{"id":266221,"date":"2025-04-16T07:48:26","date_gmt":"2025-04-15T23:48:26","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=266221"},"modified":"2025-04-15T20:58:35","modified_gmt":"2025-04-15T12:58:35","slug":"%e7%a6%8f%e5%b7%9e%e5%a4%a7%e5%ad%a6%e5%bc%a0%e4%b9%85%e4%bf%8a%e9%99%a2%e5%a3%ab%e3%80%81%e6%b8%85%e5%8d%8e%e5%a4%a7%e5%ad%a6%e5%90%95%e7%91%9e%e6%b6%9b%e6%95%99%e6%8e%88energy-environ-sci-%ef%bc%9a","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=266221","title":{"rendered":"\u798f\u5dde\u5927\u5b66\u5f20\u4e45\u4fca\u9662\u58eb\u3001\u6e05\u534e\u5927\u5b66\u5415\u745e\u6d9b\u6559\u6388Energy Environ. Sci.\uff1a\u52a8\u6001\u50ac\u5316\u5242\u8c03\u63a7\u754c\u9762\u6c22\u952e\u4fc3\u8fdb\u785d\u9178\u6839\u7535\u8fd8\u539f\u4ea7\u6c28"},"content":{"rendered":"

\"\"<\/sup>\u00a0<\/strong><\/p>\n

\u7b2c\u4e00\u4f5c\u8005\uff1a\u4e07\u5b87\u9a70\u526f\u6559\u6388<\/p>\n

\u901a\u8baf\u4f5c\u8005\uff1a\u5de6\u94f6\u6cfd\u526f\u6559\u6388\u3001\u5f20\u4e45\u4fca\u9662\u58eb\u3001\u5415\u745e\u6d9b\u6559\u6388<\/p>\n

\u901a\u8baf\u5355\u4f4d\uff1a\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u3001\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662<\/p>\n

\u8bba\u6587\u94fe\u63a5\uff1a https:\/\/doi.org\/10.1039\/D5EE00597C<\/p>\n

 <\/p>\n

    \n
  1. \u7814\u7a76\u80cc\u666f<\/strong><\/li>\n<\/ol>\n

    \u6c28\uff08NH3<\/sub>\uff09\u4f5c\u4e3a\u4e00\u79cd\u6e05\u6d01\u6c22\u6e90\uff0c\u540c\u65f6\u4e5f\u662f\u5316\u80a5\u3001\u5316\u5de5\u751f\u4ea7\u7684\u4e3b\u8981\u539f\u6599\uff0c\u7136\u800c\u5176\u5de5\u4e1a\u5408\u6210\u4e3b\u8981\u4f9d\u8d56\u4e8e\u9ad8\u80fd\u8017\u3001\u9ad8\u78b3\u6392\u653e\u7684Haber-Bosch\u6280\u672f\u3002\u7535\u50ac\u5316\u785d\u9178\u6839\u8fd8\u539f\uff08NO3<\/sub>–<\/sup>RR\uff09\u53ef\u4ee5\u5229\u7528\u7eff\u8272\u7535\u80fd\u540c\u65f6\u5b9e\u73b0\u6e05\u6d01\u7684\u6c28\u5408\u6210\u548c\u5de5\u4e1a\u5e9f\u6c34\u5904\u7406\uff0c\u5b9e\u73b0\u53d8\u5e9f\u4e3a\u5b9d\u3002\u94b4\u57fa\u50ac\u5316\u5242\u7531\u4e8e\u5176\u9002\u5f53\u7684NO3<\/sub>–<\/sup>\u5438\u9644\u80fd\u529b\u548c\u5feb\u901f\u7684NO2<\/sub>–<\/sup>\u53bb\u9664\u80fd\u529b\uff0c\u88ab\u8ba4\u4e3a\u662f\u4e00\u79cd\u6781\u5177\u6f5c\u529b\u7684\u7535\u5316\u5b66\u5408\u6210\u6c28\u50ac\u5316\u5242\u3002\u7136\u800c\uff0c\u94b4\u57fa\u50ac\u5316\u5242\u5728\u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u8fc7\u7a0b\u4e2d\u901a\u5e38\u4f1a\u53d1\u751f\u91cd\u6784\uff0c\u91cd\u6784\u8fc7\u7a0b\u4e0d\u53ef\u9006\u4e14\u96be\u4ee5\u8c03\u63a7\u3002\u4e14\u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u6d89\u53ca\u591a\u6b65\u8d28\u5b50\u8026\u5408\u7535\u5b50\u53cd\u5e94\u8fc7\u7a0b\uff0c\u5176\u4e2d\u6c22\u5316\u6b65\u9aa4\u9700\u8981\u6301\u7eed\u4f9b\u5e94\u6d3b\u6027\u6c22\uff08*<\/sup>H\uff09\uff0c\u76ee\u524d\u754c\u9762\u6c22\u952e\u5bf9NO3<\/sub>–<\/sup>RR\u6027\u80fd\u7684\u5f71\u54cd\u5c1a\u672a\u5f97\u5230\u5145\u5206\u89e3\u91ca\u3002\u56e0\u6b64\uff0c\u4e9f\u9700\u8fdb\u4e00\u6b65\u63a2\u7d22\u94b4\u57fa\u50ac\u5316\u5242\u7684\u52a8\u6001\u91cd\u6784\u673a\u5236\u4ee5\u53ca\u754c\u9762\u6c22\u952e\u8c03\u63a7\u5bf9NO3<\/sub>–<\/sup>RR\u7535\u5316\u5b66\u52a0\u6c22\u5408\u6210\u6c28\u6027\u80fd\u7684\u5f71\u54cd\u3002<\/p>\n

     <\/p>\n

      \n
    1. \u6587\u7ae0\u7b80\u4ecb<\/strong><\/li>\n<\/ol>\n

      \u8fd1\u65e5\uff0c\u798f\u5dde\u5927\u5b66\u5f20\u4e45\u4fca\u9662\u58eb\u3001\u6e05\u534e\u5927\u5b66\u5415\u745e\u6d9b\u6559\u6388\u7b49\u5728Energy & Environmental Science<\/em>\u53d1\u8868\u7814\u7a76\u6587\u7ae0\u201cInterfacial hydrogen bond modulation of dynamic catalysts for nitrate electroreduction to ammonia\u201d\u3002\u8be5\u5de5\u4f5c\u91c7\u7528\u4e86Cr\u63ba\u6742\u7b56\u7565\u4ee5\u8c03\u63a7Co\u57fa\u52a8\u6001\u50ac\u5316\u5242\u754c\u9762\u6c22\u952e\u76f8\u4e92\u4f5c\u7528\uff0c\u4ece\u800c\u4fc3\u8fdb\u7535\u50ac\u5316NO3<\/sub>–<\/sup>\u8fd8\u539f\u5408\u6210\u6c28\u3002\u6240\u5236\u5907\u7684Cr\u63ba\u6742Co\u57fa\u52a8\u6001\u50ac\u5316\u5242\u5728-0.4\u00a0V vs. RHE\u4e0b\u7684\u4ea7\u6c28\u6cd5\u62c9\u7b2c\u6548\u7387\u8fbe\u523097.36%\uff0c\u5728-0.7\u00a0V vs. RHE\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\u8fbe\u523058.92 mg h-1<\/sup>\u00a0cm-2<\/sup>\u3002\u539f\u4f4d\u8868\u5f81\u548c\u7406\u8bba\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0cCr\u63ba\u6742\u53ef\u4ee5\u8c03\u63a7Co\u57fa\u50ac\u5316\u5242\u7684\u91cd\u6784\u8fc7\u7a0b\uff0c\u5f62\u6210Co(OH)2<\/sub>\u4e0e\u91d1\u5c5eCo\u7684\u52a8\u6001\u5e73\u8861\u3002\u540c\u65f6\u754c\u9762H2<\/sub>O\u4e0eCr-Co(OH)2<\/sub>\u8868\u9762\u7684\u5f3a\u6c22\u952e\u4f5c\u7528\u4fc3\u4f7fH2<\/sub>O\u7f51\u7edc\u4e2d\u5f62\u6210\u66f4\u591a\u7684\u81ea\u7531\u6c34\u5e76\u4fc3\u8fdbH2<\/sub>O\u7684\u89e3\u79bb\uff0c\u5f62\u6210*<\/sup>H\u4ee5\u52a0\u901f\u5728\u91d1\u5c5eCo\u4f4d\u70b9\u4e0aNO3<\/sub>–<\/sup>\u7684\u52a0\u6c22\u8fc7\u7a0b\uff0c\u4ece\u800c\u63d0\u5347\u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u5408\u6210\u6c28\u6027\u80fd\u3002<\/p>\n

       <\/p>\n

        \n
      1. \u56fe\u6587\u89e3\u6790<\/strong><\/li>\n<\/ol>\n

        3.1 <\/strong>\u7406\u8bba\u8ba1\u7b97\u4e0e\u5206\u6790<\/strong><\/p>\n

        \u5206\u5b50\u52a8\u529b\u5b66\uff08MD\uff09\u6a21\u62df\u7ed3\u679c\u8868\u660e\uff0cCr-Co(OH)2<\/sub>\u53ef\u4ee5\u589e\u5f3a\u4e0e\u754c\u9762\u6c34\u7684\u5206\u5b50\u76f8\u4e92\u4f5c\u7528\u5e76\u524a\u5f31\u6c34\u5206\u5b50\u4e4b\u95f4\u7684\u6c22\u952e\u7f51\u7edc\uff0c\u4fc3\u4f7f\u66f4\u591a\u7684\u6c34\u5206\u5b50\u53c2\u4e0e\u52a0\u6c22\u53cd\u5e94\u8fc7\u7a0b\u3002\u5bc6\u5ea6\u6cdb\u51fd\u7406\u8bba\uff08DFT\uff09\u8ba1\u7b97\u8868\u660e\uff0cCr-Co(OH)2<\/sub>\u53ef\u4ee5\u4fc3\u8fdbH2<\/sub>O\u7684\u89e3\u79bb\u4ee5\u53ca*<\/sup>H\u7684\u4ea7\u751f\u3002\u4e0eCr-Co(OH)2<\/sub>\u548cCo(OH)2<\/sub>\u76f8\u6bd4\uff0c\u91d1\u5c5eCo\u4f4d\u70b9\u7684NO3<\/sub>–<\/sup>RR\u51b3\u901f\u6b65\u9aa4\u7684\u53cd\u5e94\u80fd\u5792\u66f4\u4f4e\u3002\u56e0\u6b64Cr-Co(OH)2<\/sub>\u4e0e\u91d1\u5c5eCo\u4e4b\u95f4\u5b58\u5728\u663e\u8457\u7684\u534f\u540c\u6548\u5e94\uff1aCr-Co(OH)2<\/sub>\u8868\u9762\u53d1\u751fH2<\/sub>O\u7684\u89e3\u79bb\u5e76\u4ea7\u751f*<\/sup>H\uff0c\u4fc3\u8fdb\u91d1\u5c5eCo\u4f4d\u70b9\u4e0aNO3<\/sub>–<\/sup>\u52a0\u6c22\u53cd\u5e94\u5408\u6210\u6c28\uff08\u56fe1\uff09\u3002<\/p>\n

        \"\"<\/sup><\/p>\n

        \u56fe1\u00a0\u754c\u9762\u6c22\u952e\u7ed3\u6784\u53caNO3<\/sub>–<\/sup>RR\u53cd\u5e94\u673a\u7406\u8ba1\u7b97<\/p>\n

         <\/p>\n

        3.<\/strong>2<\/strong>\u00a0<\/strong>\u6750\u6599\u5236\u5907\u4e0e\u8868\u5f81<\/strong><\/p>\n

        \u901a\u8fc7\u5bf9ZIF-67\u91c7\u7528\u79bb\u5b50\u4ea4\u6362\u6cd5\u5e76\u7ed3\u5408\u968f\u540e\u7684\u7145\u70e7\u8fc7\u7a0b\uff0c\u5f62\u6210\u4e86\u5206\u6563\u5728\u6c2e\u63ba\u6742\u78b3\u57fa\u5e95\u7684Cr\u63ba\u6742CoOx<\/sub>\u7eb3\u7c73\u9897\u7c92\u3002\u5728\u79bb\u5b50\u4ea4\u6362\u8fc7\u7a0b\u4e2d\uff0cZIF-67\u7684\u914d\u4f53\u88abCrO4<\/sub>2-<\/sup>\u90e8\u5206\u53d6\u4ee3\uff1b\u968f\u540e\u5728\u6c22\/\u6c29\u6df7\u5408\u6c14\u6c1b\u7145\u70e7\u8fc7\u7a0b\u4e2d\uff0cCr\u63ba\u6742ZIF-67\u7eb3\u7c73\u7247\u8f6c\u53d8\u4e3aCr-CoOx<\/sub>\u9897\u7c92\u3002\u901a\u8fc7XANES\u548cEXAFS\u7814\u7a76\u4e86\u50ac\u5316\u5242\u4e2dCo\u7684\u4ef7\u6001\u4ee5\u53ca\u914d\u4f4d\u7ed3\u6784\uff0c\u8bc1\u5b9e\u4e86Cr\u7684\u6210\u529f\u63ba\u6742\uff08\u56fe2\uff09\u3002<\/p>\n

        \"\"<\/sup><\/p>\n

        \u56fe2 Cr-CoOx<\/sub>\u50ac\u5316\u5242\u7684\u5236\u5907\u4e0e\u8868\u5f81<\/p>\n

         <\/p>\n

        3.<\/strong>3<\/strong>\u00a0<\/strong>\u7535\u50ac\u5316<\/strong>NO<\/strong>3<\/sub><\/strong>–<\/sup><\/strong>RR<\/strong>\u6027\u80fd\u6d4b\u8bd5<\/strong><\/p>\n

        \u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u6027\u80fd\u6d4b\u8bd5\u7ed3\u679c\u8868\u660e\uff0cCr-CoOx<\/sub>\u50ac\u5316\u5242\u5728-0.4\u00a0V vs. RHE\u4e0b\u7684\u4ea7\u6c28\u6cd5\u62c9\u7b2c\u6548\u7387\u8fbe\u523097.36%\uff0c\u5728-0.7\u00a0V vs. RHE\u4e0b\u7684\u4ea7\u6c28\u901f\u7387\u8fbe\u523058.92 mg h-1<\/sup>\u00a0cm-2<\/sup>\u3002\u4ea7\u6c28\u901f\u7387\u548c\u6cd5\u62c9\u7b2c\u6548\u7387\u572850\u5c0f\u65f6\u7684\u8fde\u7eed\u6d4b\u8bd5\u8fc7\u7a0b\u4e2d\u4fdd\u6301\u76f8\u5bf9\u7a33\u5b9a\u3002\u5176\u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u7efc\u5408\u6027\u80fd\u8d85\u8fc7\u591a\u6570\u540c\u671f\u62a5\u9053\u7684\u50ac\u5316\u5242\uff08\u56fe3\uff09\u3002<\/p>\n

        \"\"<\/sup><\/p>\n

        \u56fe3 \u7535\u50ac\u5316\u785d\u9178\u6839\u8fd8\u539f\u4ea7\u6c28\u6027\u80fd\u6d4b\u8bd5<\/p>\n

         <\/p>\n

        3.<\/strong>4\u50ac\u5316\u5242\u52a8\u6001\u91cd\u6784\u7814\u7a76<\/strong><\/p>\n

        \u539f\u4f4d\u62c9\u66fc\u6d4b\u8bd5\u7ed3\u679c\u9a8c\u8bc1\u4e86NO3<\/sub>–<\/sup>RR\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u7684Co(OH)2<\/sub>\u5f62\u6210\u3002\u539f\u4f4dXRD\u7ed3\u679c\u8868\u660e\uff0c\u968f\u7740\u53cd\u5e94\u7535\u4f4d\u7684\u8d1f\u79fb\uff0cCo(OH)2<\/sub>\u884d\u5c04\u5cf0\u5f3a\u5ea6\u9010\u6e10\u589e\u5f3a\uff0c\u800c\u91d1\u5c5eCo\u884d\u5c04\u5cf0\u5f3a\u5ea6\u9010\u6e10\u51cf\u5f31\uff1b\u5f53\u65bd\u52a0\u7535\u4f4d\u8fbe\u5230-0.4\u00a0V vs. RHE\u540e\uff0cCo(OH)2<\/sub>\u4e0e\u91d1\u5c5eCo\u7684XRD\u884d\u5c04\u5cf0\u5f3a\u5ea6\u4fdd\u6301\u76f8\u5bf9\u7a33\u5b9a\uff0c\u8868\u660eCo(OH)2<\/sub>\u4e0e\u91d1\u5c5eCo\u4e4b\u95f4\u5f62\u6210\u52a8\u6001\u5e73\u8861\u3002\u6839\u636e\u4e0a\u8ff0\u539f\u4f4d\u6d4b\u8bd5\u7ed3\u679c\uff0cCr-CoOx<\/sub>\u50ac\u5316\u5242\u5728NO3<\/sub>–<\/sup>RR\u53cd\u5e94\u8fc7\u7a0b\u4f1a\u53d1\u751f\u52a8\u6001\u91cd\u6784\u8fc7\u7a0b\uff0c\u5f62\u6210Co(OH)2<\/sub>\u4e0e\u91d1\u5c5eCo\u53cc\u7ec4\u5206\u4e4b\u95f4\u7684\u52a8\u6001\u5e73\u8861\uff08\u56fe4\uff09\u3002<\/p>\n

        \"\"<\/sup><\/strong><\/p>\n

        \u56fe4 \u52a8\u6001\u91cd\u6784\u8fc7\u7a0b\u7684\u539f\u4f4d\u6d4b\u8bd5<\/p>\n

        \u00a0<\/strong><\/p>\n

        3.<\/strong>5<\/strong>\u00a0<\/strong>\u53cd\u5e94\u673a\u5236\u89e3\u6790<\/strong><\/p>\n

        \u539f\u4f4d\u62c9\u66fc\u548c\u539f\u4f4d\u7ea2\u5916\u68c0\u6d4bNO3<\/sub>–<\/sup>RR\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u7684\u4e2d\u95f4\u4ea7\u7269\u3002\u6b64\u5916\uff0c\u539f\u4f4d\u7ea2\u5916\u6d4b\u8bd5\u7ed3\u679c\u8868\u660eCr\u63ba\u6742\u53ef\u4ee5\u6709\u6548\u8c03\u8282\u754c\u9762\u6c34\u7ed3\u6784\uff0c\u4ece\u800c\u589e\u52a0\u9ad8\u6d3b\u6027\u81ea\u7531\u6c34\u7684\u76f8\u5bf9\u542b\u91cf\u3002\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0cCr-Co(OH)2<\/sub>\u8868\u9762\u7f9f\u57fa\u4e0e\u754c\u9762\u6c34\u5206\u5b50\u5f62\u6210\u5f3a\u6c22\u952e\uff0c\u4fc3\u4f7fH2<\/sub>O\u7f51\u7edc\u4e2d\u5f62\u6210\u66f4\u591a\u7684\u81ea\u7531\u6c34\u53c2\u4e0eNO3<\/sub>–<\/sup>RR\u4e2d\u7684\u52a0\u6c22\u8fc7\u7a0b\uff0c\u4fc3\u8fdbNO3<\/sub>–<\/sup>\u8f6c\u5316\u4e3aNH3<\/sub>\uff08\u56fe5\uff09\u3002<\/p>\n

        \"\"<\/p>\n

        \u56fe5\u00a0\u754c\u9762\u6c34\u53ca\u53cd\u5e94\u4e2d\u95f4\u4ea7\u7269\u68c0\u6d4b<\/p>\n

         <\/p>\n

          \n
        1. 4<\/strong>.<\/strong>\u603b\u7ed3<\/strong>\u5c55\u671b<\/strong><\/li>\n<\/ol>\n

          \u8be5\u6587\u91c7\u7528Cr\u63ba\u6742\u7b56\u7565\u8c03\u8282Co\u57fa\u50ac\u5316\u5242\u52a8\u6001\u91cd\u6784\u8fc7\u7a0b\u548c\u754c\u9762\u6c22\u952e\u76f8\u4e92\u4f5c\u7528\u3002MD\u7ed3\u5408DFT\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0cCr-Co(OH)2<\/sub>\u53ef\u4ee5\u7834\u574f\u6c34\u5206\u5b50\u4e4b\u95f4\u7684\u6c22\u952e\u7f51\u7edc\u5e76\u4fc3\u8fdb\u754c\u9762\u6c34\u7684\u89e3\u79bb\u5f62\u6210*<\/sup>H\uff0c\u4ece\u800c\u52a0\u901f\u91d1\u5c5eCo\u4f4d\u70b9\u4e0a\u7684NO3<\/sub>–<\/sup>\u52a0\u6c22\u8fc7\u7a0b\u3002\u4f5c\u4e3a\u9a8c\u8bc1\uff0c\u901a\u8fc7\u79bb\u5b50\u4ea4\u6362\u6cd5\u7ed3\u5408\u7145\u70e7\u8fc7\u7a0b\u5236\u5907\u4e86Cr\u63ba\u6742Co\u57fa\u50ac\u5316\u5242\u3002\u8be5\u50ac\u5316\u5242\u7684\u4ea7\u6c28\u6cd5\u62c9\u7b2c\u6548\u7387\u53ef\u4ee5\u8fbe\u523097.38%\uff0c\u4e14\u4ea7\u6c28\u901f\u7387\u8fbe\u523058.92 mg h-1<\/sup>\u00a0cm-2<\/sup>\u3002\u539f\u4f4dXRD\u3001\u539f\u4f4d\u62c9\u66fc\u548cDFT\u8ba1\u7b97\u7ed3\u679c\u8868\u660eCr\u63ba\u6742\u53ef\u4ee5\u8c03\u63a7\u50ac\u5316\u5242\u7684\u91cd\u6784\u8fc7\u7a0b\uff0c\u5b9e\u73b0Co(OH)2<\/sub>\u548c\u91d1\u5c5eCo\u4e4b\u95f4\u7684\u52a8\u6001\u5e73\u8861\u3002\u539f\u4f4d\u7ea2\u5916\u6d4b\u8bd5\u548cDFT\u8ba1\u7b97\u8fdb\u4e00\u6b65\u8bc1\u660e\uff0cCr\u63ba\u6742\u53ef\u4ee5\u4fc3\u8fdbCo(OH)2<\/sub>\u4e0e\u754c\u9762\u6c34\u4e4b\u95f4\u5f62\u6210\u5f3a\u6c22\u952e\u76f8\u4e92\u4f5c\u7528\uff0c\u63d0\u5347\u754c\u9762\u81ea\u7531\u6c34\u542b\u91cf\uff0c\u5b9e\u73b0\u7535\u50ac\u5316NO3<\/sub>–<\/sup>RR\u5408\u6210\u6c28\u6027\u80fd\u7684\u63d0\u5347\u3002<\/p>\n

           <\/p>\n

            \n
          1. 5<\/b><\/strong>. <\/b><\/strong>\u4e3b\u8981<\/b><\/strong>\u4f5c\u8005\u4ecb\u7ecd<\/b><\/strong><\/li>\n<\/ol>\n

            \u4e07\u5b87\u9a70<\/b><\/strong>\uff0c\u535a\u58eb\u6bd5\u4e1a\u4e8e\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\uff0c\u73b0\u4efb\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u526f\u6559\u6388\uff0c\u798f\u5efa\u7701\u9ad8\u5c42\u6b21\u4eba\u624d\u3002\u4e3b\u8981\u4ece\u4e8b\u78b3\u57fa\u590d\u5408\u6750\u6599\u7684\u8bbe\u8ba1\u4e0e\u7535\u50ac\u5316\u6027\u80fd\u8c03\u63a7\u7814\u7a76\u5de5\u4f5c\uff0c\u4ee5\u7b2c\u4e00\u4f5c\u8005\u5728Adv. Mater.<\/em>\u3001Energy Environ. Sci.<\/em>\u3001Adv. Energy Mater.<\/em>\u3001<\/em>Adv. Funct. Mater.<\/em>\u3001ACS Nano<\/em>\u3001Materials Today<\/em>\u7b49\u56fd\u9645\u671f\u520a\u4e0a\u53d1\u8868SCI\u8bba\u658710\u4f59\u7bc7\u3002\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u798f\u5efa\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u7b49\u8d44\u52a9\u3002<\/p>\n

             <\/p>\n

            \u5de6\u94f6\u6cfd<\/strong>\uff0c\u4e0a\u6d77\u5e02\u201c\u8d85\u7ea7\u535a\u58eb\u540e\u201d\uff0c\u5e08\u4ece\u5f20\u4e45\u4fca\u9662\u58eb\uff0c\u798f\u5efa\u7701\u9ad8\u5c42\u6b21\u5f15\u8fdb\u4eba\u624d\uff0c\u4e3b\u8981\u4ece\u4e8b\u65b0\u80fd\u6e90\u50a8\u80fd\u7535\u6c60\u7535\u6781\u53ca\u50ac\u5316\u6750\u6599\u5408\u6210\u65b9\u6cd5\u5b66\u7814\u7a76\uff0c\u65b0\u80fd\u6e90\u50a8\u80fd\u7535\u6c60\u8868\u754c\u9762\u6784\u5efa\u53ca\u5176\u5728\u5145\u653e\u7535\u8fc7\u7a0b\u4e2d\u539f\u4f4d\u68c0\u6d4b\u4e0e\u7406\u8bba\u6a21\u62df\u7814\u7a76\uff0c\u4ee5\u53ca\u65b0\u80fd\u6e90\u7535\u6c60\u653e\u5927\u5316\u751f\u4ea7\u7684\u7814\u7a76\u3002\u76ee\u524d\u5728Electrochem. Energy Rev.\u3001Energy & Environ. Sci.\u3001Adv. Mater.\u3001Angew. Chem. Int. Ed.\u3001Adv. Energy Mater.\u3001Adv. Funct. Mater.\u3001Energy Storage Mater.<\/em>\u00a0\u7b49\u56fd\u9645\u671f\u520a\u53d1\u8868\u8bba\u658740\u4f59\u7bc7\uff0c\u6388\u6743\u4e13\u522910\u4f59\u9879\u3002<\/p>\n

             <\/p>\n

            \u5f20\u4e45\u4fca<\/strong>\uff0c\u4e2d\u56fd\u5de5\u7a0b\u9662\u5916\u7c4d\u9662\u58eb\uff0c\u52a0\u62ff\u5927\u7687\u5bb6\u79d1\u5b66\u9662\u9662\u58eb\u3001\u52a0\u62ff\u5927\u5de5\u7a0b\u9662\u9662\u58eb\u3001\u52a0\u62ff\u5927\u5de5\u7a0b\u7814\u7a76\u9662\u9662\u58eb\u3001\u56fd\u9645\u7535\u5316\u5b66\u5b66\u4f1a\u4f1a\u58eb\u3001\u82f1\u56fd\u7687\u5bb6\u5316\u5b66\u4f1a\u4f1a\u58eb\u3001\u56fd\u9645\u5148\u8fdb\u6750\u6599\u534f\u4f1a\u4f1a\u58eb\u3001\u56fd\u9645\u7535\u5316\u5b66\u80fd\u6e90\u79d1\u5b66\u9662\uff08IAOEES\uff09\u4e3b\u5e2d\u3001\u4e2d\u56fd\u5185\u71c3\u673a\u5b66\u4f1a\u5e38\u52a1\u7406\u4e8b\u517c\u71c3\u6599\u7535\u6c60\u53d1\u52a8\u673a\u5206\u4f1a\u4e3b\u4efb\u59d4\u5458\uff0c\u73b0\u4efb\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u9662\u957f\u3001\u65b0\u80fd\u6e90\u6750\u6599\u4e0e\u5de5\u7a0b\u7814\u7a76\u9662\u9662\u957f\u3002\u957f\u671f\u4ece\u4e8b\u7535\u5316\u5b66\u80fd\u6e90\u5b58\u50a8\u548c\u8f6c\u6362\u53ca\u5176\u6750\u6599\u7684\u7814\u7a76\u548c\u4ea7\u4e1a\u5316\u5e94\u7528\u5f00\u53d1\uff0c\u5305\u62ec\u71c3\u6599\u7535\u6c60\u3001\u9ad8\u6bd4\u80fd\u4e8c\u6b21\u7535\u6c60\u3001\u8d85\u7ea7\u7535\u5bb9\u5668\u3001CO2<\/sub>\u7535\u5316\u5b66\u8fd8\u539f\u548c\u7535\u89e3\u6c34\u7b49\u3002<\/p>\n

             <\/p>\n

            \u5415\u745e\u6d9b<\/strong>\uff0c\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\u526f\u9662\u957f\uff0c\u957f\u8058\u6559\u6388\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\u3002\u4e3b\u8981\u4ece\u4e8b\u78b3\u57fa\u4f4e\u7ef4\u6750\u6599\u7f3a\u9677\u8bbe\u8ba1\u53ca\u6027\u80fd\u8c03\u63a7\u7814\u7a76\uff0c\u4fa7\u91cd\u4e8e\u6676\u683c\u7f3a\u9677\u7684\u53ef\u63a7\u6784\u7b51\u3001\u539f\u5b50\u7ea7\u6784\u578b\u89e3\u6790\u4ee5\u53ca\u5728\u5206\u5b50\u63a2\u6d4b\u3001\u9ad8\u6027\u80fd\u50ac\u5316\u7b49\u9886\u57df\u7684\u5e94\u7528\u30022017\u5e74\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4-\u4f18\u79c0\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\u8d44\u52a9\uff0c2019\u5e74\u83b7\u6559\u80b2\u90e8\u81ea\u7136\u79d1\u5b66\u4e00\u7b49\u5956\uff0c2022\u5e74\u83b7\u4e2d\u56fd\u6750\u6599\u7814\u7a76\u5b66\u4f1a\u79d1\u5b66\u6280\u672f\u5956\uff08\u57fa\u7840\u7814\u7a76\uff09\u4e00\u7b49\u5956\u3002<\/p>\n

             <\/p>\n","protected":false},"excerpt":{"rendered":"

            \u00a0 \u7b2c\u4e00\u4f5c\u8005\uff1a\u4e07\u5b87\u9a70\u526f\u6559\u6388 \u901a\u8baf\u4f5c\u8005\uff1a\u5de6\u94f6\u6cfd\u526f\u6559\u6388\u3001\u5f20\u4e45\u4fca\u9662\u58eb\u3001\u5415\u745e\u6d9b\u6559\u6388 \u901a\u8baf\u5355\u4f4d\uff1a\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u3001\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662 \u8bba\u6587\u94fe\u63a5\uff1a https:\/\/…<\/p>\n","protected":false},"author":14360,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[2],"tags":[],"class_list":["post-266221","post","type-post","status-publish","format-standard","hentry","category-keji"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266221"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/14360"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=266221"}],"version-history":[{"count":4,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266221\/revisions"}],"predecessor-version":[{"id":266232,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/266221\/revisions\/266232"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=266221"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=266221"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=266221"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}