{"id":29464,"date":"2016-07-29T08:00:20","date_gmt":"2016-07-29T00:00:20","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=29464"},"modified":"2016-07-28T14:22:16","modified_gmt":"2016-07-28T06:22:16","slug":"%e9%a1%b6%e5%88%8a%e5%8a%a8%e6%80%81-nature%e5%ad%90%e5%88%8ajacsangew%e7%ad%89%e8%bf%91%e6%9c%9fmof%e6%9d%90%e6%96%99%e7%a0%94%e7%a9%b6%e8%bf%9b%e5%b1%95%e6%b1%87%e6%80%bb%e3%80%90mof%e6%9d%90","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=29464","title":{"rendered":"\u9876\u520a\u52a8\u6001 | Nature\u5b50\u520a\/JACS\/Angew\u7b49\u8fd1\u671fMOF\u6750\u6599\u7814\u7a76\u8fdb\u5c55\u6c47\u603b\u3010MOF\u6750\u6599\u7b2c6\u671f\u3011"},"content":{"rendered":"

1\u3001Angew | \u4e2d\u5c71\u5927\u5b66\u901a\u8fc7\u53ef\u9006\u540e\u5408\u6210\u53ef\u53d8\u9694\u5c42\u7ec4\u88c5\u6539\u826f\u6269\u5f20\u5ea6\u548c\u5438\u9644\u6027<\/strong><\/p>\n

\u91d1\u5c5e-\u6709\u673a\u6846\u67b6(MOFs)\u5316\u5408\u7269\uff0c\u6216\u79f0\u4f5c\u591a\u5b54\u914d\u4f4d\u805a\u5408\u7269(PCPs)\uff0c\u662f\u7531\u91d1\u5c5e\u79bb\u5b50\u548c\u6709\u673a\u914d\u4f53\u901a\u8fc7\u8f83\u5f3a\u7684\u914d\u4f4d\u4f5c\u7528\u7ec4\u88c5\u5f62\u6210\u7684\u4e00\u7c7b\u6676\u4f53\u6750\u6599\u3002MOFs\u7684\u540e\u5408\u6210\u4fee\u9970\u4e3a\u5f15\u5165\u65b0\u5b98\u80fd\u56e2\u63d0\u4f9b\u6709\u529b\u65b9\u5f0f\uff0c\u540c\u65f6\u4e5f\u89e3\u51b3\u4e86\u90e8\u5206MOF\u6309\u5e38\u89c4\u65b9\u6cd5\u65e0\u6cd5\u5efa\u6784\u7684\u96be\u9898\u3002\u800c\u5728\u539f\u6709MOFs\u6846\u67b6\u57fa\u7840\u4e0a\u5f15\u5165\u7b2c\u4e8c\u79cd\u914d\u4f53\u7684\u4fee\u9970\u65b9\u6cd5\u76ee\u524d\u4ecd\u7136\u5c11\u89c1\u3002<\/p>\n

\u4e2d\u5c71\u5927\u5b66\u82cf\u6210\u52c7\u8bfe\u9898\u7ec4\u62a5\u9053\u4e86\u57fa\u4e8e\u7a33\u5b9a\u800c\u7075\u6d3b\u7684Zr6-MOF\u7684\u4e00\u79cd\u540e\u5408\u6210\u53ef\u53d8\u9694\u5c42\u7ec4\u88c5\u7b56\u7565\uff08PVSI\uff09\uff0c\u5373\u7528\u4e0d\u540c\u957f\u5ea6\u548c\u5b98\u80fd\u56e2\u7684\u7ebf\u6027\u9694\u5c42\u914d\u4f53\u9009\u62e9\u6027\u5730\u7cbe\u786e\u66ff\u6362Zr6\u7c07\u4e0a\u672b\u7aef\u6c34\u5206\u5b50\u3002\u5e76\u4e14\u8be5\u8fc7\u7a0b\u662f\u6c34\u6eb6\u6db2\u9a71\u52a8\u7684\u4ece\u5c0f\u5b54\u5230\u5927\u5b54\u7684\u5355\u6676\u5230\u5355\u6676\uff08SC-SC)\u7684\u7ed3\u6784\u8f6c\u53d8\uff0c\u4e14\u5728\u6e29\u548c\u6761\u4ef6\u4e0b\u8868\u73b0\u4e3a\u52a8\u529b\u5b66\u53ef\u9006\u3002<\/p>\n

\"\u56fe\u72471\"
\n\u56fe1<\/strong> PVSI\u6d41\u7a0b\u56fe\u53ca\u9694\u5c42\u914d\u4f53 L2\u2013L6\u7684\u7ec4\u88c5\u53ca\u5378\u8f7d<\/p>\n

\u540e\u5408\u6210\u53ef\u53d8\u9694\u5c42\u7ec4\u88c5\u7b56\u7565\uff08PVSI\uff09\u6d89\u53ca\u5230\u4e86SC-SC\u7684\u7ed3\u6784\u8f6c\u53d8\u3002\u76f8\u6bd4\u4e8e\u4f20\u7edf\u7684MOFs\u7684\u540e\u5408\u6210\u4fee\u9970\u548c\u76f4\u63a5\u5408\u6210\uff0c\u8fd9\u79cd\u5bf9\u9694\u5c42\u914d\u4f53\u7684\u53ef\u9006\u6027\u7ec4\u88c5\u53ef\u5378\u8f7d\u4e0d\u4ec5\u53ef\u4ee5\u7cbe\u786e\u8c03\u63a7MOFs\u672c\u8eab\u7684\u201c\u547c\u5438\u6548\u5e94\u201d\uff0c\u4e5f\u80fd\u901a\u8fc7\u8c03\u8c10MOFs\u5b54\u9699\u8868\u9762\u6765\u6539\u5584\u5176\u5bf9\u6c14\u4f53\u7684\u5438\u9644\u548c\u5206\u79bb\u80fd\u529b\uff0c\u589e\u52a0BET\u8868\u9762\u79ef\uff0c\u7a33\u5b9a\u6846\u67b6\u7ed3\u6784\u7b49\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Precise Modulation of the Breathing Behavior and Pore Surface in Zr-MOFs by Reversible Post-Synthetic Variable-Spacer Installation to Fine-Tune the Expansion Magnitude and Sorption Properties<\/a>\uff08Angewandte Chemie International Edition\uff0c2016\uff0cDOI: 10.1002\/anie.201604023\uff09<\/p>\n

2\u3001Angew | \u798f\u5efa\u7269\u6784\u6240\u63d0\u51fa\u7528\u4e8e\u78b3\u50a8\u5b58\u548c\u5206\u79bb\u7684\u591a\u5b54\u6709\u673a\u5206\u5b50\u6846\u67b6\uff08POMF\uff09<\/strong><\/p>\n

\u591a\u5b54\u6709\u673a\u5206\u5b50\u6846\u67b6\uff08POMF\uff09\u7531\u8f7b\u5143\u7d20\uff08\u901a\u5e38\u4e3aH\u3001C\u3001N\u3001O\u3001B\uff09\u7ec4\u6210\uff0c\u76f8\u8f83\u4e8e\u91d1\u5c5e\u6709\u673a\u6846\u67b6\uff08MOFs\uff09\uff0c\u5176\u4f4e\u5bc6\u5ea6\u6027\u3001\u5fae\u6bd2\u6027\u3001\u6676\u4f53\u5b66\u53ef\u63a7\u6027\u53ca\u53ef\u518d\u751f\u6027\u7684\u4f18\u52bf\u6210\u4e3a\u4e00\u79cd\u66f4\u4e3a\u5148\u8fdb\u7684\u65b0\u578b\u6750\u6599\u3002<\/p>\n

\u798f\u5efa\u7269\u6784\u6240\u7ed3\u6784\u5316\u5b66\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u66f9\u8363\u8bfe\u9898\u7ec4\u91cd\u70b9\u62a5\u9053\u4e86\u53ef\u5b9e\u73b0\u7684\u63a7\u5236\u591a\u5b54\u6709\u673a\u5206\u5b50\uff08POMS\uff09\u7684\u7ec4\u88c5\u65b9\u6cd5\uff0c\u5305\u62ec\u56fa\u76f8\u6761\u4ef6\u548c\u6db2\u76f8\u6761\u4ef6\uff0c\u5e76\u6982\u8ff0\u4e86\u5355\u7ec4\u5206\u548c\u591a\u7ec4\u5206POMS\u7684\u6709\u6548\u7ec4\u88c5\u7b56\u7565\u3002\u5176\u4e2d\uff0c\u57fa\u4e8e\u5b9a\u5411\u548c\u53ef\u9884\u6d4b\u6027\u7684\u8d85\u5206\u5b50\u95f4\u6c22\u952e\u7684HOF\u578b\u591a\u5b54\u6709\u673a\u5206\u5b50\uff0c\u56e0\u5176\u590d\u6742\u6027\u8fd8\u9700\u8981\u8db3\u591f\u6df1\u5165\u7684\u7814\u7a76\u3002<\/p>\n

\"\u56fe\u72472-13\"
\n\u56fe2<\/strong> HOF-8\u4e09\u7ef4\u8d85\u5206\u5b50\u7ed3\u6784\u53ca\u5728298K\u65f6\u6c14\u4f53\u5438\u9644\u7b49\u6e29\u7ebf<\/p>\n

\u76f8\u6bd4\u4e4b\u4e0b\uff0c\u5229\u7528\u591a\u7ec4\u5206\u8d85\u5206\u5b50\u4f53\u7cfb\u4f5c\u7528\uff0c\u5982\u5364\u952e\uff0c\u03c0\u2013\u03c0\u4f5c\u7528\u548c\u758f\u6c34\u6027\u7b49\u4e3aPOMF\u6750\u6599\u7814\u7a76\u63d0\u4f9b\u4e86\u65b0\u89c6\u89d2\u548c\u7075\u611f\u3002\u672c\u6587\u8fd8\u63d0\u53ca\u4e86POMF\u6750\u6599\u5728\u78b3\u50a8\u5b58\u548c\u5206\u79bb\u7684\u7684\u5e94\u7528\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Porous Organic Molecular Frameworks with Extrinsic Porosity: Platform for Carbon Storage and Separation<\/a>\uff08Angewandte Chemie International Edition\uff0c2016\uff0cDOI: 10.1002\/anie.201602116\uff09<\/p>\n

3\u3001Nature Energy | MOF@GO \u9694\u819c\u89e3\u51b3\u9502\u786b\u7535\u6c60\u4e2d\u591a\u786b\u5316\u7269\u201c\u7a7f\u68ad\u201d\u95ee\u9898<\/strong><\/p>\n

\u9502-\u786b\u7535\u6c60\u5177\u6709\u76f8\u5bf9\u8f83\u4f4e\u7684\u6210\u672c\u548c\u8f83\u9ad8\u7684\u7406\u8bba\u80fd\u91cf\u5bc6\u5ea6\uff0c\u662f\u975e\u5e38\u6709\u524d\u666f\u7684\u80fd\u91cf\u5b58\u50a8\u4f53\u7cfb\u3002<\/p>\n

\u65e5\u672c\u4ea7\u4e1a\u6280\u672f\u7efc\u5408\u7814\u7a76\u6240\uff08AIST\uff09\u3001\u7b51\u6ce2\u5927\u5b66\u548c\u5357\u4eac\u5927\u5b66\u7684\u5468\u8c6a\u614e\u7814\u7a76\u56e2\u961f\u62a5\u9053\u4e86\u4e00\u79cd\u57fa\u4e8eMOF\/GO\u7684\u590d\u5408\u9694\u819c\uff0c\u5728\u9502-\u786b\u7535\u6c60\u4e2d\u53ef\u4ee5\u5f88\u597d\u5730\u6291\u5236\u591a\u786b\u5316\u5408\u7269\u201c\u7a7f\u68ad\u6548\u5e94\u201d\uff0c\u63d0\u9ad8\u4e86\u9502-\u786b\u7535\u6c60\u957f\u671f\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n

\"\u56fe\u72473-9\"<\/p>\n

\u56fe3<\/strong> MOF@GO\u590d\u5408\u9694\u819c\u5728\u9502\u786b\u7535\u6c60\u7684\u4f5c\u7528<\/p>\n

\u7814\u7a76\u8868\u660e\uff0cMOF@GO\u9694\u819c\u5728\u9502-\u786b\u7535\u6c60\u4e2d\u8d77\u5230\u4e86\u4e00\u79cd\u79bb\u5b50\u7b5b\u7684\u4f5c\u7528\uff0c\u80fd\u591f\u6709\u6548\u5730\u7b5b\u9009\u9502\u79bb\u5b50\u901a\u8fc7\uff0c\u540c\u65f6\u6291\u5236\u591a\u786b\u5316\u7269\u8fc1\u79fb\u5230\u8d1f\u6781\u3002\u5728\u6b64\u57fa\u7840\u4e0a\uff0c\u7814\u7a76\u4eba\u5458\u5229\u7528\u542b\u786b\u91cf\u7ea670%\u7684\u4ecb\u5b54\u78b3\u6750\u6599\u4f5c\u4e3a\u6b63\u6781\u6750\u6599\uff0c\u6240\u5f97\u5230\u7684\u9502-\u786b\u7535\u6c60\u8868\u73b0\u51fa\u4f4e\u5bb9\u91cf\u8870\u51cf\u7387\uff081500\u5faa\u73af\u4e2d\u7ea6\u6bcf\u5faa\u73af\u8870\u51cf0.019%\uff09\uff0c\u800c\u4e14\u8d77\u59cb\u7684100\u6b21\u5faa\u73af\u51e0\u4e4e\u6ca1\u6709\u5bb9\u91cf\u8870\u51cf\u3002\u8fd9\u4e00\u7814\u7a76\u5c55\u793a\u4e86MOF@GO\u9694\u819c\u5728\u80fd\u91cf\u5b58\u50a8\u4e2d\u5177\u6709\u91cd\u8981\u7684\u5e94\u7528\u6f5c\u529b\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Metal-organic framework-based separator for lithium-sulfur batteries<\/a>\uff08Nature Energy\uff0c2016\uff0cDOI: 10.1038\/nenergy.2016.94\uff09<\/p>\n

4\u3001JACS | \u901a\u8fc7\u914d\u4f53\u540e\u7ec4\u88c5\u6cd5\u5bf9Zr-MOF\u529f\u80fd\u6027\u7cbe\u786e\u5b9a\u5411\u6765\u4fee\u9970\u5b54\u7a74\u73af\u5883<\/strong><\/p>\n

\u7f8e\u56fd\u5fb7\u514b\u8428\u65afA&M\u5927\u5b66\u5468\u5b8f\u624d\u7814\u7a76\u7ec4\u5de7\u5999\u5730\u8fd0\u7528\u542b\u591a\u4e2a\u5b98\u80fd\u56e2\u7684\u914d\u4f53\u540e\u7ec4\u88c5\u5230\u9ad8\u5ea6\u6709\u5e8f\u7684MOFs\u7684\u7279\u5b9a\u4f4d\u70b9\u4ece\u800c\u5bf9\u6750\u6599\u7684\u5b54\u7a74\u73af\u5883\u8fdb\u884c\u4fee\u9970\u4ee5\u6ee1\u8db3\u66f4\u5148\u8fdb\u7684\u5e94\u7528\u3002\u6587\u4e2d\u63d0\u5230\u4e00\u79cd\u547d\u540d\u4e3aPCN-700\u7684Zr-MOF\u6700\u521d\u662f\u5728\u52a8\u529b\u5b66\u63a7\u5236\u4e0b\u6784\u5efa\u7684\uff0c\u5176\u4e2dZr\u7c07\u4e0a\u542b\u6709\u4e0d\u9971\u548c\u914d\u4f4d\u70b9\uff0c\u8fd9\u5c31\u4e3a\u8d1f\u8f7d\u8fc7\u5b98\u80fd\u56e2\u7684\u914d\u4f53\u540e\u7ec4\u88c5\u5230\u6846\u67b6\u5185\u63d0\u4f9b\u4e86\u826f\u597d\u7684\u6761\u4ef6\u3002<\/p>\n

\"\u56fe\u72474\"
\n\u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0 \u00a0\u56fe4<\/strong> \u901a\u8fc7\u914d\u4f53\u540e\u7ec4\u88c5\u5728Zr-MOF\u4e2d\u5f15\u5165\u591a\u79cd\u5b98\u80fd\u56e2\u5b9e\u73b0\u529f\u80fd\u7684\u7cbe\u786e\u5b9a\u5411<\/p>\n

\u8be5\u7814\u7a76\u7ec4\u5206\u522b\u5728PCN-700\u6846\u67b6\u4e0a\u540e\u7ec4\u88c5\u4e0d\u540c\u957f\u5ea6\u7684\u914d\u4f53\u5f97\u523011\u4e2d\u65b0\u578bMOFs\uff0c\u4e14\u6bcf\u4e00\u79cd\u90fd\u5728\u9884\u5b9a\u4f4d\u7f6e\u6210\u529f\u63a5\u51653\u79cd\u5b98\u80fd\u56e2\u3002\u8fd9\u79cd\u914d\u4f53\u540e\u7ec4\u88c5\u6cd5\u5b9e\u73b0\u4e86\u6750\u6599\u5b54\u9699\u4f53\u79ef\u548c\u5b54\u7a74\u73af\u5883\u7684\u4fee\u9970\uff0c\u5e76\u534f\u540c\u63d0\u5347\u4e86\u5bf9H2\u7684\u5438\u9644\u91cf\u8fbe57%\u3002\u5e76\u4e14\u5728\u5177\u6709\u5c3a\u5bf8\u6548\u5e94\u7684\u4e59\u9187\u6709\u6c27\u50ac\u5316\u6c27\u5316\u4f53\u7cfb\u4e2d\uff0c\u4f5c\u4e3a\u50ac\u5316\u5242\uff0c\u901a\u8fc7\u914d\u4f53\u540e\u7ec4\u88c5\u4fee\u9970\u7684PCN-700\u8868\u73b0\u51fa\u5f88\u9ad8\u7684\u50ac\u5316\u6d3b\u6027\u548c\u53ef\u8c03\u8c10\u7684\u5c3a\u5bf8\u9009\u62e9\u6027\u3002<\/p>\n

\u5229\u7528\u542b\u6709\u914d\u4f4d\u4e0d\u9971\u548c\u4f4d\u70b9\u7684\u7a33\u5b9aMOF\uff0c\u901a\u8fc7\u914d\u4f53\u540e\u7ec4\u88c5\u6cd5\u5f15\u5165\u591a\u79cd\u5b98\u80fd\u56e2\uff0c\u4ece\u800c\u4fee\u9970\u6750\u6599\u7684\u5b54\u7a74\u73af\u5883\u4ee5\u8fdb\u4e00\u6b65\u5b9e\u73b0\u5728\u6c14\u4f53\u5438\u9644\u3001\u50ac\u5316\u6216\u5176\u5b83\u8bf8\u5982\u4f20\u611f\u53ca\u7535\u5b66\u7b49\u6027\u8d28\u5e94\u7528\u4e2d\u7684\u6027\u80fd\u6539\u826f\u3002\u8fd9\u4e3aMOF\u6750\u6599\u7684\u591a\u65b9\u9762\u6027\u8d28\u8c03\u63a7\u53ca\u5e94\u7528\u53c8\u589e\u6dfb\u4e00\u7b14\u5149\u5f69\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1aLinker Installation: Engineering Pore Environment with Precisely Placed Functionalities in Zirconium MOFs<\/a>\uff08Journal of the American Chemical Society\uff0c2016\uff0c DOI: 10.1021\/jacs.6b04501\uff09<\/p>\n

5\u3001Angew | \u57fa\u4e8e\u7075\u6d3b\u7684Zr-MOF\u7684\u53ef\u5207\u6362\u7684\u4eff\u751f\u50ac\u5316\u5f00\u5173<\/strong><\/p>\n

\u7075\u6d3b\u7684MOFs\u7531\u4e8e\u5176\u8fd1\u4e4e\u65e0\u9650\u7684\u7ed3\u6784\/\u529f\u80fd\u7684\u591a\u6837\u6027\u548c\u53ef\u63a7\u7684\u7a7a\u9699\u7ed3\u6784\u6210\u4e3a\u4e3b\u5ba2\u4f53\u5316\u5b66\u7684\u7814\u7a76\u70ed\u70b9\u3002<\/p>\n

\"\u56fe\u72478-2\"<\/p>\n

\u56fe5<\/strong> \u914d\u4f53\u540e\u7ec4\u88c5\u8c03\u63a7\u7ed3\u6784\u6027\u201c\u547c\u5438\u201d\u8f6c\u5316\u53ca\u4f5c\u4e3a\u50ac\u5316\u5f00\u5173\u7684\u53ef\u9006\u5207\u6362\u793a\u610f\u56fe<\/p>\n

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\u8fd9\u79cd\u53ef\u63a7\u6027\u50ac\u5316\u5f00\u5173\u7684\u6982\u5ff5\u4e0d\u4ec5\u4f1a\u5f15\u9886\u65b0\u4e00\u4ee3\u50ac\u5316\u5242\u7814\u7a76\uff0c\u4e5f\u4f1a\u62d3\u5bbdMOF\u6750\u6599\u7684\u7814\u7a76\u8303\u56f4\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong>Flexible Zirconium Metal-Organic Frameworks as Bioinspired Switchable Catalysts<\/a>\uff08Angewandte Chemie International Edition\uff0c2016\uff0cDOI: 10.1002\/anie.201606587\uff09<\/p>\n

\u672c\u6587\u7531\u6750\u6599\u4eba\u7f16\u8f91\u90e8MOF\u7ec4\u4f9b\u7a3f\uff0c\u6750\u6599\u725b\u7f16\u8f91\u6574\u7406\u3002<\/p>\n

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