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\u4e8c\u3001\u521b\u65b0\u6210\u679c<\/strong><\/p>\n

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\u56fe<\/strong>1 <\/strong>\u7532\u9178\u5206\u89e3\u7684\u7406\u8bba\u6a21\u62df\uff1b<\/strong>\u00a9 2024 Springer Nature Limited<\/strong><\/p>\n

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\"\"<\/p>\n

\u56fe<\/strong>2 <\/strong>\u7eaf\u8424\u77f3<\/strong>ZrO2<\/sub><\/strong>\u7684\u5408\u6210\u4e0e\u8868\u5f81\uff1b<\/strong>\u00a9 2024 Springer Nature Limited<\/strong><\/p>\n

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\"\"<\/p>\n

\u56fe<\/strong>3 <\/strong>\u70ed\u50ac\u5316\u7532\u9178\u5206\u89e3\u6027\u80fd\u7684\u50ac\u5316\u5242\uff1b<\/strong>\u00a9 2024 Springer Nature Limited<\/strong><\/p>\n

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\u56fe<\/strong>4 <\/strong>\u7532\u9178\u5206\u89e3\u4e2d\u95f4\u4f53\u7684\u8868\u5f81\uff1b<\/strong>\u00a9 2024 Springer Nature Limited<\/strong><\/p>\n

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\"\"<\/p>\n

\u56fe<\/strong>5 <\/strong>\u5149\u70ed\u7532\u9178\u8131\u6c34\u793a\u610f\u56fe\uff1b<\/strong>\u00a9 2024 Springer Nature Limited<\/strong><\/p>\n

\u7532\u9178\u7684\u8131\u6c34\u662f\u4e00\u4e2a\u5438\u70ed\u53cd\u5e94\uff08\u0394H = 26.45 kJ mol\u22121<\/sup>\uff09\uff0c\u9700\u8981\u4e8c\u6b21\u80fd\u91cf\u7684\u8f93\u5165\u3002\u4e3a\u89e3\u51b3\u4e8c\u6b21\u80fd\u8017\u95ee\u9898\uff0c\u7814\u7a76\u4eba\u5458\u6784\u5efa\u4e86\u5149\u70ed\u7532\u9178\u5206\u89e3\u7cfb\u7edf\u3002\u5c06F-ZrO2<\/sub>\u653e\u5165TiC\/Cu\u57fa\u5149\u70ed\u53cd\u5e94\u5668\u4e2d\uff0c\u8be5\u7cfb\u7edf\u4ec5\u7531\u592a\u9633\u5149\u9a71\u52a8\u3002\u57280.1 kW m\u22122<\/sup>\u7684\u592a\u9633\u5149\u7167\u5c04\u4e0b\uff0c\u7532\u9178\u53d1\u751f\u5149\u70ed\u5206\u89e3\uff0c\u50ac\u5316\u5242\u6e29\u5ea6\u8fbe\u5230130 \u2103\u3002\u5f53\u5149\u7167\u5f3a\u5ea6\u589e\u52a0\u52300.5 kW m\u22122<\/sup>\u65f6\uff0c\u50ac\u5316\u5242\u6e29\u5ea6\u4e0a\u5347\u5230278 \u2103\uff0cCO\u751f\u6210\u901f\u7387\u663e\u8457\u589e\u52a0\u523083 mmol g\u22121<\/sup> h\u22121<\/sup>\u3002\u7ed3\u679c\u8868\u660e\uff0c\u5149\u70ed\u7532\u9178\u5206\u89e3\u53ef\u4ee5\u5728\u5fae\u5f31\u7684\u81ea\u7136\u5149\u7167\u4e0b\u76f4\u63a5\u8fdb\u884c\u3002\u7531\u4e8eF-ZrO2<\/sub>\u53ef\u4ee5\u89c4\u6a21\u5316\u5408\u6210\uff0c\u56e0\u6b64\u91c7\u752840 g\u7c92\u72b6F-ZrO2<\/sub>\u8fdb\u884c\u89c4\u6a21\u5316\u5149\u70ed\u7532\u9178\u50ac\u5316\u5206\u89e3\uff0c\u5176\u4e2d\u7814\u7a76\u4eba\u5458\u4f7f\u7528\u7684TiC\/Cu\u57fa\u53cd\u5e94\u5668\u7684\u65e5\u7167\u7167\u5c04\u9762\u79ef\u4e3a0.036 m2<\/sup>\u3002\u5f53\u5149\u7167\u5bc6\u5ea6\u4e3a0.15 kW m\u22122<\/sup>\uff0cCO\u751f\u6210\u901f\u7387\u4e3a~0.55 l h\u22121<\/sup>\uff0c\u7532\u9178\u8f6c\u5316\u7387\u9ad8\u4e8e63%\u3002\u5f53\u5149\u7167\u5bc6\u5ea6\u63d0\u5347\u81f30.5 kW m\u22122<\/sup>\uff0c\u7532\u9178\u8f6c\u5316\u7387\u9ad8\u8fbe92.4%\u3002\u8be5\u7814\u7a76\u5c55\u793a\u7684\u5149\u70ed\u7cfb\u7edf\u4e8e2023\u5e7410\u670810\u65e5\u5728\u4e2d\u56fd\u6cb3\u5317\u7701\u4fdd\u5b9a\u5e02\u8fdb\u884c\u4e86\u6d4b\u8bd5\u3002\u5728\u5ba4\u5916\u9633\u5149\u7167\u5c04\u4e0b\uff0c\u5ba4\u5916\u7cfb\u7edf\u7684\u7eafCO\u4ea7\u7387\u4ece4.1 l h\u2212<\/sup>1<\/sup>\u8c03\u6574\u52309.6 l h\u2212<\/sup>1<\/sup>\uff0c\u603b\u7eafCO\u4ea7\u7387\u4e3a55.4 l \/\u5929\uff0c\u76f8\u5f53\u4e8e1538 l m\u2212<\/sup>2<\/sup> \/\u5929\u3002\u6db2\u4f53\u7532\u9178\u6bcf\u65e5\u7528\u91cf\u4e3a150 ml\uff0c\u5de5\u4f5c\u65e5\u7532\u9178\u5e73\u5747\u8f6c\u5316\u7387\u9ad8\u4e8e60%\u3002\u901a\u8fc7\u8ba1\u7b97\u5206\u6790\uff0c\u7814\u7a76\u4eba\u5458\u8868\u660e\u8be5\u50ac\u5316-\u5149\u70ed\u7cfb\u7edf\u80fd\u591f\u5c55\u73b0\u51fa\u5de8\u5927\u7684\u7ecf\u6d4e\u4ef7\u503c\uff0c\u6709\u671b\u88ab\u89c4\u6a21\u5316\u5e94\u7528\u3002<\/p>\n

\u8be5\u65b9\u6cd5\u6210\u529f\u63a2\u7d22\u51fa\u4e86\u4e0d\u4f9d\u8d56\u51c0\u5316\u548c\u4e8c\u6b21\u80fd\u6e90\u751f\u4ea7\u9ad8\u7eaf\u5ea6CO\u7684\u4f4e\u6210\u672c\u3001\u7eff\u8272\u6a21\u5f0f\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cHigh-purity carbon monoxide production via photothermal formic acid decomposition over fluorite ZrO2<\/sub><\/em><\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u8457\u540d\u671f\u520aNature Catalysis<\/em><\/strong>\u4e0a\u3002<\/p>\n

\"\"<\/p>\n

\u4e09\u3001\u79d1\u5b66\u542f\u8fea<\/strong><\/p>\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u7814\u7a76\u4eba\u5458\u62a5\u544a\u4e86\u4e00\u79cd\u6237\u5916\u9633\u5149\u9a71\u52a8\u7684\u9ad8\u7eaf\u5ea6CO\u751f\u4ea7\u7cfb\u7edf\u3002\u901a\u8fc7\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\u8ba1\u7b97\u548c\u539f\u4f4d\u8868\u5f81\u7684\u7814\u7a76\u8868\u660e\uff0c\u7eaf\u8424\u77f3ZrO2<\/sub>\u53ef\u4ee5\u901a\u8fc7\u81f4\u5bc6\u7684\u8868\u9762\u6676\u683c\u6c27\u81ea\u7136\u6392\u65a5HCOO*\u4e2d\u95f4\u4f53\uff0c\u4ece\u800c\u5b8c\u5168\u907f\u514d\u7532\u9178\u751f\u6210H2<\/sub>\u526f\u4ea7\u7269\u3002\u7206\u70b8\u6cd5\u5236\u5907\u7684\u7eaf\u8424\u77f3ZrO2<\/sub>\u7eb3\u7c73\u7247\u5728250 \u2103\u4e0b\u65e0H2<\/sub>\u526f\u4ea7\u7269\u6742\u8d28\uff0c\u70ed\u7532\u9178CO\u4ea7\u7387\u7a33\u5b9a\u572855 mmol g\u22121<\/sup> h\u22121<\/sup>\u3002\u5728TiC\/Cu\u57fa\u5149\u70ed\u53cd\u5e94\u5668\u7684\u8f85\u52a9\u4e0b\uff0c\u57280.5 kW m\u22122<\/sup>\u592a\u9633\u7167\u5c04\u4e0b\uff0c\u7eaf\u8424\u77f3ZrO2<\/sub>\u7eb3\u7c73\u7247\u7684\u5149\u70edCO\u4ea7\u7387\u4e3a83 mmol g\u22121<\/sup> h\u22121<\/sup>\u3002\u6b64\u5916\uff0c\u5728\u73af\u5883\u592a\u9633\u7167\u5c04\u4e0b\uff0c\u8be5\u7cfb\u7edf\u6bcf\u5929\u7684\u7eafCO\u4ea7\u91cf\u4e3a1,538 l m\u22122<\/sup>\uff0c\u6709\u7740\u5de8\u5927\u7684\u5546\u4e1a\u4ef7\u503c\u3002\u8be5\u7814\u7a76\u63d0\u51fa\u4e86\u4e00\u79cd\u8bbe\u8ba1\u9971\u548c\u914d\u4f4d\u8868\u9762\u6c27\u7684\u7b56\u7565\uff0c\u4ee5\u6dec\u706d\u7532\u9178\u50ac\u5316\u751f\u6210CO\u8fc7\u7a0b\u4e2d\u4ea7\u751f\u526f\u4ea7\u7269H2<\/sub>\u3002\u5149\u70ed\u793a\u8303\u63a2\u7a76\u4e3a\u7532\u9178\u884d\u751fCO\u751f\u4ea7\u63d0\u4f9b\u4e86\u4e00\u6761\u4e0d\u6d88\u8017\u4e8c\u6b21\u80fd\u6e90\u7684\u9014\u5f84\uff0c\u8fd9\u662f\u9ad8\u7eaf\u5ea6\u6c14\u4f53\u5de5\u4e1a\u7684\u91cd\u8981\u6210\u679c\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>High-purity carbon monoxide production via photothermal formic acid decomposition over fluorite ZrO2<\/sub><\/strong>\uff0c<\/strong>2024<\/strong>\uff0c<\/strong>https:\/\/doi.org\/10.1038\/s41929-024-01249-7<\/strong>\uff09<\/strong><\/p>\n

\u00a0<\/strong><\/p>\n

\u672c\u6587\u7531LWB\u4f9b\u7a3f\u3002<\/p>\n

 <\/p>\n","protected":false},"excerpt":{"rendered":"

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