{"id":266007,"date":"2025-04-07T07:42:24","date_gmt":"2025-04-06T23:42:24","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=266007"},"modified":"2025-04-06T22:47:14","modified_gmt":"2025-04-06T14:47:14","slug":"%e5%90%b4%e5%ae%87%e6%81%a9-%e8%ae%b8%e6%9d%b0-%e5%90%b4%e9%93%9c%e4%bc%9f-%e8%83%a1%e6%9e%97jacs%ef%bc%9a%e7%a3%81%e5%9c%ba%e5%a2%9e%e5%bc%ba%e9%95%8d%e5%8d%95%e5%8e%9f%e5%ad%90%e9%85%b8%e6%80%a7co2","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=266007","title":{"rendered":"\u5434\u5b87\u6069\/\u8bb8\u6770\/\u5434\u94dc\u4f1f\/\u80e1\u6797JACS\uff1a\u78c1\u573a\u589e\u5f3a\u954d\u5355\u539f\u5b50\u9178\u6027CO2\u7535\u8fd8\u539f\u53cd\u5e94\u6d3b\u6027"},"content":{"rendered":"<p><strong><b>\u00a0<img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-266009\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72471-7.png\" alt=\"\" width=\"700\" height=\"260\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72471-7.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72471-7-300x111.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/>\u00a0\u00a0\u00a0\u00a0 <\/b><\/strong><\/p>\n<p><strong><b>\u7b2c\u4e00\u4f5c\u8005\uff1a\u5b8b\u4f73\u3001\u4f55\u5927\u5bc5\u3001\u9a6c\u5baa\u8f89<\/b><\/strong><\/p>\n<p><strong><b>\u901a\u8baf\u4f5c\u8005\uff1a\u8bb8\u6770\u3001\u5434\u94dc\u4f1f\u3001\u80e1\u6797\u3001\u5434\u5b87\u6069<\/b><\/strong><\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>\u7814\u7a76\u80cc\u666f<\/b><\/strong><\/p>\n<p>&nbsp;<\/p>\n<p>\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u53cd\u5e94(CO<sub>2<\/sub>RR)\u662f\u6700\u6709\u524d\u9014\u7684\u56fa\u78b3\u51cf\u6392\u6280\u672f\u4e4b\u4e00\uff0c\u5176\u9009\u62e9\u6027\u5728\u751f\u6210CO\u3001HCOOH\u548cC<sub>2<\/sub>H<sub>4<\/sub>\u7b49\u9ad8\u9644\u52a0\u503c\u4ea7\u7269\u4e2d\u8d77\u7740\u81f3\u5173\u91cd\u8981\u7684\u4f5c\u7528\u3002\u7279\u522b\u662f\u5728\u9178\u6027\u7535\u89e3\u73af\u5883\u4e2d\uff0cCO<sub>2<\/sub>RR\u5f80\u5f80\u4f34\u968f\u7740\u53cd\u5e94\u52a8\u529b\u5b66\u66f4\u5feb\u7684\u7ade\u4e89\u6027\u6790\u6c22\u53cd\u5e94(HER)\uff0c\u8fd9\u4f1a\u663e\u8457\u964d\u4f4eCO<sub>2<\/sub>\u7684\u8f6c\u5316\u6548\u7387\u3002\u5916\u90e8\u78c1\u573a\u7684\u5e94\u7528\u76f8\u6bd4\u4e8e\u4f20\u7edf\u7684\u4fa7\u91cd\u4e8e\u6d3b\u6027\u4f4d\u70b9\u7ed3\u6784\u8c03\u8282\u7684\u50ac\u5316\u5242\u6539\u6027\u7b56\u7565\u800c\u8a00\uff0c\u63d0\u4f9b\u4e86\u4e00\u79cd\u7075\u6d3b\u3001\u53ef\u8c03\u3001\u975e\u63a5\u89e6\u7684\u65b9\u6cd5\uff0c\u53ef\u4ee5\u5728\u4e0d\u6539\u53d8\u6216\u66f4\u6362\u50ac\u5316\u5242\u672c\u8eab\u7684\u60c5\u51b5\u4e0b\u5b9e\u65f6\u8c03\u6574\u50ac\u5316\u5242\u7684\u6d3b\u6027\u548c\u9009\u62e9\u6027\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>\u7814\u7a76\u8981\u70b9<\/b><\/strong><\/p>\n<p>&nbsp;<\/p>\n<p>\u8fd1\u65e5\uff0c\u4e2d\u56fd\u79d1\u5b66\u6280\u672f\u5927\u5b66\u5434\u5b87\u6069\u3001\u6e29\u5dde\u5927\u5b66\u8bb8\u6770\u3001\u7535\u5b50\u79d1\u6280\u5927\u5b66\u5434\u94dc\u4f1f\u3001\u4e2d\u56fd\u79d1\u5b66\u9662\u5408\u80a5\u7269\u8d28\u79d1\u5b66\u7814\u7a76\u9662\u80e1\u6797\u7b49\u4eba\u5408\u4f5c\u5728<em><i>Journal of the American Chemical Society<\/i><\/em>\u671f\u520a\u53d1\u8868\u9898\u4e3a\u201cMagnetic Field-Enhanced Acidic CO<sub>2<\/sub>\u00a0Electroreduction Reaction on Single Nickel-Site Catalysts\u201d\u7684\u7814\u7a76\u8bba\u6587\u3002\u5728\u672c\u6587\u4e2d\u5f15\u5165\u4e86\u4e00\u4e2a\u8fde\u7eed\u53ef\u8c03\u7684\u5916\u78c1\u573a\uff0c\u4ee5\u63d0\u9ad8\u9178\u6027CO<sub>2<\/sub>\u8fd8\u539f\u53cd\u5e94(CO<sub>2<\/sub>RR)\u7684\u6027\u80fd\u3002\u5728\u9178\u6027\u7535\u89e3\u6db2(pH = 0.91)\u4e2d\uff0cCO<sub>2<\/sub>RR\u5bf9CO\u7684\u521d\u59cb\u6cd5\u62c9\u7b2c\u6548\u7387(FE)\u4ec5\u4e3a18%\uff0c\u65bd\u52a02 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http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72472-7-300x176.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/b><\/strong><\/p>\n<p>\u56fe1. \u5b9e\u9a8c\u88c5\u7f6e\u4e0e\u50ac\u5316\u5242\u7ed3\u6784\u8868\u5f81\u56fe\u3002<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-266011\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72473-8.png\" alt=\"\" width=\"700\" height=\"593\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72473-8.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72473-8-300x254.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/b><\/strong><\/p>\n<p>\u56fe2. \u50ac\u5316\u5242\u7684\u7ed3\u6784\u4e0e\u7535\u5b50\u6027\u8d28\u5206\u6790\u3002<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-266012\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72474-7.png\" alt=\"\" width=\"700\" height=\"356\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72474-7.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72474-7-300x153.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/b><\/strong><\/p>\n<p>\u56fe3. \u78c1\u573a\u5bf9CO<sub>2<\/sub>RR\u50ac\u5316\u6027\u80fd\u7684\u5f71\u54cd\u3002<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-266013\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72475-8.png\" alt=\"\" width=\"700\" height=\"399\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72475-8.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72475-8-300x171.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/b><\/strong><\/p>\n<p>\u56fe4. \u53cd\u5e94\u8fc7\u7a0b\u4e2d\u7684\u7535\u5316\u5b66\u5206\u6790\u3002<\/p>\n<p><strong><b><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-266014\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72476-6.png\" alt=\"\" width=\"700\" height=\"796\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72476-6.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/04\/\u56fe\u72476-6-264x300.png 264w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/b><\/strong><\/p>\n<p>\u56fe5. \u7406\u8bba\u8ba1\u7b97\u5206\u6790\u53cd\u5e94\u673a\u5236\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>\u603b\u7ed3\u4e0e\u5c55\u671b<\/b><\/strong><\/p>\n<p>&nbsp;<\/p>\n<p>\u6b64\u7814\u7a76\u63ed\u793a\u4e86\u5916\u52a0\u9ad8\u78c1\u573a\u53ef\u663e\u8457\u63d0\u5347Ni-N<sub>5<\/sub>-C\u50ac\u5316\u5242\u5728CO<sub>2<\/sub>RR\u4e2d\u7684\u6027\u80fd\u3002\u78c1\u573a\u589e\u5f3a\u4e86\u6d3b\u6027\u954d\u4e2d\u5fc3\u7684\u78c1\u77e9\uff0c\u4f18\u5316\u4e86CO<sub>2<\/sub>\u7684\u5438\u9644\u8fc7\u7a0b\uff0c\u4ece\u800c\u6709\u6548\u63d0\u9ad8\u4e86CO\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff0c\u4e3aCO<sub>2<\/sub>RR\u53cd\u5e94\u6d3b\u6027\u7684\u63d0\u5347\u5f00\u8f9f\u4e86\u65b0\u65b9\u5411\u3002\u4ece\u5b9e\u9645\u5e94\u7528\u89d2\u5ea6\u770b\uff0c\u6280\u672f\u7ecf\u6d4e\u5206\u6790\u8868\u660e\uff0c\u5373\u4f7f\u8003\u8651\u78c1\u573a\u8bbe\u5907\u7684\u989d\u5916\u6210\u672c\uff0c\u6709\u78c1\u573a\u53c2\u4e0e\u65f6\u751f\u4ea7\u6bcf\u5428CO\u7684\u6210\u672c\u4ecd\u663e\u8457\u4f4e\u4e8e\u65e0\u78c1\u573a\u60c5\u51b5\uff0c\u8fd9\u4e3a\u8be5\u6280\u672f\u7684\u5de5\u4e1a\u5316\u5e94\u7528\u63d0\u4f9b\u4e86\u6709\u529b\u7684\u7ecf\u6d4e\u652f\u6491\u3002<\/p>\n<p>\u5728\u672a\u6765\uff0c\u78c1\u573a\u8f85\u52a9\u50ac\u5316\u6280\u672f\u6709\u671b\u5728\u66f4\u591a\u9886\u57df\u5f97\u5230\u62d3\u5c55\u3002\u4e00\u65b9\u9762\uff0c\u53ef\u4ee5\u8fdb\u4e00\u6b65\u4f18\u5316\u78c1\u573a\u6761\u4ef6\u548c\u50ac\u5316\u5242\u4f53\u7cfb\uff0c\u63a2\u7d22\u4e0d\u540c\u7c7b\u578b\u50ac\u5316\u5242\u4e0e\u78c1\u573a\u7684\u534f\u540c\u6548\u5e94\uff0c\u63d0\u9ad8CO<sub>2<\/sub>RR\u7684\u9009\u62e9\u6027\u548c\u6d3b\u6027\uff0c\u5b9e\u73b0\u66f4\u591a\u9ad8\u9644\u52a0\u503c\u4ea7\u7269\u7684\u9ad8\u6548\u5236\u5907\uff1b\u53e6\u4e00\u65b9\u9762\uff0c\u5c06\u8be5\u6280\u672f\u4e0e\u5176\u4ed6\u5148\u8fdb\u7684\u7535\u5316\u5b66\u6280\u672f\u76f8\u7ed3\u5408\uff0c\u5f00\u53d1\u66f4\u52a0\u9ad8\u6548\u3001\u7a33\u5b9a\u7684\u4e8c\u6c27\u5316\u78b3\u8f6c\u5316\u7cfb\u7edf\uff0c\u4e3a\u5168\u7403\u78b3\u51cf\u6392\u76ee\u6807\u7684\u5b9e\u73b0\u8d21\u732e\u66f4\u591a\u529b\u91cf\u3002<\/p>\n<p>&nbsp;<\/p>\n<p><strong><b>\u6587\u732e\u6765\u6e90<\/b><\/strong><\/p>\n<p>&nbsp;<\/p>\n<p>Magnetic Field-Enhanced Acidic CO<sub>2<\/sub>\u00a0Electroreduction Reaction on Single Nickel-Site Catalysts.\u00a0<strong><em><b><i>J. Am. Chem. Soc.<\/i><\/b><\/em><\/strong>\u00a02025.<\/p>\n<p>DOI\uff1a10.1021\/jacs.5c00858<\/p>\n<p>https:\/\/doi.org\/10.1021\/jacs.5c00858<\/p>\n<p>&nbsp;<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u00a0\u00a0\u00a0\u00a0\u00a0 \u7b2c\u4e00\u4f5c\u8005\uff1a\u5b8b\u4f73\u3001\u4f55\u5927\u5bc5\u3001\u9a6c\u5baa\u8f89 \u901a\u8baf\u4f5c\u8005\uff1a\u8bb8\u6770\u3001\u5434\u94dc\u4f1f\u3001\u80e1\u6797\u3001\u5434\u5b87\u6069 &nbsp; \u7814\u7a76\u80cc\u666f &nbsp; \u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u53cd\u5e94(CO2RR)\u662f\u6700\u6709\u524d\u9014&#8230;<\/p>\n","protected":false},"author":14360,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[2],"tags":[],"class_list":["post-266007","post","type-post","status-publish","format-standard","hentry","category-keji"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266007"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/14360"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=266007"}],"version-history":[{"count":3,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266007\/revisions"}],"predecessor-version":[{"id":266016,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266007\/revisions\/266016"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=266007"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=266007"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=266007"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}