{"id":263446,"date":"2024-11-23T13:21:42","date_gmt":"2024-11-23T05:21:42","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=263446"},"modified":"2024-11-23T13:21:42","modified_gmt":"2024-11-23T05:21:42","slug":"%e4%b8%80%e7%a7%8d%e5%88%a9%e7%94%a8%e9%98%b4%e5%bd%b1%e7%90%83%e5%85%89%e5%88%bb%e6%8a%80%e6%9c%af%e4%bc%98%e5%8c%96%e7%ba%b3%e7%b1%b3%e5%88%b6%e9%80%a0%e7%9a%84%e9%80%9a%e7%94%a8%e6%a1%86%e6%9e%b6","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=263446","title":{"rendered":"\u4e00\u79cd\u5229\u7528\u9634\u5f71\u7403\u5149\u523b\u6280\u672f\u4f18\u5316\u7eb3\u7c73\u5236\u9020\u7684\u901a\u7528\u6846\u67b6\uff1a\u624b\u6027\u7eb3\u7c73\u5b54\u9635\u5217\u7684\u6848\u4f8b\u7814\u7a76"},"content":{"rendered":"

\u4e00\u3001\u3010\u5bfc\u8bfb\u3011<\/b><\/strong><\/h3>\n

\u968f\u7740\u7eb3\u7c73\u6280\u672f\u7684\u8fc5\u901f\u53d1\u5c55\uff0c\u5236\u9020\u590d\u6742\u7eb3\u7c73\u7ed3\u6784\u7684\u9700\u6c42\u4e5f\u5728\u4e0d\u65ad\u589e\u52a0\u3002\u9634\u5f71\u7403\u5149\u523b\uff08SSL\uff09\u662f\u4e00\u79cd\u5229\u7528\u81ea\u7ec4\u88c5\u80f6\u4f53\u7403\u4f5c\u4e3a\u63a9\u6a21\u7684\u5148\u8fdb\u7eb3\u7c73\u5236\u9020\u6280\u672f\uff0c\u80fd\u591f\u901a\u8fc7\u6750\u6599\u6c89\u79ef\u521b\u5efa\u590d\u6742\u7eb3\u7c73\u7ed3\u6784\u3002\u8fd9\u79cd\u65b9\u6cd5\u4e0d\u4ec5\u7ecf\u6d4e\u9ad8\u6548\uff0c\u8fd8\u80fd\u591f\u5b9e\u73b0\u5927\u89c4\u6a21\u751f\u4ea7\uff0c\u975e\u5e38\u9002\u5408\u5de5\u4e1a\u5e94\u7528\u3002\u7136\u800c\uff0c\u7531\u4e8e\u53c2\u6570\u7a7a\u95f4\u7684\u5e9e\u5927\uff0c\u4f18\u5316\u8fd9\u4e9b\u7ed3\u6784\u4ecd\u7136\u5177\u6709\u6311\u6218\u6027\u3002\u8fd9\u4e3b\u8981\u662f\u56e0\u4e3aSSL\u6d89\u53ca\u7684\u53c2\u6570\u7a7a\u95f4\u6781\u5176\u5e7f\u6cdb\uff0c\u5305\u62ec\u6750\u6599\u9009\u62e9\u3001\u6c89\u79ef\u89d2\u5ea6\u53ca\u95f4\u9694\u3001\u7403\u4f53\u76f4\u5f84\u7b49\u3002\u4f20\u7edf\u8bd5\u9519\u6cd5\u96be\u4ee5\u5e94\u5bf9\u5982\u6b64\u590d\u6742\u7684\u53c2\u6570\u7ec4\u5408\uff0c\u56e0\u6b64\u4e9f\u9700\u4e00\u79cd\u901a\u7528\u4f18\u5316\u6846\u67b6\uff0c\u80fd\u9ad8\u6548\u5f15\u5bfc\u7eb3\u7c73\u7ed3\u6784\u7684\u8bbe\u8ba1\u4e0e\u4f18\u5316\u3002<\/p>\n

\u4e8c\u3001\u3010\u6210\u679c\u63a0\u5f71\u3011<\/b><\/strong><\/h3>\n

\u6700\u8fd1\uff0c\u91cd\u5e86\u5927\u5b66\u5fae\u7535\u5b50\u4e0e\u901a\u4fe1\u5de5\u7a0b\u5b66\u9662\u535a\u58eb\u7814\u7a76\u751f\u9648\u5fc3\u6021\u5728\u827e\u658c\u7814\u7a76\u5458\u7684\u6307\u5bfc\u4e0b\uff0c\u53d1\u8868\u4e86\u4e00\u7bc7\u9898\u4e3a\u300aA general optimization framework for nanofabrication using shadow sphere Lithography: A case study on chiral nanohole arrays\u300b\u7684\u8bba\u6587\u3002\u8be5\u8bba\u6587\u53d1\u8868\u4e8eELSEVIER\u7684\u4e2d\u79d1\u9662\u4e00\u533a\u671f\u520a\u300aJournal of Colloid and Interface Science\u300b\u3002\u8be5\u7814\u7a76\u56e2\u961f\u63d0\u51fa\u4e86\u4e00\u79cd\u7528\u4e8eSSL\u5236\u9020\u7eb3\u7c73\u7ed3\u6784\u7684\u901a\u7528\u4f18\u5316\u6846\u67b6\uff0c\u5e76\u901a\u8fc7\u624b\u6027\u65cb\u8f6c\u7eb3\u7c73\u5b54\u9635\u5217\uff08RHA\uff09\u8fdb\u884c\u4e86\u9a8c\u8bc1\u3002\u8fd9\u9879\u7814\u7a76\u7ed3\u5408\u81ea\u5b9a\u4e49SSL\u7a0b\u5e8f\u3001\u7528\u4e8e\u6d88\u9664\u5197\u4f59\u7ed3\u6784\u7684\u65b0\u6570\u5b66\u6a21\u578b\uff0c\u4ee5\u53ca\u7ed3\u5408\u6709\u9650\u5dee\u5206\u65f6\u57df\uff08FDTD\uff09\u6a21\u62df\u7684\u673a\u5668\u5b66\u4e60\u5206\u6790\u3002\u901a\u8fc7\u8fd9\u4e2a\u65b9\u6cd5\uff0c\u9ad8\u6548\u5206\u6790\u4e867200\u79cd\u7ed3\u6784\u53c2\u6570\uff0c\u6210\u529f\u8bc6\u522b\u51fa\u5706\u4e8c\u8272\u6027\uff08CD\uff09\u4e0e\u4e0d\u5bf9\u79f0\u56e0\u5b50\u5747\u4f18\u5f02\u7684\u6700\u4f73\u53c2\u6570\u914d\u7f6e\u3002<\/p>\n

\"\"\u00a0\u00a0\u00a0\u00a0<\/p>\n

\u4e09\u3001\u3010\u6838\u5fc3\u521b\u65b0\u70b9\u3011<\/b><\/strong><\/h3>\n

\u8be5\u5de5\u4f5c\u901a\u8fc7\u81ea\u5b9a\u4e49SSL\u7a0b\u5e8f\u7684\u5f00\u53d1\uff0c<\/strong>\u6839\u636e\u5236\u9020\u53c2\u6570\u81ea\u52a8\u751f\u6210\u5927\u91cf\u7eb3\u7c73\u5b54\u7ed3\u6784\u3002\u901a\u8fc7\u5f15\u5165\u65b0\u6570\u5b66\u6a21\u578b\uff0c\u6d88\u9664\u91cd\u590d\u7ed3\u6784\uff0c\u663e\u8457\u4f18\u5316\u8ba1\u7b97\u6548\u7387\u3002\u91c7\u7528CatBoost\u7b97\u6cd5\u7ed3\u5408FDTD\u6a21\u62df\u6570\u636e\uff0c\u5206\u6790\u5e76\u627e\u51fa\u5bf9\u7ed3\u6784\u6027\u80fd\u5f71\u54cd\u6700\u5927\u7684\u5236\u9020\u53c2\u6570\u3002\u8fd9\u9879\u7814\u7a76\u5bf97200\u79cd\u53c2\u6570\u914d\u7f6e\u7684RHAs\u8bc6\u522b\u51fa\u6700\u4f73\u53c2\u6570\u914d\u7f6e\uff0c\u7ed3\u5408\u6570\u5b66\u6a21\u578b\u6d88\u9664\u5197\u4f59\u7ed3\u6784\uff0c\u51cf\u5c1186%\u7684\u6570\u636e\u96c6\uff0c\u964d\u4f4e\u4e86\u8ba1\u7b97\u548c\u5b9e\u9a8c\u6210\u672c\u3002\u4f18\u5316\u540e\u7684RHAs\u5b9e\u9a8c\u7ed3\u679c\u4e0e\u9884\u6d4b\u9ad8\u5ea6\u4e00\u81f4\uff0c\u6700\u5927CD\u548cg\u56e0\u5b50\u5206\u522b\u8fbe\u52303.23\u02da\u548c0.28\uff0c\u663e\u8457\u4f18\u4e8e\u5927\u591a\u6570\u4e8c\u7ef4\u7eb3\u7c73\u7ed3\u6784\u7684\u624b\u6027\u54cd\u5e94\u3002\u8be5\u65b9\u6cd5\u6709\u671b\u52a0\u901f\u7eb3\u7c73\u5149\u5b50\u5b66\u3001\u7b49\u79bb\u5b50\u4f53\u5b66\u548c\u624b\u6027\u4f20\u611f\u9886\u57df\u7684\u5e94\u7528\u5f00\u53d1\u3002<\/p>\n

\u56db\u3001\u3010\u6570\u636e\u6982\u89c8\u3011<\/b><\/strong><\/h3>\n

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Fig. 1<\/strong>.\u00a0Optimization framework\u00a0workflow.<\/p>\n

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Fig. 2<\/strong>. An SSL program to generate nanostructures automatically. (a)\u00a0Schematic showing the principle to develop the SSL program. \u00a0(b) The fabrication configuration and major parameters varied to generate different\u00a0RHAs. (c) Examples of the RHAs with different fabrication parameters based on the SSL program. (d) Stereoscopic views of the RHAs and showing the mirror symmetry of the enantiomers.<\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

F<\/b><\/strong>ig. 3<\/b><\/strong>. Schematic showing the general\u00a0symmetry, mirror symmetry, and 60\u02da<\/strong>\u00a0differential rotation. The images were generated by the SSL program with the fabrication parameters depicted\u00a0in the above rows and side columns.<\/p>\n

\"\"\u00a0<\/b><\/strong><\/p>\n

Fig. 4<\/b><\/strong>. Chiroptical properties\u00a0of the Au-Ag RHAs. (a) T<\/i><\/em>R<\/sub>(\u03bb<\/i><\/em>) and\u00a0T<\/i><\/em>L<\/sub>(\u03bb<\/i><\/em>) and of the RHA\u00a0with the max CD. The inset shows the corresponding morphology.\u00a0(b) CD spectra of the RHAs\u00a0with the max CD. (c) Relative frequency distribution of the CD for the Au-Ag RHAs. (d) Plan Views of the Top 5 Au-Ag RHAs. (e) Scatter plotting\u00a0of the CD for the Au-Ag and Ag-Au RHAs. Colormaps of the CD distribution\u00a0for the\u00a0Au-Ag RHAs: (f) \u0394\u03c6<\/em>-\u0394\u03b8<\/em>\u00a0and\u00a0(g)\u00a0\u03c6<\/em>1<\/sub>–\u03b8<\/em>1<\/sub>.<\/p>\n

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Fig. 5<\/b><\/strong>.<\/b><\/strong>\u00a0<\/b><\/strong>ML Algorithms\u00a0for calculating the contribution of each fabrication parameter. (a) Using algorithms of CatBoost, RF, and LightGBM to train the dataset. The max CD of each CD spectra and the fabrication parameters\u00a0are the input and labels, respectively. (b)\u00a0The\u00a0R2<\/sup>\u00a0and RMSE of the three algorithms. (c) Diagram illustrating the gradient boosting decision tree in the CatBoost model algorithm. (d) Feature importance and permutation importance of\u00a0\u03c6<\/em>1<\/sub>, \u03b8<\/em>1<\/sub>, \u0394\u03c6<\/em>, \u0394\u03b8<\/em>, \u03c6<\/em>2<\/sub>, and \u03b8<\/em>2<\/sub>)\u00a0calculated by CatBoost.<\/p>\n

\u00a0\"\"<\/b><\/strong><\/p>\n

Fig. 6<\/b><\/strong>. Experimental samples and practical chiral responses. SEM images with EDS mapping for the Au-Ag (a) m-RHA and (b) r-RHA. The left bottom insets show the corresponding calculated morphology.\u00a0T<\/em>R<\/sub>(\u03bb<\/i><\/em>) and T<\/em>L<\/sub>(\u03bb<\/i><\/em>)\u00a0of the (c)\u00a0experimental and (d) corresponding calculated\u00a0m-RHA and r-RHA. (e)\u00a0CD\u00a0<\/em>spectra of the experimental and calculated\u00a0m-RHA and r-RHA. (f) Plotting of the experimental and calculated CD in this work and those in previous works. (g) |\u2206E<\/em>\/E<\/em>0<\/sub>| and (<\/strong>h) <\/strong>C<\/em>\/|C<\/em>0<\/sub>| of the m-RHA and r-RHA.<\/p>\n

\u4e94\u3001\u3010\u6210\u679c\u542f\u793a\u3011<\/b><\/strong><\/h3>\n

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\u7b2c\u4e00\u4f5c\u8005\u4e3a\u91cd\u5e86\u5927\u5b66\u5fae\u7535\u5b50\u4e0e\u901a\u4fe1\u5de5\u7a0b\u5b66\u9662\u9648\u5fc3\u6021\uff0c\u901a\u8baf\u4f5c\u8005\u4e3a\u91cd\u5e86\u5927\u5b66\u5fae\u7535\u5b50\u4e0e\u901a\u4fe1\u5de5\u7a0b\u5b66\u9662\u827e\u658c\u7814\u7a76\u5458\u3002\u8be5\u7814\u7a76\u5f97\u5230\u4e86\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4\u548c\u91cd\u5e86\u5e02\u7814\u7a76\u751f\u79d1\u7814\u521b\u65b0\u9879\u76ee\u7684\u8d44\u52a9\uff0c\u5e76\u7531\u91cd\u5e86\u5927\u5b66\u3001\u676d\u5dde\u7535\u5b50\u79d1\u6280\u5927\u5b66\u548c\u5409\u6797\u5927\u5b66\u7684\u7814\u7a76\u4eba\u5458\u5171\u540c\u5b8c\u6210\uff0c\u5176\u4e2d\u5305\u62ec\u5409\u6797\u5927\u5b66\u5f20\u521a\u6559\u6388\u7b49\u53c2\u4e0e\u5de5\u4f5c\u7814\u7a76\u3002\u60f3\u4e86\u89e3\u66f4\u591a\u5173\u4e8e\u8fd9\u4e00\u7814\u7a76\u7684\u7ec6\u8282\u548c\u5b9e\u9645\u5e94\u7528\u6f5c\u529b\uff1f\u8bf7\u8bbf\u95ee\u8bfe\u9898\u7ec4https:\/\/www.ailabcqu.com\/page112<\/a>\u3002\u8ba9\u6211\u4eec\u4e00\u540c\u89c1\u8bc1\u7eb3\u7c73\u79d1\u6280\u7684\u672a\u6765\uff01\u672c\u5b9e\u9a8c\u5ba4\u4e13\u6ce8\u4e8e\u667a\u80fd\u5fae\u7eb3\u4f20\u611f\u7cfb\u7edf\uff0c\u5c06\u4eba\u5de5\u667a\u80fd\u548c\u7269\u8054\u7f51\u6280\u672f\u4e0e\u4f20\u7edf\u5316\u5b66\u3001\u7269\u7406\u548c\u6750\u6599\u7b49\u5b66\u79d1\u7ed3\u5408\uff0c\u5f00\u53d1\u65b0\u578b\u5fae\u7eb3\u5236\u5907\u6280\u672f\u3001\u65b0\u578b\u5fae\u7eb3\u5149\u7535\u5b50\u4f20\u611f\u5668\u548c\u751f\u7269\u68c0\u6d4b\u529f\u80fd\u7cfb\u7edf\u3002<\/p>\n

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\u6587\u7ae0\u6765\u6e90\uff1a\u539f\u521b<\/p>\n

\u8bba\u6587\u94fe\u63a5\uff1ahttps:\/\/doi.org\/10.1016\/j.jcis.2024.11.086<\/a><\/p>\n

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\u901a\u4fe1\u4f5c\u8005\u7b80\u4ecb<\/strong><\/p>\n

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