{"id":267305,"date":"2025-06-06T07:01:15","date_gmt":"2025-06-05T23:01:15","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=267305"},"modified":"2025-06-05T22:11:58","modified_gmt":"2025-06-05T14:11:58","slug":"advanced-materials-%e6%b2%b3%e5%8d%97%e5%a4%a7%e5%ad%a6%e9%99%88%e7%8f%82%e8%af%be%e9%a2%98%e7%bb%84%e5%9c%a8%e4%ba%8c%e7%bb%b4%e8%bf%87%e6%b8%a1%e9%87%91%e5%b1%9e%e7%a2%b2%e5%8c%96%e7%89%a9%e7%9a%84","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=267305","title":{"rendered":"Advanced Materials: \u6cb3\u5357\u5927\u5b66\u9648\u73c2\u8bfe\u9898\u7ec4\u5728\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u78b2\u5316\u7269\u7684\u53ef\u63a7\u751f\u957f\u9886\u57df\u53d6\u5f97\u91cd\u8981\u7814\u7a76\u8fdb\u5c55"},"content":{"rendered":"<p>&nbsp;<\/p>\n<p>2025\u5e746\u67083\u65e5\uff0c\u6cb3\u5357\u5927\u5b66\u9648\u73c2\u6559\u6388\u4e0e\u9ec4\u660e\u4e3e\u6559\u6388\u3001\u4e2d\u79d1\u9662\u6df1\u5733\u5148\u8fdb\u6280\u672f\u7814\u7a76\u9662\u4e01\u5cf0\u6559\u6388\u3001\u4e2d\u56fd\u4eba\u6c11\u5927\u5b66\u5218\u707f\u6559\u6388\u5408\u4f5c\u5728\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u78b2\u5316\u7269\u7684\u53ef\u63a7\u751f\u957f\u7814\u7a76\u65b9\u9762\u53d6\u5f97\u91cd\u8981\u8fdb\u5c55\uff0c\u7814\u7a76\u6210\u679c\u4ee5\u201cSiliconizing-Driven Layer-by-Layer Growth of Two-Dimensional Tellurides with Controlled Crystallization\u201d\u4e3a\u9898\uff0c\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520a\u300a\u5148\u8fdb\u6750\u6599\u300b\uff08Advanced Materials\uff09\u4e0a\u5728\u7ebf\u53d1\u8868\uff08DOI: 10.1002\/adma.202501451\uff09\uff0c\u6cb3\u5357\u5927\u5b66\u4e3a\u7b2c\u4e00\u901a\u8baf\u5355\u4f4d\u3002<\/p>\n<p>1.\u80cc\u666f\u4ecb\u7ecd<\/p>\n<p>\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u78b2\u5316\u7269\uff08TMTs\uff09\u8fd1\u5e74\u6765\u56e0\u5176\u72ec\u7279\u7684\u7269\u7406\u6027\u8d28\u5907\u53d7\u5173\u6ce8\u3002\u5b83\u4eec\u5c55\u73b0\u51fa\u5ba4\u6e29\u94c1\u78c1\u6027\u3001\u8d85\u5bfc\u6027\u3001\u624b\u6027\u53cd\u5e38\u6548\u5e94\u4ee5\u53ca\u5404\u5411\u5f02\u6027\u8d1f\u78c1\u963b\u7b49\u7279\u6027\u4f7f\u5176\u5728\u81ea\u65cb\u7535\u5b50\u5b66\u3001\u62d3\u6251\u91cf\u5b50\u5668\u4ef6\u548c\u5149\u7535\u9886\u57df\u5177\u6709\u5e7f\u9614\u5e94\u7528\u524d\u666f\u3002\u7136\u800c\uff0c\u76f8\u8f83\u4e8e\u8fc7\u6e21\u91d1\u5c5e\u786b\u5316\u7269\u548c\u7852\u5316\u7269\u5df2\u7ecf\u88ab\u5e7f\u6cdb\u5236\u5907\uff0c\u78b2\uff08Te\uff09\u4e0e\u8fc7\u6e21\u91d1\u5c5e\u95f4\u952e\u80fd\u5f31\u3001\u9ad8\u6e29\u5408\u6210\u4e2d\u76f8\u63a7\u56f0\u96be\u7b49\u95ee\u9898\uff0c\u4e25\u91cd\u9650\u5236\u4e86\u9ad8\u8d28\u91cfTMTs\u7684\u53ef\u63a7\u5236\u5907\uff0c\u6b64\u5916\uff0c\u4f20\u7edf\u65b9\u6cd5\u4f9d\u8d56\u9ad8Te\u84b8\u6c14\u901a\u91cf\uff0c\u6613\u5bfc\u81f4\u4ea7\u7269\u76f8\u7ec4\u6210\u590d\u6742\u3001\u7ed3\u6676\u5ea6\u4e0d\u5747\uff0c\u4e14\u96be\u4ee5\u5b9e\u73b0\u5927\u5c3a\u5bf8\u5747\u5300\u751f\u957f\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>2\u3001\u6210\u679c\u7b80\u4ecb<\/p>\n<p>\u672c\u7814\u7a76\u63d0\u51fa\u4e00\u79cdSi\u539f\u5b50\u9a71\u52a8\u9010\u5c42\u751f\u957f\u7b56\u7565\uff0c\u6210\u529f\u5408\u6210\u9ad8\u7ed3\u6676\u5ea6\u3001\u539a\u5ea6\u53ef\u63a7\u7684\u4e8c\u7ef4ZrTe<sub>2<\/sub>\u548cZrTe<sub>3<\/sub>\u6676\u4f53\u3002\u901a\u8fc7\u5f15\u5165Si-Te\u4e8c\u805a\u4f53\uff0c\u663e\u8457\u964d\u4f4e\u53cd\u5e94\u4f53\u7cfb\u4e2dTe<sub>2<\/sub>\u5206\u538b\uff0c\u5e76\u901a\u8fc7Si\u539f\u5b50\u7684\u6e17\u900f\u4e0e\u9694\u79bb\u4f5c\u7528\uff0c\u5b9e\u73b0Zr\u819c\u7684\u539f\u5b50\u7ea7\u7cbe\u5ea6\u7684\u53ef\u63a7\u78b2\u5316\u3002\u57fa\u4e8e\u8fd9\u4e00\u7b56\u7565\u5408\u6210\u7684ZrTe<sub>2<\/sub>\u6676\u4f53\u5c55\u73b0\u51faII\u578bWeyl\u534a\u91d1\u5c5e\u7279\u6027\uff08\u8d1f\u78c1\u963b\u6548\u5e94\uff0c2K, 9 T\u4e0b\u78c1\u963b\u8fbe30%\uff09\uff0c\u800cZrTe<sub>3<\/sub>\u5219\u5b58\u5728\u7535\u8377\u5bc6\u5ea6\u6ce2(~34 K)\u548c\u672c\u5f81\u8d85\u5bfc\u6027(~3 K)\u3002\u7406\u8bba\u7814\u7a76\u8868\u660e\uff0cSi\u539f\u5b50\u80fd\u591f\u9010\u5c42\u6e17\u900fZr\u819c\u5c06\u5176\u9010\u5c42\u53ef\u63a7\u78b2\u5316\u3002<\/p>\n<p>\u8be5\u5de5\u4f5c\u4e3a\u4e8c\u7ef4TMTs\u7684\u7cbe\u51c6\u53ef\u63a7\u5408\u6210\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u7684\u601d\u8def\uff0c\u5b9e\u73b0\u4e86\u7845\u5316\u9a71\u52a8\u4e8c\u7ef4\u78b2\u5316\u9506\u6676\u4f53\u7684\u53ef\u63a7\u751f\u957f\uff0c\u4e3a\u53ef\u63a7\u76f8\u7ed3\u6784\u7684\u9ad8\u8d28\u91cf\u4e8c\u7ef4\u8fc7\u6e21\u91d1\u5c5e\u78b2\u5316\u7269\u7684\u5927\u89c4\u6a21\u5408\u6210\u63d0\u4f9b\u4e86\u65b0\u8def\u5f84\uff0c\u5e76\u4e3a\u57fa\u4e8e\u4e8c\u7ef4\u62d3\u6251\u6750\u6599\u7684\u81ea\u65cb\u7535\u5b50\u5668\u4ef6\u521b\u65b0\u63d0\u4f9b\u4e86\u6750\u6599\u57fa\u7840\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>3\u3001\u56fe\u6587\u5bfc\u8bfb<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-267307\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72471-6.png\" alt=\"\" width=\"800\" height=\"540\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72471-6.png 800w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72471-6-300x203.png 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72471-6-768x518.png 768w\" sizes=\"(max-width: 800px) 100vw, 800px\" \/>\u00a0<\/p>\n<p>\u56fe1\uff1aSi\u539f\u5b50\u9a71\u52a8\u4e8c\u7ef4\u78b2\u5316\u9506\u6676\u4f53\u751f\u957f\u793a\u610f\u56fe\u3002\u76f4\u63a5\u78b2\u5316Zr\u8584\u819c\u7684\u4ea7\u7269\u5448\u73b0\u65e0\u5e8f\u6210\u6838\u548c\u5c9b\u72b6\u751f\u957f\u7684Zr-Te\u5408\u91d1\u9897\u7c92\uff0c\u76f8\u7ec4\u6210\u590d\u6742\uff08\u8def\u5f84I\uff09\u3002\u5728Si\u539f\u5b50\u8f85\u52a9\u4e0b\uff0c\u53ef\u5206\u522b\u5728\u9ad8\u6e29\u548c\u4f4e\u6e29\u6761\u4ef6\u4e0b\u751f\u957f\u5747\u5300\u7684\u4e8c\u7ef4ZrTe<sub>2<\/sub>\u548cZrTe<sub>3<\/sub>\u6676\u4f53\uff08\u8def\u5f84II\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-267308\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72472-8.png\" alt=\"\" width=\"800\" height=\"820\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72472-8.png 800w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72472-8-293x300.png 293w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72472-8-768x787.png 768w\" sizes=\"(max-width: 800px) 100vw, 800px\" \/><\/p>\n<p>\u56fe2\uff1a\u4e8c\u7ef4ZrTe<sub>2<\/sub>\u6676\u4f53\u7684\u53ef\u63a7\u5408\u6210\u4e0e\u8868\u5f81\u3002a) ZrTe<sub>2<\/sub>\u8584\u7247\u7684AFM\u56fe\u50cf\u3002b) ZrTe<sub>2<\/sub>\u7684\u62c9\u66fc\u5149\u8c31\uff0c\u63d2\u56fe\u4e3aA<sub>1g<\/sub>\u548cE<sub>g<\/sub>\u6a21\u5f0f\u7684\u62c9\u66fc\u5f3a\u5ea6\u5206\u5e03\u56fe\u3002c, d) ZrTe<sub>2<\/sub>\u7684Zr 3d\u548cTe 3d\u9ad8\u5206\u8fa8XPS\u80fd\u8c31\u3002e) ZrTe<sub>2<\/sub>\u6676\u4f53\u7684SAED\u56fe\u8c31\u3002f) ZrTe<sub>2<\/sub>\u6676\u4f53HAADF-STEM\u56fe\u50cf\u53ca\u5bf9\u5e94\u7684EDS\u5143\u7d20mapping\u3002g) ZrTe<sub>2<\/sub>\u6676\u4f53\u7684\u539f\u5b50\u5206\u8fa8HAADF-STEM\u56fe\u50cf\u3002h) g\u56fe\u4e2d\u7ea2\u8272\u548c\u84dd\u8272\u77e9\u5f62\u6807\u8bb0\u533a\u57df\u7684\u5f3a\u5ea6\u7ebf\u626b\u63cf\u56fe\u3002i) \u4f7f\u75281 nm\u539a\u5ea6Zr\u819c\u5728\u4e0d\u540c\u6e29\u5ea6\u4e0b\u5408\u6210\u7684ZrTe<sub>2<\/sub>\u6a2a\u5411\u6676\u7c92\u5c3a\u5bf8\u7edf\u8ba1\uff0c\u63d2\u56fe\u4e3a\u76f8\u5e94\u7684OM\u56fe\u50cf\uff08\u6bd4\u4f8b\u5c3a\u5747\u4e3a10 \u03bcm\uff09\u3002j) ZrTe<sub>2<\/sub>\u8584\u819c\u539a\u5ea6\u968f\u6e85\u5c04Zr\u819c\u539a\u5ea6\u7684\u53d8\u5316\u5173\u7cfb\u3002k-o) 30\u00b0\u626d\u8f6c\u53cc\u5c42ZrTe<sub>2<\/sub>\u7684\u8868\u5f81\uff1a(k) \u5149\u5b66\u56fe\u50cf\uff1b(l) \u626d\u8f6c\u89d2\u793a\u610f\u56fe\uff1b(m) SAED\u56fe\u8c31\uff1b(n) \u539f\u5b50\u5206\u8fa8HAADF-STEM\u56fe\u50cf\uff1b(o) \u76f8\u5e94\u7684\u83ab\u5c14\u6761\u7eb9\u793a\u610f\u56fe\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"alignnone size-full wp-image-267309\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72473-5.png\" alt=\"\" width=\"1000\" height=\"709\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72473-5.png 1000w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72473-5-300x213.png 300w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/06\/\u56fe\u72473-5-768x545.png 768w\" sizes=\"(max-width: 1000px) 100vw, 1000px\" \/><\/p>\n<p>\u56fe3\uff1a\u7845\u5316\u9a71\u52a8\u4e8c\u7ef4ZrTe<sub>2<\/sub>\u9010\u5c42\u751f\u957f\u7684\u673a\u5236\u3002a) \u57fa\u4e8e\u7b2c\u4e00\u6027\u539f\u7406\u548c\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u83b7\u5f97\u7684\u4e8c\u7ef4ZrTe<sub>2<\/sub>\u751f\u957f\u8fc7\u7a0b\uff1a1000 K\u4e0bSi-Te\u4e8c\u805a\u4f53\u4e0eZr\u819c\u4f53\u7cfb\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df1 ps\uff08i\uff09\u548c5 ps\uff08ii\uff09\u7684\u7ed3\u6784\uff1b300 K\u4e0bZr-Te\u5c42\u4e0eSi\u949d\u5316Zr\u819c\u4f53\u7cfb\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df5 ps\u7684\u7ed3\u6784\uff08iii\uff09\uff1bSi\u949d\u5316Zr\u8868\u9762ZrTe<sub>2<\/sub>\u5c42\u7684\u4f18\u5316\u6784\u578b\uff08iv\uff09\u3002b) \u4e8c\u7ef4ZrTe<sub>2<\/sub>\u751f\u957f\u8fc7\u7a0b\u793a\u610f\u56fe\u3002c) Si\u539f\u5b50\u5728Zr\u8868\u9762\u79fb\u52a8\u7684\u7ed3\u6784\u53ca\u521d\u6001\uff08IS\uff09\u3001\u8fc7\u6e21\u6001\uff08TS\uff09\u3001\u7ec8\u6001\uff08FS\uff09\u7684\u76f8\u5bf9\u80fd\u91cf\u3002d) \u5355\u5c42ZrTe<sub>2<\/sub>\u4e0e\u886c\u5e95\u4e4b\u95f4\u7684\u7535\u5b50\u5b9a\u57df\u51fd\u6570\u56fe\uff08\u84dd\u8272\u3001\u6a59\u8272\u3001\u7d2b\u8272\u7403\u4f53\u5206\u522b\u4ee3\u8868Zr\u3001Te\u3001Si\u539f\u5b50\uff09\u3002<\/p>\n<p>&nbsp;<\/p>\n<p>\u6cb3\u5357\u5927\u5b66\u5218\u536b\u6d9b\u535a\u58eb\u3001\u5317\u4eac\u5927\u5b66\u738b\u537f\u8d6b\u535a\u58eb\u3001\u5927\u8fde\u7406\u5de5\u5927\u5b66\u8d75\u5706\u5706\u535a\u58eb\u4e3a\u8bba\u6587\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\uff0c\u6cb3\u5357\u5927\u5b66\u9648\u73c2\u6559\u6388\u548c\u9ec4\u660e\u4e3e\u6559\u6388\u3001\u4e2d\u79d1\u9662\u6df1\u5733\u5148\u8fdb\u6280\u672f\u7814\u7a76\u9662\u4e01\u5cf0\u6559\u6388\u3001\u4e2d\u56fd\u4eba\u6c11\u5927\u5b66\u5218\u707f\u6559\u6388\u4e3a\u8bba\u6587\u7684\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff0c\u5317\u4eac\u5927\u5b66\u5218\u5f00\u8f89\u6559\u6388\u3001\u9ad8\u9e4f\u6559\u6388\u3001\u9648\u53ec\u9f99\u7814\u7a76\u5458\uff0c\u5357\u65b9\u79d1\u6280\u5927\u5b66\u6768\u70fd\u6559\u6388\u7b49\u53c2\u4e0e\u4e86\u5408\u4f5c\u7814\u7a76\uff0c\u6cb3\u5357\u5927\u5b66\u4e3a\u7b2c\u4e00\u901a\u8baf\u5355\u4f4d\u3002\u672c\u7814\u7a76\u5f97\u5230\u4e86\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u56fd\u5bb6\u4e07\u4eba\u8ba1\u5212\u548c\u6cb3\u5357\u7701\u4e2d\u539f\u82f1\u624d\u8ba1\u5212\u7b49\u9879\u76ee\u652f\u6301\u3002\u8bba\u6587\u94fe\u63a5\uff1a<\/p>\n<p><a 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