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\u666f\u884c<\/p>\n\n\n\n

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\u56fe<\/strong>1<\/strong>\u7535\u5b50\u4f20\u8f93\u5c42\uff08<\/strong>ETL<\/strong>\uff09\u7684\u8868\u5f81\u3002\uff08<\/strong>a<\/strong>\uff09\u5c55\u793a\u9178\u78b1\u53cd\u5e94\u8f85\u52a9\u5408\u6210<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA<\/strong>\u548c<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-OAm<\/strong>\u7684\u793a\u610f\u56fe\uff08<\/strong>R-NH<\/strong>2<\/sub><\/strong>\u542b\u6b63\u4e01\u80fa\u3001\u03b2<\/strong>–<\/strong>\u82ef\u4e59\u80fa\u7b49\uff09\uff1b\uff08<\/strong>b<\/strong>\uff09\u4e3a<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-OAm<\/strong>\u7eb3\u7c73\u9897\u7c92\u7684<\/strong>TEM<\/strong>\u56fe\u50cf\uff1b\uff08<\/strong>c<\/strong>\uff09<\/strong>TGA<\/strong>\u3001<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA<\/strong>\u53ca<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-OAm<\/strong>\u7684\u62c9\u66fc\u5149\u8c31\uff1b\uff08<\/strong>d<\/strong>\uff09\u4e0d\u540c<\/strong>ETL<\/strong>\u5728<\/strong>FTO<\/strong>\u57fa\u5e95\u4e0a\u7684\u53cd\u5c04\u7387\uff1b\uff08<\/strong>e<\/strong>\uff09\u6fc0\u5b50\u6269\u6563\u957f\u5ea6\u4e0e\u5149\u81f4\u53d1\u5149\u5bff\u547d\u5173\u7cfb\u56fe\u3002<\/strong>\u00a9 2026 Springer Nature<\/strong><\/p>\n\n\n\n

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\u56fe<\/strong>2<\/strong>\u63a9\u57cb\u754c\u9762\u5904<\/strong>2D\/3D<\/strong>\u5f02\u8d28\u7ed3\u7684\u5f62\u6210\u3002\uff08<\/strong>a<\/strong>\uff09\u4e3a\u65f6\u95f4\u5206\u8fa8\u5149\u81f4\u53d1\u5149\u5149\u8c31\u5206\u6790\uff08<\/strong>EA<\/strong>\u4e3a\u4e59\u9178\u4e59\u916f\uff09\uff1b\uff08<\/strong>b<\/strong>\uff09\uff08<\/strong>c<\/strong>\uff09\u5206\u522b\u662f<\/strong>Alfa SnO<\/strong>2<\/sub><\/strong>\uff08\u5bf9\u7167\u7ec4\uff09\u548c<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-OAm<\/strong>\uff08\u76ee\u6807\u7ec4\uff09\u4e0a\u63a9\u57cb\u9499\u949b\u77ff\u7684<\/strong>GIWAXS<\/strong>\u56fe\u8c31\uff1b\uff08<\/strong>d<\/strong>\uff09\u4e24\u7ec4\u9499\u949b\u77ff\u8584\u819c\u7684\u65b9\u4f4d\u89d2\u56fe\u8c31\uff0c\u8bc1\u5b9e\u76ee\u6807\u7ec4\uff08<\/strong>100<\/strong>\uff09\u6676\u9762\u62e9\u4f18\u53d6\u5411\uff1b\uff08<\/strong>e<\/strong>\uff09\u4e0d\u540c\u5165\u5c04\u89d2\u4e0b\u7684<\/strong>GIXRD<\/strong>\u884d\u5c04\u89d2\u8d8b\u52bf\uff1b\uff08<\/strong>f<\/strong>\uff09\u80cc\u5165\u5c04<\/strong>PL<\/strong>\u5149\u8c31\uff0c\u63d2\u56fe\u663e\u793a<\/strong>n=1<\/strong>\u7684<\/strong>2D<\/strong>\u9499\u949b\u77ff\u53d1\u5c04\u5cf0\uff1b\uff08<\/strong>g<\/strong>\uff09\u5668\u4ef6\u622a\u9762<\/strong>SEM<\/strong>\u56fe\u50cf\uff0c\u9499\u949b\u77ff\u5c42\u5448\u5355\u6676\u7c92\u7ed3\u6784\uff1b\uff08<\/strong>h<\/strong>\uff09\uff08<\/strong>i<\/strong>\uff09\u4e3a\u5bf9\u7167\u7ec4\u4e0e\u76ee\u6807\u7ec4\u9499\u949b\u77ff\u8584\u819c\u7684<\/strong>C 1s XPS<\/strong>\u5149\u8c31\uff0c\u8bc1\u5b9e<\/strong>OAm<\/strong>\u914d\u4f53\u5b58\u5728\u3002<\/strong>\u00a9 2026 Springer Nature<\/strong><\/p>\n\n\n\n

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\u56fe<\/strong>3<\/strong>\u63a9\u57cb\u754c\u9762\u5904\u7684\u79bb\u5b50\u4ea4\u6362\u53cd\u5e94\u3002\uff08<\/strong>a<\/strong>\uff09<\/strong>OAm<\/strong>\u3001<\/strong>TGA<\/strong>\u53ca\u5176\u6df7\u5408\u7269\u7684<\/strong>FTIR<\/strong>\u5149\u8c31\uff0c<\/strong>OAm<\/strong>\u7684<\/strong>N\u2013H<\/strong>\u5cf0\u5411\u4f4e\u6ce2\u6570\u4f4d\u79fb\uff0c\u8868\u660e<\/strong>-NH<\/strong>2<\/sub><\/strong>\u8d28\u5b50\u5316\uff1b\uff08<\/strong>b<\/strong>\uff09\uff08<\/strong>c<\/strong>\uff09\u5206\u522b\u4e3a<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA<\/strong>\u3001<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-OAm<\/strong>\u53ca<\/strong>SnO<\/strong>2<\/sub><\/strong>-TGA-FA<\/strong>\u7684<\/strong>FTIR<\/strong>\u7c89\u672b\u5149\u8c31\u4e0e<\/strong>13<\/sup><\/strong>C<\/strong>\u56fa\u4f53<\/strong>NMR<\/strong>\u5149\u8c31\uff1b\uff08<\/strong>d<\/strong>\uff09\u6dfb\u52a0<\/strong>FAI<\/strong>\u540e\uff0c<\/strong>OAm<\/strong>\u7684<\/strong>C\u2013H<\/strong>\u5cf0\u6d88\u5931\uff0c\u51fa\u73b0<\/strong>FA<\/strong>\u207a<\/strong>\u7684<\/strong>N\u2013H<\/strong>\u5cf0\uff0c\u8bc1\u5b9e\u79bb\u5b50\u4ea4\u6362\uff1b\uff08<\/strong>e<\/strong>\uff09\uff08<\/strong>f<\/strong>\uff09\u4e3a<\/strong>2D\/3D<\/strong>\u5f02\u8d28\u7ed3\u5f62\u6210\u673a\u7406\u793a\u610f\u56fe\u53ca<\/strong>FAI<\/strong>\u4e0e<\/strong>RA-TGA<\/strong>\u7684\u79bb\u5b50\u4ea4\u6362\u53cd\u5e94\u65b9\u7a0b\u5f0f\u3002<\/strong>\u00a9 2026 Springer Nature<\/strong><\/p>\n\n\n\n

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\u56fe<\/strong>4<\/strong>\u63a9\u57cb\u754c\u9762\u5904\u8f7d\u6d41\u5b50\u590d\u5408\u7684\u6291\u5236\u3002\uff08<\/strong>a<\/strong>\uff09\u5bf9\u7167\u7ec4\u4e0e\u76ee\u6807\u7ec4\u7eaf\u7535\u5b50\u5668\u4ef6\u7684\u7a7a\u95f4\u7535\u8377\u9650\u5236\u7535\u6d41\uff08<\/strong>SCLC<\/strong>\uff09\u56fe\u8c31\uff1b\uff08<\/strong>b<\/strong>\uff09\u70ed\u5bfc\u7eb3\u8c31\u6d4b\u5f97\u7684\u9677\u9631\u6001\u5bc6\u5ea6\uff0c\u76ee\u6807\u7ec4\u6d45<\/strong>\/<\/strong>\u6df1\u9677\u9631\u5bc6\u5ea6\u5747\u964d\u4f4e\uff1b\uff08<\/strong>c<\/strong>\uff09\u9499\u949b\u77ff<\/strong>\/SnO<\/strong>\u2082<\/strong>\u754c\u9762\u9677\u9631\u5bc6\u5ea6\u4ece<\/strong>1.13\u00d71016<\/sup> cm-3<\/sup><\/strong>\u964d\u81f3<\/strong>9.06\u00d710\u00b9\u2074 cm-3<\/sup><\/strong>\uff1b\uff08<\/strong>d<\/strong>\uff09\uff08<\/strong>e<\/strong>\uff09\u4e0d\u540c\u5149\u7167\u5f3a\u5ea6\u4e0b\u7684<\/strong>C-V<\/strong>\u56fe\u8c31\uff1b\uff08<\/strong>f<\/strong>\uff09\u83ab\u7279<\/strong>–<\/strong>\u8096\u7279\u57fa\u56fe\u8c31\u663e\u793a\u76ee\u6807\u7ec4\u5185\u5efa\u7535\u52bf\u66f4\u9ad8\uff08<\/strong>1.19 V<\/strong>\uff09\uff1b\uff08<\/strong>g<\/strong>\uff09<\/strong>Voc<\/sub><\/strong>\u4e0e\u5149\u7167\u5f3a\u5ea6\u5173\u7cfb\u8bc1\u5b9e\u7535\u8377\u8f6c\u79fb\u6539\u5584\uff1b\uff08<\/strong>h<\/strong>\uff09\u5fae\u5206\u8f7d\u6d41\u5b50\u5bff\u547d\u8868\u660e\u76ee\u6807\u7ec4\u8f7d\u6d41\u5b50\u8f6c\u79fb\u66f4\u5feb\u3002<\/strong>\u00a9 2026 Springer Nature<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe<\/strong>5<\/strong>\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u5149\u4f0f\u6027\u80fd\u4e0e\u7a33\u5b9a\u6027\u3002\uff08<\/strong>a<\/strong>\uff09\u4e24\u7ec4\u5668\u4ef6<\/strong>PCE<\/strong>\u7684\u7edf\u8ba1\u5206\u5e03\uff1b\uff08<\/strong>b<\/strong>\uff09\u6b63\u5411<\/strong>\/<\/strong>\u53cd\u5411\u626b\u63cf<\/strong>J-V<\/strong>\u66f2\u7ebf\uff1b\uff08<\/strong>c<\/strong>\uff09\u76ee\u6807\u7ec4\u7a33\u6001\u529f\u7387\u8f93\u51fa\u6d4b\u8bd5\uff1b\uff08<\/strong>d<\/strong>\uff09\u672a\u5c01\u88c5\u5668\u4ef6<\/strong>MPP<\/strong>\u8ddf\u8e2a\u7ed3\u679c\uff0c\u76ee\u6807\u7ec4<\/strong>3000 h<\/strong>\u540e\u4fdd\u7559<\/strong>95%<\/strong>\u521d\u59cb\u6548\u7387\uff1b\uff08<\/strong>e<\/strong>\uff09<\/strong>6<\/strong>\u00d7<\/strong>6 cm2<\/sup><\/strong>\u9499\u949b\u77ff\u6a21\u7ec4\u7167\u7247\uff1b\uff08<\/strong>f<\/strong>\uff09\uff08<\/strong>g<\/strong>\uff09<\/strong>6<\/strong>\u00d7<\/strong>6 cm2<\/sup><\/strong>\u6a21\u7ec4<\/strong>J-V<\/strong>\u66f2\u7ebf\uff0c\u5b54\u5f84\u9762\u79ef<\/strong>21.54 cm2<\/sup><\/strong>\u65f6<\/strong>PCE=23.44%<\/strong>\uff08\u8ba4\u8bc1<\/strong>22.68%<\/strong>\uff09\uff1b\uff08<\/strong>h<\/strong>\uff09<\/strong>10<\/strong>\u00d7<\/strong>10 cm2<\/sup><\/strong>\u5927\u6a21\u7ec4<\/strong>J-V<\/strong>\u66f2\u7ebf\uff0c\u5b54\u5f84\u9762\u79ef<\/strong>64.80 cm2<\/sup><\/strong>\u65f6<\/strong>PCE=22.22%<\/strong>\uff1b\uff08<\/strong>i<\/strong>\uff09\u5df2\u62a5\u9053<\/strong>2D\/3D<\/strong>\u9499\u949b\u77ff\u5668\u4ef6<\/strong>PCE<\/strong>\u968f\u9762\u79ef\u53d8\u5316\u7684\u7edf\u8ba1\u5bf9\u6bd4\u3002<\/strong>\u00a9 2026 Springer Nature<\/strong><\/p>\n\n\n\n

\u4f5c\u8005\u901a\u8fc7FTIR\u3001\u56fa\u6001\u6838\u78c1\u5171\u632f\u7b49\u8868\u5f81\u8bc1\u5b9e\u4e86\u5def\u57fa\u4e59\u9178\uff08TGA\uff09\u4e0e\u6cb9\u80fa\uff08OAm\uff09\u7684\u9178\u78b1\u53cd\u5e94\u53ca\u540e\u7eed\u4e0e\u7532\u8112\u7898\uff08FAI\uff09\u7684\u79bb\u5b50\u4ea4\u6362\u673a\u5236\uff0c\u660e\u786eOAm\u901a\u8fc7\u79bb\u5b50\u952e\u7a33\u5b9a\u63a5\u679d\u4e8eSnO2<\/sub>\u8868\u9762\uff0c\u70ed\u9000\u706b\u65f6\u5b9a\u5411\u91ca\u653e\u5e76\u4e0e\u754c\u9762PbI2<\/sub>\u53cd\u5e94\u5f62\u62102D\u9499\u949b\u77ff\uff0c\u4e3a\u63a9\u57cb\u754c\u97622D\/3D\u5f02\u8d28\u7ed3\u7684\u7cbe\u51c6\u6784\u5efa\u63d0\u4f9b\u4e86\u5316\u5b66\u57fa\u7840\uff1b\u540c\u65f6\uff0c\u501f\u52a9\u7a7a\u95f4\u7535\u8377\u9650\u5236\u7535\u6d41\u3001\u70ed\u5bfc\u7eb3\u8c31\u3001\u7535\u5bb9-\u7535\u538b\u7b49\u7535\u5b66\u6d4b\u8bd5\uff0c\u9a8c\u8bc1\u4e86\u8be5\u5f02\u8d28\u7ed3\u4f7f\u9499\u949b\u77ff\/SnO2<\/sub>\u754c\u9762\u7f3a\u9677\u6d53\u5ea6\u964d\u4f4e\u8d85\u5341\u500d\uff0c\u6709\u6548\u6291\u5236\u8f7d\u6d41\u5b50\u590d\u5408\u4e0e\u7535\u8377\u79ef\u7d2f\uff0c\u63d0\u5347\u5185\u5efa\u7535\u52bf\u548c\u7535\u8377\u4f20\u8f93\u6548\u7387\uff1b\u6700\u540e\uff0c\u6587\u7ae0\u5448\u73b0\u4e86\u8be5\u7b56\u7565\u5728\u4e0d\u540c\u5c3a\u5bf8\u5668\u4ef6\u4e0a\u7684\u5149\u4f0f\u6027\u80fd\u4e0e\u7a33\u5b9a\u6027\u4f18\u52bf\uff0c\u5c0f\u9762\u79ef\u5668\u4ef6\u5149\u7535\u8f6c\u6362\u6548\u7387\u8fbe26.19%\uff08\u8ba4\u8bc126.04%\uff09\uff0c21.54 cm2<\/sup>\u548c64.80 cm2<\/sup>\u5927\u5c3a\u5bf8\u6a21\u7ec4\u6548\u7387\u5206\u522b\u8fbe23.44%\uff08\u8ba4\u8bc122.68%\uff09\u548c22.22%\uff0c\u4e14\u672a\u5c01\u88c5\u5668\u4ef6\u5728\u8fde\u7eed\u8fd0\u884c3000 h\u540e\u4ecd\u4fdd\u755995%\u4ee5\u4e0a\u521d\u59cb\u6548\u7387\uff0c\u5145\u5206\u8bc1\u660e\u4e86\u8be5\u754c\u9762\u5de5\u7a0b\u7b56\u7565\u7684\u5b9e\u7528\u6027\u4e0e\u89c4\u6a21\u5316\u5e94\u7528\u6f5c\u529b\u3002<\/p>\n\n\n\n

\u8be5\u7814\u7a76\u5b9e\u73b0\u4e86\u4e00\u79cd\u9ad8\u6027\u80fdn\u2013i\u2013p\u578b\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\uff0c\u4ee5\u201cBuried 2D\/3D heterojunction in n\u2013i\u2013p perovskite solar cells through solid-state ligand-exchange reaction<\/strong>\u201d\u4e3a\u9898\u53d1\u8868\u5728\u56fd\u9645\u9876\u7ea7\u671f\u520aNature Energy<\/strong>\u4e0a\uff0c\u5f15\u8d77\u4e86\u76f8\u5173\u9886\u57df\u7814\u7a76\u4eba\u5458\u70ed\u8bae\u3002<\/strong><\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u4e09\u3001\u3010\u79d1\u5b66\u542f\u8fea\u3011<\/strong><\/p>\n\n\n\n

\u7efc\u4e0a\u6240\u8ff0\uff0c\u8be5\u7814\u7a76\u901a\u8fc7\u56fa\u6001\u914d\u4f53\u4ea4\u6362\u7b56\u7565\uff0c\u6210\u529f\u5728<\/a>n\u2013i\u2013p<\/a>\u578b\u9499\u949b\u77ff\u592a\u9633\u80fd\u7535\u6c60\u7684\u63a9\u57cb\u754c\u9762\u7cbe\u51c6\u6784\u5efa2D\/3D\u5f02\u8d28\u7ed3\uff0c\u89e3\u51b3\u4e86\u4f20\u7edf\u914d\u4f53\u6613\u6eb6\u89e3\u30012D\u76f8\u96be\u4ee5\u5b9a\u4f4d\u5f62\u6210\u7684\u5173\u952e\u96be\u9898\u3002\u6539\u6027\u540e\u7684SnO\u2082-TGA-OAm\u7535\u5b50\u4f20\u8f93\u5c42\u663e\u8457\u63d0\u5347\u4e86\u9499\u949b\u77ff\u8584\u819c\u7684\u7ed3\u6676\u8d28\u91cf\uff0c\u4f7f\u754c\u9762\u7f3a\u9677\u6d53\u5ea6\u964d\u4f4e\u8d85\u5341\u500d\uff0c\u5668\u4ef6\u6548\u7387\u4e0e\u7a33\u5b9a\u6027\u5b9e\u73b0\u534f\u540c\u7a81\u7834\uff0c\u5c0f\u9762\u79ef\u5668\u4ef6\u6548\u7387\u8fbe26.19%\uff0c\u5927\u5c3a\u5bf8\u6a21\u7ec4\u6548\u7387\u4fdd\u6301\u572822%\u4ee5\u4e0a\uff0c\u4e3a\u9499\u949b\u77ff\u7535\u6c60\u7684\u754c\u9762\u5de5\u7a0b\u63d0\u4f9b\u4e86\u5168\u65b0\u601d\u8def\u3002<\/p>\n\n\n\n

\u672a\u6765\u53ef\u8fdb\u4e00\u6b65\u4f18\u5316\u914d\u4f53\u7ed3\u6784\u4e0e\u7ec4\u5206\uff0c\u62d3\u5c55\u8be5\u7b56\u7565\u5728\u4e0d\u540c\u4f53\u7cfb\u9499\u949b\u77ff\u7535\u6c60\u4e2d\u7684\u9002\u7528\u6027\uff1b\u540c\u65f6\u63a8\u52a8\u5de5\u827a\u4e0e\u4ea7\u4e1a\u5316\u6210\u819c\u6280\u672f\u7684\u6df1\u5ea6\u9002\u914d\uff0c\u51cf\u5c11\u5927\u9762\u79ef\u5236\u5907\u4e2d\u7684\u6548\u7387\u8870\u51cf\u3002\u6b64\u5916\uff0c\u7ed3\u5408\u5168\u754c\u9762\u949d\u5316\u4e0e\u53e0\u5c42\u7535\u6c60\u8bbe\u8ba1\uff0c\u6709\u671b\u7a81\u7834\u5355\u7ed3\u5668\u4ef6\u6548\u7387\u6781\u9650\uff0c\u52a0\u901f\u9499\u949b\u77ff\u5149\u4f0f\u6280\u672f\u7684\u5546\u4e1a\u5316\u843d\u5730\u3002<\/p>\n\n\n\n

\u539f\u6587\u8be6\u60c5<\/strong>\uff1aZhao, Q., Zhang, B., Hui, W. et al. Buried 2D\/3D heterojunction in n\u2013i\u2013p perovskite solar cells through solid-state ligand-exchange reaction. Nat Energy (2026). https:\/\/doi.org\/10.1038\/s41560-026-01980-4<\/p>\n\n\n\n

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