{"id":269683,"date":"2025-11-30T11:50:00","date_gmt":"2025-11-30T03:50:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=269683"},"modified":"2025-11-30T11:50:01","modified_gmt":"2025-11-30T03:50:01","slug":"%e5%9b%bd%e7%a7%91%e5%a4%a7%e6%9d%ad%e5%b7%9e%e9%ab%98%e7%ad%89%e7%a0%94%e7%a9%b6%e9%99%a2%e6%9b%be%e6%bb%94-%e9%87%91%e6%80%9d%e4%bd%b3nat-commun-%ef%bd%9c%e9%ab%98%e9%85%8d%e4%bd%8d%e7%bc%ba","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=269683","title":{"rendered":"\u56fd\u79d1\u5927\u676d\u5dde\u9ad8\u7b49\u7814\u7a76\u9662\u66fe\u6ed4\/\u91d1\u601d\u4f73Nat. Commun.\uff5c\u9ad8\u914d\u4f4d\u7f3a\u9677\u8fdc\u7a0b\u8c03\u63a7\u5355\u539f\u5b50Fe-N5\u4f4d\u70b9\u4ee5\u589e\u5f3a\u7c7b\u82ac\u987f\u6c34\u51c0\u5316\u6027\u80fd"},"content":{"rendered":"\n

\u4e00\u3001\u8bba\u6587\u76f8\u5173\u4fe1\u606f<\/strong><\/p>\n\n\n\n

\u8bba\u6587\u622a\u56fe<\/strong><\/p>\n\n\n\n

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\u8bba\u6587<\/strong> DOI<\/strong>\uff1ahttps:\/\/doi.org\/10.1038\/s41467-025-65425-4<\/p>\n\n\n\n

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1\ufe0f<\/strong>\u20e3<\/strong> <\/strong>\u5168\u6587\u901f\u89c8<\/strong><\/p>\n\n\n\n

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\u8bba\u6587\u94fe\u63a5\uff1ahttps:\/\/www.nature.com\/articles\/s41467-025-65425-4<\/a><\/p>\n\n\n\n

2\ufe0f<\/strong>\u20e3<\/strong> <\/strong>\u80cc\u666f\u4ecb\u7ecd<\/strong><\/p>\n\n\n\n

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4\ufe0f<\/strong>\u20e3<\/strong> <\/strong>\u56fe\u6587\u89e3\u6790<\/strong><\/p>\n\n\n\n

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\"\"<\/figure>\n\n\n\n

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1. <\/strong>\u5355\u539f\u5b50Fe\uff0c\u7535\u5b50\u72b6\u6001\u7cbe\u51c6\u8c03\u63a7<\/strong><\/p>\n\n\n\n

\u9ad8\u5206\u8fa8XPS\u663e\u793aFe\u4ee5Fe2+<\/sup>\u548cFe3+<\/sup>\u5f62\u5f0f\u5b58\u5728\uff0c\u672a\u53d1\u73b0Fe0<\/sup>\u4fe1\u53f7\uff0c\u786e\u8ba4\u539f\u5b50\u7ea7\u5206\u6563\uff0c\u6ca1\u6709\u91d1\u5c5e\u56e2\u7c07\u6216\u7eb3\u7c73\u9897\u7c92\u3002Fe2+<\/sup>\u548cFe3+<\/sup>\u7684\u7ed3\u5408\u80fd\u6b63\u5411\u504f\u79fb0.74\u20131.30 eV\uff0c\u8bf4\u660e\u7f3a\u9677\u5f15\u53d1\u7684\u9ad8\u9636\u914d\u4f4d\u8c03\u63a7\u589e\u5f3a\u4e86Fe\u4e2d\u5fc3\u4e0e\u5916\u5c42\u7535\u5b50\u7684\u76f8\u4e92\u4f5c\u7528\uff08\u56fe2a\uff09\u3002<\/p>\n\n\n\n

2. <\/strong>\u7f3a\u9677\u63d0\u5347Fe\u4ef7\u6001\u4e0e\u914d\u4f4d\u91cd\u6784<\/strong><\/p>\n\n\n\n

Fe K\u8fb9XAFS\u5206\u6790\u663e\u793aFeN5<\/sub>-SD2<\/sub>\u7684\u5438\u6536\u8fb9\u76f8\u5bf9FeN5<\/sub>\u660e\u663e\u53f3\u79fb\uff0c\u8868\u660e\u7f3a\u9677\u6210\u529f\u63d0\u5347Fe\u4ef7\u6001\uff0c\u540c\u65f6\u7f3a\u5931\u65b9\u5e73\u9762FeN4<\/sub>\u7279\u5f81\u524d\u6cbf\u5cf0\uff0c\u8bf4\u660eFe\u914d\u4f4d\u73af\u5883\u88ab\u91cd\u6784\uff08\u56fe2b\uff09\u3002<\/p>\n\n\n\n

3. Fe-N5<\/sub><\/strong>\u7ed3\u6784\u7cbe\u786e\u8868\u5f81<\/strong><\/p>\n\n\n\n

EXAFS\u5206\u6790\u663e\u793a1.53 \u00c5\u7684\u4e3b\u5cf0\u5bf9\u5e94Fe\u2013N\u914d\u4f4d\uff0c\u65e0Fe\u2013Fe\u4fe1\u53f7\uff08\u56fe2c\uff09\uff0c\u5b9a\u91cf\u62df\u5408\u5f97\u5230Fe-N\u5e73\u5747\u914d\u4f4d\u6570\u4e3a5\uff0cFe\u2013N\u952e\u957f\u4eceFePc\u76841.93 \u00c5\u5ef6\u957f\u81f32.01 \u00c5\uff0c\u8bc1\u5b9e\u989d\u5916\u8f74\u5411N\u914d\u4f4d\u7684\u5f62\u6210\u3002\u5c0f\u6ce2\u53d8\u6362\u5206\u6790\u8fdb\u4e00\u6b65\u9a8c\u8bc1\u5355\u539f\u5b50\u7ed3\u6784\uff0c\u4ec5\u6709Fe\u2013N\u4fe1\u53f7\u5cf0\uff0c\u65e0Fe\u2013Fe\u6216Fe\u2013O\u7279\u5f81\uff08\u56fe2d\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe3\u7f3a\u9677\u8c03\u63a7\u5e26\u6765\u9ad8\u6548Fenton-like\u53cd\u5e94<\/strong><\/p>\n\n\n\n

\u901a\u8fc7\u5f15\u5165\u9ad8\u9636\u914d\u4f4d\u7f3a\u9677\uff08\u56fe3a-b\uff09\uff0cFeN5<\/sub>-SD2<\/sub>\u5728PMS\u6d3b\u5316\u4e2d\u8868\u73b0\u51fa\u6700\u4f73\u50ac\u5316\u6027\u80fd\uff0c\u4ec5\u970020\u5206\u949f\u5373\u53ef\u5b9e\u73b0BPA\u5b8c\u5168\u964d\u89e3\uff0c\u5176\u53cd\u5e94\u901f\u7387\u548cTOF\u5747\u663e\u8457\u9ad8\u4e8e\u5176\u4ed6FeN5<\/sub>-SDx<\/sub><\/em>\u50ac\u5316\u5242\uff0c\u8bf4\u660e\u9002\u5ea6\u7f3a\u9677\u6709\u6548\u63d0\u5347\u4e86\u50ac\u5316\u6d3b\u6027\uff08\u56fe3b-c\uff09\u3002\u540c\u65f6\uff0c\u8be5\u50ac\u5316\u5242\u5728\u5bbdpH\u8303\u56f4\uff082\u201311\uff09\u5185\u4f9d\u7136\u4fdd\u6301\u4f18\u5f02\u6027\u80fd\uff08\u56fe3d\uff09\uff0c\u5e76\u5bf9\u5e38\u89c1\u6c34\u4f53\u5e72\u6270\u7269\uff08Cl\u207b\u3001SO4<\/sub>2<\/sup>\u207b\u3001HCO3<\/sub>\u207b\u3001HA\uff09\u8868\u73b0\u51fa\u6781\u4f73\u8010\u53d7\u6027\uff08\u56fe3e\uff09\u3002\u6b64\u5916\uff0cFeN5<\/sub>-SD2<\/sub>\/PMS\u4f53\u7cfb\u53ef\u5e7f\u8c31\u964d\u89e3\u5404\u7c7b\u6c61\u67d3\u7269\uff0c\u5305\u62ec\u67d3\u6599\u3001\u6c2f\u4ee3\u915a\u548c\u836f\u7269\u7b49\uff0c\u5176\u4e2d\u7535\u5b50\u7ed9\u4f53\u5e95\u7269\u964d\u89e3\u6548\u7387\u66f4\u9ad8\uff0c\u63d0\u793a\u8be5\u4f53\u7cfb\u4e3b\u8981\u901a\u8fc7\u975e\u81ea\u7531\u57fa\u9014\u5f84\u5b9e\u73b0\u6c61\u67d3\u7269\u6e05\u9664\uff08\u56fe3f\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe4 FeN5<\/sub>-SDx<\/sub>\/PMS\u4f53\u7cfb\u4e2d\u7684\u6d3b\u6027\u6c27\u4e0e\u50ac\u5316\u673a\u7406<\/strong><\/p>\n\n\n\n

\u5728Fenton-like\u53cd\u5e94\u4e2d\uff0c\u591a\u79cd\u6d3b\u6027\u6c27\uff08ROS\uff09\u53ef\u80fd\u53c2\u4e0e\uff0c\u5305\u62ec\u81ea\u7531\u57fa\uff08\u2022OH\u3001SO4<\/sub>\u2022\u2212<\/sup>\u3001O2<\/sub>\u2022\u2212<\/sup>\uff09\u548c\u975e\u81ea\u7531\u57fa\uff081<\/sup>O2<\/sub>\u3001\u9ad8\u4ef7\u94c1-\u6c27\u7269\u79cd\u3001\u7535\u5b50\u8f6c\u79fb\u9014\u5f84\uff09\u3002\u901a\u8fc7\u7cfb\u7edf\u731d\u706d\u5b9e\u9a8c\u53d1\u73b0\uff0c\u2022OH\u548cSO4<\/sub>\u2022\u2212<\/sup>\u51e0\u4e4e\u4e0d\u53c2\u4e0eBPA\u964d\u89e3\uff0cO2<\/sub>\u2022\u2212<\/sup>\u4ec5\u4f5c\u4e3a\u4e2d\u95f4\u4f53\uff0c\u800c1<\/sup>O2<\/sub>\u624d\u662f\u4e3b\u8981\u6d3b\u6027\u6c27\uff08\u56fe4a\uff09\u3002PMS\u5206\u89e3\u5b9e\u9a8c\u663e\u793a\uff0cFeN5<\/sub>-SD2<\/sub>\u7f3a\u9677\u8bbe\u8ba1\u4e0bPMS\u5206\u89e3\u7387\u6700\u9ad8\uff0c\u5bf9\u5e94BPA\u964d\u89e3\u6548\u7387\u6700\u4f73\uff08\u56fe4b\uff09\uff1b\u9884\u5148\u4e0ePMS\u6df7\u5408\u518d\u52a0BPA\u7684\u53cd\u5e94\u88ab\u6291\u5236\uff0c\u8bf4\u660e\u76f4\u63a5\u7535\u5b50\u8f6c\u79fb\u9014\u5f84\u4e0d\u5360\u4e3b\u5bfc\uff08\u56fe4c\uff09\u3002<\/p>\n\n\n\n

EPR\u5206\u6790\u8fdb\u4e00\u6b65\u9a8c\u8bc11<\/sup>O2<\/sub>\u751f\u6210\u5f3a\u5ea6\u968f\u7f3a\u9677\u987a\u5e8f\u589e\u5f3a\uff08FeN5<\/sub>-SD2<\/sub> > FeN5<\/sub>-SD3<\/sub> > FeN5<\/sub>-SD1<\/sub> > FeN5<\/sub>\uff09\uff08\u56fe4d\uff09,9,10-\u4e8c\u82ef\u57fa\u84bd\u6c27\u5316\u5b9e\u9a8c\u4e5f\u663e\u793a1<\/sup>O2<\/sub>\u751f\u6210\u91cf\u968f\u7f3a\u9677\u589e\u52a0\u800c\u964d\u4f4e\uff08\u56fe4e\uff09\u3002\u62df\u4e00\u7ea7\u52a8\u529b\u5b66\u5206\u6790\u8868\u660e\uff0c1<\/sup>O2<\/sub>\u751f\u6210\u91cf\u4e0eBPA\u964d\u89e3\u6548\u7387\u5448\u706b\u5c71\u578b\u5173\u7cfb\uff0c\u9ad8\u5c42\u914d\u4f4d\u7f3a\u9677\u901a\u8fc7\u589e\u5f3a1<\/sup>O2<\/sub>\u751f\u6210\u663e\u8457\u63d0\u5347\u50ac\u5316\u6027\u80fd\uff08\u56fe4f-g\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe5 \u9ad8\u914d\u4f4d\u58f3\u5c42\u7f3a\u9677\u8c03\u63a7Fe\u2013N<\/strong>5<\/sub><\/strong>\u6d3b\u6027\u4f4d\u70b9\u7684\u4f5c\u7528\u673a\u5236\u3002<\/strong><\/p>\n\n\n\n

DFT\u7ed3\u679c\u8868\u660e\uff0c\u8c03\u63a7\u66f4\u9ad8\u914d\u4f4d\u58f3\u5c42\u53ef\u7cfb\u7edf\u6027\u5730\u63d0\u5347Fe\u4f4d\u70b9\u7684\u7535\u5b50\u7ed3\u6784\u3002\u968f\u7740\u7f3a\u9677\u5f15\u5165\uff0cd\u5e26\u4e2d\u5fc3\u6301\u7eed\u4e0a\u79fb\uff08Fig. 5a\uff09\uff0c\u4f7f\u53cd\u952e\u8f68\u9053\u5360\u636e\u964d\u4f4e\u3001\u7535\u5b50\u5728\u8d39\u7c73\u80fd\u7ea7\u9644\u8fd1\u66f4\u6d3b\u8dc3\uff0c\u4ece\u800c\u589e\u5f3aPMS\u5438\u9644\u80fd\u529b\u3002\u7136\u800c\uff0cPMS\u5438\u9644\u80fd\u5448\u201c\u9002\u4e2d\u6700\u4f18\u201d\u7684\u706b\u5c71\u8d8b\u52bf\uff1aFeN5<\/sub>-SD2<\/sub>\u5177\u6709\u6700\u5408\u9002\u7684\u5438\u9644\u5f3a\u5ea6\uff08Fig.5b\uff09\uff0c\u89e3\u91ca\u4e86\u5176\u6700\u9ad8\u7684\u53cd\u5e94\u901f\u7387\uff0c\u800cFeN5<\/sub>-SD3<\/sub>\u8fc7\u5f3a\u7684\u7ed3\u5408\u5bfc\u81f4\u50ac\u5316\u4f4d\u70b9\u88ab\u8fc7\u5ea6\u5360\u7528\u3002<\/p>\n\n\n\n

\u7535\u8377\u8fc1\u79fb\u5206\u6790\uff08Fig.5c\uff09\u8fdb\u4e00\u6b65\u63ed\u793aFeN5<\/sub>-SD2<\/sub>\u62e5\u6709\u6700\u5f3a\u7684Fe\u2192PMS\u7535\u5b50\u8f6c\u79fb\uff0c\u8bf4\u660e\u9002\u5ea6\u7f3a\u9677\u53ef\u663e\u8457\u964d\u4f4e\u754c\u9762\u7535\u8377\u4f20\u8f93\u963b\u529b\u3002\u7ed3\u5408\u80fd\u5792\u5206\u6790\uff08Fig.5d\u2013f\uff09\u53ef\u77e5O\u2013O\u952e\u7684\u65ad\u88c2\u59cb\u7ec8\u662f\u6700\u6613\u53d1\u751f\u7684PMS\u6d3b\u5316\u6b65\u9aa4\uff0c\u540c\u65f6\u4e5f\u662f\u751f\u62101<\/sup>O2<\/sub>\u7684\u8d77\u59cb\u8def\u5f84\u3002FeN5<\/sub>-SD2<\/sub>\u7684\u9002\u4e2d\u7f3a\u9677\u6709\u6548\u964d\u4f4e\u4e86\u51b3\u901f\u6b65\u9aa4\uff08*PMS\u2192*OH+*SO4<\/sub>\uff09\u7684\u80fd\u5792\uff0c\u5e76\u663e\u8457\u62c9\u957fO\u2013O\u952e\u957f\uff08Fig.5g\uff09\uff0c\u4ece\u800c\u52a0\u901f1<\/sup>O2<\/sub>\u7684\u751f\u6210\u52a8\u529b\u5b66\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe6 BPA\u53bb\u9664\u8def\u5f84\u3001\u6bd2\u6027\u53d8\u5316\u4e0e\u819c\u5e94\u7528\u524d\u666f<\/strong><\/p>\n\n\n\n

\u56fe6\u5c55\u793a\u4e86FeN5<\/sub>-SD2<\/sub>\/PMS\u4f53\u7cfb\u4ece\u201c\u964d\u89e3\u2014\u89e3\u6bd2\u2014\u5e94\u7528\u201d\u4e09\u65b9\u9762\u7684\u6574\u4f53\u8868\u73b0\u3002\u9996\u5148\uff0cBPA\u5728\u4f53\u7cfb\u4e2d\u6cbf\u4e24\u6761\u8def\u5f84\u88ab\u5feb\u901f\u62c6\u89e3\uff0c\u7ecf\u5386\u7f9f\u57fa\u5316\u3001\u65ad\u952e\u548c\u5f00\u73af\uff0c\u6700\u7ec8\u5b8c\u5168\u77ff\u5316\uff0c\u8fc7\u7a0b\u4e2d\u751f\u6210\u7684\u4e2d\u95f4\u4f53\u6bd2\u6027\u5927\u5e45\u4e0b\u964d\uff08\u56fe6a\u2013b\uff09\u3002\u6591\u9a6c\u9c7c\u5b9e\u9a8c\u548c\u5fae\u751f\u7269\u6d3b\u6027\u8fdb\u4e00\u6b65\u9a8c\u8bc1\u4e86\u5904\u7406\u540e\u6eb6\u6db2\u7684\u5b89\u5168\u6027\uff0c\u7ec6\u80de\u5b58\u6d3b\u7387\u663e\u8457\u63d0\u5347\uff08\u56fe6c\u2013d\uff09\u3002<\/p>\n\n\n\n

\u5728\u5e94\u7528\u7aef\uff0c\u7814\u7a76\u6784\u5efa\u4e86PVDF\/FeN5<\/sub>-SD2<\/sub>\u50ac\u5316\u8fc7\u6ee4\u819c\uff0c\u5b9e\u73b0\u6c61\u67d3\u7269\u62e6\u622a\u4e0e\u539f\u4f4d\u6c27\u5316\u7684\u534f\u540c\u6548\u5e94\u3002\u8be5\u819c\u5177\u6709\u826f\u597d\u67d4\u6027\u548c\u7a33\u5b9a\u6027\uff0c\u8fde\u7eed\u8fd0\u884c10\u5c0f\u65f6\u4ecd\u53ef\u4fdd\u6301>95%BPA\u53bb\u9664\u7387\uff0c\u5e76\u5bf94-CP\u3001SMX\u7b49\u591a\u7c7b\u96be\u964d\u89e3\u7269\u540c\u6837\u6709\u6548\uff08\u56fe6e\u2013i\uff09\u3002\u5728\u81ea\u6765\u6c34\u548c\u5730\u8868\u6c34\u4e2d\u6027\u80fd\u4f9d\u65e7\u7a33\u5b9a\uff0c\u94c1\u6d78\u51fa\u8fdc\u4f4e\u4e8e\u56fd\u5bb6\u6807\u51c6\uff08\u56fe6j\uff09\uff0c\u5c55\u793a\u51fa\u4f18\u5f02\u7684\u5de5\u7a0b\u5316\u6f5c\u529b\u3002<\/p>\n\n\n\n

5\ufe0f<\/strong>\u20e3<\/strong> <\/strong>\u603b\u7ed3\u4e0e\u5c55\u671b<\/strong><\/p>\n\n\n\n

\u672c\u7814\u7a76\u901a\u8fc7\u7cbe\u51c6\u8c03\u63a7Fe-N5<\/sub>\u6d3b\u6027\u4e2d\u5fc3\u53ca\u5176\u9ad8\u914d\u4f4d\u58f3\u5c42\u7f3a\u9677\uff0c\u6210\u529f\u6784\u5efa\u4e86\u9ad8\u6548\u3001\u7a33\u5b9a\u4e14\u65e0\u987b\u9ad8\u6e29\u7145\u70e7\u7684\u5355\u539f\u5b50\u50ac\u5316\u4f53\u7cfb\uff0c\u5728PMS\u9ad8\u9009\u62e9\u6027\u6d3b\u5316\u4e0eBPA\u6df1\u5ea6\u89e3\u6bd2\u65b9\u9762\u8868\u73b0\u7a81\u51fa\u3002\u540c\u65f6\uff0c\u96c6\u6210\u5f0fPVDF\/FeN5<\/sub>-SD2<\/sub>\u50ac\u5316\u819c\u5728\u8fde\u7eed\u6d41\u4e0e\u771f\u5b9e\u6c34\u4f53\u4e2d\u5747\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u51c0\u5316\u6027\u80fd\u548c\u5de5\u7a0b\u5316\u7a33\u5b9a\u6027\u3002\u8be5\u7b56\u7565\u4e0d\u4ec5\u63ed\u793a\u4e86PMS\u6d3b\u5316\u8fc7\u7a0b\u4e2d\u7684\u6d3b\u6027\u4f4d\u70b9\u7ed3\u6784\u2013\u6027\u8d28\u5173\u8054\uff0c\u4e5f\u4e3a\u4e0b\u4e00\u4ee3\u6c34\u51c0\u5316\u50ac\u5316\u5242\u7684\u7406\u6027\u8bbe\u8ba1\u63d0\u4f9b\u4e86\u65b0\u7684\u601d\u8def\u4e0e\u4f9d\u636e\uff0c\u6709\u671b\u63a8\u52a8\u9ad8\u7ea7\u6c27\u5316\u6280\u672f\u5728\u57ce\u5e02\u6c34\u5904\u7406\u53ca\u73af\u5883\u4fee\u590d\u9886\u57df\u7684\u5b9e\u9645\u5e94\u7528\u3002<\/p>\n\n\n\n

6\ufe0f<\/strong>\u20e3<\/strong> <\/strong>\u6587\u732e\u4fe1\u606f<\/strong><\/p>\n\n\n\n

Jin, S., Tan, W., Huang, Y. et al. Remote tuning of single-atom Fe-N5<\/sub> sites via high-coordination defects for enhanced Fenton-like water decontamination. Nat Commun 16, 10455 (2025). https:\/\/doi.org\/10.1038\/s41467-025-65425-4<\/a><\/p>\n\n\n\n

\u901a\u8baf\u4f5c\u8005\u4ecb\u7ecd<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u66fe\u6ed4\uff0c\u56fd\u79d1\u5927\u676d\u5dde\u9ad8\u7b49\u7814\u7a76\u9662\u73af\u5883\u5b66\u9662\u6559\u6388\uff0c\u6d59\u6c5f\u7701\u6770\u9752\uff0c\u6d59\u6c5f\u7701\u9ad8\u6821\u9886\u519b\u4eba\u624d\u3002\u957f\u671f\u4ece\u4e8b\u6c61\u67d3\u63a7\u5236\u4e0e\u8d44\u6e90\u5316\u6280\u672f\u7814\u7a76\uff0c\u805a\u7126\u73af\u5883\u50ac\u5316\u754c\u9762\u8fc7\u7a0b\u3001\u9ad8\u7ea7\u6c27\u5316\u8fd8\u539f\u3001\u56fa\u5e9f\u8d44\u6e90\u5316\u7b49\u65b9\u5411\u3002\u76ee\u524d\u5df2\u4e3b\u6301\u56fd\u81ea\u7136\u9762\u4e0a\u3001\u6d59\u6c5f\u7701\u6770\u51fa\u9752\u5e74\u79d1\u5b66\u57fa\u91d1\u3001\u6d59\u6c5f\u7701\u57fa\u91d1\u91cd\u70b9\u9879\u76ee\u7b49\u7eb5\u5411\u3002\u5728Nat. Commun.\u3001Adv. Sci.\u3001ACS Catal.\u3001Adv. Funct. Mater.\u3001Environ. Sci. Technol.\u7b49\u671f\u520a\u4e0a\u53d1\u8868\u5b66\u672f\u8bba\u658790\u4f59\u7bc7\uff0c\u7d2f\u8ba1\u4ed6\u5f154000\u4f59\u6b21\uff0c\u4e13\u5229\u6388\u674317\u9879\u3002\u83b7\u4e2d\u56fd\u79d1\u5b66\u9662\u9662\u957f\u5956\u3001\u6d59\u6c5f\u7701\u81ea\u7136\u79d1\u5b66\u4e09\u7b49\u5956\uff0c\u6307\u5bfc\u5b66\u751f\u83b72023\u4e2d\u56fd\u56fd\u9645\u5927\u5b66\u751f\u521b\u65b0\u5927\u8d5b\u56fd\u5bb6\u94f6\u5956\u3002\u5f53\u9009\u4e2d\u56fd\u73af\u5883\u79d1\u5b66\u5b66\u4f1a\u73af\u5883\u5316\u5b66\u5206\u4f1a\u59d4\u5458\uff1b\u62c5\u4efb\u300aJ. Environ. Health Res.\u300b\u3001\u300aGreen Carbon\u300b\u7b49\u591a\u672c\u671f\u520a\u7f16\u59d4\u6216\u9752\u5e74\u7f16\u59d4\uff1b\u53d7\u8058\u5df4\u585e\u5c14\u516c\u7ea6\u4e9a\u592a\u533a\u57df\u4e2d\u5fc3\u5316\u5b66\u54c1\u548c\u5e9f\u7269\u73af\u5883\u7ba1\u7406\u667a\u5e93\u4e13\u5bb6\u3002\u8bfe\u9898\u7ec4\u6b22\u8fce\u76f8\u5173\u65b9\u5411\u535a\u58eb\u540e\u52a0\u5165\uff0c\u53e6\u6709\u535a\u58eb\u62db\u751f\u540d\u989d\u5c11\u8bb8\u3002<\/p>\n","protected":false},"excerpt":{"rendered":"

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