{"id":271287,"date":"2026-04-02T08:33:00","date_gmt":"2026-04-02T00:33:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=271287"},"modified":"2026-04-01T23:38:17","modified_gmt":"2026-04-01T15:38:17","slug":"%e4%b8%8a%e6%b5%b7%e7%90%86%e5%b7%a5%e5%a4%a7%e5%ad%a6%e7%86%8a%e5%a9%b7%e5%9b%a2%e9%98%9fgreen-chemistry%ef%bc%9amno2%e7%95%8c%e9%9d%a2%e5%b7%a5%e7%a8%8b%e5%ae%9e%e7%8e%b0%e9%ab%98%e6%80%a7%e8%83%bd","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=271287","title":{"rendered":"\u4e0a\u6d77\u7406\u5de5\u5927\u5b66\u718a\u5a77\u56e2\u961fGreen Chemistry\uff1aMnO2\u754c\u9762\u5de5\u7a0b\u5b9e\u73b0\u9ad8\u6027\u80fd\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60"},"content":{"rendered":"\n

\u80cc\u666f\u4ecb\u7ecd<\/strong><\/strong><\/p>\n\n\n\n

\u968f\u7740\u592a\u9633\u80fd\u7b49\u53ef\u518d\u751f\u80fd\u6e90\u7684\u5feb\u901f\u53d1\u5c55\uff0c\u5982\u4f55\u5b9e\u73b0\u80fd\u91cf\u91c7\u96c6\u3001\u5b58\u50a8\u4e0e\u5229\u7528\u7684\u4e00\u4f53\u5316\uff0c\u5df2\u6210\u4e3a\u80fd\u6e90\u6750\u6599\u9886\u57df\u7684\u91cd\u8981\u7814\u7a76\u65b9\u5411\u3002\u4f20\u7edf\u592a\u9633\u80fd\u4f9b\u80fd\u7cfb\u7edf\u901a\u5e38\u91c7\u7528\u201c\u592a\u9633\u80fd\u7535\u6c60+\u50a8\u80fd\u7535\u6c60\u201d\u7684\u5206\u4f53\u5f0f\u67b6\u6784\uff0c\u867d\u7136\u6280\u672f\u8f83\u4e3a\u6210\u719f\uff0c\u4f46\u4ecd\u5b58\u5728\u5668\u4ef6\u7ed3\u6784\u590d\u6742\u3001\u80fd\u91cf\u8f6c\u6362\u635f\u8017\u8f83\u5927\u4ee5\u53ca\u7cfb\u7edf\u96c6\u6210\u6210\u672c\u8f83\u9ad8\u7b49\u95ee\u9898\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u5149\u5145\u7535\u6c60\u80fd\u591f\u5728\u5355\u4e00\u5668\u4ef6\u4e2d\u540c\u65f6\u5b9e\u73b0\u5149\u80fd\u6355\u83b7\u4e0e\u7535\u5316\u5b66\u50a8\u80fd\uff0c\u88ab\u8ba4\u4e3a\u662f\u6784\u5efa\u4e0b\u4e00\u4ee3\u81ea\u4f9b\u80fd\u7cfb\u7edf\u7684\u91cd\u8981\u5019\u9009\u65b9\u6848\u3002<\/p>\n\n\n\n

\u5728\u4f17\u591a\u50a8\u80fd\u4f53\u7cfb\u4e2d\uff0c\u950c\u79bb\u5b50\u7535\u6c60\u7531\u4e8e\u5177\u6709\u8d44\u6e90\u4e30\u5bcc\u3001\u5b89\u5168\u6027\u9ad8\u3001\u73af\u5883\u53cb\u597d\u548c\u6210\u672c\u4f4e\u7b49\u4f18\u52bf\uff0c\u8fd1\u5e74\u6765\u53d7\u5230\u5e7f\u6cdb\u5173\u6ce8\u3002\u82e5\u5c06\u5176\u4e0e\u5149\u7535\u8f6c\u6362\u8fc7\u7a0b\u8026\u5408\uff0c\u6709\u671b\u6784\u5efa\u517c\u5177\u7eff\u8272\u6027\u548c\u5b9e\u7528\u6027\u7684\u5149\u5145\u50a8\u4e00\u4f53\u5316\u5668\u4ef6\u3002\u7136\u800c\uff0c\u76ee\u524d\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u4ecd\u9762\u4e34\u4e00\u4e2a\u5173\u952e\u74f6\u9888\uff0c\u5373\u5149\u6b63\u6781\u6750\u6599\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\u504f\u4f4e\uff0c\u5bfc\u81f4\u5176\u6574\u4f53\u6027\u80fd\u53d7\u9650\u3002MnO2<\/sub>\u4f5c\u4e3a\u4e00\u79cd\u5e38\u89c1\u7684\u950c\u79bb\u5b50\u5b58\u50a8\u6750\u6599\uff0c\u5177\u6709\u7406\u8bba\u5bb9\u91cf\u8f83\u9ad8\u3001\u539f\u6599\u5ec9\u4ef7\u548c\u4f4e\u6bd2\u7b49\u4f18\u70b9\uff0c\u4f46\u5176\u5149\u751f\u8f7d\u6d41\u5b50\u5206\u79bb\u80fd\u529b\u6709\u9650\uff0c\u4e25\u91cd\u5236\u7ea6\u4e86\u5668\u4ef6\u7684\u8fdb\u4e00\u6b65\u53d1\u5c55\u3002<\/p>\n\n\n\n

\u56e0\u6b64\uff0c\u5982\u4f55\u901a\u8fc7\u754c\u9762\u5de5\u7a0b\u8c03\u63a7MnO2<\/sub>\u7535\u6781\u4e2d\u7684\u7535\u8377\u4f20\u8f93\u548cZn2+<\/sup>\u5b58\u50a8\u884c\u4e3a\uff0c\u8fdb\u800c\u63d0\u5347\u5668\u4ef6\u7684\u5149\u5145\u7535\u6027\u80fd\uff0c\u662f\u8be5\u9886\u57df\u4e9f\u5f85\u89e3\u51b3\u7684\u95ee\u9898\u3002<\/p>\n\n\n\n

\u6210\u679c\u7b80\u4ecb<\/strong><\/strong><\/p>\n\n\n\n

\u8fd1\u65e5\uff0c\u4e0a\u6d77\u7406\u5de5\u5927\u5b66\u718a\u5a77\u56e2\u961f\u5728 Green Chemistry \u4e0a\u53d1\u8868\u9898\u4e3a Interface engineering of MnO2<\/sub> for high-performance photo-rechargeable Zn ion batteries \u7684\u7814\u7a76\u8bba\u6587\u3002\u8be5\u5de5\u4f5c\u901a\u8fc7\u5728MnO2<\/sub>\u4e0eTi\u57fa\u5e95\u4e4b\u95f4\u5f15\u5165\u4e00\u5c42\u975e\u6676TiO2<\/sub>\u754c\u9762\u5c42\uff0c\u6210\u529f\u6784\u5efa\u4e86MnO2<\/sub>\/TiO2<\/sub>\u5149\u6b63\u6781\uff0c\u663e\u8457\u589e\u5f3a\u4e86\u5149\u751f\u7535\u5b50-\u7a7a\u7a74\u5bf9\u5206\u79bb\u6548\u7387\uff0c\u5e76\u52a0\u5feb\u4e86\u540e\u7eedZn2+<\/sup>\u5b58\u50a8\u52a8\u529b\u5b66\uff0c\u4ece\u800c\u5b9e\u73b0\u4e86\u9ad8\u6027\u80fd\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u3002<\/p>\n\n\n\n

\u7814\u7a76\u8868\u660e\uff0c\u8be5MnO2<\/sub>\/TiO2<\/sub>\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u5728\u5149\u7167\u6761\u4ef6\u4e0b\u53ef\u5b9e\u73b0374 mAh g-1<\/sup>\u7684\u9ad8\u6bd4\u5bb9\u91cf\uff0c\u660e\u663e\u9ad8\u4e8e\u6697\u6001\u4e0b\u7684230 mAh g-1<\/sup>\uff1b\u5728\u7eaf\u5149\u5145\u7535\u6761\u4ef6\u4e0b\uff0c\u5668\u4ef6\u5f00\u8def\u7535\u538b\u53ef\u8fbe\u52301.39 V\uff0c\u6700\u9ad8\u5149\u7535\u8f6c\u6362\u6548\u7387\u8fbe\u52301.5 %\u3002\u8fdb\u4e00\u6b65\u5730\uff0c\u4f5c\u8005\u8fd8\u6784\u5efa\u4e86\u7531\u591a\u4e2a\u5668\u4ef6\u4e32\u5e76\u8054\u7ec4\u6210\u7684\u96c6\u6210\u6a21\u5757\uff0c\u5728\u81ea\u7136\u5149\u7167\u6761\u4ef6\u4e0b\u5b8c\u6210\u5149\u5145\u7535\u540e\uff0c\u53ef\u6210\u529f\u9a71\u52a8\u65e0\u4eba\u673a\u3001\u6a21\u578b\u5c0f\u8f66\u548c\u706f\u6ce1\u7b49\u7535\u5b50\u8bbe\u5907\uff0c\u5c55\u793a\u51fa\u8be5\u4f53\u7cfb\u5728\u67d4\u6027\u3001\u81ea\u4e3b\u4f9b\u80fd\u5668\u4ef6\u4e2d\u7684\u5e94\u7528\u6f5c\u529b\u3002\u8be5\u5de5\u4f5c\u4e3aMnO2<\/sub>\u57fa\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u63d0\u4f9b\u4e86\u4e00\u79cd\u7b80\u5355\u800c\u9ad8\u6548\u7684\u754c\u9762\u8bbe\u8ba1\u7b56\u7565\uff0c\u4e5f\u4e3a\u6784\u7b51\u7eff\u8272\u3001\u4f4e\u6210\u672c\u3001\u53ef\u6301\u7eed\u7684\u5149\u5145\u50a8\u4e00\u4f53\u5316\u80fd\u6e90\u7cfb\u7edf\u63d0\u4f9b\u4e86\u65b0\u601d\u8def\u3002<\/p>\n\n\n\n

\u56fe\u6587\u7b80\u4ecb<\/strong><\/strong><\/p>\n\n\n\n

\u56fe\u4e00 \u5149\u6b63\u6781\u7684\u8bbe\u8ba1<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

(a) \u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u7684\u5e94\u7528\u793a\u610f\u56fe\uff1b<\/p>\n\n\n\n

(b) \u57fa\u4e8eMnO2<\/sub>\/TiO2<\/sub>\u5149\u6b63\u6781\u7684\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u5de5\u4f5c\u673a\u7406\u53ca\u5149\u5145\u7535\u8fc7\u7a0b\u793a\u610f\u56fe\u3002<\/p>\n\n\n\n

\u56fe\u4e8c \u5149\u6b63\u6781\u7684\u7ed3\u6784\u4e0e\u5f62\u8c8c\u8868\u5f81<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

(a) MnO2<\/sub>\u7684XRD\u56fe\u8c31\uff1b<\/p>\n\n\n\n

(b) SEM\u56fe\u50cf\uff1b<\/p>\n\n\n\n

(c) TEM\u56fe\u50cf\uff1b<\/p>\n\n\n\n

(d) HR-TEM\u56fe\u50cf\uff1b<\/p>\n\n\n\n

(e) UV-vis DRS\u5149\u8c31\u53ca\u80fd\u5e26\u7ed3\u6784\u793a\u610f\u56fe\uff1b<\/p>\n\n\n\n

(f) TiO2<\/sub>@Ti\u7684SEM \u56fe\u50cf\uff1b<\/p>\n\n\n\n

(g) XRD\u56fe\u8c31\uff1b<\/p>\n\n\n\n

(h) EDX\u80fd\u8c31\u53ca\u5143\u7d20\u5206\u5e03\u56fe\uff1b<\/p>\n\n\n\n

(i) MnO2<\/sub>@Ti\u4e0eMnO2<\/sub>\/TiO2<\/sub>@Ti\u7684\u5149\u7535\u6d41\u54cd\u5e94\u3002<\/p>\n\n\n\n

\u56fe\u4e09 MnO2<\/sub>\u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u7684\u7535\u5316\u5b66\u6027\u80fd<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

(a) \u7535\u5316\u5b66\u963b\u6297\u8c31\uff08EIS\uff09\u6d4b\u8bd5\uff1b<\/p>\n\n\n\n

(b) \u6697\u6001\u548c\u5149\u7167\u6761\u4ef6\u4e0b\u5bf9\u5e94\u7684\u6269\u6563\u6548\u7387\uff1b<\/p>\n\n\n\n

(c) 0.5 mV s-1<\/sup>\u626b\u63cf\u901f\u7387\u4e0b\u7684\u5faa\u73af\u4f0f\u5b89\uff08CV\uff09\u66f2\u7ebf\uff1b<\/p>\n\n\n\n

(d) \u5149\u7167\u6761\u4ef6\u4e0b\u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e0b\u7684 CV \u66f2\u7ebf\uff1b<\/p>\n\n\n\n

(e) \u7535\u5bb9\u8d21\u732e\uff1b<\/p>\n\n\n\n

(f) \u6d3b\u6027\u4f4d\u70b9\uff1b<\/p>\n\n\n\n

(g) 0.2 A g-1<\/sup>\u7535\u6d41\u5bc6\u5ea6\u4e0b\u7684\u5145\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n\n\n\n

(h) \u500d\u7387\u6027\u80fd\uff1b<\/p>\n\n\n\n

(i) \u6697\u6001\u548c\u5149\u7167\u6761\u4ef6\u4e0b\u7684\u80fd\u91cf\u5bc6\u5ea6\u3002<\/p>\n\n\n\n

\u56fe\u56db \u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u7684\u5149\u5145\u7535\u6027\u80fd<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

(a) \u91c7\u7528\u7535\u5316\u5b66\u5de5\u4f5c\u7ad9\u5728\u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u4e0b\u8fdb\u884c\u5149\u5145\u7535\u53ca\u540e\u7eed\u6052\u6d41\u653e\u7535\uff1b<\/p>\n\n\n\n

(b) \u5149\u5145\u7535\u540e\u5728\u5149\u7167\u6761\u4ef6\u4e0b\u548c\u6697\u6001\u6761\u4ef6\u4e0b\u653e\u7535\uff1b<\/p>\n\n\n\n

(c) \u7ecf\u8fc7\u516d\u6b21\u5149\u5145\u7535\u6d4b\u8bd5\u540e\u7684\u5bb9\u91cf\u4fdd\u6301\u7387\uff1b<\/p>\n\n\n\n

(d) \u67d4\u6027\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u793a\u610f\u56fe\uff1b<\/p>\n\n\n\n

(e) \u5355\u4e2a\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u4ee5\u53ca\u4e24\u4e2a\u5e76\u8054\u6216\u4e32\u8054\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u7684\u5149\u5145\u7535\u4e0e\u540e\u7eed\u653e\u7535\u66f2\u7ebf\uff1b<\/p>\n\n\n\n

(f) \u6240\u5236\u5907\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u5728\u4e0d\u540c\u5f2f\u6298\u72b6\u6001\u4e0b\u7684\u7535\u538b\u53d8\u5316\u3002<\/p>\n\n\n\n

\u56fe\u4e94 \u5149\u5145\u950c\u79bb\u5b50\u7535\u6c60\u7684\u5e94\u7528<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

(a) \u7531\u516d\u4e2a\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u4e32\u8054\u548c\u5e76\u8054\u7ec4\u6210\u7684\u6a21\u5757\u793a\u610f\u56fe\uff1b<\/p>\n\n\n\n

(b) \u8be5\u6a21\u5757\u5728\u6674\u5929\u6237\u5916\u5149\u71672 h\u540e\u6240\u8fbe\u5230\u7684\u7535\u538b\uff1b<\/p>\n\n\n\n

(c) \u8be5\u6a21\u5757\u4e0e\u65e0\u4eba\u673a\u96c6\u6210\u540e\u7684\u7167\u7247\uff1b<\/p>\n\n\n\n

(d) \u7531\u4e09\u4e2a\u5149\u5145\u7535\u950c\u79bb\u5b50\u7535\u6c60\u7ec4\u6210\u7684\u6a21\u5757\u793a\u610f\u56fe\uff0c\u4ee5\u53ca\u5176\u4e3a\u5c0f\u8f66 (e) \u548c\u706f\u6ce1 (f) \u4f9b\u7535\u7684\u5e94\u7528\u5c55\u793a\u3002<\/p>\n\n\n\n

\u603b\u7ed3<\/strong><\/strong><\/p>\n\n\n\n

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