{"id":260880,"date":"2024-06-16T06:37:32","date_gmt":"2024-06-15T22:37:32","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=260880"},"modified":"2024-06-15T13:42:15","modified_gmt":"2024-06-15T05:42:15","slug":"kaust%e5%bc%a0%e5%8d%8e%e5%bd%ac%e8%af%be%e9%a2%98%e7%bb%84jacs-%e5%8d%95%e5%8e%9f%e5%ad%90%e4%bd%8d%e7%82%b9%e8%b0%83%e6%8e%a7%e5%85%89%e7%83%ad%e5%82%ac%e5%8c%96co2%e7%94%b2%e7%83%b7%e5%8c%96","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=260880","title":{"rendered":"KAUST\u5f20\u534e\u5f6c\u8bfe\u9898\u7ec4JACS.: \u5355\u539f\u5b50\u4f4d\u70b9\u8c03\u63a7\u5149\u70ed\u50ac\u5316CO2\u7532\u70f7\u5316"},"content":{"rendered":"<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260883\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/\u56fe\u72471-8.png\" alt=\"\" width=\"624\" height=\"234\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/\u56fe\u72471-8.png 624w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/\u56fe\u72471-8-300x113.png 300w\" sizes=\"(max-width: 624px) 100vw, 624px\" \/><\/p>\n<p>\u5171\u540c\u4e00\u4f5c\uff1aFazal Raziq, \u51af\u7a0b\u6d0b, \u80e1\u6dfc<\/p>\n<p>\u901a\u8baf\u4f5c\u8005\uff1a\u674e\u5de7\u7ea2, Jorge Gascon, \u5f20\u534e\u5f6c<\/p>\n<p>\u901a\u8baf\u5355\u4f4d\uff1a\u6c99\u7279\u963f\u535c\u675c\u62c9\u56fd\u738b\u79d1\u6280\u5927\u5b66\uff08KAUST\uff09<\/p>\n<p>\u8bba\u6587DOI\uff1a10.1021\/jacs.4c05873<\/p>\n<p><strong>\u80cc\u666f\u4ecb\u7ecd<\/strong><\/p>\n<p>\u5149\u70ed\u52a0\u6c22\u5c06\u4e8c\u6c27\u5316\u78b3 (CO<sub>2<\/sub>) \u8f6c\u5316\u4e3a\u589e\u503c\u4ea7\u54c1\u662f\u89e3\u51b3\u80fd\u6e90\u5371\u673a\u548c\u51cf\u5c11\u4e8c\u6c27\u5316\u78b3\u6392\u653e\u7684\u7406\u60f3\u89e3\u51b3\u65b9\u6848\u3002\u7136\u800c\uff0c\u7531\u4e8e\u4e8c\u6c27\u5316\u78b3\u52a0\u6c22\u8fc7\u7a0b\u4e2d\u540c\u65f6\u53d1\u751f\u8bb8\u591a\u7ade\u4e89\u4e2d\u95f4\u53cd\u5e94\uff0c\u5b9e\u73b0\u9ad8\u4ea7\u54c1\u9009\u62e9\u6027\u4ecd\u7136\u5177\u6709\u6311\u6218\u6027\u3002\u6211\u4eec\u63d0\u51fa\u4e86\u4e00\u79cd\u65b0\u65b9\u6cd5\uff0c\u5c06\u5b64\u7acb\u7684\u5355\u539f\u5b50\u954d (Ni) \u951a\u5b9a\u5728\u6c27\u5316\u94df (In<sub>2<\/sub>O<sub>3<\/sub>) \u7eb3\u7c73\u6676\u4f53\u4e0a\uff0c\u4f5c\u4e3a\u6709\u6548\u7684\u5149\u70ed\u50ac\u5316\u5242\uff0c\u5c06\u4e8c\u6c27\u5316\u78b3\u52a0\u6c22\u6210\u7532\u70f7 (CH<sub>4<\/sub>)\uff0c\u63a5\u8fd1100%\u7684\u9009\u62e9\u6027\u3002\u5b9e\u9a8c\u548c\u7406\u8bba\u6a21\u62df\u5df2\u7ecf\u8bc1\u5b9e\uff0cIn<sub>2<\/sub>O<sub>3<\/sub> \u8868\u9762\u4e0a\u7684\u5b64\u7acb Ni \u4f4d\u70b9\u53ef\u4ee5\u6709\u6548\u7a33\u5b9a\u4e8c\u6c27\u5316\u78b3\u52a0\u6c22\u53cd\u5e94\u7684\u4e2d\u95f4\u4ea7\u7269\u5e76\u964d\u4f4e\u8fc7\u6e21\u6001\u80fd\u5792\uff0c\u4ece\u800c\u6539\u53d8\u53cd\u5e94\u8def\u5f84\u5b9e\u73b0\u8d85\u9ad8\u9009\u62e9\u6027\u7532\u70f7\u5316\u3002\u8fd9\u9879\u7814\u7a76\u4e3a\u9ad8\u9009\u62e9\u6027\u5149\u70ed\u50ac\u5316\u52a0\u6c22\u4e8c\u6c27\u5316\u78b3\u4e3a\u7532\u70f7\u7684\u5355\u539f\u5b50\u50ac\u5316\u5242\u7684\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u5168\u9762\u7684\u89c1\u89e3\u3002<\/p>\n<p><strong>\u672c\u6587\u4eae\u70b9<\/strong><\/p>\n<p>1.\u63a5\u8fd1100%\u9009\u62e9\u6027\u7684CO<sub>2<\/sub>\u5149\u70ed\u52a0\u6c22\u7532\u70f7\u5316<\/p>\n<p>2.\u63ed\u793a\u4e86\u6709\u522b\u4e8e\u4f20\u7edf\u7532\u6c27\u57fa\u8def\u5f84\u7684CO<sub>2<\/sub>\u52a0\u6c22\u8fc7\u7a0b<\/p>\n<p><strong>\u56fe\u6587\u89e3\u6790<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260884\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/2-4.jpg\" alt=\"\" width=\"700\" height=\"460\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/2-4.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/2-4-300x197.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p><strong>Figure 1. <\/strong><strong>\u50ac\u5316\u5242\u7684\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n<p>\u901a\u8fc7\u7b80\u5355\u7684\u6d78\u6e0d-\u70e7\u7ed3\u6cd5\u5236\u5907\u4e86\u4ee5In<sub>2<\/sub>O<sub>3<\/sub>\u4e3a\u57fa\u5e95\u7684Ni\u5355\u539f\u5b50\u50ac\u5316\u5242\u3002HAADF-STEM, HRTEM\u8bc1\u5b9e\u4e86Ru\u7269\u79cd\u7684\u5355\u539f\u5b50\u7ea7\u5206\u6563\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260885\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/3-4.jpg\" alt=\"\" width=\"700\" height=\"372\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/3-4.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/3-4-300x159.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p><strong>Figure 2. Ni<\/strong><strong>\u4f4d\u70b9\u7684\u914d\u4f4d\u7ed3\u6784\u8868\u5f81<\/strong><\/p>\n<p>\u901a\u8fc7\u540c\u6b65\u8f90\u5c04X\u5c04\u7ebf\u5438\u6536\u5149\u8c31\uff08XAS\uff09\u7814\u7a76\u4e86\u6240\u5236\u5907Ni\/In<sub>2<\/sub>O<sub>3<\/sub>\u50ac\u5316\u5242\u4e2dNi\u7269\u79cd\u7684\u7535\u5b50\u7ed3\u6784\u548c\u914d\u4f4d\u60c5\u51b5\u3002\u786e\u8ba4\u4e86Ni\u7269\u79cd\u7684\u539f\u5b50\u7ea7\u5206\u6563\uff0c\u5438\u6536\u8fb9\u62df\u5408\u6807\u660eNi\u7269\u79cd\u7684\u4ef7\u6001\u4e3a+2.1\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260887\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/4-4.jpg\" alt=\"\" width=\"700\" height=\"387\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/4-4.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/4-4-300x166.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p><strong>Figure 3.<\/strong><strong>\u5149\u70ed<\/strong><strong>CO<sub>2<\/sub><\/strong><strong>\u52a0\u6c22\u6d3b\u6027\u6d4b\u8bd5<\/strong><\/p>\n<p>Ni\u4f4d\u70b9\u7684\u5f15\u5165\u5f7b\u5e95\u6539\u53d8\u4e86CO2\u5149\u70ed\u52a0\u6c22\u4ea7\u7269\uff0c\u7531CO\u8f6c\u53d8\u4e3aCH4\uff0c\u9009\u62e9\u6027\u63a5\u8fd1100%\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260888\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/5-4.jpg\" alt=\"\" width=\"700\" height=\"392\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/5-4.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/5-4-300x168.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p><strong>Figure 4<\/strong><strong>.<\/strong><strong>\u8d85\u5feb\u5149\u8c31\u548c\u539f\u4f4d\u8868\u5f81<\/strong><\/p>\n<p>\u7ed3\u5408\u8d85\u5feb\u5149\u8c31\u4e0e\u6362\u4f4d\u5b9e\u9a8c\uff0c\u63a2\u8ba8\u4e86\u5149\u751f\u7535\u5b50\u7684\u8fc1\u79fb\u884c\u4e3a\u3002\u7ed3\u679c\u8868\u660e\uff0c\u5149\u6fc0\u53d1\u4e0bIn<sub>2<\/sub>O<sub>3<\/sub>\u4ea7\u751f\u7684\u5149\u751f\u7535\u5b50\u4f1a\u5411Ni\u4f4d\u70b9\u8f6c\u79fb\uff0c\u5f62\u6210\u5bcc\u7535\u5b50\u7684\u53cd\u5e94\u6d3b\u6027\u533a\uff0c\u6709\u5229\u4e8eCO<sub>2<\/sub>\u7684\u8fd8\u539f\u3002\u66f4\u91cd\u8981\u7684\u662f\uff0c\u539f\u4f4d\u5b9e\u9a8c\u8bc1\u660eNi\u4f4d\u70b9\u5bf9\u5173\u952e\u4e2d\u95f4\u4ea7\u7269*CO\u7684\u5f3a\u5438\u9644\u4f5c\u7528\u5bfc\u81f4\u4e86\u9009\u62e9\u6027\u7684\u8f6c\u53d8\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-260889\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/7-2.jpg\" alt=\"\" width=\"700\" height=\"483\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/7-2.jpg 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2024\/06\/7-2-300x207.jpg 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p><strong>Figure 5. <\/strong><strong>\u673a\u7406\u7814\u7a76\u548c\u7406\u8bba\u8ba1\u7b97<\/strong><\/p>\n<p>\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u63ed\u793a\u4e86Ni\u4f4d\u70b9\u4e0aCO<sub>2<\/sub>\u5149\u70ed\u52a0\u6c22\u7684\u53cd\u5e94\u8def\u5f84\uff0c\u63d0\u51fa\u4e86\u6709\u522b\u4e8e\u4f20\u7edf\u7532\u6c27\u57fa\u8def\u5f84\u7684CO<sub>2<\/sub>\u52a0\u6c22\u8fc7\u7a0b\u3002<\/p>\n<p><strong>\u603b\u7ed3\u4e0e\u5c55\u671b<\/strong><\/p>\n<p>\u7efc\u4e0a\u6240\u8ff0\uff0c In<sub>2<\/sub>O<sub>3<\/sub> \u8868\u9762\u4e0a\u539f\u5b50\u7ea7\u5206\u6563\u7684 Ni \u53ef\u4ee5\u4fc3\u8fdb\u5149\u70ed CO<sub>2<\/sub> \u52a0\u6c22\uff0cCH<sub>4<\/sub> \u9009\u62e9\u6027\u9ad8\u8fbe 99%\u3002\u901a\u8fc7\u4e00\u7cfb\u5217\u8868\u5f81\u3001\u539f\u4f4d\u5b9e\u9a8c\u548c\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\uff0c\u63a2\u7a76\u4e86\u7269\u7406\u5316\u5b66\u5c5e\u6027\uff0c\u786e\u5b9a\u4e86\u9650\u901f\u6b65\u9aa4\u5e76\u63d0\u51fa\u4e86\u53cd\u5e94\u9014\u5f84\u3002\u6240\u5f00\u53d1\u50ac\u5316\u5242\u7684\u4f18\u5f02\u6027\u80fd\u53ef\u4ee5\u5f52\u56e0\u4e8e\u5b64\u7acb\u7684 Ni \u4f4d\u70b9\u5bf9 CO*\u7684\u7a33\u5b9a\uff0c\u964d\u4f4e\u5173\u952e\u6b65\u9aa4\u7684\u53cd\u5e94\u80fd\u5792\uff0c\u52a0\u901f H<sub>2<\/sub> \u89e3\u79bb\uff0c\u4ece\u800c\u4fc3\u8fdb CO<sub>2<\/sub> \u52a0\u6c22\uff0c\u5bfc\u81f4 \u9ad8\u9009\u62e9\u6027CH<sub>4<\/sub>\u751f\u6210\u3002<\/p>\n<p><strong>\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n<p><strong>\u5f20\u534e\u5f6c<\/strong>\u6559\u6388\u7b80\u4ecb\uff1a2020\u5e7412\u6708\u52a0\u5165\u963f\u535c\u675c\u62c9\u56fd\u738b\u79d1\u6280\u5927\u5b66\uff08KAUST\uff09, \u5316\u5b66\u79d1\u5b66\u7cfb\uff0c\u62c5\u4efb\u72ec\u7acbPI, \u535a\u58eb\u751f\u5bfc\u5e08\u3002\u66fe\u8363\u83b7\u5f97\u56fd\u5bb6\u9ad8\u5c42\u6b21\u9752\u5e74\u4eba\u624d\u548c\u4e2d\u79d1\u9662\u767e\u4eba\u8ba1\u5212\u7b49\u79f0\u53f7\u3002\u5f20\u534e\u5f6c\u535a\u58eb\u4e8e2013\u5e74\u4e8e\u4e2d\u56fd\u79d1\u5b66\u9662\u83b7\u5f97\u535a\u58eb\u5b66\u4f4d\uff0c\u540c\u5e74\u4e8e\u4e2d\u56fd\u79d1\u5b66\u9662\u62c5\u4efb\u52a9\u7406\u7814\u7a76\u5458\u30022014\u5e74\u81f32017\u5e74\u4e8e\u65e5\u672c\u56fd\u7acb\u7269\u8d28\u7814\u7a76\u6240\u8fdb\u884c\u535a\u58eb\u540e\u7814\u7a76\u3002\u5e76\u4e8e2017\u5e743\u6708\u4efd\u52a0\u5165\u65b0\u52a0\u5761\u5357\u6d0b\u7406\u5de5\u5927\u5b66(Research fellow)\u3002\u957f\u671f\u81f4\u529b\u4e8e\u6784\u7b51\u5355\u539f\u5b50\u50ac\u5316\u5242\u5728\u80fd\u6e90\u8f6c\u5316\u4e0e\u73af\u5883\u4f18\u5316\u9886\u57df\u7684\u5e94\u7528\u3002\u76ee\u524d\u5df2\u53d1\u8868\u8bba\u6587\/\u4e13\u8457\u7ae0\u8282150\u4f59\u7bc7\uff0c\u6587\u7ae0\u5f15\u7528\u6b21\u657017000\u4f59\u6b21\uff0cH\u56e0\u5b5065\u3002\u5176\u4e2d\u591a\u7bc7\u6587\u7ae0\u4ee5\u7b2c\u4e00\/\u901a\u8baf\u4f5c\u8005\u53d1\u8868\u5728Sci. Adv., PNAS, Joule, Adv. Mater., Energy Environ. Sci., Angew. Chem. Int. Ed., J. Am. Chem. Soc., Adv. Energy Mater., Adv. Funct. Mater., ACS Nano, Nano Energy\u7b49\u56fd\u9645\u8457\u540d\u671f\u520a\u3002<\/p>\n<p><strong>\u8bfe\u9898\u7ec4\u4ecb\u7ecd<\/strong><\/p>\n<p><strong>https:\/\/acse.kaust.edu.sa\/<\/strong><\/p>\n<p>Advanced Catalysis of Sustainable Energy (ACSE), headed by Huabin Zhang (Assistant Professor of Chemistry) in the KAUST Catalysis Center.<\/p>\n<p>Lab of ACSE focuses on the development of single-atom catalysts with the particular configuration for sustainable energy conversion, including photocatalysis, electrocatalysis, and thermal catalysis. Our research also extends to the operando investigation for monitoring the structural evolution of the reactive centers, as well as the mutual interaction between the reactive center and reactant in the catalytic process.<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u5171\u540c\u4e00\u4f5c\uff1aFazal Raziq, \u51af\u7a0b\u6d0b, \u80e1\u6dfc \u901a\u8baf\u4f5c\u8005\uff1a\u674e\u5de7\u7ea2, Jorge Gascon, \u5f20\u534e\u5f6c \u901a\u8baf\u5355\u4f4d\uff1a\u6c99\u7279\u963f\u535c\u675c\u62c9\u56fd\u738b\u79d1\u6280\u5927\u5b66\uff08KAUST\uff09 \u8bba&#8230;<\/p>\n","protected":false},"author":2,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[215],"tags":[],"class_list":["post-260880","post","type-post","status-publish","format-standard","hentry","category-jiedu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/260880"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/2"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=260880"}],"version-history":[{"count":3,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/260880\/revisions"}],"predecessor-version":[{"id":260891,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/260880\/revisions\/260891"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=260880"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=260880"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=260880"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}