54\u9699\u7387\u548c\u7535\u8377\uff08Fe-PB-2\uff08P\uff09\uff09\u8f6c\u5316\u7684\u5e73\u9762\u5206\u5b50\u50ac\u5316\u5242Fe-TPP\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\uff08c\uff09\u5728\u9971\u548cCO2<\/sub>\u6c14\u6c1b\u4e0b\uff0cFeTPP\u3001Fe-PB-3\uff08N\uff09\u3001Fe-PB-2\uff08P\uff09\u548cFe-P-TMA\u7684\u5149\u50ac\u5316CO2<\/sub>RR\u6d3b\u6027\u5bf9\u6bd4\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>5\u00a0 <\/strong>\u7528\u4e8e<\/strong>CO2<\/sub>RR<\/strong>\u7684\u4ee3\u8868\u6027\u91d1\u5c5e<\/strong>–<\/strong>\u6709\u673a\u7269\u7b3c\u50ac\u5316\u5242<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\uff08a\uff09IrIII<\/sup>-MOC-NH2<\/sub>\u7684\u4ee3\u8868\u6027\u7ed3\u6784\u3002<\/p>\n

\uff08b\uff09IrIII<\/sup>-MOC-NH2<\/sub>\u3001\u4f53IrIII<\/sup>-MOC-NH2<\/sub>\u3001\u4ee5\u53caMOF\u7c7b\u4f3c\u7269\u7684\u5149\u50ac\u5316CO2RR\u6d3b\u6027\u3002<\/p>\n

 <\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>6\u00a0 <\/strong>\u7528\u4e8e<\/strong>CO<\/strong>\u8fd8\u539f\u7684\u4ee3\u8868\u6027<\/strong>\u5206\u5b50\u6750\u6599\u7b3c\u50ac\u5316\u5242<\/strong>\u00a9 2023 Wiley<\/strong><\/p>\n

\uff08a\uff09\u4e00\u79cd\u6742\u5316\u5206\u5b50\u6750\u6599\u7684\u793a\u610f\u56fe\uff0c\u8be5\u6750\u6599\u7531\u5e73\u9762\u535f\u5549\u5206\u5b50\u548c\u7535\u6d3b\u6027\u91d1\u5c5e\u7535\u6781\u8868\u9762\u4e4b\u95f4\u7684\u8d85\u5206\u5b50\u81ea\u7ec4\u88c5\u4ea7\u751f\u6c38\u4e45\u5b54\u9699\u7387\u3002<\/p>\n

\uff08b-c\uff09\u4e0d\u540clinker\u957f\u5ea6\u548c\u6d3b\u6027\u4e2d\u5fc3\u91d1\u5c5e\u5bf9\u7535\u5316\u5b66CO\u8fd8\u539f\u5f62\u6210\u7684C-C\u4ea7\u7269\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u7684\u5f71\u54cd\u3002<\/p>\n

\u00a0<\/strong><\/p>\n

\u8868<\/strong>3. <\/strong>\u4ee3\u8868\u6027\u591a\u5b54\u5206\u5b50\u7b3c\u4e0e\u6742\u5316\u6750\u6599\u50ac\u5316\u5242\u7684<\/strong>CO2<\/sub>RR<\/strong>\u50ac\u5316\u6d3b\u6027<\/strong> \u00a9 2023 Wiley<\/strong><\/p>\n

\u00a0\"\"<\/strong><\/p>\n

\u00a0<\/strong><\/p>\n

\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/strong><\/p>\n

\u5206\u5b50\u6750\u6599\u7cfb\u7edf\u662f\u6781\u5177\u4ef7\u503c\u7684CO2<\/sub>RR\u50ac\u5316\u5242\uff0c\u5b83\u53ef\u4ee5\u901a\u8fc7\u53ef\u6301\u7eed\u7684\u7535\u6216\u592a\u9633\u80fd\u6765\u9a71\u52a8\u3002\u4e8b\u5b9e\u4e0a\uff0c\u8be5\u7cfb\u7edf\u878d\u5408\u4e86\u529f\u80fd\u50ac\u5316\u5242\u5f00\u53d1\u4e2d\u6700\u91cd\u8981\u7684\u4e24\u4e2a\u65b9\u9762\uff1a\u6a21\u5757\u6027\u548c\u8010\u7528\u6027\uff0c\u7279\u522b\u662f\u663e\u793a\u51fa\u6c38\u4e45\u5b54\u9699\u7387\u7684\u529f\u80fd\u6027\u5206\u5b50\u6750\u6599\u50ac\u5316\u5242\u7684\u5f00\u53d1\uff0c\u5305\u62ecCOFs\u3001MOFs\u548c\u591a\u5b54\u5206\u5b50\u7b3c\u3002\u76ee\u524d\u5df2\u7ecf\u6539\u8fdb\u4e86\u8bbe\u8ba1\u539f\u7406\uff0c\u8fd9\u4e9b\u539f\u7406\u5229\u7528\u4e86\u5747\u5300\u7cfb\u7edf\u4e2d\u7684\u5206\u5b50\u7cbe\u5ea6\u548c\u975e\u5747\u5300\u5bf9\u5e94\u7269\u7684\u8010\u4e45\u6027\u3002\u5728CO2<\/sub>RR\u4e2d\uff0c\u5206\u5b50\u6750\u6599\u4e2d\u7684\u4e00\u4e2a\u5173\u952e\u7279\u6027\u662f\u5b54\u9699\u7387\uff0c\u5b83\u53ef\u4ee5\u589e\u5f3aCO2<\/sub>\u5e95\u7269\u7684\u6269\u6563\u548c\u6355\u83b7\uff0c\u5e76\u5c06\u5176\u5f15\u5bfc\u5411\u50ac\u5316\u5242\u7684\u6d3b\u6027\u4f4d\u70b9\u3002\u6700\u540e\uff0c\u4f5c\u8005\u8ba4\u4e3a\u5728\u8be5\u9886\u57df\u4e2d\u672a\u6765\u5e94\u5f53\u5bfb\u6c42\u5c06\u5feb\u901f\u51fa\u73b0\u7684\u65b0\u7684\u6700\u5148\u8fdb\u7684\u5206\u5b50\u50ac\u5316\u5242\u4f53\u591a\u76f8\u5316\u4e3a\u591a\u5b54\u7ed3\u6784\uff1b\u4f18\u5316\u7535\u6781\u7684\u7ed3\u6784\uff0c\u4ee5\u63d0\u9ad8\u6750\u6599\u7684\u5bfc\u7535\u6027\u548c\u50ac\u5316\u4f4d\u70b9\u7684\u7535\u6d3b\u6027\uff1b\u5173\u6ce8\u4e8c\u6b21\u914d\u4f4d\u7403\u7684\u8d21\u732e\u5e76\u5229\u7528\u8fd9\u4e9b\u53d7\u9650\u7a7a\u95f4\u5fae\u73af\u5883\u589e\u5f3aCO2RR\u53cd\u5e94\u6027\u4ee5\u53ca\u57fa\u4e8e\u9644\u52a0\u6c22\u952e\u6216\u9759\u7535\u90e8\u5206\u7684\u5206\u5b50\u914d\u4f4d\u7edc\u5408\u7269\u5f00\u53d1\u7528\u4e8e\u8054\u5408\u78b3\u6355\u83b7\u548c\u56fa\u5b9a\u7684\u4e0b\u4e00\u4ee3\u50ac\u5316\u5242\u7b49\u3002<\/p>\n

\u539f\u6587\u8be6\u60c5<\/strong>\uff1aPorosity as a Design Element for Developing Catalytic Molecular Materials for Electrochemical and Photochemical Carbon Dioxide Reduction <\/a>(Adv. Mater. <\/em>2023<\/strong>, 2302122)<\/p>\n

\u672c\u6587\u7531\u5927\u5175\u54e5\u4f9b\u7a3f\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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