{"id":271862,"date":"2026-05-14T08:38:00","date_gmt":"2026-05-14T00:38:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=271862"},"modified":"2026-05-14T22:42:43","modified_gmt":"2026-05-14T14:42:43","slug":"%e4%b8%89%e7%bb%b4%e5%87%a0%e4%bd%95%e9%98%bb%e6%8c%ab%e6%96%b0%e8%bf%9b%e5%b1%95-3d-%e8%bf%87%e6%b8%a1%e9%87%91%e5%b1%9e%e7%83%a7%e7%bb%bf%e7%9f%b3%e7%a3%81%e4%bd%93","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=271862","title":{"rendered":"\u4e09\u7ef4\u51e0\u4f55\u963b\u632b\u65b0\u8fdb\u5c55 | 3d \u8fc7\u6e21\u91d1\u5c5e\u70e7\u7eff\u77f3\u78c1\u4f53"},"content":{"rendered":"\n<p><strong>\u79d1\u7814\u8fdb\u5c55\u5bfc\u8bfb<\/strong><strong><\/strong><\/p>\n\n\n\n<p>\u8fd1\u65e5\uff0c\u5357\u65b9\u79d1\u6280\u5927\u5b66\u90ed\u6292\u8bfe\u9898\u7ec4\uff0c\u8054\u5408\u5357\u65b9\u79d1\u6280\u5927\u5b66\u5434\u7559\u9501\u8bfe\u9898\u7ec4\u548c\u5927\u6e7e\u533a\u5927\u5b66\u76db\u6d01\u660e\u8bfe\u9898\u7ec4\uff0c\u5728\u4e09\u7ef4\u51e0\u4f55\u963b\u632b\u78c1\u6027\u6750\u6599\u7814\u7a76\u9886\u57df\u53d6\u5f97\u91cd\u8981\u8fdb\u5c55\u3002\u7814\u7a76\u56e2\u961f\u57fa\u4e8e\u5316\u5b66\u88c1\u526a\u7b56\u7565\uff0c\u6210\u529f\u8bbe\u8ba1\u5e76\u5408\u6210\u4e86\u4e00\u79cd\u5168\u65b0\u7684\u6beb\u7c73\u7ea7\u9530\u57fa\u70e7\u7eff\u77f3\u53cd\u94c1\u78c1\u4f53\uff0c\u7cfb\u7edf\u63ed\u793a\u4e86\u5176\u8106\u5f31\u7684\u53cd\u94c1\u78c1\u6709\u5e8f\u4e0e\u5f3a\u91cf\u5b50\u81ea\u65cb\u6da8\u843d\u5171\u5b58\u7684\u72ec\u7279\u7269\u7406\u56fe\u50cf\u3002\u76f8\u5173\u7814\u7a76\u6210\u679c\u4ee5\u201cA Mn<sup>2+<\/sup>\u2010Based Pyrochlore Magnet with Fragile Magnetic Order and Strong Spin Fluctuations\u201d\u4e3a\u9898\uff0c\u4e8e2026\u5e743\u67083\u65e5\u5728\u56fd\u9645\u5b66\u672f\u671f\u520aAdvanced Materials\u4e0a\u6b63\u5f0f\u53d1\u8868\u3002<\/p>\n\n\n\n<p><strong>\u5185\u5bb9\u6982\u8ff0<\/strong><\/p>\n\n\n\n<p>\u70e7\u7eff\u77f3\u6676\u683c\u7531\u56db\u9762\u4f53\u4ee5\u5171\u9876\u89d2\u5f62\u5f0f\u6784\u5efa\u6210\u4e09\u7ef4\u7f51\u72b6\u7ed3\u6784\uff0c\u662f\u7814\u7a76\u51e0\u4f55\u963b\u632b\u7684\u7ecf\u5178\u4e09\u7ef4\u6750\u6599\u5e73\u53f0\u3002\u5728\u8be5\u7ed3\u6784\u4e2d\uff0c\u7531\u4e8e\u51e0\u4f55\u9650\u5236\u81ea\u65cb\u4e4b\u95f4\u7684\u53cd\u94c1\u78c1\u76f8\u4e92\u4f5c\u7528\u65e0\u6cd5\u540c\u65f6\u6ee1\u8db3\uff0c\u5f80\u5f80\u5448\u73b0\u51fa\u9ad8\u5ea6\u7b80\u5e76\u7684\u57fa\u6001\uff0c\u8fdb\u800c\u8bf1\u5bfc\u4ea7\u751f\u81ea\u65cb\u51b0\u3001\u91cf\u5b50\u81ea\u65cb\u6db2\u4f53\u7b49\u65b0\u5947\u91cf\u5b50\u6001\u3002\u7136\u800c\uff0c\u5df2\u6709\u7814\u7a76\u4e3b\u8981\u96c6\u4e2d\u5728\u7a00\u571f\u79bb\u5b50\uff084<em>f<\/em>\u7535\u5b50\uff09\u4f53\u7cfb\uff0c\u800c\u8fc7\u6e21\u91d1\u5c5e\uff083<em>d<\/em>\u7535\u5b50\uff09\u70e7\u7eff\u77f3\u6750\u6599\u5374\u975e\u5e38\u7f55\u89c1\u3002\u56e0\u6b64\uff0c\u5982\u4f55\u5728\u4e09\u7ef4\u70e7\u7eff\u77f3\u6676\u683c\u4e2d\u5f15\u5165\u4e0d\u540c\u91cf\u5b50\u81ea\u65cb\u6570\u76843<em>d<\/em>\u8fc7\u6e21\u91d1\u5c5e\u79bb\u5b50\uff0c\u5e76\u5c06\u78c1\u76f8\u4e92\u4f5c\u7528\u6709\u6548\u8c03\u63a7\u5230\u4f4e\u80fd\u5c3a\u5ea6\uff0c\u4e00\u76f4\u662f\u8be5\u9886\u57df\u7684\u91cd\u8981\u6311\u6218\u3002<\/p>\n\n\n\n<ol class=\"wp-block-list\">\n<li><strong>\u5316\u5b66\u88c1\u526a\u8bbe\u8ba1\u601d\u8def\u4e0e\u6676\u4f53\u5408\u6210<\/strong><\/li>\n<\/ol>\n\n\n\n<p>\u7814\u7a76\u56e2\u961f\u4ee5Na<sub>3<\/sub>Mn(CO<sub>3<\/sub>)<sub>2<\/sub>Cl\u4e3a\u7ed3\u6784\u6a21\u7248\uff0c\u63d0\u51fa\u4e86\u6e05\u6670\u7684\u5316\u5b66\u88c1\u526a\u7684\u7ed3\u6784\u8bbe\u8ba1\u601d\u8def\u3002\u9996\u5148\uff0c\u4ee5&nbsp;A<sub>3<\/sub>B(C)<sub>2<\/sub>X \u4e3a\u901a\u5f0f\uff0c\u901a\u8fc7\u8c03\u8282A<sup>+<\/sup>\u4f4d\u9633\u79bb\u5b50\u5c3a\u5bf8\uff0c\u63a7\u5236\u201c\u547c\u5438\u578b\u7acb\u65b9\u9aa8\u67b6\u201d\u7684\u7a7a\u95f4\u5c3a\u5ea6\uff1b\u8fdb\u4e00\u6b65\uff0c\u7528\u4e0d\u540c\u7684\u6865\u952e\u57fa\u56e2\u5982MoO<sub>4<\/sub><sup>2-<\/sup>\u56db\u9762\u4f53\u53d6\u4ee3\u539f\u6709\u7684CO<sub>3<\/sub><sup>2-<\/sup>\u4e09\u89d2\u5e73\u9762\u57fa\u56e2\uff0c\u5728\u4fdd\u6301\u7ed3\u6784\u7a33\u5b9a\u6027\u7684\u540c\u65f6\u62c9\u5927\u78c1\u79bb\u5b50\u95f4\u8ddd\uff1b\u6700\u540e\uff0c\u7528\u8d1f\u7535\u8377\u7684\u5364\u7d20\u79bb\u5b50&nbsp;Cl\u207b \u4f5c\u4e3a\u7535\u8377\u5e73\u8861\u8c03\u8282\u5242\uff0c\u4ece\u800c\u5b9e\u73b0\u6676\u4f53\u7ed3\u6784\u7684\u7535\u4e2d\u6027\u548c\u7ed3\u6784\u7a33\u5b9a\u6027\u3002\u5728\u6837\u54c1\u5408\u6210\u4e0a\uff0c\u901a\u8fc7\u9ad8\u6e29\u81ea\u52a9\u7194\u5242\u6cd5\u6210\u529f\u5408\u6210\u65b0\u578b\u9530\u57fa\u70e7\u7eff\u77f3\u53cd\u94c1\u78c1\u4f53\u3002\u57fa\u4e8e\u5355\u6676XRD\u5b9e\u9a8c\uff0c\u786e\u5b9a\u8be5\u6750\u6599\u5316\u5b66\u5f0f\u8fd1\u4f3c\u4e3aK<sub>3<\/sub>Mn(MoO<sub>4<\/sub>)<sub>2<\/sub>Cl\uff0c\u7ed3\u6676\u4e8e\u7acb\u65b9\u6676\u7cfb<em>Fd<\/em>-3\u7a7a\u95f4\u7fa4\uff0c\u4e8c\u4ef7Mn\u79bb\u5b50\u6784\u7b51\u7406\u60f3\u4e09\u7ef4\u70e7\u7eff\u77f3\u6676\u683c\uff0c\u6700\u8fd1\u90bbMn\u2013Mn\u8ddd\u79bb\u8fbe\u52305.78&nbsp;\u00c5\uff0c\u663e\u8457\u5927\u4e8e\u4f20\u7edf\u70e7\u7eff\u77f3\u4f53\u7cfb\uff0c\u4ece\u7ed3\u6784\u5c42\u9762\u524a\u5f31\u4e86\u78c1\u4ea4\u6362\u4f5c\u7528\u3002\u540c\u65f6\uff0c\u6beb\u7c73\u7ea7\u5355\u6676\u6837\u54c1\u7684\u5236\u5907\uff0c\u4e3a\u540e\u7eed\u5fae\u89c2\u7269\u7406\u673a\u5236\u7814\u7a76\u63d0\u4f9b\u4e86\u575a\u5b9e\u6750\u6599\u57fa\u7840\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"600\" height=\"526\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2026\/05\/2382c315a6ba396-14.png\" alt=\"\" class=\"wp-image-271864\"\/><\/figure>\n\n\n\n<p><strong>\u56fe<\/strong><strong>1.<\/strong>&nbsp;\u5316\u5b66\u88c1\u526a\u601d\u8def\u548c\u6676\u4f53\u7ed3\u6784<\/p>\n\n\n\n<ul class=\"wp-block-list\">\n<li><strong>\u5f3a<\/strong><strong>\u78c1<\/strong><strong>\u963b\u632b<\/strong><strong>\u4e0e\u8106\u5f31<\/strong><strong>\u6709\u5e8f<\/strong><strong>\u6001<\/strong><\/li>\n<\/ul>\n\n\n\n<p>\u8be5\u6750\u6599\u7684\u78c1\u5316\u7387\u5728\u9ad8\u6e29\u533a\u4e25\u683c\u9075\u5faa\u5c45\u91cc\u2013\u5916\u65af\u884c\u4e3a\uff0cWeiss \u6e29\u5ea6 \u0398 \u2248 \u221219.2 K\uff0c\u8868\u660e\u663e\u8457\u53cd\u94c1\u78c1\u76f8\u4e92\u4f5c\u7528\u3002\u7ed3\u5408 Mn<sup>2+<\/sup>\uff08<em>S<\/em>&nbsp;= 5\/2\uff09\u7279\u6027\uff0c\u4f30\u7b97\u6700\u8fd1\u90bb\u4ea4\u6362\u5e38\u6570 J \u2248 1.1 K\u3002\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u957f\u7a0b\u6709\u5e8f\u4ec5\u5728\u6781\u4f4e\u6e29 <em>T<\/em><sub>N<\/sub>&nbsp;\u2248 0.26 K \u624d\u51fa\u73b0\uff0c\u963b\u632b\u56e0\u5b50 <em>f<\/em>&nbsp;&gt; 80\uff0c\u8868\u660e\u4f53\u7cfb\u5904\u4e8e\u9ad8\u5ea6\u78c1\u963b\u632b\u72b6\u6001\u3002\u6cbf [111] \u65b9\u5411\u78c1\u5316\u66f2\u7ebf\u5728 ~6.8 T \u51fa\u73b0\u8fd1\u534a\u9971\u548c\u7279\u5f81\uff08<em>M<\/em>&nbsp;\u2248 0.5 <em>M<\/em><sub>sat<\/sub>\uff09\u3002\u4e0d\u540c\u4e8e\u7ecf\u5178\u5206\u6570\u91cf\u5b50\u5316\u5e73\u53f0\uff0c\u8be5\u884c\u4e3a\u66f4\u53ef\u80fd\u5bf9\u5e94\u77ed\u7a0b\u5173\u8054\u589e\u5f3a\u6216\u4ea4\u53c9\u533a\u884c\u4e3a\uff0c\u51f8\u663e\u5176\u590d\u6742\u81ea\u65cb\u5173\u8054\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"800\" height=\"415\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2026\/05\/ce6e2814f207c93-13.png\" alt=\"\" class=\"wp-image-271865\"\/><\/figure>\n\n\n\n<p><strong>\u56fe<\/strong><strong>2.<\/strong>&nbsp;\u57fa\u672c\u78c1\u5316\u884c\u4e3a<\/p>\n\n\n\n<ul class=\"wp-block-list\">\n<li><strong>\u78c1\u5173\u8054\u6a21\u578b\u4e0e\u78c1\u76f8\u53d8<\/strong><\/li>\n<\/ul>\n\n\n\n<p>\u96f6\u78c1\u573a\u4e0b\u7684\u6bd4\u70ed\u6d4b\u91cf\u4e3a\u63ed\u793aK<sub>3<\/sub>Mn(MoO<sub>4<\/sub>)<sub>2<\/sub>Cl\u7684\u5173\u952e\u7269\u7406\u56fe\u50cf\u3002\u78c1\u6bd4\u70ed\u7ed3\u679c\u663e\u793a\uff0c\u57283\u201310&nbsp;K \u6e29\u533a\u5185\uff0c\u968f\u964d\u6e29\u9010\u6e10\u4e0a\u5347\u5e76\u5f62\u6210\u4e00\u4e2a\u5bbd\u5cf0\uff0c\u8868\u660e\u9ad8\u6e29\u5df2\u5efa\u7acb\u663e\u8457\u77ed\u7a0b\u5173\u8054\u3002\u8be5\u6e29\u533a\u5185\u7684\u5b9e\u9a8c\u7ed3\u679c\u4e0e\u70e7\u7eff\u77f3\u6676\u683c\u4e0a<em>S<\/em>&nbsp;= 5\/2\u6d77\u68ee\u5821\u6a21\u578b\u7684\u9ad8\u6e29\u7ea7\u6570\u5c55\u5f00\u8ba1\u7b97\u7ed3\u679c\u9ad8\u5ea6\u4e00\u81f4\uff0c\u5bf9\u5e94\u6700\u8fd1\u90bb\u4ea4\u6362\u4f5c\u7528\u80fd\u6807\u7ea6\u4e3a<em>J<\/em>&nbsp;\u2248&nbsp;1.1 K\u3002\u540c\u65f6\u78c1\u6bd4\u70ed\u5728\u7ea6 2.4 K \u9644\u8fd1\u51fa\u73b0\u660e\u663e\u7684\u5bbd\u7f13\u5cf0\u7ed3\u6784\uff0c\u6e05\u695a\u6307\u793a\u5f3a\u51e0\u4f55\u963b\u632b\u80cc\u666f\u4e0b\u77ed\u7a0b\u78c1\u5173\u8054\u7684\u6301\u7eed\u589e\u5f3a\u3002\u76f4\u81f3\u6781\u4f4e\u6e29 <em>T<\/em><sub>N<\/sub>&nbsp;\u2248 0.26 K \u624d\u51fa\u73b0\u6e05\u6670\u03bb\u578b\u78c1\u8f6c\u3002\u78c1\u71b5\u5206\u6790\u663e\u793a\uff0c\u5728\u8fd9\u4e00\u78c1\u76f8\u53d8\u6e29\u5ea6\u5904\u4ec5\u91ca\u653e\u4e86\u7ea6 11-15% \u7684 Rln(6) \u7406\u8bba\u78c1\u71b5\uff0c\u8bf4\u660e\u8fdb\u5165\u6709\u5e8f\u76f8\u540e\u4ecd\u4fdd\u7559\u5927\u91cf\u81ea\u65cb\u6da8\u843d\u4e0e\u7b80\u5e76\u81ea\u7531\u5ea6\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"800\" height=\"236\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2026\/05\/7f88dbbcaa77a1d-12.png\" alt=\"\" class=\"wp-image-271866\"\/><\/figure>\n\n\n\n<p><strong>\u56fe<\/strong><strong>3. <\/strong>\u96f6\u573a\u6bd4\u70ed\u884c\u4e3a<\/p>\n\n\n\n<ul class=\"wp-block-list\">\n<li><strong>\u78c1\u573a\u8bf1\u5bfc\u7684\u81ea\u65cb\u65e0\u5e8f\u6001<\/strong><\/li>\n<\/ul>\n\n\n\n<p>\u8be5\u53cd\u94c1\u78c1\u957f\u7a0b\u5e8f\u5bf9\u5916\u754c\u6270\u52a8\u6781\u5176\u654f\u611f\uff0c\u4ec5\u7ea60.4 T&nbsp;\u78c1\u573a\u5373\u53ef\u8fc5\u901f\u538b\u5236\u8be5\u78c1\u6709\u5e8f\uff0c\u8868\u660e\u8be5\u6709\u5e8f\u6001\u6781\u5176\u201c\u8106\u5f31\u201d\u3002\u8be5\u957f\u7a0b\u5e8f\u6d88\u5931\u540e\uff0c\u4f53\u7cfb\u8fdb\u5165\u4e86\u78c1\u573a\u8bf1\u5bfc\u7684\u65b0\u5947\u81ea\u65cb\u65e0\u5e8f\u6001\uff0c\u800c\u975e\u7b80\u5355\u81ea\u65cb\u6781\u5316\u6001\u3002\u8be5\u65e0\u5e8f\u6001\u662f\u5426\u4e3a\u91cf\u5b50\u81ea\u65cb\u6db2\u4f53\uff0c\u4ecd\u9700\u901a\u8fc7\u975e\u5f39\u6027\u4e2d\u5b50\u6563\u5c04\u7b49\u5b9e\u9a8c\u8fdb\u4e00\u6b65\u9a8c\u8bc1\u3002<\/p>\n\n\n\n<figure class=\"wp-block-image size-full\"><img loading=\"lazy\" decoding=\"async\" width=\"800\" height=\"229\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2026\/05\/4e9a0ba2491dfde-12.png\" alt=\"\" class=\"wp-image-271867\"\/><\/figure>\n\n\n\n<p><strong>\u56fe<\/strong><strong>4.<\/strong>&nbsp;\u6cbf\u7740[111]\u65b9\u5411\u7684\u5f31\u78c1\u573a\u6bd4\u70ed\u884c\u4e3a<\/p>\n\n\n\n<ul 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