{"id":68429,"date":"2017-03-02T06:30:25","date_gmt":"2017-03-01T22:30:25","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=68429"},"modified":"2017-03-01T20:03:09","modified_gmt":"2017-03-01T12:03:09","slug":"nature%e5%ad%90%e5%88%8a%ef%bc%9a%e4%b8%80%e7%a7%8d%e9%80%9a%e8%bf%87c-c%e5%81%b6%e8%81%94%e5%8f%8d%e5%ba%94%e5%90%88%e6%88%90%e7%9a%84%e4%ba%8c%e7%bb%b4%e5%85%b1%e8%bd%ad%e8%8a%b3%e9%a6%99%e8%81%9a","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=68429","title":{"rendered":"Nature\u5b50\u520a\uff1a\u4e00\u79cd\u901a\u8fc7C-C\u5076\u8054\u53cd\u5e94\u5408\u6210\u7684\u4e8c\u7ef4\u5171\u8f6d\u82b3\u9999\u805a\u5408\u7269"},"content":{"rendered":"<p><strong>\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n<p>\u77f3\u58a8\u70ef\u7684\u53d1\u73b0\u662f\u6750\u6599\u9886\u57df\u7684\u91cd\u5927\u7a81\u7834\u4e4b\u4e00\uff0c\u56e0\u4e3a\u5b83\u7684\u5e26\u9699\u4e3a\u96f6\u3002\u4f46\u662f\u77f3\u58a8\u70ef\u5728\u534a\u5bfc\u4f53\u884c\u4e1a\u4e2d\u7684\u5e94\u7528\u6f5c\u529b\u4e00\u76f4\u6ca1\u6709\u88ab\u5f00\u53d1\u51fa\u6765\uff0c\u56e0\u6b64\uff0c\u7814\u7a76\u8005\u975e\u5e38\u5e0c\u671b\u80fd\u5408\u6210\u4e0e\u77f3\u58a8\u70ef\u5177\u6709\u76f8\u540c\u7279\u6027\u7684\u6709\u673a\u7c7b\u77f3\u58a8\u70ef\u3002<\/p>\n<p>\u77f3\u58a8\u70ef\u662f\u81ea\u7136\u754c\u6700\u5927\u7684\u4e8c\u7ef4\u5171\u8f6d\u4f53\u7cfb\uff0c\u5b83\u7684\u03c0\u7535\u5b50\u5728\u5355\u53cc\u952e\u4ea4\u66ff\u7684\u5e73\u9762\u5185\u53d1\u751f\u79fb\u4f4d\uff0c\u8fd9\u4f7f\u5f97\u77f3\u58a8\u70ef\u6750\u6599\u5177\u6709\u826f\u597d\u7684\u673a\u68b0\u6027\u80fd\u548c\u5149\u7535\u6027\u80fd\u3002\u56e0\u6b64\uff0c\u7814\u7a76\u4eba\u5458\u4e00\u76f4\u81f4\u529b\u4e8e\u5728\u5206\u5b50\u5c3a\u5ea6\u5408\u6210\u5b8c\u5168\u5171\u8f6d\u548c\u5b9a\u5411\u4e8c\u7ef4\u7684\u7ed3\u6784\u3002\u76ee\u524d\uff0c\u5408\u6210\u65b9\u6cd5\u4e3b\u8981\u6709\u4e09\u79cd\uff1a\u5171\u4ef7\u6709\u673a\u6846\u67b6\u7ed3\u6784\uff08CFOs\uff09\u6cd5\u3001\u8868\u9762\u8f85\u52a9\u805a\u5408\u6cd5\u548c\u56fa\u6001\u5c40\u90e8\u805a\u5408\u6cd5\u3002\u6bcf\u4e00\u79cd\u65b9\u6cd5\uff0c\u5bf9\u6700\u7ec8\u4ea7\u54c1\u7684\u7a33\u5b9a\u6027\u8d77\u51b3\u5b9a\u6027\u4f5c\u7528\u7684\u662f\u76f8\u4e92\u53d1\u751f\u53cd\u5e94\u7684\u5206\u5b50\u95f4\u6240\u5f62\u6210\u7684\u5316\u5b66\u952e\u7684\u7c7b\u578b\u548c\u5f3a\u5ea6\u3002\u5171\u4ef7\u6709\u673a\u6846\u67b6\u7ed3\u6784\uff08CFOs\uff09\u6cd5\u662f\u901a\u8fc7\u53d1\u751f\u52a8\u6001\u53ef\u9006\u7684\u53cd\u5e94\u5f62\u6210\u5171\u4ef7\u952e\uff0c\u8fd9\u79cd\u53cd\u5e94\u80fd\u81ea\u52a8\u4fee\u590d\u5728\u5408\u6210\u8fc7\u7a0b\u4e2d\u53d1\u751f\u7684\u7ed3\u6784\u7f3a\u9677\u3002\u9057\u61be\u7684\u662f\uff0c\u5927\u591a\u6570\u5171\u4ef7\u6709\u673a\u6846\u67b6\u7ed3\u6784\u4e0d\u7a33\u5b9a\uff0c\u4e00\u822c\u6761\u4ef6\u4e0b\u5bb9\u6613\u5206\u89e3\u3002\u4f46\u662f\uff0c\u7531\u53ef\u9006\u5171\u4ef7\u53cc\u952e\u7ec4\u6210\u7684\u4e8c\u7ef4\u5171\u8f6d\u5171\u4ef7\u6709\u673a\u6846\u67b6\u6700\u8fd1\u5df2\u88ab\u5408\u6210\u51fa\u6765\uff0c\u5f97\u5230\u4e86100\u03bcm\u957f\u7684\u7247\u72b6\u6676\u4f53\u3002\u8868\u9762\u8f85\u52a9\u805a\u5408\u6cd5\uff0c\u53ef\u4ee5\u5728\u4ec5\u4ec5\u51e0\u5e73\u65b9\u7eb3\u7c73\u7684\u8303\u56f4\u5185\u751f\u6210\u5e73\u6574\u7684\u5171\u8f6d\u805a\u5408\u7269\u3002\u800c\u56fa\u6001\u5c40\u90e8\u805a\u5408\u6cd5\uff0c\u5176\u53cd\u5e94\u53d1\u751f\u5728\u7b26\u5408\u4e00\u5b9a\u8ddd\u79bb\u548c\u65b9\u5411\u7684\u5355\u4f53\u5206\u5b50\u4e4b\u95f4\uff0c\u5355\u4f53\u53d1\u751f\u53cd\u5e94\u540e\u5f62\u6210\u6676\u4f53\u3002\u6709\u62a5\u9053\u663e\u793a\uff0c\u7528\u8fd9\u79cd\u65b9\u6cd5\u53ef\u5b9e\u73b0\u6676\uff0d\u6676\u578b\u5355\u4f53\u5411\u5c42\u578b\u805a\u5408\u7269\u7684\u8f6c\u53d8\u3002\u4f46\u662f\uff0c\u8fd9\u79cd\u805a\u5408\u7269\u5e76\u4e0d\u662f\u5b8c\u5168\u5171\u8f6d\u7684\u4e8c\u7ef4\u805a\u5408\u7269\uff0c\u800c\u4e14\u53ea\u80fd\u901a\u8fc7\u52a0\u70ed\u3001\u6eb6\u5242\u5904\u7406\u6216\u8005\u540c\u65f6\u7528\u4e24\u79cd\u65b9\u6cd5\u5904\u7406\u53d1\u751f\u5265\u843d\u3002<\/p>\n<p><strong>\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u65b0\u52a0\u5761\u56fd\u7acb\u5927\u5b66\u7684Su Ying Quek<\/strong>\u548c<strong>Kian Ping Loh\uff08\u5171\u540c\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u7b49\u4eba\uff0c\u901a\u8fc7\u56db\u6eb4\u591a\u82b3\u9999\u65cf\u5355\u4f53\u95f4\u7684C\u2014C\u5076\u8054\u53cd\u5e94\uff0c\u5408\u6210\u4e86\u4e8c\u7ef4\u5171\u8f6d\u82b3\u9999\u805a\u5408\u7269 (2D-CAP)\u3002\u4ed6\u4eec\u5229\u7528\u5185\u6e90\u6027\u56fa\u6001\u805a\u5408\u6cd5\uff0c\u5408\u6210\u4e86\u7ed3\u6676\u5171\u805a\u7269\uff0c\u5171\u805a\u7269\u81ea\u52a8\u5265\u843d\u540e\uff0c\u5f97\u5230\u4e861nm\u539a\u7684\u5c42\u72b6\u7269\u3002\u7b49\u6e29\u6c14\u4f53\u5438\u9644\u6d4b\u91cf\u8868\u660e\uff0c\u5c42\u72b6\u7269\u5927\u90e8\u5206\u7684\u5b54\u9699\u4e3a\uff5e0.6 nm\uff0c\u8fd9\u8bf4\u660e\u5c42\u95f4\u5177\u6709\u4e00\u81f4\u7684\u5f00\u653e\u901a\u9053\u3002\u5e38\u6e29\u4e0b\uff0c\u5f53\u4f5c\u4e3a\u6709\u673a\u9633\u6781\u5e94\u7528\u4e8e\u94a0\u79bb\u5b50\u7535\u6c60\u65f6\uff0c\u5b83\u80fd\u4f7f\u94a0\u79bb\u5b50\u7535\u6c60\u5feb\u901f\u5145\u653e\u7535\uff0c\u4e14\u8fd9\u79cd\u5145\u653e\u7535\u5177\u6709\u826f\u597d\u7684\u53ef\u9006\u5bb9\u91cf\u3001\u500d\u7387\u6027\u80fd\u4ee5\u53ca\u7a33\u5b9a\u6027\u80fd\u3002\u76f8\u5173\u6210\u679c\u4ee5\u201cA two-dimensional conjugated aromatic polymer via C\u2013C coupling reaction\u201d\u4e3a\u9898\uff0c\u53d1\u8868\u5728\u8fd1\u671f\u7684Nature Chemistry\u6742\u5fd7\u4e0a\u3002<\/p>\n<p><strong>\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n<p><strong>\u56fe1\uff1a\u7528\u8868\u9762\u8f85\u52a9\u805a\u5408\u6cd5\u5728\u91d1\u8868\u9762\u5236\u5907\u51fa\u7684\u5355\u5c42CAP\u7684STM\u8868\u5f81\u56fe<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-68431\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72471-29.png\" alt=\"\" width=\"657\" height=\"396\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72471-29.png 657w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72471-29-300x181.png 300w\" sizes=\"(max-width: 657px) 100vw, 657px\" \/><\/p>\n<p>\uff08a\uff09 \u901a\u8fc7\u91d1\u5c5e\u8868\u9762\u8f85\u52a9\u805a\u5408\u6cd5\u7528\u524d\u4f532-TBQP\u5408\u6210\u7684CAP\uff1b<\/p>\n<p>\uff08b\uff09 \u751f\u957f\u5728Au(111)\u8868\u9762\u7684\u5355\u5c42CAP\uff1b<\/p>\n<p>\uff08c\uff09 Au(111)\u8868\u9762\u4e0a\u4e24\u4e2a\u5b9a\u5411\u5f02\u5e38\u7684\u4e8c\u7ef4CAP\u57df\uff1b<\/p>\n<p>\uff08d\uff09 \u56fec\u4e2d\u4ea4\u53c9\u90e8\u5206i\uff08\u7ea2\u8272\uff09\u548cii\uff08\u9ec4\u8272\uff09\u5206\u522b\u5bf9\u5e94\u7684\u9ad8\u5ea6\uff1b<\/p>\n<p>\uff08e\uff09 \u751f\u957f\u5728Au(110)\u8868\u9762\u7684\u5355\u5c42CAP\u3002<\/p>\n<p><strong>\u56fe2\uff1a 2D-CAP\uff08\u5185\u6e90\u6027\u56fa\u6001\u805a\u5408\u6cd5\u5408\u6210\uff09\u7684\u5408\u6210\u548c\u8868\u5f81<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-68432\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72472-16.png\" alt=\"\" width=\"700\" height=\"711\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72472-16.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72472-16-295x300.png 295w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><br \/>\n \uff08a\uff09 \u524d\u4f532-TBQP\u7684\u805a\u5408\u53cd\u5e94\u6761\u4ef6\u548c\u6676\u4f53\u5806\u79ef\uff0c\u7403\uff0d\u6746\u6a21\u578b\uff08\u9876\uff0d\u9876\u89c6\u56fe\uff0c\u5e95\uff0d\u4fa7\u89c6\u56fe\uff09\u5982\u56fe\u6240\u793a\uff1b<\/p>\n<p>\uff08b\uff09 \u524d\u4f532-TBQP\u548c2D-CAP\u7684Br 3p\u5149\u8c31\u56fe\uff1b<\/p>\n<p>\uff08c\uff09 \u524d\u4f532-TBQP\u6676\u4f53\u7684SEM\u56fe\uff1b<\/p>\n<p>\uff08d\uff09 \u672a\u5904\u74062D-CAP\u6676\u4f53\u7684SEM\u56fe\uff1b<\/p>\n<p>\uff08e\uff09 \u5265\u843d\u540e2D-CAP\u7684TEM\u56fe\uff1b<\/p>\n<p>\uff08f\uff09 \u5728\u7845\u7247\u4e0a\u5265\u843d\u540e2D-CAP\u5c42\u7684AFM\u62d3\u6251\u56fe\uff1b<\/p>\n<p>\uff08g\uff09 f\u56fe\u4e2d\uff0c\u4e09\u89d2\u5f62\u5c42\u9762\u7684AFM\u62d3\u6251\u56fe\uff08\u7d2b\u8272\u865a\u7ebf\u65b9\u6846\uff09\uff1b<\/p>\n<p>\uff08h\uff09 \u56feg\u4e2d\u4ea4\u53c9\u90e8\u5206\u5bf9\u5e94\u7684AFM\u9ad8\u5ea6\uff08\u9ed1\u7ebf\uff09\u663e\u793a\u9636\u8dc3\u8fb9\u7f18\u4e3a\uff5e1nm\uff0ca.u.\u4efb\u610f\u5355\u4f4d\u3002<\/p>\n<p><strong>\u56fe3\uff1aAr\u6c14\u5438\u9644\u7b49\u6e29\u7ebf\u548c2D-CAP\u6676\u4f53\u7ed3\u6784\u5206\u6790\u56fe<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-68433\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72473-15.png\" alt=\"\" width=\"700\" height=\"336\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72473-15.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72473-15-300x144.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><br \/>\n \uff08a\uff092D-CAP\u7684Ar\u6c14\u5438\u9644\u548c\u8131\u9644\u7b49\u6e29\u7ebf\uff1b<\/p>\n<p>\uff08b\uff09\u6839\u636eAr\u6c14\u5438\u9644\u6570\u636e\u548c\u975e\u5c40\u90e8DFT\u6a21\u578b\u8ba1\u7b97\u76842D-CAP\u5b54\u9699\u5206\u5e03\u56fe\uff1b<\/p>\n<p>\uff08c\uff092D-CAP\u4e24\u4e2a\u76f8\u90bb\u5c42\u95f4\u4e0d\u540c\u95f4\u8ddd\u7684\u80fd\u91cf\u9762\uff1b<\/p>\n<p>\uff08d\uff092D-CAP\u7684Bader\u7535\u8377\u5206\u6790\u56fe\uff1b<\/p>\n<p>\uff08e\uff09XRD\u56fe\uff0c\u84dd\u8272\u8868\u793a\u75282D-CAP\u6d4b\u8bd5\uff0c\u7d2b\u8272\u8868\u793a\u7528\u91cd\u53e0\u5806\u79ef\u6a21\u578b\u6a21\u62df\uff0c\u7eff\u8272\u8868\u793a\u7528\u9519\u5217\u5806\u79ef\u6a21\u578b\u6a21\u62df\uff0c\u9ed1\u8272\u8868\u793a\u75281D-CAP\u6d4b\u8bd5\uff1b<\/p>\n<p>\uff08f\uff09\u91cd\u53e0\u5806\u79ef\u6a21\u578b\u4e2d\uff0c\u6700\u4f182D-CAP\u7684\u4fef\u89c6\u56fe\uff1b<\/p>\n<p>\uff08g\uff09\u9519\u5217\u5806\u79ef\u6a21\u578b\u4e2d\uff0c\u6700\u4f182D-CAP\u7684\u4fef\u89c6\u56fe\u3002<\/p>\n<p><strong>\u56fe4\uff1a\u53cd\u5e94\u673a\u7406\u5206\u6790<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-68434\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72474-12.png\" alt=\"\" width=\"700\" height=\"372\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72474-12.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72474-12-300x159.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/><\/p>\n<p>\uff08a\uff09 2-TBQP\u5355\u6676\u4e2d\u7684\u5355\u5143\u6676\u683c\uff0c\u6b64\u5355\u6676\u4e2d\u542b\u6709\u4e24\u4e2a\u5927\u7ea6\u76f8\u4e92\u5782\u76f4\u7684\u5355\u4f53\uff0cO\u662f\u539f\u59cb\u5750\u6807\u7cfb\uff1b<\/p>\n<p>\uff08b\uff09 2-TBQP\u5355\u6676\u4e2d\u76f8\u90bb\u5355\u4f53\u7684\u6676\u4f53\u53c2\u6570\uff1b<\/p>\n<p>\uff08c\uff09 \u4e0d\u542bBr\u76842-TBQP\u6676\u4f53\u5206\u5b50\u52a8\u529b\u5b66\u6a21\u62df\u8fc7\u7a0b\u4e2d\u7684\u7ed3\u6784\u53d8\u5316\uff1b<\/p>\n<p>\uff08d\uff09 \u5ba4\u6e29\u4e0b\u5185\u6e90\u6027\u56fa\u6001\u805a\u5408\u53cd\u5e94\u751f\u6210\u7684\u6676\u4f53\u6837\u54c1\u5206\u89e3\u524d\uff08\u5de6\uff09\u540e\uff08\u53f3\uff09\u8bb0\u5f55\u56fe\u3002<\/p>\n<p><strong>\u56fe5\uff1a0.005-2.5V\u7684\u7535\u538b\u8303\u56f4\u5185\uff0c2D\uff0dCAP\u7535\u6781\u94a0\u79bb\u5b50\u50a8\u5b58\u91cf\u53d8\u5316\u56fe<\/strong><\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"aligncenter size-full wp-image-68435\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72475-8.png\" alt=\"\" width=\"700\" height=\"480\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72475-8.png 700w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/02\/\u56fe\u72475-8-300x206.png 300w\" sizes=\"(max-width: 700px) 100vw, 700px\" \/>\uff08e\uff09 0.1\uff0c0.5\uff0c1.0\uff0c3.0\uff0c5.0\u548c10.0 A g\u22121\u7684\u6761\u4ef6\u4e0b\uff0c2D\uff0dCAP\u7535\u6781\u7684\u7535\u5bb9\u91cf\u53d8\u5316\uff1b<\/p>\n<p>\uff08f\uff09 \u4e0d\u540c\u7535\u6d41\u5bc6\u5ea6\u7684\u6761\u4ef6\u4e0b\uff0c2D-CAP\u7684Galvanostatic\u5145\u653e\u7535\u56fe\uff1b<\/p>\n<p>\uff08g\uff09 5.0 A g\u22121\u6761\u4ef6\u4e0b\uff0c2D-CAP\u7684\u5faa\u73af\u6027\u80fd\u56fe\uff08\u6700\u9ad87700\u6b21\u5faa\u73af\uff09\u3002<\/p>\n<p><strong>\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n<p>1\u3001 \u901a\u8fc7\u5185\u6e90\u6027\u56fa\u6001\u805a\u5408\u6cd5\uff0c\u5206\u5b50\u95f4\u53d1\u751fC-C\u5076\u8054\u53cd\u5e94\uff0c\u6210\u529f\u5408\u6210\u4e86\u4e8c\u7ef4\u5171\u8f6d\u82b3\u9999\u805a\u5408\u7269\uff082D-CAP\uff09\u3002<\/p>\n<p>2\u3001 2D-CAP\u5177\u6709\u591a\u5c42\u7ed3\u6784\uff0c\u5b54\u9699\u4e3a\uff5e0.6nm\uff0c\u80fd\u5265\u79bb\u6210\u539a\u5ea61nm\u7684\u8d85\u8584\u5355\u5c42\u3002<\/p>\n<p>3\u3001 \u56e0\u4e3a\u5177\u6709\u5c42\u95f4\u5171\u8f6d\u548c\u5b9a\u5411\u5f00\u653e\u7684\u4e00\u7ef4\u901a\u9053\uff0c\u4e00\u822c\u6761\u4ef6\u4e0b\uff0c2D-CAP\u53ef\u4f5c\u4e3a\u94a0\u79bb\u5b50\u7535\u6c60\u7684\u7535\u6781\uff0c\u5faa\u73af\u6027\u80fd\u7a33\u5b9a\uff0c\u7535\u5bb9\u91cf\u9ad8\uff0c\u500d\u7387\u6027\u80fd\u597d\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/www.nature.com\/nchem\/journal\/vaop\/ncurrent\/full\/nchem.2696.html\" target=\"_blank\">A two-dimensional conjugated aromatic polymer via C\u2013C coupling reaction<\/a><\/strong>\uff08Nature Chem., 2017, 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