{"id":268796,"date":"2025-10-08T02:56:00","date_gmt":"2025-10-07T18:56:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=268796"},"modified":"2025-10-08T15:00:38","modified_gmt":"2025-10-08T07:00:38","slug":"%e6%b8%85%e5%8d%8e%e5%a4%a7%e5%ad%a6%e5%90%95%e7%91%9e%e6%b6%9b%e6%95%99%e6%8e%88%e3%80%81%e7%a6%8f%e5%b7%9e%e5%a4%a7%e5%ad%a6%e4%b8%87%e5%ae%87%e9%a9%b0%e5%89%af%e6%95%99%e6%8e%88adv-mater-%ef%bc%9a","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=268796","title":{"rendered":"\u6e05\u534e\u5927\u5b66\u5415\u745e\u6d9b\u6559\u6388\u3001\u798f\u5dde\u5927\u5b66\u4e07\u5b87\u9a70\u526f\u6559\u6388Adv. Mater.\uff1a\u754c\u9762\u6c22\u6ea2\u6d41\u534f\u540c\u7535\u5b50\u8f6c\u79fb\u4fc3\u8fdb\u785d\u9178\u6839\u8fd8\u539f\u4ea7\u6c28"},"content":{"rendered":"\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"313\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/2382c315a6ba396-7.png\" alt=\"\" class=\"wp-image-268797\"\/><\/figure>\n\n\n\n<p>\u7b2c\u4e00\u4f5c\u8005\uff1a\u90d1\u6c90\u4e91<\/p>\n\n\n\n<p>\u901a\u8baf\u4f5c\u8005\uff1a\u5415\u745e\u6d9b\u6559\u6388\u3001\u4e07\u5b87\u9a70\u526f\u6559\u6388<\/p>\n\n\n\n<p>\u901a\u8baf\u5355\u4f4d\uff1a\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\u3001\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662<\/p>\n\n\n\n<p>\u8bba\u6587DOI\uff1a10.1002\/adma.202514834<\/p>\n\n\n\n<p><strong>1. \u7814\u7a76\u80cc\u666f<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u5de5\u4e1a\u548c\u519c\u4e1a\u5e9f\u6c34\u4e2d\u7684\u785d\u9178\u76d0\u6c61\u67d3\u53ef\u80fd\u5bfc\u81f4\u6c34\u4f53\u5bcc\u8425\u517b\u5316\uff0c\u5a01\u80c1\u4eba\u7c7b\u5065\u5eb7\u3002\u5de5\u4e1aHaber-Bosch\u6cd5\u5408\u6210\u6c28\u80fd\u8017\u9ad8\u3001\u78b3\u6392\u653e\u5de8\u5927\uff0c\u56e0\u6b64\u8feb\u5207\u9700\u8981\u5f00\u53d1\u7eff\u8272\u5408\u6210\u6c28\u9014\u5f84\u3002\u800c\u7535\u50ac\u5316\u785d\u9178\u76d0\u8fd8\u539f\u53cd\u5e94\uff08NO<sub>3<\/sub><sup>\u2212<\/sup>RR\uff09\u6709\u671b\u5229\u7528\u53ef\u518d\u751f\u80fd\u6e90\u5c06\u785d\u9178\u76d0\u8f6c\u5316\u4e3a\u6c28\uff0c\u5176\u7406\u8bba\u80fd\u8017\uff086.5 kWh kg<sup>\u2212<\/sup><sup>1<\/sup>\uff09\u8fdc\u4f4e\u4e8eHaber\u2212Bosch\u6cd5\uff0810\u201313 kWh kg<sup>-1<\/sup>\uff09\uff0c\u6709\u671b\u540c\u65f6\u5b9e\u73b0\u5e9f\u6c34\u5904\u7406\u548c\u7eff\u6c28\u5408\u6210\u3002\u7136\u800c\uff0cNO<sub>3<\/sub><sup>\u2212<\/sup>RR\u9886\u57df\u4ecd\u7136\u5b58\u5728\u6311\u6218\uff0c\u5982\u590d\u6742\u7684\u53cd\u5e94\u8def\u5f84\u5bfc\u81f4\u6c28\u9009\u62e9\u6027\u548c\u4ea7\u7387\u4f4e\u3002\u56e0\u6b64\uff0c\u4f18\u5316\u53cd\u5e94\u9014\u5f84\u548c\u8bbe\u8ba1\u9ad8\u6548\u50ac\u5316\u5242\u662f\u4fc3\u8fdb\u7535\u50ac\u5316\u785d\u9178\u76d0\u8fd8\u539f\u5408\u6210\u6c28\u8d70\u5411\u672a\u6765\u5de5\u4e1a\u5e94\u7528\u7684\u5173\u952e\u3002<\/p>\n\n\n\n<p><strong>2. <\/strong><strong>\u6587\u7ae0\u7b80\u4ecb<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u8fd1\u65e5\uff0c\u6e05\u534e\u5927\u5b66\u5415\u745e\u6d9b\u6559\u6388\u3001\u798f\u5dde\u5927\u5b66\u4e07\u5b87\u9a70\u526f\u6559\u6388\u56e2\u961f\u5728\u7535\u50ac\u5316\u9886\u57df\u53d6\u5f97\u91cd\u8981\u8fdb\u5c55\uff0c\u5b9e\u73b0\u4e86\u5927\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7535\u50ac\u5316\u785d\u9178\u76d0\u8fd8\u539f\u5408\u6210\u6c28\uff0c\u7b2c\u4e00\u4f5c\u8005\u4e3a\u6e05\u534e\u5927\u5b66\u535a\u58eb\u751f\u90d1\u6c90\u4e91\u3002\u7814\u7a76\u56e2\u961f\u91c7\u7528\u7535\u6c27\u5316\/\u7535\u6c89\u79ef\u7b56\u7565\uff0c\u5236\u5907\u51faCu<sub>2<\/sub>O\u7eb3\u7c73\u7ebf\u9635\u5217\u8d1f\u8f7d\u7684CoNi\u2013LDH\u7eb3\u7c73\u7247\u81ea\u652f\u6491\u7535\u6781\u3002\u8be5\u7535\u6781\u5728\u78b1\u6027\u6761\u4ef6\u4e0b\u5747\u8868\u73b0\u51fa\u5353\u8d8a\u7684\u7535\u50ac\u5316\u785d\u9178\u76d0\u8fd8\u539f\u53cd\u5e94\uff08NO<sub>3<\/sub><sup>\u2212<\/sup>RR\uff09\u5408\u6210\u6c28\u6027\u80fd\uff0c\u5728\u7ea61 A cm<sup>\u2212<\/sup><sup>2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5b9e\u73b0\u4e8675.2 mg h<sup>\u2212<\/sup><sup>1<\/sup>&nbsp;cm<sup>\u2212<\/sup><sup>2<\/sup>\u4ea7\u6c28\u901f\u7387\uff0c\u5728\u22120.3 V vs. RHE\u7535\u4f4d\u4e0b\u5b9e\u73b0\u4e8697.8%\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201c<em>Interfacial Synergistic Hydrogen Spillover and Electron Transfer for Boosting Electrocatalytic Nitrate Reduction to Ammonia<\/em>\u201d\u4e3a\u9898\uff0c\u4e8e2025\u5e7410\u67086\u65e5\u53d1\u8868\u5728\u56fd\u9645\u671f\u520a\u300a\u5148\u8fdb\u6750\u6599\u300b\uff08<em>Advanced Materials<\/em>\uff09\u4e0a\u3002<\/p>\n\n\n\n<p><strong>3. <\/strong><strong>\u56fe\u6587\u89e3\u6790<\/strong><strong><\/strong><\/p>\n\n\n\n<p><strong>3.1 <\/strong><strong>\u6750\u6599\u5236\u5907\u4e0e\u8868\u5f81<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u8be5\u5de5\u4f5c\u91c7\u7528\u4e86\u4e00\u79cd\u7535\u6c27\u5316\u7ed3\u5408\u7535\u6c89\u79ef\u7684\u7b56\u7565\uff0c\u5728\u6ce1\u6cab\u94dc\u57fa\u5e95\u4e0a\u751f\u957f\u4e86CoNi\u2013LDH@Cu<sub>2<\/sub>O\u5f02\u8d28\u7ed3\u6784\u3002\u9996\u5148\u901a\u8fc7\u9633\u6781\u7535\u6c27\u5316\u65b9\u6cd5\u5236\u5907Cu(OH)<sub>2<\/sub>\u7eb3\u7c73\u7ebf\u9635\u5217\uff0c\u5728\u7a7a\u6c14\u4e2d\u70ed\u89e3\u5236\u5907CuO\u7eb3\u7c73\u7ebf\u9635\u5217\uff0c\u91c7\u7528\u7535\u6c89\u79ef\u6cd5\u8d1f\u8f7dCoNi\u2013LDH\u7eb3\u7c73\u7247\uff0c\u5728\u6b64\u8fc7\u7a0b\u4e2dCuO\u7eb3\u7c73\u7ebf\u9635\u5217\u539f\u4f4d\u7535\u8fd8\u539f\u4e3aCu<sub>2<\/sub>O\u7eb3\u7c73\u7ebf\u9635\u5217\u3002\uff08\u56fe1\uff09\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"828\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/ce6e2814f207c93-6.png\" alt=\"\" class=\"wp-image-268798\"\/><\/figure>\n\n\n\n<p>\u56fe1 CoNi\u2013LDH@Cu<sub>2<\/sub>O\u50ac\u5316\u5242\u7684\u5236\u5907\u4e0e\u8868\u5f81<\/p>\n\n\n\n<p><strong>3.2 <\/strong><strong>\u7535\u50ac\u5316<\/strong><strong>NO<\/strong><strong><sub>3<\/sub><\/strong><strong><sup>&#8211;<\/sup><\/strong><strong>RR<\/strong><strong>\u6027\u80fd\u6d4b\u8bd5<\/strong><strong><\/strong><\/p>\n\n\n\n<p>CoNi\u2013LDH@Cu<sub>2<\/sub>O\u7535\u50ac\u5316\u5242\u5728\u22120.3 V vs. RHE\u7535\u4f4d\u4e0b\u5b9e\u73b0\u4e8697.8%\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\uff0c\u5728\u7ea61 A cm<sup>\u2212<\/sup><sup>2<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u5b9e\u73b0\u4e8675.2 mg h<sup>\u2212<\/sup><sup>1<\/sup>&nbsp;cm<sup>\u2212<\/sup><sup>2<\/sup>\u4ea7\u6c28\u901f\u7387\uff0c\u7a33\u5b9a\u6027\u8d85\u8fc724 h\uff0c\u6027\u80fd\u8d85\u8fc7\u5bf9\u6bd4\u6837\u54c1\u548c\u5927\u591a\u6570\u5df2\u62a5\u9053\u6587\u732e\u3002\u540c\u65f6\u5236\u5907\u4e86CoFe\u2013LDH@Cu<sub>2<\/sub>O\u7535\u50ac\u5316\u5242\u3001NiFe\u2013LDH@Cu<sub>2<\/sub>O\u7535\u50ac\u5316\u5242\uff0c\u5747\u5b9e\u73b0\u4e86\u5927\u7535\u6d41\u5bc6\u5ea6\u4e0b\u9ad8\u6027\u80fdNO<sub>3<\/sub><sup>\u2212<\/sup>RR\uff0c\u8fdb\u4e00\u6b65\u8bc1\u660e\u4e86\u6750\u6599\u6784\u7b51\u7b56\u7565\u7684\u666e\u9002\u6027\u3002\uff08\u56fe2\uff09\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"525\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/7f88dbbcaa77a1d-5.png\" alt=\"\" class=\"wp-image-268799\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/7f88dbbcaa77a1d-5.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/7f88dbbcaa77a1d-5-200x150.png 200w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/figure>\n\n\n\n<p>\u56fe2 \u7535\u50ac\u5316\u785d\u9178\u6839\u8fd8\u539f\u4ea7\u6c28\u6027\u80fd\u6d4b\u8bd5<\/p>\n\n\n\n<p><strong>3.3 <\/strong><strong>\u53cd\u5e94\u673a\u5236\u89e3\u6790<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u539f\u4f4dEPR\u5b9e\u9a8c\u7ed3\u679c\u8868\u660e\uff0c\u52a0\u5165\u53cd\u5e94\u7269\u785d\u9178\u76d0\u540eDMPO-H\u5cf0\u6d88\u5931\uff0cCV\u4e2d\u52a0\u5165\u53cd\u5e94\u7269\u785d\u9178\u76d0\u540eH<sub>ads<\/sub>\u5cf0\u6d88\u5931\uff0c\u8bf4\u660e*H\u53c2\u4e0eNO<sub>3<\/sub><sup>\u2212<\/sup>RR\u4e2d\u7684\u52a0\u6c22\u8fd8\u539f\u6b65\u9aa4\u800c\u88ab\u6d88\u8017\u3002TBA\u6dec\u706d*H\u5b9e\u9a8c\u4e2d\uff0c\u968fTBA\u52a0\u5165\u91cf\u589e\u52a0\u800c\u4ea7\u6c28\u6027\u80fd\u4e0b\u964d\uff0c\u57281000 mM TBA\u4e2d\u83b7\u5f97\u548c\u5bf9\u6bd4\u6837\u54c1Cu foam\u63a5\u8fd1\u7684\u6027\u80fd\uff0c\u8bf4\u660e*H\u7684\u53c2\u4e0e\u662f\u5b9e\u73b0\u9ad8\u6027\u80fdNO<sub>3<\/sub><sup>\u2212<\/sup>RR\u7684\u5173\u952e\uff0c\u800cCoNi\u2013LDH\u7684\u5f15\u5165\u53ef\u4ee5\u6709\u6548\u4fc3\u8fdb*H\u7684\u4ea7\u751f\u3002\u5728\u22120.4 V vs. RHE\u7535\u4f4d\u4e0b\uff0c\u539f\u4f4dDEMS\u5b9e\u9a8c\u68c0\u6d4b\u53cd\u5e94\u4e2d\u95f4\u4f53\uff0c\u5176\u4e2dNH\u5cf0\u5f3a\u5ea6\u660e\u663e\u9ad8\u4e8eNH<sub>2<\/sub>OH\u5cf0\uff0c\u8bf4\u660e\u53cd\u5e94\u8def\u5f84\u4e3aNOH\u8def\u5f84\uff1a*NO<sub>3<\/sub>\u2192*NO<sub>2<\/sub>\u2192*NO\u2192*NOH\u2192*N\u2192*NH\u2192*NH<sub>2<\/sub>\u2192*NH<sub>3<\/sub>\uff08\u56fe3\uff09\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"529\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/4e9a0ba2491dfde-5.png\" alt=\"\" class=\"wp-image-268800\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/4e9a0ba2491dfde-5.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/4e9a0ba2491dfde-5-200x150.png 200w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/figure>\n\n\n\n<p>\u56fe3 \u53cd\u5e94\u673a\u5236\u89e3\u6790<\/p>\n\n\n\n<p><strong>3.4 <\/strong><strong>\u5143\u7d20\u4ef7\u6001\u539f\u4f4d\u5206\u6790<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u5728\u22120.4 V vs. RHE\u7535\u4f4d\u4e0b\uff0c\u4f7f\u7528\u539f\u4f4dXPS\u8868\u5f81NO<sub>3<\/sub><sup>\u2212<\/sup>RR\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u50ac\u5316\u5242\u7684\u5143\u7d20\u4ef7\u6001\u53d8\u5316\u3002\u53cd\u5e94\u8fc7\u7a0b\u4e2dCo\u4ef7\u6001\u4fdd\u6301\u7a33\u5b9a\uff0c\u800cNi\u4ef7\u6001\u7565\u6709\u5347\u9ad8\uff1bCu LMM\u7684\u5cf0\u4f4d\u5411\u52a8\u80fd\u589e\u52a0\u7684\u65b9\u5411\u79fb\u52a8\uff0c\u8868\u660e\u7ed3\u5408\u80fd\u964d\u4f4e\uff0cCu 2p\u7684\u5cf0\u4f4d\u4e5f\u76f4\u63a5\u89c2\u5bdf\u5230\u5411\u7ed3\u5408\u80fd\u964d\u4f4e\u7684\u65b9\u5411\u79fb\u52a8\uff0c\u4ee5\u4e0a\u8868\u660eCu\u7684\u4ef7\u6001\u964d\u4f4e\u3002\u4e0a\u8ff0\u539f\u4f4dXPS\u5206\u6790\u7ed3\u679c\u8868\u660e\uff0c\u5728NO<sub>3<\/sub><sup>\u2212<\/sup>RR\u53cd\u5e94\u8fc7\u7a0b\u4e2d\u53d1\u751f\u4eceCoNi\u2013LDH\u5411Cu<sub>2<\/sub>O\u7684\u7535\u5b50\u8f6c\u79fb\u3002\uff08\u56fe4\uff09\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"261\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/b14210e1ee30421-5.png\" alt=\"\" class=\"wp-image-268801\"\/><\/figure>\n\n\n\n<p>\u56fe4 \u539f\u4f4dXPS\u5206\u6790<\/p>\n\n\n\n<p><strong>3.5 <\/strong><strong>\u7406\u8bba\u8ba1\u7b97<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u5438\u9644\u81ea\u7531\u80fd\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0cCu<sub>2<\/sub>O\u663e\u793a\u51fa\u6bd4CoNi\u2013LDH\u66f4\u8d1f\u7684*NO<sub>3<\/sub>\u5438\u9644\u81ea\u7531\u80fd\uff1bpCOHP\u8ba1\u7b97\u7ed3\u679c\u8868\u660e\uff0c*NO<sub>3<\/sub>\u548cCu<sub>2<\/sub>O\u4e4b\u95f4\u7684\u76f8\u4e92\u4f5c\u7528\u66f4\u5f3a\u3002\u56e0\u6b64\uff0c*NO<sub>3<\/sub>\u66f4\u503e\u5411\u4e8e\u5438\u9644\u5728Cu<sub>2<\/sub>O\uff08111\uff09\u8868\u9762\uff0c\u800c\u975eCoNi\u2013LDH\u3002NO<sub>3<\/sub><sup>\u2212<\/sup>RR\u81ea\u7531\u80fd\u53f0\u9636\u56fe\u8868\u660e\uff0c\u53cd\u5e94\u8def\u5f84\u7684\u51b3\u901f\u6b65\uff08RDS\uff09\u4e3a*NO\u2192*NOH\uff0c\u800cCoNi\u2013LDH@Cu<sub>2<\/sub>O\u663e\u793a\u51fa\u6700\u4f4e\u7684\u51b3\u901f\u6b65\u9aa4\u80fd\u5792\uff0c\u5bf9\u5e94\u4e8e\u6700\u9ad8\u7684NO<sub>3<\/sub><sup>\u2212<\/sup>RR\u6d3b\u6027\u3002\u6b64\u5916\uff0c*NOH\u2192*N\u5728\u70ed\u529b\u5b66\u4e0a\u6bd4*NOH\u2192*NHOH\u6b65\u9aa4\u66f4\u6709\u5229\uff0c\u4e0eDEMS\u7ed3\u679c\u4e00\u81f4\u3002\u5dee\u5206\u7535\u8377\u5bc6\u5ea6\u8868\u660e\uff0c\u7535\u8377\u7d2f\u79ef\u4e8e\u754c\u9762\u7684\u914d\u4f4d\u4e0d\u9971\u548cCu\u539f\u5b50\u9644\u8fd1\uff1b\u6b64\u5916\uff0cCoNi\u2013LDH\u7684\u529f\u51fd\u6570\u5c0f\u4e8eCu<sub>2<\/sub>O\uff0c\u8868\u660e\u7535\u5b50\u5bb9\u6613\u4eceCoNi\u2013LDH\u8f6c\u79fb\u81f3Cu<sub>2<\/sub>O\uff1bBader\u7535\u8377\u5206\u6790\u8868\u660e\uff0c\u5f53\u5f62\u6210CoNi\u2013LDH\u548cCu<sub>2<\/sub>O\u754c\u9762\u65f6\uff0c\u4e0d\u9971\u548cCu\u539f\u5b50\u7684\u4ef7\u6001\u964d\u4f4e\u3002\u4e0a\u8ff0\u7ed3\u679c\u53ef\u4ee5\u8bf4\u660e\uff0c\u7535\u5b50\u503e\u5411\u4e8e\u4eceCoNi\u2013LDH\u8f6c\u79fb\u5230Cu<sub>2<\/sub>O\uff0c\u800c\u8fd9\u4e00\u8fc7\u7a0b\u4e2d\u4e0d\u9971\u548cCu\u539f\u5b50\u7684\u4ef7\u7535\u5b50\u589e\u52a0\u6709\u5229\u4e8e\u5438\u9644\u7684*NO<sub>3<\/sub>\u7684\u8fd8\u539f\u3002\u6b64\u5916\uff0c\u5728Cu<sub>2<\/sub>O\u4e2d\u5f15\u5165CoNi\u2013LDH\u53ef\u4ee5\u5927\u5927\u964d\u4f4e\u6c34\u89e3\u79bb\u7684\u80fd\u5792\u3002\u5f62\u6210\u7684*H\u53ef\u4ee5\u81ea\u53d1\u5730\u53d1\u751f\u6c22\u6ea2\u6d41\u8fc7\u7a0b\uff0c\u4eceCoNi\u2013LDH\u8f6c\u79fb\u5230Cu<sub>2<\/sub>O\uff0c\u4ece\u800c\u52a0\u901fNO<sub>3<\/sub><sup>\u2212<\/sup>RR\u7684\u52a0\u6c22\u52a8\u529b\u5b66\u3002\u57fa\u4e8e\u4e0a\u8ff0\u7406\u8bba\u5206\u6790\u7ed3\u679c\uff0c\u754c\u9762\u6c22\u6ea2\u6d41\u534f\u540c\u7535\u5b50\u8f6c\u79fb\u53ef\u4ee5\u4fc3\u8fdbNO<sub>3<\/sub><sup>\u2212<\/sup>RR\u7684\u591a\u8d28\u5b50\u548c\u7535\u5b50\u53c2\u4e0e\u8fc7\u7a0b\uff0c\u4ece\u800c\u663e\u8457\u63d0\u5347\u7535\u50ac\u5316\u5408\u6210\u6c28\u6027\u80fd\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"562\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/de5bcf7d8eaea98-4.png\" alt=\"\" class=\"wp-image-268802\"\/><\/figure>\n\n\n\n<p>\u56fe5 \u7406\u8bba\u8ba1\u7b97<\/p>\n\n\n\n<p><strong>4<\/strong><strong>.<\/strong><strong>&nbsp;<\/strong><strong>\u603b\u7ed3<\/strong><strong>\u5c55\u671b<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u8be5\u7814\u7a76\u63d0\u51fa\u4e86\u4e00\u79cd\u754c\u9762\u6c22\u6ea2\u51fa\u534f\u540c\u7535\u5b50\u8f6c\u79fb\u7684\u754c\u9762\u8c03\u63a7\u7b56\u7565\uff0c\u901a\u8fc7\u6784\u5efaCoNi\u2013LDH@Cu<sub>2<\/sub>O\u7535\u50ac\u5316\u5242\u5728\u5927\u7535\u6d41\u5bc6\u5ea6\u4e0b\u83b7\u5f9775.2 mg h<sup>\u2212<\/sup><sup>1<\/sup>&nbsp;cm<sup>\u2212<\/sup><sup>2<\/sup>\u4ea7\u6c28\u901f\u7387\u548c\u22120.3 V vs. RHE\u7535\u4f4d\u4e0b97.8%\u7684\u6cd5\u62c9\u7b2c\u6548\u7387\u3002\u539f\u4f4dDEMS\u9274\u522b\u53cd\u5e94\u4e2d\u95f4\u4f53\u5e76\u786e\u5b9aNOH\u53cd\u5e94\u8def\u5f84\uff0c\u539f\u4f4dEPR\u548c\u5176\u4ed6\u5b9e\u9a8c\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u5f15\u5165CoNi\u2013LDH\u53ef\u4ee5\u964d\u4f4e\u6c34\u89e3\u79bb\u7684\u80fd\u5792\uff0c\u4fc3\u8fdb*H\u7684\u4ea7\u751f\uff0c\u5e76\u5728\u754c\u9762\u5904\u81ea\u53d1\u7684\u5b9e\u73b0\u6c22\u6ea2\u6d41\uff0c\u4fc3\u8fdb\u542b\u6c2e\u7269\u79cd\u7684\u6c22\u5316\u8fd8\u539f\u3002\u539f\u4f4dXPS\u5b9e\u9a8c\u7ed3\u5408\u7406\u8bba\u8ba1\u7b97\u8868\u660e\uff0c\u7535\u5b50\u5728\u754c\u9762\u5904\u4eceCoNi\u2013LDH\u8f6c\u79fb\u5230Cu<sub>2<\/sub>O\uff0c\u8fd9\u6709\u52a9\u4e8e\u8fd8\u539f\u4e0d\u9971\u548cCu\u4f4d\u70b9\u4e0a\u5438\u9644\u7684*NO<sub>3<\/sub>\u3002\u8fd9\u9879\u5de5\u4f5c\u4e3a\u754c\u9762\u8bbe\u8ba1\u7b56\u7565\u63d0\u4f9b\u4e86\u65b0\u7684\u89c1\u89e3\uff0c\u5e76\u5236\u5907\u4e86\u4e00\u7cfb\u5217LDH@Cu<sub>2<\/sub>O\u7535\u50ac\u5316\u5242\uff0c\u5b9e\u73b0\u4e86\u5e9f\u6c34\u4e2d\u785d\u9178\u76d0\u5904\u7406\u548c\u9ad8\u6027\u80fd\u7eff\u6c28\u5408\u6210\u3002<\/p>\n\n\n\n<p><strong>\u4f5c\u8005\u4ecb\u7ecd\uff1a<\/strong><strong><\/strong><\/p>\n\n\n\n<p><strong>\u3010\u7b2c\u4e00\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><strong><\/strong><\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"260\" height=\"344\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/aa3023e0288002c-2.png\" alt=\"\" class=\"wp-image-268803\"\/><\/figure>\n\n\n\n<p><strong>\u90d1\u6c90\u4e91<\/strong>\uff0c\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\u535a\u58eb\u7814\u7a76\u751f\uff08\u5bfc\u5e08\uff1a\u5415\u745e\u6d9b\u6559\u6388\uff09\u3002\u4e3b\u8981\u4ece\u4e8b\u8fc7\u6e21\u91d1\u5c5e\u7535\u50ac\u5316\u785d\u9178\u76d0\u8fd8\u539f\u5408\u6210\u6c28\u9886\u57df\u7814\u7a76\uff0c\u4ee5\u7b2c\u4e00\u4f5c\u8005\u5728<em>Adv. Mater.<\/em>, <em>J. Energy Chem.<\/em>\u7b49\u671f\u520a\u4e0a\u53d1\u8868\u591a\u7bc7\u8bba\u6587\u3002\u66fe\u83b7\u6e05\u534e\u5927\u5b66\u7efc\u5408\u4f18\u79c0\u5956\u3001\u6e05\u534e\u5927\u5b66\u672a\u6765\u5b66\u8005\u5956\u5b66\u91d1\u7b49\u3002<\/p>\n\n\n\n<p><strong>\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><strong><\/strong><\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"969\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/e2f457ec632c1f6-1.png\" alt=\"\" class=\"wp-image-268804\"\/><\/figure>\n\n\n\n<p>\u4e07\u5b87\u9a70\uff0c\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662\u526f\u6559\u6388\uff0c\u798f\u5efa\u7701\u9ad8\u5c42\u6b21\u4eba\u624d\u30022023\u5e74\u83b7\u6e05\u534e\u5927\u5b66\u535a\u58eb\u5b66\u4f4d\uff0c\u5e08\u4ece\u5415\u745e\u6d9b\u6559\u6388\uff1b\u540c\u5e74\u52a0\u5165\u798f\u5dde\u5927\u5b66\u5f20\u4e45\u4fca\u9662\u58eb\u56e2\u961f\u3002\u4e3b\u8981\u4ece\u4e8b\u4f4e\u7ef4\u8d1f\u8f7d\u578b\u6750\u6599\u7684\u8bbe\u8ba1\u4e0e\u7535\u50ac\u5316\u6027\u80fd\u8c03\u63a7\u7814\u7a76\u5de5\u4f5c\uff0c\u4ee5\u7b2c\u4e00\u4f5c\u8005\/\u901a\u8baf\u4f5c\u8005\u5728<em>Adv. Mater.<\/em>\uff082\u7bc7\uff09\u3001<em>Energy Environ. Sci.<\/em>\u3001<em>Adv. Energy Mater.<\/em>\u3001<em>Adv. Funct. Mater.<\/em>\u3001<em>ACS Nano<\/em>\u3001<em>Materials Today<\/em>\u7b49\u56fd\u9645\u671f\u520a\u4e0a\u53d1\u8868SCI\u8bba\u658710\u4f59\u7bc7\uff0c\u5176\u4e2d\u591a\u7bc7\u5165\u9009ESI\u9ad8\u88ab\u5f15\u8bba\u6587\u3002\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9752\u5e74\u9879\u76ee\u3001\u798f\u5efa\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u9762\u4e0a\u9879\u76ee\u7b49\u9879\u76ee\u8d44\u52a9\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"700\" height=\"862\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2025\/10\/bf2e94a56e16c6a-1.png\" alt=\"\" class=\"wp-image-268805\"\/><\/figure>\n\n\n\n<p>\u5415\u745e\u6d9b\uff0c\u6e05\u534e\u5927\u5b66\u957f\u8058\u6559\u6388\uff0c\u6750\u6599\u5b66\u9662\u526f\u9662\u957f\u30022009\u5e74\u83b7\u6e05\u534e\u5927\u5b66\u535a\u58eb\u5b66\u4f4d\uff0c2009\u5e74-2013\u5e74\u5148\u540e\u5728\u6e05\u534e\u5927\u5b66\u548c\u7f8e\u56fd\u5bbe\u5915\u6cd5\u5c3c\u4e9a\u5dde\u7acb\u5927\u5b66\u7269\u7406\u7cfb\u505a\u535a\u58eb\u540e\u7814\u7a76\u3002\u4e3b\u8981\u7814\u7a76\u65b9\u5411\u4e3a\u4f4e\u7ef4\u6750\u6599\u7f3a\u9677\u8c03\u63a7\u4e0e\u529f\u80fd\u521b\u5236\u3002\u5728<em>Science<\/em>\u3001<em>Nat. Commun.<\/em>\u3001<em>Adv. Mater.<\/em>\u7b49\u671f\u520a\u53d1\u8868\u8bba\u6587200\u4f59\u7bc7\uff0c\u88ab\u5f1520,400\u4f59\u6b21\uff0cH\u56e0\u5b5068\u30022017\u5e74\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4-\u4f18\u79c0\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\u8d44\u52a9\uff0c2022\u5e74\u83b7\u4e2d\u56fd\u6750\u6599\u7814\u7a76\u5b66\u4f1a\u79d1\u5b66\u6280\u672f\u5956\uff08\u57fa\u7840\u7814\u7a76\uff09\u4e00\u7b49\u5956\uff0c2025\u5e74\u83b7\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u59d4-\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u9879\u76ee\uff08A\u7c7b\uff09\uff08\u539f\u56fd\u5bb6\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\uff09\u8d44\u52a9\u3002<\/p>\n\n\n\n<p><strong>\u6587\u732e\u4fe1\u606f<\/strong><strong><\/strong><\/p>\n\n\n\n<p>Muyun Zheng, Yuchi Wan*, Zheng-Hong Huang, Feiyu Kang, Ruitao Lv*.&nbsp;Interfacial Synergistic Hydrogen Spillover and Electron Transfer for Boosting Electrocatalytic Nitrate Reduction to Ammonia. <strong><em>Adv. Mater. <\/em><\/strong>(2025): e14834. https:\/\/doi.org\/10.1002\/adma.202514834<\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u7b2c\u4e00\u4f5c\u8005\uff1a\u90d1\u6c90\u4e91 \u901a\u8baf\u4f5c\u8005\uff1a\u5415\u745e\u6d9b\u6559\u6388\u3001\u4e07\u5b87\u9a70\u526f\u6559\u6388 \u901a\u8baf\u5355\u4f4d\uff1a\u6e05\u534e\u5927\u5b66\u6750\u6599\u5b66\u9662\u3001\u798f\u5dde\u5927\u5b66\u6750\u6599\u79d1\u5b66\u4e0e\u5de5\u7a0b\u5b66\u9662 \u8bba\u6587DOI\uff1a10.1002\/adma.202514&#8230;<\/p>\n","protected":false},"author":31345,"featured_media":0,"comment_status":"open","ping_status":"","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[2],"tags":[],"class_list":["post-268796","post","type-post","status-publish","format-standard","hentry","category-keji"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/268796"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/31345"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=268796"}],"version-history":[{"count":1,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/268796\/revisions"}],"predecessor-version":[{"id":268806,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/268796\/revisions\/268806"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=268796"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=268796"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=268796"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}