{"id":270060,"date":"2025-12-29T08:00:00","date_gmt":"2025-12-29T00:00:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=270060"},"modified":"2025-12-28T22:32:21","modified_gmt":"2025-12-28T14:32:21","slug":"%e4%b8%9c%e5%8d%97%e5%a4%a7%e5%ad%a6%e6%9d%8e%e4%b9%83%e6%97%ad%e6%95%99%e6%8e%88nature-communications-%e6%b0%a7%e8%b0%83%e6%8e%a7cu0-cu%e7%95%8c%e9%9d%a2%e5%b7%a5%e7%a8%8b%e5%ae%9e%e7%8e%b0","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=270060","title":{"rendered":"\u4e1c\u5357\u5927\u5b66\u674e\u4e43\u65ed\u6559\u6388Nature Communications: \u6c27\u8c03\u63a7Cu0\u2013Cu+\u754c\u9762\u5de5\u7a0b\u5b9e\u73b0\u5149\u70ed\u50ac\u5316\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u5236\u4e59\u70ef"},"content":{"rendered":"\n
\"\"<\/figure>\n\n\n\n

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\u8bba\u6587DOI\uff1a<\/strong>10.1038\/s41467-025-67844-9<\/p>\n\n\n\n

1\ufe0f<\/strong>\u20e3<\/strong> \u5168\u6587\u901f\u89c8<\/strong><\/strong><\/p>\n\n\n\n

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2\ufe0f<\/strong>\u20e3<\/strong> \u80cc\u666f\u4ecb\u7ecd<\/strong><\/strong><\/p>\n\n\n\n

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3\ufe0f<\/strong>\u20e3<\/strong>\u672c\u6587\u4eae\u70b9<\/strong><\/strong><\/p>\n\n\n\n

1. \u7a81\u7834\u4f20\u7edf\u8010\u6c27\u684e\u688f\uff1a\u539f\u521b\u201c\u6c27\u4ecb\u5bfc-\u52a8\u6001\u754c\u9762\u91cd\u6784\u201d\u7b56\u7565<\/strong><\/strong><\/p>\n\n\n\n

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2. \u4f18\u5f02\u6027\u80fd<\/strong>\uff1a\u592a\u9633\u80fd\u9a71\u52a8\u9ad8\u9009\u62e9\u6027C<\/strong>2<\/sub><\/strong><\/sub><\/strong>H<\/strong>4<\/sub><\/strong><\/sub><\/strong>\u5408\u6210<\/strong><\/p>\n\n\n\n

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3. <\/strong>\u673a\u5236\u6df1\u5ea6\u89e3\u6790\uff1a\u5149\u70ed<\/strong>\u6548\u5e94<\/strong>\u8026\u5408-\u754c\u9762\u7535\u8377\u534f\u540c\u9a71\u52a8\u78b3\u94fe\u589e\u957f<\/strong><\/strong><\/p>\n\n\n\n

\u9996\u63ed\u201c\u5f3a\u5149\u70ed\u8026\u5408\u6548\u5e94 \u2192 O2<\/sub>\u5bcc\u96c6 \u2192 \u52a8\u6001\u754c\u9762\u91cd\u6784\u201d\u7684\u7ea7\u8054\u6548\u5e94\uff0c\u901a\u8fc7\u7406\u8bba\u8ba1\u7b97\u548c\u539f\u4f4d\u5149\u8c31\u8bc1\u5b9e\u754c\u9762\u7535\u8377\u7ea7\u8054\u8f6c\u79fb\u4e0e\u51e0\u4f55\u4f4d\u70b9\u534f\u540c\u4f5c\u7528\uff0c\u70ed\u529b\u5b66\u5b9e\u73b0C1 <\/sub>\u2192 C2<\/sub>\u4ea7\u7269\u6839\u672c\u6027\u8de8\u8d8a\uff0c\u5f00\u8f9f\u78b3\u94fe\u5b9a\u5411\u5408\u6210\u65b0\u9014\u5f84\u3002<\/p>\n\n\n\n

4\ufe0f<\/strong>\u20e3<\/strong> \u56fe\u6587\u89e3\u6790<\/strong><\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. 1 | <\/strong>Mechanistic evolution <\/strong>in<\/strong> <\/strong>multiscale<\/strong> metal<\/strong>-site <\/strong>catalysis<\/strong>.<\/strong><\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. <\/strong>2<\/strong> | <\/strong>Structural and electronic characterization<\/strong> of<\/strong> <\/strong>Ru<\/strong>0.6<\/sub><\/strong><\/sub><\/strong>Cu<\/strong>1<\/sub><\/strong><\/sub><\/strong>\/CeO<\/strong>2<\/sub><\/strong><\/sub><\/strong>.<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. 3 | O<\/strong>2<\/sub><\/strong><\/sub><\/strong>-mediated photothermal catalytic CO<\/strong>2<\/sub><\/strong><\/sub><\/strong> reduction performance.<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. 4 | Active site<\/strong>s<\/strong> verification and operando characterization of C<\/strong>2<\/sub><\/strong><\/sub><\/strong>H<\/strong>4<\/sub><\/strong><\/sub><\/strong>-formation intermediates.<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. <\/strong>5<\/strong> | Theoretical calculation.<\/strong><\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

Fig. <\/strong>6<\/strong> |<\/strong> <\/strong>CO<\/strong>2<\/sub><\/strong><\/sub><\/strong> reduction mechanism<\/strong>.<\/strong><\/p>\n\n\n\n

5\ufe0f<\/strong>\u20e3<\/strong> \u603b\u7ed3\u4e0e\u5c55\u671b<\/strong><\/strong><\/p>\n\n\n\n

\u672c\u7814\u7a76\u7ed3\u5408\u591a\u5c3a\u5ea6\u7406\u8bba\u5efa\u6a21\u4e0e\u5b9e\u9a8c\u5206\u6790\uff0c\u63ed\u793a\u5149\u70ed\u8026\u5408\u6548\u5e94\u5bf9\u91d1\u5c5e\u6d3b\u6027\u4f4d\u70b9\u52a8\u6001\u91cd\u6784\u7684\u9a71\u52a8\u673a\u5236\u3002\u7814\u7a76\u53d1\u73b0\uff0c\u5355\u539f\u5b50Ru\u53d6\u4ee3Ce\u6676\u683c\u5f62\u6210\u626d\u66f2\u4e09\u89d2\u68f1\u67f1\u914d\u4f4d\u7ed3\u6784\uff0c\u663e\u8457\u4fc3\u8fdb\u8d28\u5b50\u8026\u5408\u7535\u5b50\u8f6c\u79fb\u8fc7\u7a0b\uff0c\u8fdb\u800c\u52a0\u901fH2<\/sub>O\u89e3\u79bb\u3002\u50ac\u5316\u8fc7\u7a0b\u4e2d\uff0c\u539f\u4f4d\u4ea7\u751f\u7684O2<\/sub>\u6709\u6548\u8bf1\u5bfc\u5177\u5907\u7535\u8377\u68af\u5ea6\u7684Cu0<\/sup>\u2013Cu+<\/sup>\u754c\u9762\u5f62\u6210\u3002\u8fd9\u79cd\u5f3a\u5149\u70ed\u8026\u5408\u6548\u5e94\u9a71\u52a8\u7684\u52a8\u6001\u81ea\u7ec4\u88c5\u4f4d\u70b9\u4e0d\u4ec5\u4f18\u5316\u5bf9\u5173\u952e\u4e2d\u95f4\u4f53*<\/sup>CHOCO\u7684\u5438\u9644\u884c\u4e3a\uff0c\u8fd8\u91cd\u6784C\u2013C\u5076\u8054\u8def\u5f84\u3002\u901a\u8fc7\u539f\u4f4d\u5149\u8c31\u4e0e\u7535\u5b50\u7ed3\u6784\u5206\u6790\u8bc1\u5b9e\uff0c\u7535\u8377\u68af\u5ea6\u754c\u9762\u4e0e\u51e0\u4f55\u4f4d\u70b9\u7684\u534f\u540c\u4f5c\u7528\u662f\u5b9e\u73b0C2<\/sub>\u4ea7\u7269\u9ad8\u6548\u9009\u62e9\u6027\u7684\u5173\u952e\u3002\u57fa\u4e8e\u6b64\u673a\u7406\u8bbe\u8ba1\u7684Ru0.6<\/sub>Cu1<\/sub>(Cu0<\/sup>\u2013Cu1+<\/sup>)\/CeO2<\/sub>\u50ac\u5316\u5242\uff0c\u5728\u805a\u96c6\u592a\u9633\u80fd\u8f90\u7167\u4e0b\u5b9e\u73b0\u4e86549 \u00b1 20 \u03bcmol\u00b7g\u20131<\/sup>\u7684C2<\/sub>H4<\/sub>\u9ad8\u9009\u62e9\u6027\u751f\u6210\uff0874.3%\uff09\uff0c\u5176\u592a\u9633\u80fd\u81f3\u5316\u5b66\u80fd\u8f6c\u5316\u6548\u7387\uff080.5%\uff09\u76f8\u6bd4\u975e\u805a\u96c6\u592a\u9633\u80fd\u6761\u4ef6\u663e\u8457\u63d0\u534725\u500d\u3002\u8be5\u7814\u7a76\u6df1\u523b\u9610\u660e\u4e86\u5f3a\u5149\u70ed\u8026\u5408\u6548\u5e94\u8bf1\u5bfcO2<\/sub>\u79ef\u7d2f\u3001\u8fdb\u800c\u4ecb\u5bfc\u7535\u8377\u68af\u5ea6\u754c\u9762\u539f\u4f4d\u5f62\u6210\u7684\u673a\u5236\uff0c\u4e3a\u89e3\u51b3\u50ac\u5316\u78b3\u94fe\u589e\u957f\u4e2d\u6d3b\u6027-\u9009\u62e9\u6027-\u7a33\u5b9a\u6027\u76f8\u4e92\u63a3\u8098\u7684\u4e09\u91cd\u56f0\u5883\u63d0\u4f9b\u4e86\u65b0\u7b56\u7565\u3002<\/p>\n\n\n\n

6\ufe0f<\/strong>\u20e3<\/strong> \u6587\u732e\u4fe1\u606f<\/strong><\/strong><\/p>\n\n\n\n

Oxygen-modulated engineering of Cu0<\/sup>\u2013Cu+<\/sup> interfaces for CO2<\/sub>-to-C2<\/sub>H4<\/sub> photoreduction. Nature Communications.<\/em> 2025<\/p>\n\n\n\n

DOI\uff1ahttps:\/\/doi.org\/10.1038\/s41467-025-67844-9<\/p>\n\n\n\n

7\ufe0f<\/strong>\u20e3<\/strong>\u4f5c\u8005\u4ecb\u7ecd<\/strong><\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u4efb\u5b87\u5947\uff0c\u73b0\u4e3a\u4e1c\u5357\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u535a\u58eb\u7814\u7a76\u751f\uff0c\u7814\u7a76\u65b9\u5411\u4e3aCO2<\/sub>\u8d44\u6e90\u5316\u8f6c\u5316\u4e0e\u5229\u7528\u3002\u4ee5\u7b2c\u4e00\u4f5c\u8005\u53ca\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u8eab\u4efd\u5728Nature Communications (2\u7bc7), Angewandte Chemie International Edition\uff0cACS Nano\uff0cACS Catalysis (2\u7bc7). \u7b49SCI\u6536\u5f55\u520a\u7269\u4e0a\u53d1\u8868\u7814\u7a76\u8bba\u658715\u7bc7\uff0c\u7d2f\u8ba1\u53d1\u886818\u7bc7\u3002\u4e3b\u63012025\u548c2026\u5e74\u5ea6\u4e1c\u5357\u5927\u5b66\u535a\u58eb\u7814\u7a76\u751f\u521b\u65b0\u80fd\u529b\u63d0\u5347\u8ba1\u5212\uff0c\u5e76\u6210\u529f\u5165\u9009\u9996\u5c4a\u4e2d\u56fd\u79d1\u534f\u9752\u5e74\u79d1\u6280\u4eba\u624d\u57f9\u80b2\u5de5\u7a0b\u535a\u58eb\u751f\u4e13\u9879\u8ba1\u5212\uff08\u4e2d\u56fd\u80fd\u6e90\u7814\u7a76\u4f1a\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u7a0b\u6dfc\uff0c\u73b0\u4e3a\u4e1c\u5357\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u535a\u58eb\u7814\u7a76\u751f\uff0c\u7814\u7a76\u65b9\u5411\u4e3a\u57fa\u4e8e\u7b2c\u4e00\u6027\u539f\u7406\u8ba1\u7b97\u6a21\u62df\u8bbe\u8ba1\u7528\u4e8e\u5149\/\u7535\u50ac\u5316\u6c34\u5206\u89e3\u3001\u4e8c\u6c27\u5316\u78b3\u8fd8\u539f\u53ca\u751f\u7269\u8d28\u8f6c\u5316\u7684\u65b0\u578b\u9ad8\u6548\u50ac\u5316\u5242\u3002\u4ee5\u7b2c\u4e00\u4f5c\u8005\u53ca\u5171\u540c\u7b2c\u4e00\u4f5c\u8005\u8eab\u4efd\u5728Journal of the American Chemical Society\u3001Journal of Materials Chemistry A\u3001Applied Catalysis B: Environment and Energy\u3001Nano Letters. \u7b49SCI\u6536\u5f55\u520a\u7269\u4e0a\u53d1\u8868\u7814\u7a76\u8bba\u658710\u7bc7\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u8d3a\u7ea2\u658c\uff0c\u73b0\u4e3a\u4e1c\u5357\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u535a\u58eb\u7814\u7a76\u751f\uff0c\u7814\u7a76\u65b9\u5411\u4e3a\u8fde\u7eed\u6d41\u975e\u5747\u76f8\u50ac\u5316CO2<\/sub>\u8d44\u6e90\u5316\u8f6c\u5316\u4e0e\u5229\u7528\u3002\u5728ACS Catalysis, Applied Catalysis B: Environment and Energy, Nano energy, Small. \u7b49SCI\u6536\u5f55\u520a\u7269\u4e0a\u53d1\u8868\u7814\u7a76\u8bba\u658716\u7bc7\uff0c\u7533\u8bf7\/\u6388\u6743\u56fd\u5bb6\u4e13\u52299\u9879\u3002\u66fe\u83b7\u5b9d\u94a2\u4f18\u79c0\u5b66\u751f\u5956\u3001\u7814\u7a76\u751f\u56fd\u5bb6\u5956\u5b66\u91d1\u7b49\u8363\u8a89\uff0c\u5728\u7b2c\u4e5d\u5c4a\u4e2d\u56fd\u7814\u7a76\u751f\u80fd\u6e90\u88c5\u5907\u521b\u65b0\u8bbe\u8ba1\u5927\u8d5b\u7b49\u5b66\u79d1\u7ade\u8d5b\u4e2d\u4ee5\u7b2c\u4e00\u5b8c\u6210\u4eba\u83b7\u5f97\u56fd\u5bb6\u7ea7\u5956\u52b15\u9879\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u674e\u4e43\u65ed\u73b0\u4e3a\u4e1c\u5357\u5927\u5b66\u5316\u5b66\u5316\u5de5\u5b66\u9662\u6559\u6388\uff0c\u535a\/\u7855\u5bfc\u30022003\u5e74~2014\u5e74\u4e8e\u4e1c\u5357\u5927\u5b66\u5206\u522b\u5b8c\u6210\u672c\u79d1\u3001\u7855\u58eb\u548c\u535a\u58eb\u7684\u5b66\u4e60\u548c\u7814\u7a76\u9636\u6bb5\uff1b\u671f\u95f42011\u5e74~2013\u5e74\u5728\u56fd\u5bb6\u7559\u5b66\u57fa\u91d1\u59d4\u7684\u652f\u6301\u4e0b\uff0c\u4e8e\u7f8e\u56fd\u4f50\u6cbb\u4e9a\u7406\u5de5\u5b66\u9662\u8fdb\u884c\u8054\u5408\u57f9\u517b\uff0c\u5bfc\u5e08\u4e3aYounan Xia\u548cKrista Walton\u6559\u6388\u3002\u5165\u9009\u6c5f\u82cf\u7701\u201c333\u9ad8\u5c42\u6b21\u4eba\u624d\u57f9\u517b\u5de5\u7a0b\u201d\u4e2d\u9752\u5e74\u5b66\u672f\u6280\u672f\u5e26\u5934\u4eba\u3001\u5510\u4ef2\u82f1\u57fa\u91d1\u4f1a\u201c\u4ef2\u82f1\u9752\u5e74\u5b66\u8005\u201d\u3001\u6c5f\u82cf\u7701\u201c\u53cc\u521b\u8ba1\u5212\u201d\u79d1\u6280\u526f\u603b\u9879\u76ee\u3001\u5357\u4eac\u9ad8\u5c42\u6b21\u521b\u4e1a\u4eba\u624d\u5f15\u8fdb\u8ba1\u5212\u3002\u4e3b\u6301\u56fd\u5bb6\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u6c5f\u82cf\u7701\u6559\u6539\u9879\u76ee\/\u6c5f\u82cf\u7701\u81ea\u7136\u79d1\u5b66\u57fa\u91d1\u3001\u4f01\u4e1a\u6a2a\u5411\u7b49\u9879\u76ee\u3002\u4ee5\u7b2c\u4e00\u6216\u901a\u8baf\u4f5c\u8005\u5728Nature Communications, Journal of the American Chemical Society, Angewandte Chemie International Edition, ACS Nano, ACS Catalysis, Science Bulletin, Advanced Functional Materials, Nano Energy, AIChE Journal.\u7b49\u5b66\u672f\u671f\u520a\u53d1\u8868\u7814\u7a76\u8bba\u6587100\u4f59\u7bc7\uff1b\u7533\u8bf7\u56fd\u5bb6\u53d1\u660e\u4e13\u522969\u4ef6\uff0c\u6388\u674340\u4ef6\u3002<\/p>\n\n\n\n

\u8bfe\u9898\u7ec4\u5b98\u7f51\uff1ahttps:\/\/www.x-mol.com\/groups\/linaixu191.<\/p>\n","protected":false},"excerpt":{"rendered":"

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