{"id":272727,"date":"2026-08-06T09:01:00","date_gmt":"2026-08-06T01:01:00","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=272727"},"modified":"2026-08-05T23:18:17","modified_gmt":"2026-08-05T15:18:17","slug":"%e8%a5%bf%e5%ae%89%e5%bb%ba%e5%a4%a7%e4%ba%91%e6%96%af%e5%ae%81%e6%95%99%e6%8e%88journal-of-materials-chemistry-a%ef%bc%9a-%e5%b7%a7%e5%80%9f%e7%94%b5%e8%b4%9f%e6%80%a7%e6%a2%af%e5%ba%a6%e6%9e%84","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=272727","title":{"rendered":"\u897f\u5b89\u5efa\u5927\u4e91\u65af\u5b81\u6559\u6388Journal of Materials Chemistry A\uff1a \u5de7\u501f\u7535\u8d1f\u6027\u68af\u5ea6\u6784\u7b51\u5185\u5efa\u7535\u573a\u7684\u9ad8\u71b5\u5408\u91d1\u951a\u5b9a\u516b\u9762\u4f53\u6c2e\u63ba\u6742\u78b3\uff1a\u534f\u540c\u754c\u9762\u52a0\u901f\u6790\u6c22\u53ca\u4e09\u7898\u5316\u7269\/\u94dc\u8fd8\u539f\u53cd\u5e94"},"content":{"rendered":"\n
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\"\"<\/figure>\n\n\n\n

\u56fe3. (a) HEA-NC\u7684XPS\u626b\u63cf\u8c31\u3002MEA-NC\u548cHEA-NC\u4e2d(b)Fe\u3001(c) Cr\u3001(d) Cu\u548c(e) Co\u5143\u7d20\u7684\u7cbe\u7ec6\u8c31\u3002(f) HEA-NC\u4e2dMn\u5143\u7d20\u7684\u7cbe\u7ec6\u8c31\u3002<\/p>\n\n\n\n

\u8981\u70b9\u4e09\uff1a<\/strong>\u9ad8\u6548\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\u6027\u80fd\u53ca\u7a33\u5b9a\u6027<\/strong><\/strong><\/p>\n\n\n\n

\u5c06HEA-NC\u7528\u4e8e\u78b1\u6027\u7535\u89e3\u6c34\u6790\u6c22\u53cd\u5e94\uff08\u56fe4\uff09\u3002\u7535\u5316\u5b66\u6d4b\u8bd5\u8868\u660e\uff0c\u5f97\u76ca\u4e8eHEA\u5185\u90e8”Mn\u2192Cu\/Co”\u5b9a\u5411\u7535\u8377\u8f6c\u79fb\uff0c\u9ad8\u71b5HEA-NC\u6709\u6548\u964d\u4f4e\u4e86HER\u53cd\u5e94\u80fd\u5792\uff0c\u52a0\u5feb\u4e86\u7535\u5b50\u8f6c\u79fb\u8fc7\u7a0b\u3002\u572810 mA cm\u207b\u00b2\u4e0b\u8fc7\u7535\u4f4d\u4ec599 mV\uff0c\u4f4e\u4e8e\u4e2d\u71b5MEA-NC\uff08120 mV\uff09\u3001Cu-NC\uff08146 mV\uff09\u548cNF\uff08224 mV\uff09\uff1b\u9ad8\u71b5HEA-NC\u7684Tafel\u659c\u7387\u4e3a64 mV dec\u207b\u00b9\uff0c\u4f4e\u4e8e\u4e2d\u71b5MEA-NC\uff08102 mV dec\u207b\u00b9\uff09\u548cCu-NC\uff08138 mV dec\u207b\u00b9\uff09\uff0c\u8868\u660e\u5176\u9075\u5faa\u9ad8\u6548\u7684Volmer-Heyrovsky\u673a\u5236\uff08\u56fe4a-b\uff09\u3002\u7535\u5316\u5b66\u963b\u6297\u5206\u6790\u8fdb\u4e00\u6b65\u8bc1\u5b9e\uff0cHEA-NC\u7684\u7535\u8377\u8f6c\u79fb\u7535\u963b\uff08Rct<\/sub>=5.32 \u03a9 cm2<\/sup>\uff09\u663e\u8457\u4f4e\u4e8e\u5bf9\u6bd4\u7ec4\uff08\u56fe4c\uff09\uff0c\u5f52\u56e0\u4e8e\u5185\u5efa\u7535\u573a\u4e3aHeyrovsky\u6b65\u9aa4\u4e2d\u7535\u5b50\u8f6c\u79fb\u63d0\u4f9b\u4e86\u5feb\u901f\u901a\u9053\u3002\u7535\u5316\u5b66\u6d3b\u6027\u9762\u79ef\u6d4b\u8bd5\u8868\u660eHEA-NC\u5177\u6709\u6700\u5927\u7684Cdl\uff084.61 mF cm\u207b\u00b2\uff09\u548cECSA\uff08115.25 cm\u00b2\uff09\uff08\u56fe4d-e\uff09\uff0c\u516b\u9762\u4f53\u4e09\u7ef4\u7ed3\u6784\u63d0\u4f9b\u4e86\u9ad8\u6bd4\u8868\u9762\u79ef\u548c\u4e30\u5bcc\u7684\u591a\u91d1\u5c5e\u6d3b\u6027\u4f4d\u70b9\u3002\u7a33\u5b9a\u6027\u6d4b\u8bd5\u8868\u660e\uff08\u56fe4f-g\uff09\uff0c\u7ecf1000\u5708CV\u5faa\u73af\u540eLSV\u66f2\u7ebf\u51e0\u4e4e\u91cd\u5408\uff0c30 h\u6052\u7535\u6d41\u6d4b\u8bd5\u540e\u8fc7\u7535\u4f4d\u4fdd\u6301\u7387\u8fbe96.4%\uff0c\u9ad8\u6784\u578b\u71b5\u8d4b\u4e88\u7684\u50ac\u5316\u5242\u7684\u7ed3\u6784\u7a33\u5b9a\u6027\u548cCr\u5143\u7d20\u7684\u8010\u8150\u8680\u6027\uff0c\u5171\u540c\u4fdd\u969c\u4e86\u5176\u957f\u671f\u8010\u4e45\u6027\u3002\u4e0a\u8ff0\u7ed3\u679c\u8868\u660e\uff0c\u9ad8\u71b5\u5408\u91d1HEA\u4e2d\u7684\u5b9a\u5411\u7535\u8377\u8f6c\u79fb\u80fd\u591f\u6709\u6548\u4fc3\u8fdbHER\u8fc7\u7a0b\u4e2d\u7684\u7535\u8377\u4f20\u8f93\u4e0e\u53cd\u5e94\u52a8\u529b\u5b66\uff0c\u4f7fHEA-NC\u5728\u78b1\u6027HER\u4e2d\u5c55\u73b0\u51fa\u4f18\u4e8e\u591a\u6570\u5df2\u62a5\u9053\u975e\u8d35\u91d1\u5c5e\u50ac\u5316\u5242\u7684\u6790\u6c22\u6027\u80fd\uff08\u56fe4h\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe4. (a) \u50ac\u5316\u5242\u7684LSV\u66f2\u7ebf\uff0c(b) Tafel\u6781\u5316\u66f2\u7ebf\uff0c(c) Nyquist\u56fe<\/a>\uff0c(d) Cdl\u503c\u3002(e) \u50ac\u5316\u5242\u7684ECSA\u503c\u3002(f) \u50ac\u5316\u5242\u57281000\u6b21CV\u5faa\u73af\u524d\u540e\u7684LSV\u66f2\u7ebf\u548c(g)\u6052\u7535\u4f4d\u65f6\u95f4\u66f2\u7ebf\u3002(h)\u672c\u7814\u7a76\u4e2d\u7684\u50ac\u5316\u5242 HEA-NC\u4e0e\u5df2\u6709\u50ac\u5316\u5242\u7684\u6790\u6c22\u6027\u80fd\u6bd4\u8f83\u3002<\/p>\n\n\n\n

\u8981\u70b9\u56db\uff1a<\/strong>\u8d85\u8d8aPt\u5bf9\u7535\u6781\u7684<\/strong>\u592a\u9633\u80fd<\/strong>\u5149\u4f0f\u6027\u80fd\u53ca\u7a33\u5b9a\u6027\uff08IRR\/CRR\uff09<\/strong><\/strong><\/p>\n\n\n\n

\u5c06HEA-NC\u7528\u4f5c\u592a\u9633\u80fd\u7535\u6c60\u5bf9\u7535\u6781\uff0c\u8003\u5bdf\u5176\u5728IRR\u548cCRR\u8fc7\u7a0b\u4e2d\u7684\u50ac\u5316\u6027\u80fd\uff08\u56fe5\uff09\u3002\u5faa\u73af\u4f0f\u5b89\u6d4b\u8bd5\u8868\u660e\uff0cHEA-NC\u5177\u6709\u66f4\u9ad8\u7684\u6c27\u5316-\u8fd8\u539f\u5cf0\u7535\u6d41\u5bc6\u5ea6\uff08-2.51 mA cm\u207b\u00b2\uff09\u548c\u66f4\u5c0f\u7684\u5cf0\u7535\u4f4d\u5206\u79bb\uff080.41 V\uff09\uff0c\u4f18\u4e8eMEA-NC\u548cCu-NC\uff08\u56fe5a<\/a>-c\uff09\uff0c\u8868\u660e\u5176\u80fd\u591f\u6709\u6548\u4fc3\u8fdbI\u2083\u207b\/I\u207b\u6c27\u5316\u8fd8\u539f\u53cd\u5e94\u52a8\u529b\u5b66\u3002\u5728\u7898\u7535\u5bf9\u4f53\u7cfb\uff08<\/a>\u56fe5d-f\uff09\u548c\u94dc\u7535\u5bf9\u4f53\u7cfb\uff08\u56fe5g-i\uff09\u4e2d\uff0c\u7535\u5316\u5b66\u963b\u6297\u8c31\u548c\u5854\u83f2\u5c14\u66f2\u7ebf\u5206\u6790\u8fdb\u4e00\u6b65\u8bc1\u660e\uff0cHEA\u8868\u9762\u5bcc\u7535\u5b50\u533a\u57df\u964d\u4f4e\u4e86I\u2083\u207b\u8fd8\u539f\u7684\u6d3b\u5316\u80fd\u5792\uff0c\u800cHEA\u5185\u90e8\u591a\u91d1\u5c5e\u6d3b\u6027\u4f4d\u70b9\u4e0eHEA\u2192NC\u754c\u9762\u5185\u5efa\u7535\u573a\u7684\u534f\u540c\u4f5c\u7528\u964d\u4f4e\u4e86\u754c\u9762\u7535\u8377\u4f20\u8f93\u963b\u529b\uff0c\u52a0\u5feb\u4e86\u7535\u5b50\u8f6c\u79fb\u8fc7\u7a0b\uff08\u56fe5d-e\uff09\u3002HEA-NC\u8868\u73b0\u51fa\u4f18\u5f02\u7684\u7535\u50ac\u5316\u6d3b\u6027\uff0c\u5728IRR\u548cCRR\u4e2d\u5206\u522b\u5b9e\u73b0\u4e868.52%\u548c5.82%\u7684\u5149\u7535\u8f6c\u6362\u6548\u7387\uff08\u56fe5f\uff0ci\uff09\uff0c\u9ad8\u4e8ePt\u5bf9\u7535\u6781\uff087.34%\u548c4.53%\uff09\u4ee5\u53ca\u5927\u591a\u6570\u5df2\u62a5\u9053\u7684\u540c\u7c7b\u50ac\u5316\u6750\u6599\uff08\u56fe5j\uff09\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe5. (a) \u56db\u79cd\u50ac\u5316\u5242\u7684\u5faa\u73af\u4f0f\u5b89\u66f2\u7ebf\u3002(b) \u4e0d\u540c\u626b\u63cf\u901f\u7387\u4e0b\u7684HEA-NC\u7684\u5faa\u73af\u4f0f\u5b89\u66f2\u7ebf\u3002(c) Ip<\/sub>\u4e0e\u626b\u63cf\u901f\u7387\u5e73\u65b9\u6839\u4e4b\u95f4\u7684\u7ebf\u6027\u5173\u7cfb\u3002(d-e) \u50ac\u5316\u5242<\/a>\u5728 I3<\/sub>\u2212<\/sup>\/I\u2212<\/sup>\u4f53\u7cfb\u4e2d\u7684Nyquist\u56fe\u548cTafel\u6781\u5316\u66f2\u7ebf\u3002(f) \u50ac\u5316\u5242\u5728N719-I<\/a>3<\/sub>\u2212<\/sup>\/I\u2212<\/sup>\u4f53\u7cfb\u4e2d<\/a>\u7684J\u2013V\u66f2\u7ebf\u3002(g-h) \u50ac\u5316\u5242<\/a>\u5728<\/a>Cu2+<\/sup>\/Cu+<\/sup>\u4f53\u7cfb\u4e2d\u7684Nyquist\u56fe\u548cTafel\u6781\u5316\u66f2\u7ebf\u3002(i) \u50ac\u5316\u5242\u5728D35-Cu2+<\/sup>\/Cu+<\/sup>\u4f53\u7cfb\u4e2d\u7684J\u2013V\u66f2\u7ebf\u3002(h) \u4e0d\u540c\u50ac\u5316\u5242\u5728I3<\/sub>\u2212<\/sup>\/I\u2212<\/sup>\u4f53\u7cfb\u548c\u5728Cu2+<\/sup>\/Cu+<\/sup>\u4f53\u7cfb\u4e2d\u7684\u592a\u9633\u80fd\u5149\u7535\u8f6c\u6362\u6548\u7387PCE\u6bd4\u8f83\u3002<\/p>\n\n\n\n

\u8fdb\u4e00\u6b65\u7684\u7a33\u5b9a\u6027\u6d4b\u8bd5\u8868\u660e\uff08\u56fe6\uff09\uff0cHEA-NC\u5bf9\u7535\u6781\u572850\u5708\u8fde\u7eedCV\u626b\u63cf\u540e\u66f2\u7ebf\u9ad8\u5ea6\u91cd\u5408\uff0c\u5149\u5f00\u5173\u5faa\u73af\u6d4b\u8bd5\u540e\u5149\u7535\u6d41\u4fdd\u6301\u7387\u8fbe97.2%\uff0c\u9ad8\u71b5\u5408\u91d1\u7684\u70ed\u529b\u5b66\u7a33\u5b9a\u6027\u548cCr\u8bf1\u5bfc\u7684\u8010\u8150\u8680\u6027\u4f7f\u5176\u5728\u8150\u8680\u6027\u7898\u7535\u89e3\u6db2\u4e2d\u5c55\u73b0\u51fa\u663e\u8457\u4f18\u4e8ePt\u57fa\u7535\u6781\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u548c\u6301\u7eed\u5149\u7535\u54cd\u5e94\u80fd\u529b\u3002\u4e0a\u8ff0\u7ed3\u679c\u8868\u660e\uff0c\u7535\u8d1f\u6027\u68af\u5ea6\u9a71\u52a8\u7684\u5185\u5efa\u7535\u573a\u4e0e\u53cc\u7535\u5b50\u901a\u8def\u80fd\u591f\u6709\u6548\u63d0\u5347\u7535\u5b50\u4f20\u8f93\u548c\u53cd\u5e94\u52a8\u529b\u5b66\uff0c\u4f7fHEA-NC\u5728IRR\u548cCRR\u4e2d\u5c55\u73b0\u51fa\u4f18\u5f02\u7684\u50ac\u5316\u6027\u80fd\uff0c\u5c55\u73b0\u51fa\u5176\u5728\u65b0\u578b\u592a\u9633\u80fd\u7535\u6c60\u4e2d\u7684\u5e94\u7528\u6f5c\u529b\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe6. (a) HEA-NC\u3001(b) MEA-NC\u548c(c) Cu-NC \u768450\u6b21\u5faa\u73afCV\u66f2\u7ebf\u3002(d-f) \u50ac\u5316\u5242\u7684\u6c27\u5316-\u8fd8\u539f\u5cf0\u7535\u6d41\u5bc6\u5ea6\u3002(g) \u5149\u7535\u54cd\u5e94\u6d4b\u8bd5\u53ca(h) \u50ac\u5316\u5242\u7684\u7535\u6d41\u5bc6\u5ea6\u8010\u4e45\u6027\u5bf9\u6bd4\u3002<\/p>\n\n\n\n

\u8981\u70b9\u4e94\uff1a<\/strong>\u5185\u5efa\u7535\u573a\u4e0e\u53cc\u7535\u5b50\u901a\u8def\u534f\u540c\u673a\u7406<\/strong><\/strong><\/p>\n\n\n\n

DFT\u8ba1\u7b97\u63ed\u793a\u4e86HEA\u5185\u90e8\u7535\u5b50\u5206\u5e03\uff08\u56fe7a-b\uff09\u3002Mn\u539f\u5b50\u5468\u56f4\u7535\u5b50\u5bc6\u5ea6\u964d\u4f4e\uff08\u4f9b\u4f53\uff09\uff0cFe\/Cr\/Co\/Cu\u5468\u56f4\u589e\u52a0\uff08\u53d7\u4f53\uff09\uff0c\u9a8c\u8bc1\u4e86\u201cMn\u2192Cu\/Co\u201d\u7535\u8377\u8f6c\u79fb\uff08\u56fe7c\uff09<\/a>\u3002HEA-NC\u754c\u9762\u7535\u8377\u5bc6\u5ea6\u5dee\u663e\u793a\u7535\u5b50\u4eceHEA\u5411NC\u8f7d\u4f53\u51c0\u8fc1\u79fb\uff0cNC\u4fa7\u5bcc\u7535\u5b50\uff0cHEA\u4fa7\u7f3a\u7535\u5b50\uff0c\u5f62\u6210\u5185\u5efa\u7535\u573a\uff08\u56fe7d\uff09\u3002\u7ed3\u5408UPS\/XPS\u8bc1\u5b9e\uff0c\u786e\u7acb\u4e86\u53cc\u7535\u5b50\u901a\u8def\uff1a\u2460\u5408\u91d1\u5185\u7535\u8d1f\u6027\u68af\u5ea6\u9a71\u52a8\u5b9a\u5411\u7535\u8377\u8f6c\u79fb\uff0c\u4f18\u5316\u6d3b\u6027\u4f4d\u70b9\u7535\u5b50\u7ed3\u6784\uff1b\u2461\u754c\u9762\u5904\u7535\u5b50\u6301\u7eed\u8fc1\u79fb\u81f3NC\u8f7d\u4f53\uff0c\u964d\u4f4e\u6574\u4f53\u529f\u51fd\u6570\uff0c\u4e3aHeyrovsky\u6b65\u9aa4\u548cIRR\u521d\u59cb\u7535\u5b50\u8f6c\u79fb\u63d0\u4f9b\u5feb\u901f\u901a\u9053\uff08\u56fe7e-g\uff09\u3002\u8be5\u534f\u540c\u673a\u5236\u52a0\u901f\u4e86HER\u548cIRR\/CRR\u7684\u53cd\u5e94\u52a8\u529b\u5b66\uff0c\u662fHEA-NC\u4f18\u5f02\u7efc\u5408\u6027\u80fd\u7684\u5fae\u89c2\u6839\u6e90\u3002<\/p>\n\n\n\n

\"\"<\/figure>\n\n\n\n

\u56fe7. (a) Cu-NC\u3001MEA-NC\u548cHEA-NC\u7684\u529f\u51fd\u6570\u3002(b) MEA-NC\u4e0eHEA-NC\u4e2d\u5404\u5143\u7d20\u7ed3\u5408\u80fd\u7684\u6bd4\u8f83\u3002(c) MEA\u548cHEA\u4e2d\u7684\u7535\u5b50\u5bc6\u5ea6\u5206\u5e03\u3002(d) HEA-NC\u754c\u9762\u5904\u5dee\u5206\u7535\u8377\u5bc6\u5ea6\uff08CDD\uff09\u56fe\u3002(e) \u7535\u5b50\u4f20\u8f93\u8def\u5f84\u793a\u610f\u56fe\u3002(f) HEA-NC\u5728\u6790\u6c22\u53cd\u5e94HER\u4e2d\u7684\u793a\u610f\u56fe\u3002(g) HEA-NC\u5728<\/a>IRR\u50ac\u5316\u4e2d\u7684\u793a\u610f\u56fe<\/a>\u3002<\/p>\n\n\n\n

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\u3010\u6587\u7ae0\u94fe\u63a5\u3011<\/strong><\/strong><\/p>\n\n\n\n

<\/a>Internal Electric Field Engineered High-Entropy Alloy on Octahedral N-Doped Carbon via Electronegativity Gradient: Synergistic Interfaces Accelerating Hydrogen Evolution and Triiodide\/Copper Reduction Reactions<\/p>\n\n\n\n

<\/a>Juntao Wang, Sining Yun,* Tianxiang Yang, Leifei Wang, Yang Yang, Zhiguo Wang, Haijiang Yang, Rou Feng, Ting Lu and Zechang Liu<\/p>\n\n\n\n

https:\/\/doi.org\/10.1039\/d6ta02832b<\/a><\/p>\n\n\n\n

\u3010\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\u3011<\/strong><\/strong><\/p>\n\n\n\n

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https:\/\/xajzkj.teacher.360eol.com\/teacherBasic\/preview?teacherId=21532<\/a><\/p>\n\n\n\n

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