{"id":261031,"date":"2024-06-26T06:46:43","date_gmt":"2024-06-25T22:46:43","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=261031"},"modified":"2024-06-25T20:50:51","modified_gmt":"2024-06-25T12:50:51","slug":"nature-energy%ef%bc%9a%e9%9d%9e%e7%a8%a0%e7%8e%af%e6%9c%89%e6%9c%ba%e5%85%89%e4%bc%8f%e6%80%a7%e8%83%bd%e6%96%b0%e8%ae%b0%e5%bd%95","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=261031","title":{"rendered":"Nature Energy\uff1a\u975e\u7a20\u73af\u6709\u673a\u5149\u4f0f\u6027\u80fd\u65b0\u8bb0\u5f55"},"content":{"rendered":"

\u4e00\u3001\u3010\u79d1\u5b66\u80cc\u666f\u3011 \u00a0<\/strong><\/p>\n

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\u4e8c\u3001\u3010\u521b\u65b0\u6210\u679c\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e0a\u6d77\u4ea4\u901a\u5927\u5b66\u548c\u9752\u5c9b\u5927\u5b66\u7684\u7814\u7a76\u4eba\u5458\u5408\u4f5c\uff0c\u62a5\u9053\u4e86\u4e00\u79cd\u6df7\u5408\u6eb6\u5242\u52a0\u5de5\u7b56\u7565\uff0c\u901a\u8fc7\u5e73\u8861\u5feb\u6325\u53d1\u826f\u6eb6\u5242\u4e0e\u6162\u6325\u53d1\u4e0d\u826f\u6eb6\u5242\u7684\u6eb6\u5ea6\u6027\u8d28\u4e0e\u6bd4\u4f8b\uff0c\u8bf1\u5bfc\u5171\u8f6d\u805a\u5408\u7269\u5728\u9002\u5ea6\u4e0d\u826f\u6eb6\u5242\u4e2d\u5f62\u6210\u7ea4\u7ef4\u7ed3\u6676\uff0c\u4fc3\u4f7fNFREAs\u5728\u7ea4\u7ef4\u8868\u9762\u4e0e\u95f4\u4ecb\u9010\u6b65\u53d6\u5411\u4e0e\u7ed3\u6676\uff0c\u6700\u7ec8\u5f62\u6210\u53cc\u7ea4\u7ef4\u7ed3\u6784\u4e92\u7a7f\u7f51\u7edc\u8584\u819c\uff0c\u89e3\u51b3\u7ed9\u53d7\u4f53\u6750\u6599\u4e92\u6eb6\u6027\u5f3a\u4e0e\u7ed3\u6676\u6027\u5dee\u7684\u95ee\u9898\u3002\u5229\u7528\u4e0a\u8ff0\u7b56\u7565\u6210\u529f\u5730\u5c06NFREAs\u6709\u673a\u5149\u4f0f\u6548\u7387\u63d0\u5347\u81f319.02%\u3002<\/p>\n

\"\"<\/p>\n

\u56fe1\u6750\u6599\u548c\u6eb6\u5242\u9009\u62e9\u3002\uff08a\uff09D18\u30012BTh-2F-C2\u53ca\u76f8\u5173\u6eb6\u5242\u7684\u5316\u5b66\u7ed3\u6784\u3002\uff08b\uff09D18\u5728\u4e0d\u540c\u6eb6\u5242\u4e2d\u7684\u6eb6\u89e3\u5ea6\u3002\uff08c\uff09D18\u5728\u4e0d\u540c\u6eb6\u5242\u4e2d\u7684\u5f52\u4e00\u5316\u5438\u6536\u3002\uff08d\uff09\u57fa\u4e8e\u84b8\u6c7d\u538b\u548c\u6eb6\u89e3\u5ea6\u7684\u6eb6\u5242\u5206\u7c7b\u56fe\uff0c\uff08e\uff09\u6c2f\u4eff\uff08CF\uff09&\u90bb\u4e8c\u7532\u82ef\uff08OXY\uff09\u4e8c\u5143\u6eb6\u5242\u4e2d\u84b8\u6c7d\u538b\u4e0e\u4f53\u79ef\u5206\u6570\u7684\u5173\u7cfb\u3002CF\u6761\u4ef6\u4e0b( f )\u3001OXY\u6761\u4ef6\u4e0b( g )\u548cCF&OXY\u6761\u4ef6\u4e0b( h )\u7684D18:2BTh-2F-C2\u6df7\u5408\u524d\u4f53\u6eb6\u6db2\u7684\u539f\u4f4d\u7d2b\u5916-\u53ef\u89c1\u5438\u6536\u5149\u8c31\u7684\u65f6\u95f4\u4f9d\u8d56\u7b49\u503c\u7ebf\u56fe\u3002\u00a9<\/strong>\u00a02023 Springer Nature<\/strong><\/p>\n

\u4e3a\u4e86\u5236\u5907\u9002\u5f53\u7684\u6eb6\u5242\u6df7\u5408\u7269\u4ee5\u5b8c\u5168\u8bf1\u5bfcD18\u539f\u7ea4\u7ef4\u6837\u805a\u96c6\uff0c\u6c27\u6d53\u5ea6\u5e94\u8bbe\u5b9a\u5728\u6c27\u6eb6\u6db2\u53bb\u9664\u66f2\u7ebf\u7684\u504f\u8f6c\u70b9\u4e4b\u4e0a(\u7ea6\u4e3a\u6c27\u6e7f\u819c\u603b\u539a\u5ea6\u76848%)\u3002\u5728\u76ee\u524d\u7684\u60c5\u51b5\u4e0b\uff0c\u53d1\u73b0CF&OXY\u4e2d12%\u7684OXY\u662f\u6700\u4f73\u7684\u3002D18\u94fe\u5728CF\u84b8\u53d1\u540e\u5f00\u59cb\u7ec4\u88c5\u6210\u539f\u7ea4\u7ef4\u3002\u5728\u8fde\u7eed\u9664\u53bb\u542b\u6c27\u6b8b\u4f59\u6eb6\u5242\u540e\uff0c\u6eb6\u89e3\u5ea6\u6781\u9650\u8feb\u4f7f\u66f4\u591a\u7684D18\u4ee5\u672a\u6324\u538b\u7684\u65b9\u5f0f\u6c89\u6dc0\uff0c\u5f62\u6210\u539f\u7ea4\u7ef4\u7f51\u7edc\u3002\u540c\u65f6\uff0c\u6d41\u52a8\u76f8\u5bcc\u96c62BTh-2F-C2\u5e76\u9010\u6e10\u76f8\u7eaf\u5316\u3002\u521d\u7ea7D18\u7f51\u7edc\u76f8\u51b3\u5b9a\u4e86\u5f62\u6001\uff0c\u7136\u540e2BTh-2F-C2\u5206\u5b50\u5728D18\u539f\u7ea4\u7ef4\u7f51\u4e2d\u6709\u5e8f\u6392\u5217\uff0c\u5f62\u6210\u6b21\u7ea72BTh-2F-C2\u7f51\u7edc\u3002\u56e0\u6b64\uff0c\u6750\u6599\u7ed3\u6676\u589e\u5f3a\uff0c\u6df7\u5408\u533a\u57df\u5c3a\u5bf8\u51cf\u5c0f\uff0c\u76f8\u5206\u79bb\u7684\u957f\u5ea6\u8303\u56f4\u4e3b\u8981\u7531\u539f\u7ea4\u7ef4\u76f4\u5f84\u7684\u5c3a\u5bf8\u51b3\u5b9a\u3002\u8fd9\u79cd\u63a2\u7d22\u76f8\u5206\u79bb\u8fc7\u7a0b\u4ee5\u8bf1\u5bfc\u968f\u540e\u7684\u539f\u7ea4\u7ef4\u5f62\u6210\u7684\u5de5\u827a\u5bf9\u4e8e\u592a\u9633\u80fd\u7535\u6c60\u88c5\u7f6e\u6765\u8bf4\u662f\u975e\u5e38\u6709\u5229\u7684\uff0c\u56e0\u4e3a\u7ed3\u6676\u5728\u5e73\u8861\u4e2d\u5f97\u5230\u589e\u5f3a\u3002<\/p>\n

\"\"<\/p>\n

\u56fe2\u5668\u4ef6\u6027\u80fd\u3002\uff08a\uff09\u5728<\/strong>AM 1.5G, 100 mA cm<\/strong>\u22122<\/sup><\/strong>\u4e0d\u540c\u6761\u4ef6\u4e0b\u7684<\/strong>J-V<\/strong>\u66f2\u7ebf\u548c\u8be6\u7ec6\u53c2\u6570\u3002\uff08b\uff09\u5bf9\u5e94\u6761\u4ef6\u4e0b\u7684<\/strong>EQE<\/strong>\u5149\u8c31\u548c\u79ef\u5206<\/strong>J<\/strong>SC<\/sub><\/strong>\u3002\uff08c\uff09\u5728<\/strong>AM 1.5G, 100 mA cm<\/strong>\u22122<\/sup><\/strong>\u6761\u4ef6\u4e0b\uff0c\u6839\u636e<\/strong>20<\/strong>\u4e2a\u72ec\u7acb\u7684\u5b9e\u9a8c\u6570\u636e\u70b9\u83b7\u5f97\u7684\u8bbe\u5907<\/strong>PCE<\/strong>\u6d4b\u91cf\u7684\u76f4\u65b9\u56fe\u3002\uff08d\uff09\u6587\u732e\u4e2d\u62a5\u9053\u7684\u9ad8\u6548<\/strong>NFREAs<\/strong>\u7684<\/strong>PCE<\/strong>\u4e0e<\/strong>J<\/strong>SC<\/sub><\/strong>\u7684\u56fe\u8868\u3002\uff08e\uff09\u57fa\u4e8e<\/strong>ITIC-4F<\/strong>\u3001<\/strong>Y6<\/strong>\u3001<\/strong>L8-BO<\/strong>\u548c<\/strong>2BTh-2F-C2<\/strong>\u7684\u7efc\u5408<\/strong>\u6027\u80fd<\/strong>\u7684\u5b8f\u89c2\u56e0\u5b50\u77e9\u9635\u3002\uff08f\uff09\u5728<\/strong>AM 1.5G, 100 mA cm<\/strong>\u22122<\/sup><\/strong>\u4e0b\uff0c\u4e0d\u540c\u6eb6\u5242\u7ec4\u5408\u7684\u6548\u7387\u3002\u00a9<\/strong>\u00a02023 Springer Nature<\/strong><\/p>\n

\u4f5c\u8005\u4f7f\u7528\u4f18\u5316\u7684\u5668\u4ef6\u5236\u9020\u65b9\u6cd5\uff0c\u83b7\u5f97\u4e86\u5668\u4ef6\u6027\u80fd\u7684\u663e\u8457\u6539\u5584\u3002J-V\u66f2\u7ebf\u548c\u592a\u9633\u80fd\u7535\u6c60\u6027\u80fd\u603b\u7ed3\u5728\u56fe2\u3002CF\u3001OXY\u548cCF&OXY\u5904\u7406\u7684\u592a\u9633\u80fd\u7535\u6c60\u7684PCE\u5206\u522b\u4e3a15.59% (VOC<\/sub>\u00a0= 0.915 V\uff0cJSC <\/sub>= 24.53\u00a0mA cm–<\/sup>2<\/sup>\uff0cFF=69.49%)\uff0c17.50% (VOC<\/sub>\u00a0= 0.911 V\uff0cJSC<\/sub>\u00a0= 25.68\u00a0mA cm–<\/sup>2<\/sup>\uff0cFF=74.83%)\u548c19.02% (VOC <\/sub>= 0.913 V\uff0cJSC <\/sub>= 26.71\u00a0mA cm–<\/sup>2<\/sup>\uff0cFF=77.98%)\u3002\u8ba4\u8bc1\u7684PCE\u8fbe\u523018.63%\uff0c\u8fd9\u662fNFREA\u57fa\u6709\u673a\u5149\u4f0f\u7684\u6700\u9ad8\u503c\u3002CF&OXY\u88c5\u7f6e\u4e2d\u8f83\u9ad8\u7684JSC<\/sub>\u548cFF\u8868\u660e\u8f7d\u6d41\u5b50\u4ea7\u751f\u548c\u8f7d\u6d41\u5b50\u4f20\u8f93\u90fd\u5f97\u5230\u4e86\u4f18\u5316\uff0c\u8fd9\u8868\u660e\u83b7\u5f97\u4e86\u66f4\u6709\u5229\u7684\u53cc\u8fde\u7eed\u5f62\u6001\u3002<\/p>\n

\"\"<\/p>\n

\u56fe3\u8584\u819c\u5f62\u6001\u3002\u5728<\/strong>CF (a)<\/strong>\u3001<\/strong>OXY (b)<\/strong>\u548c<\/strong>CF&OXY (c)<\/strong>\u6761\u4ef6\u4e0b\uff0c<\/strong>D18:2BTh-2F-C2<\/strong>\u6df7\u5408\u7269\u5728<\/strong>1,700 cm<\/strong>\u22121<\/sup><\/strong>\u6ce2\u6570\u5904\u7684<\/strong>AFM<\/strong>\u8868\u5f81<\/strong>\u3002<\/strong>\uff08d\uff09\u4e0d\u540c\u6761\u4ef6\u4e0b<\/strong>D18:2BTh-2F-C2<\/strong>\u6df7\u5408\u7269\u7684<\/strong>GIWXAS<\/strong>\u5256\u9762\u3002<\/strong>CF-<\/strong>\u3001<\/strong>OXY-<\/strong>\u548c<\/strong>CF&OXY<\/strong>\u57fa\u524d\u4f53\u6eb6\u6db2\u5728<\/strong>50 nm<\/strong>\u5c3a\u5ea6<\/strong>(e)<\/strong>\u548c<\/strong>100 nm<\/strong>\u5c3a\u5ea6<\/strong>(f)<\/strong>\u7684\u51b7\u51bb\u900f\u5c04\u7535\u955c\u56fe\u50cf\u3002\u00a9<\/strong>\u00a02023 Springer Nature<\/strong><\/p>\n

CF&OXY\u5904\u7406\u7684\u8584\u819c\u663e\u793a\u76f4\u5f84\u589e\u52a0\u523025.9 nm\u7684\u539f\u7ea4\u7ef4\u5f62\u6001\u3002\u56e0\u6b64\uff0c\u6eb6\u5242\u6df7\u5408\u7b56\u7565\u5728\u8bf1\u5bfc2BTh-2F-C2\u7ec4\u88c5\u4e2d\u7684\u4f18\u52bf\u662f\u663e\u800c\u6613\u89c1\u7684\u3002\u9700\u8981\u6ce8\u610f\u7684\u662f\uff0cOXY\u5bf9D18\u7684\u6eb6\u89e3\u5ea6\u975e\u5e38\u6709\u9650\uff0c\u6df7\u5408\u8584\u819c\u9700\u8981\u5728\u6eb6\u6db2\u8fd8\u662f\u70ed\u7684\u65f6\u5019\u8fdb\u884c\u5904\u7406\u3002CF&OXY\u6eb6\u6db2\u66f4\u5bb9\u6613\u5904\u7406\u548c\u518d\u73b0\uff0c\u5e76\u4e14\u901a\u8fc7\u968f\u540e\u7684\u84b8\u53d1\u7684\u52a8\u6001\u6eb6\u6db2\u8d28\u91cf\u52a3\u5316\u53ef\u4ee5\u66f4\u597d\u5730\u8bf1\u5bfcNFREA\u5171\u6df7\u7269\u7684\u53cc\u8fde\u7eed\u76f8\u5206\u79bb\u3002<\/p>\n

\"\"<\/p>\n

\u56fe<\/strong>4<\/strong>\u6d41\u53d8\u6027\u8d28\u548c\u5927\u9762\u79ef\u5668\u4ef6\u3002\uff08a\uff09\u5728CF\u3001OXY\u548cCF&OXY\u6761\u4ef6\u4e0b\uff0c\u57fa\u4e8e\u7845\u7247\u6d4b\u91cf\u7684\u539a\u5ea6\u548c\u8868\u9762\u8f6e\u5ed3\u7ebf\u5207\u5272\u3002\uff08b\uff09D18\u5728CB\u548cOXY\u6eb6\u6db2\u4e2d\u7684\u6d41\u53d8\u6d4b\u91cf\uff0c\u7528Herschel-Bulkley\u6a21\u578b\u62df\u5408\u3002\uff08c\uff09CF\u3001OXY\u548cCF&OXY\u6761\u4ef6\u4e0b\u8bbe\u5907\u539a\u5ea6\u548c\u6548\u7387\u5206\u5e03\u3002\uff08d\uff09CF\u3001OXY\u548cCF&OXY\u6761\u4ef6\u4e0b5.2 mm<\/strong>2<\/sup><\/strong>(\u5b9e\u7ebf)\u548c1 cm<\/strong>2<\/sup><\/strong>(\u865a\u7ebf)\u8bbe\u5907\u7684J-V\u66f2\u7ebf\u548c\u8be6\u7ec6\u53c2\u6570\u3002\uff08e\uff09\u4e0d\u540c\u6761\u4ef6\u4e0b\u7684\u8868\u9762\u7c97\u7cd9\u5ea6(S<\/strong>a<\/sub><\/strong>)\u3001\u4e32\u8054\u7535\u963b(R<\/strong>s<\/sub><\/strong>)\u3001\u6f0f\u7535\u7535\u963b(R<\/strong>sh<\/sub><\/strong>)\u548c\u5927\u9762\u79ef\u8bbe\u5907\u635f\u8017\u3002\u00a9<\/strong>\u00a02023 Springer Nature<\/strong><\/p>\n

\u6700\u540e\uff0c\u4f5c\u8005\u5236\u9020\u4e86\u5927\u9762\u79ef\u6709\u673a\u5149\u4f0f\u5668\u4ef6(1 cm2<\/sup>)\uff0c\u4ee5\u8bc4\u4f30\u4e0e\u5c0f\u9762\u79ef\u5668\u4ef6(5.2 mm2<\/sup>)\u76f8\u6bd4\u7684\u6027\u80fd\u4e0b\u964d\u3002\u7528CF\u3001OXY\u548cCF&OXY\u5236\u9020\u76845.2 mm2<\/sup>\u5668\u4ef6\u7684PCE\u5206\u522b\u4e3a15.38%\u300117.36%\u548c18.72%\uff0c\u7528CF\u3001OXY\u548cCF&OXY\u5236\u9020\u76841 cm2<\/sup>\u5668\u4ef6\u7684PCE\u5206\u522b\u4e3a11.67%\u300114.86%\u548c17.28%\u3002\u6548\u7387\u4fdd\u6301\u56e0\u5b50(Pr<\/sub>)\uff0c\u5373\u5927\u9762\u79ef\u5668\u4ef6\u4e0e\u5c0f\u9762\u79ef\u5668\u4ef6\u7684PCE\u6bd4\uff0c\u7528\u4e8e\u8bc4\u4f30\u5668\u4ef6\u9762\u79ef\u4e0a\u7684\u54c1\u8d28\u56e0\u5b50\u3002CF\u3001OXY\u548cCF&OXY\u6eb6\u6db2\u5904\u7406\u5668\u4ef6\u7684Pr<\/sub>\u503c\u5206\u522b\u4e3a75.9%\u300185.6%\u548c92.3%\uff0cCF&OXY\u6eb6\u6db2\u5904\u7406\u5668\u4ef6\u83b7\u5f97\u4e86\u66f4\u597d\u7684\u6027\u80fd\u3002<\/p>\n

\u8be5\u7814\u7a76\u5b9e\u73b0\u4e86\u4e00\u79cd\u9ad8\u6027\u80fd\u975e\u7a20\u73af\u6709\u673a\u5149\u4f0f\uff0c\u4ee5\u201cAchieving 19% efficiency in non-fused ring electron acceptor solar cells via solubility control of donor and acceptor crystallization<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520aNature Energy<\/strong>\u4e0a\uff0c\u5f15\u8d77\u4e86\u76f8\u5173\u9886\u57df\u7814\u7a76\u4eba\u5458\u70ed\u8bae\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u3010\u79d1\u5b66\u542f\u8fea\u3011<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u672c\u6587\u5efa\u7acb\u4e86\u4e00\u79cd\u8f83\u4e3a\u5b9e\u7528\u7684\u5171\u6df7\u6eb6\u5242\u52a8\u529b\u5b66\u8def\u5f84\u63a7\u5236\u65b9\u6cd5\uff0c\u5229\u7528\u4e0d\u540c\u6750\u6599\u5728\u4e0d\u540c\u6eb6\u5242\u4e2d\u7684\u6eb6\u89e3\u6027\u8d28\u7684\u5dee\u5f02\uff0c\u5e76\u4e14\u901a\u8fc7\u6325\u53d1\u6027\u8c03\u63a7\u5728\u52a8\u529b\u5b66\u8def\u5f84\u4e0a\u6709\u6548\u5b9e\u73b0\u4e86\u4e0d\u540c\u6750\u6599\u7684\u5206\u6b65\u5f0f\u5f62\u6001\u8c03\u8282\uff0c\u5728\u6210\u819c\u52a8\u529b\u5b66\u4e0a\u83b7\u5f97\u7a81\u7834\uff0c\u89e3\u51b3\u4e86NFREAs\u4f53\u7cfb\u5f62\u8c8c\u4f18\u5316\u7684\u96be\u9898\uff0c\u5e76\u4e14\u80fd\u591f\u5b9e\u73b0\u5236\u5907\u9762\u79ef\u653e\u5927\u65f6\u8584\u819c\u7684\u5e73\u6574\u6027\uff0c\u51cf\u5c0f\u4e86\u5668\u4ef6\u9762\u79ef\u653e\u5927\u65f6\u7684\u6548\u7387\u4e0b\u964d\uff0c\u4e3a\u9ad8\u6548\u7387\u6709\u673a\u5149\u4f0f\u7684\u5236\u5907\u63d0\u4f9b\u4e86\u65b0\u601d\u8def\u3002<\/p>\n

 <\/p>\n

\u539f\u6587\u8be6\u60c5<\/strong>\uff1aZeng, R., Zhang, M., Wang, X. et al. Achieving 19% efficiency in non-fused ring electron acceptor solar cells via solubility control of donor and acceptor crystallization. Nat. Energy (2024). https:\/\/doi.org\/10.1038\/s41560-024-01564-0<\/p>\n

 <\/p>\n

\u672c\u6587\u7531\u666f\u884c\u64b0\u7a3f<\/strong><\/p>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

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