{"id":81040,"date":"2017-05-18T06:30:10","date_gmt":"2017-05-17T22:30:10","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=81040"},"modified":"2017-05-16T17:26:30","modified_gmt":"2017-05-16T09:26:30","slug":"nano-lett-%e4%b8%ad%e7%a7%91%e9%99%a2%e4%b8%8a%e6%b5%b7%e7%a1%85%e9%85%b8%e7%9b%90%e7%a0%94%e7%a9%b6%e6%89%80%e7%a0%94%e5%8f%91%e4%ba%9a%e7%a8%b3%e6%80%81%e9%87%91%e5%b1%9e%e7%a1%ab%e5%8c%96%e7%89%a9","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=81040","title":{"rendered":"Nano Lett. \u4e2d\u79d1\u9662\u4e0a\u6d77\u7845\u9178\u76d0\u7814\u7a76\u6240\u7814\u53d1\u4e9a\u7a33\u6001\u91d1\u5c5e\u786b\u5316\u7269\u50ac\u5316\u5242"},"content":{"rendered":"

\u3010\u5f15\u8a00\u3011<\/strong><\/p>\n

\u5f00\u53d1\u9ad8\u6548\u7684\u50a8\u80fd\u50ac\u5316\u5242\u8f6c\u6362\u8fc7\u7a0b\uff0c\u5982Li-O2<\/sub>\u7535\u6c60\u548c\u6790\u6c22\u53cd\u5e94\uff08HER\uff09\uff0c\u4ecd\u7136\u662f\u5177\u6709\u6311\u6218\u6027\u7684\u5de5\u4f5c\u3002\u6539\u6027\u8868\u9762\u7535\u5b50\u7ed3\u6784\u901a\u8fc7\u6676\u683c\u8c03\u5236\u663e\u8457\u63d0\u9ad8\u7535\u50ac\u5316\u6027\u80fd\u3002\u7531\u4e8e\u4e2d\u95f4\u5c42\u7684\u63a7\u5236\u529b\u5f31\u8303\u5fb7\u534e\u4e0a\u7684\u683c\u5b50\u7ed3\u6784\uff0c\u65b0\u9896\u76842D\u6676\u4f53\u53ef\u4ee5\u4f5c\u4e3a\u76f4\u63a5\u5f15\u5165\u7684\u7406\u60f3\u5e95\u7269\u6676\u683c\u5e94\u53d8\uff0c\u53d8\u5f62\uff0c\u538b\u7f29\u6216\u62c9\u4f38\uff0c\u4ee5\u53ca\u8fdb\u4e00\u6b65\u8c03\u8282\u50ac\u5316\u6d3b\u6027\u3002\u5168\u534a\u5bfc\u4f53\u5f02\u8d28\u7ed3\u6784\u7684\u6784\u9020\u901a\u8fc7\u5782\u76f4\u5806\u53e0\u4e0d\u540c\u7684LTMD\u6216\u5207\u6362\u65e0\u7f1d\u5730\u5728\u4e00\u8d77\u3002\u6784\u5efa\u56fa\u6eb6\u4f53\u7ed3\u6784\u6216\u6742\u539f\u5b50\u63ba\u6742\u4e5f\u901a\u5e38\u7528\u4e8e\u8c03\u8282\u539f\u5b50\u7ed3\u6784\u6216\u5f15\u5165\u6d3b\u6027\u4f4d\u70b9\u3002\u589e\u5f3a\u50ac\u5316\u548c\u7535\u5316\u5b66\u6027\u80fd\u786e\u8ba4\u8fd9\u4e9b\u65b9\u6cd5\u7684\u6548\u7387\u3002\u800c\u8fc7\u7a0b\u5927\u90e8\u5206\u662f\u7531\u9ad8\u6e29\u8fdb\u884c\u7684\u56fa\u76f8\u5408\u6210\u8def\u7ebf\u3002\u5728\u9000\u706b\u8fc7\u7a0b\u4e2d\uff0c\u6742\u539f\u5b50\u88ab\u5f15\u5165\u5230\u672c\u5f81\u6676\u4f53\u7ed3\u6784\u4e2d\uff0c\u540c\u65f6\u9ad8\u6e29\u89e6\u53d1\u539f\u5b50\u7ed3\u6784\u5b9e\u73b0\u70ed\u529b\u5b66\u7a33\u5b9a\u6027\u5e76\u5f62\u6210\u65b0\u7684\u7a33\u5b9a\u76f8\u3002\u6709\u6548\u7684\u65b0\u65b9\u6cd5\u7075\u6d3b\u5730\u8bf1\u5bfc\u6676\u683c\u7578\u53d8\u800c\u4e0d\u5f15\u5165\u9700\u8981\u989d\u5916\u7684\u6548\u679c\u3002\u56e0\u6b64\uff0c\u5f00\u53d1\u4e86\u4f4e\u6210\u672c\u548c\u6f5c\u5728\u7684\u6269\u5927\u89c4\u6a21\u8def\u7ebf\u5408\u6210\u4e09\u7ef4\u4e9a\u7a33\u6001MoSSe\u56fa\u4f53\u5177\u6709\u9ad8\u5ea6\u5c40\u90e8\u6676\u683c\u7684\u89e3\u51b3\u65b9\u6848\u5931\u771f\u3002\u51c6\u5907\u76843D M-MoSSe\u5177\u6709\u5f88\u9ad8\u7684\u7a33\u5b9a\u6027\u548c\u8d85\u8584MoSSe\u5c42\u5f00\u653e\u5fae\u7ed3\u6784\u3002\u6b64\u5916\uff0c\u6676\u683c\u7578\u53d8\u7ed3\u6784\u5177\u6709\u4e0d\u7b49\u5f0f\u76f8\u540c\u6676\u4f53\u5e73\u9762\u4e4b\u95f4\u7684\u9762\u95f4\u8ddd\u53ef\u5728\u5355\u72ec\u7684MoSSe\u7eb3\u7c73\u7247\u4e2d\u83b7\u5f97\u3002<\/p>\n

\u3010\u6210\u679c\u7b80\u4ecb\u3011<\/strong><\/p>\n

\u8fd1\u65e5\uff0c\u4e2d\u79d1\u9662\u4e0a\u6d77\u7845\u9178\u76d0\u7814\u7a76\u6240\u6e29\u5146\u94f6\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u548c\u4f0a\u5229\u8bfa\u4f0a\u5927\u5b66\u829d\u52a0\u54e5\u5206\u6821<\/strong>Reza Shahbazian-Yassar<\/strong>\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u8bfe\u9898\u7ec4\u5728Nano Lett.<\/strong>\u4e0a\u53d1\u8868\u4e86\u9898\u4e3a\u201cLocal Lattice Distortion Activate Metastable Metal Sulfide as Catalyst with Stable Full Discharge-Charge Capability for Li-O2<\/sub> Batteries<\/strong>\u201d\u7684\u6587\u7ae0\u3002\u8be5\u7814\u7a76\u56e2\u961f\u5f00\u53d1\u76f4\u63a5\u6676\u683c\u5e94\u53d8\u53ef\u4ee5\u6709\u6548\u5730\u6539\u53d8\u50ac\u5316\u5242\u7684\u56fa\u6709\u7535\u50ac\u5316\u6027\u80fd\u3002\u901a\u8fc7\u6784\u5efa\u4e9a\u7a33\u6001MoSSe\u56fa\u6eb6\u4f53\u6765\u626d\u66f2\u6676\u683c\u7ed3\u6784\uff0c\u4ece\u800c\u8c03\u8282\u5bf9Li-O2<\/sub>\u7535\u6c60\u7684\u50ac\u5316\u6d3b\u6027\u3002\u540c\u65f6\u5728\u539f\u4f4d\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u548c\u50cf\u5dee\u6821\u6b63\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u7684\u5404\u4e2aMoSSe\u7eb3\u7c73\u7247\u4e2d\u76f4\u63a5\u89c2\u5bdf\u5230\u5728\u76f8\u540c\u6676\u9762\u4e4b\u95f4\u5177\u6709\u4e0d\u7b49\u5f0f\u9762\u95f4\u8ddd\u7684\u6676\u683c\u7578\u53d8\u7ed3\u6784\u3002\u6b64\u5916\uff0c\u539f\u4f4d\u900f\u5c04\u7535\u5b50\u663e\u5fae\u955c\u5206\u6790\u663e\u793a\u6574\u4e2a\u4e9a\u7a33\u6001\u7ed3\u6784\u7684\u5feb\u901fLi+<\/sup>\u6269\u6563\u3002<\/p>\n

\u3010\u56fe\u6587\u5bfc\u8bfb\u3011<\/strong><\/p>\n

\u56fe<\/strong>1\u00a0<\/strong>\u5177\u6709\u5931\u771f\u6676\u683c\u7ed3\u6784\u7684<\/strong>3D M-MoSSe<\/strong>\u7684\u5408\u6210\u7a0b\u5e8f\u7684\u793a\u610f\u56fe<\/strong><\/p>\n

\"\"<\/p>\n

\u5177\u6709\u5931\u771f\u6676\u683c\u7ed3\u6784\u76843D M-MoSSe\u7684\u5408\u6210\u7a0b\u5e8f\u7684\u793a\u610f\u56fe\u3002<\/p>\n

\u56fe<\/strong>2 MoS2<\/sub><\/strong>\uff0c<\/strong>MoSe2<\/sub><\/strong>\u7eb3\u7c73\u7247\uff0c<\/strong>3D S-MoSSe<\/strong>\u548c<\/strong>3D M-MoSSe<\/strong>\u56fa\u6eb6\u4f53\u7684\u7269\u7406\u5316\u5b66\u6027\u8d28\u8868\u5f81<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u76f8\u540c\u7684\u8def\u7ebf\u5236\u5907\u7684MoS2<\/sub>\uff0cMoSe2<\/sub>\u7eb3\u7c73\u7247\uff0c3D S-MoSSe\u548c3D M-MoSSe\u56fa\u6eb6\u4f53\u7684XRD\u56fe\uff1b<\/p>\n

\uff08b\uff093D M-MoSSe\u56fa\u6eb6\u4f53\u7684SEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\uff08b\uff09\u4e2d\u9ec4\u8272\u533a\u57df\u7684\u76f8\u5e94\u653e\u5927\u7684FESEM\u56fe\u50cf\uff1b<\/p>\n

\uff08d\uff093D M-MoSSe\u56fa\u6eb6\u4f53\u7684TEM\u56fe\u50cf\uff1b<\/p>\n

\uff08e\uff09\uff08d\uff09\u4e2d\u533a\u57df2\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n

\uff08f\uff09\uff08d\uff09\u4e2d\u533a\u57df1\u7684HRTEM\u56fe\u50cf\uff1b<\/p>\n

\uff08g\uff09\uff08f\uff09\u4e2d\u6cbf\u9ec4\u7ebf\u76843D M-MoSSe\u56fa\u6eb6\u4f53\u7684\u7ebf\u626b\u63cfEDS\u5206\u6790\uff1b<\/p>\n

\uff08h\uff0ci\uff093D M-MoSSe\u56fa\u6eb6\u4f53\u7684HRTEM\u56fe\u50cf\uff0c\u8868\u660e\uff08002\uff09\u9762\u7684d\u95f4\u8ddd\u4e0d\u4e00\u81f4\u3002<\/p>\n

\u56fe<\/strong>3. 3D M-MoSSe<\/strong>\u7684<\/strong>STEM<\/strong>\u56fe\u50cf<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff093D M-MoSSe\u7684\u5c42\u7684HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

\uff08b\uff093D M-MoSSe\u7684\u57fa\u9762\u7684HAADF-STEM\u56fe\u50cf\uff1b<\/p>\n

\uff08c\uff09\u6cbf\u7740\uff08b\uff09\u4e2d\u7684HAADF\u56fe\u50cf\u8ba1\u7b97\u7684\u6cbfxx\u65b9\u5411\u62cd\u6444\u7684\u5e94\u53d8\u56fe\uff1b<\/p>\n

\uff08d\uff09\u6cbf\u7740\uff08b\uff09\u4e2d\u7684HAADF\u56fe\u50cf\u8ba1\u7b97\u7684\u6cbfyy\u65b9\u5411\u62cd\u6444\u7684\u5e94\u53d8\u56fe\uff1b<\/p>\n

\uff08e\uff09Mo\uff0c\uff08f\uff09Se\u548c\uff08g\uff09S\u7684\u76f8\u5e94\u5143\u7d20\u5206\u5e03\u56fe\uff1b<\/p>\n

\uff08h\uff093D\u4e9a\u7a33\u6001MoSSe\u56fa\u6eb6\u4f53\u4e2d\u7684\u9762\u5185\u548c\u5916\u5e73\u9762\u6676\u683c\u5206\u5e03\u7684\u7ed3\u6784\u6a21\u578b\u3002<\/p>\n

\u56fe<\/strong>4. 3D M-MoSSe<\/strong>\uff0c<\/strong>3D S-MoSSe<\/strong>\uff0c<\/strong>MoS2<\/sub><\/strong>\u548c<\/strong>MoSe2<\/sub><\/strong>\u7eb3\u7c73\u7247\u7684<\/strong>XPS<\/strong>\u5206\u6790<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff093D M-MoSSe\uff0c3D S-MoSSe\uff0cMoS2<\/sub>\u548cMoSe2<\/sub>\u7684Mo3d<\/sub>\u7684\u9ad8\u5206\u8fa8\u7387\uff1b<\/p>\n

\uff08b\uff093D M-MoSSe\uff0c3D S-MoSSe\u548cMoS2<\/sub>\u7684S2p<\/sub>\u7684\u9ad8\u5206\u8fa8\u7387\uff1b<\/p>\n

\uff08c\uff093D M-MoSSe\uff0c3D S-MoSSe\u548cMoSe2<\/sub>\u7684Se3d<\/sub>\u7684\u9ad8\u5206\u8fa8\u7387\u3002<\/p>\n

\u56fe<\/strong>5. MoS2<\/sub><\/strong>\uff0c<\/strong>MoSe2<\/sub><\/strong>\uff0c<\/strong>3DS-MoSSe<\/strong>\u548c<\/strong>3DM-MoSSe<\/strong>\u9634\u6781\u6750\u6599\u7684\u7535\u5316\u5b66\u6027\u80fd\u6d4b\u8bd5<\/strong><\/p>\n

\"\"<\/p>\n

\uff08a\uff09\u572850mAg-1\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0bMoS2<\/sub>\uff0cMoSe2<\/sub>\uff0c3DS-MoSSe\u548c3DM-MoSSe\u9634\u6781\u7684\u7b2c\u4e00\u6b21\u5faa\u73af\u653e\u7535-\u7535\u8377\u66f2\u7ebf\uff1b<\/p>\n

\uff08b\uff09\u572850\u301c300mAg-1<\/sup>\u7684\u7535\u6d41\u5bc6\u5ea6\u4e0b\uff0c\u7b2c\u4e00\u6b21\u5faa\u73af\u4e2d\u7684\u4e09\u7ef4\u4e9a\u7a33\u6001MoSSe\u9634\u6781\u7684\u7535\u6d41\u653e\u7535\u548c\u7535\u8377\u66f2\u7ebf\uff1b<\/p>\n

\uff08c\uff09\u5177\u67093D M-MoSSe\u9634\u6781\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u5b8c\u5168\u653e\u7535\u7535\u8377\u66f2\u7ebf\uff1b<\/p>\n

\uff08d\uff09\u5177\u67093D\u4e9a\u7a33MoSSe\u9634\u6781\u7684Li-O2<\/sub>\u7535\u6c60\u7684\u5faa\u73af\u7a33\u5b9a\u6027\u3002<\/p>\n

\u3010\u5c0f\u7ed3\u3011<\/strong><\/p>\n

\u8be5\u7814\u7a76\u56e2\u961f\u901a\u8fc7\u9ad8\u5ea6\u901a\u7528\u7684\u65b9\u6cd5\uff0c\u6784\u5efa\u4e9a\u7a33\u56fa\u6eb6\u4f53\u7ed3\u6784\u5728MoS2<\/sub>\u57fa\u50ac\u5316\u5242\u4e2d\u8bf1\u5bfc\u6676\u683c\u7578\u53d8\u3002\u53d1\u73b0\u9002\u5f53\u5b9a\u5236\u7684\u539f\u5b50\u7ed3\u6784\u5728\u663e\u7740\u6539\u5584\u7535\u5316\u5b66\u6d3b\u6027\u548c\u4fc3\u8fdb\u5feb\u901f\u79bb\u5b50\u8f6c\u8fd0\u65b9\u9762\u662f\u6709\u6548\u7684\u3002 \u5f53\u7528\u4f5cLi-O2<\/sub>\u7535\u6c60\u548c\u6790\u6c22\u53cd\u5e94\u7684\u50ac\u5316\u5242\u65f6\uff0c3D\u5f00\u653e\u5f0f\u4e9a\u7a33\u56fa\u6eb6\u4f53\u7cfb\u7ed3\u6784\u8868\u73b0\u51fa\u6781\u5927\u5730\u63d0\u9ad8\u7684\u7535\u5316\u5b66\u6027\u80fd\u3002\u5bf9\u4e9a\u7a33\u6001\u56fa\u6eb6\u4f53\u7ed3\u6784\u7684\u539f\u5b50\u7ed3\u6784\u548c\u6784\u9020\u8fdb\u884c\u5927\u4fee\u6539\u7684\u53ef\u80fd\u6210\u4e3a\u4e0b\u4e00\u4ee3\u50ac\u5316\u6750\u6599\u7684\u8bbe\u8ba1\u94fa\u8def\u3002\u540c\u65f6\u4e3a\u7814\u53d1\u4e9a\u7a33\u6001\u91d1\u5c5e\u786b\u5316\u7269\u50ac\u5316\u5242\u63d0\u4f9b\u4e86\u4e00\u79cd\u65b0\u9896\u7684\u65b9\u6cd5\u3002<\/p>\n

\u6587\u732e\u94fe\u63a5\uff1a<\/strong> Local Lattice Distortion Activate Metastable Metal Sulfide as Catalyst with Stable Full Discharge-Charge Capability for Li-O2<\/sub> Batteries<\/a> \uff08Nano Lett. 2017, DOI: 10.1021\/acs.nanolett.7b00603\uff09<\/p>\n

\u901a\u8baf\u4f5c\u8005\u7b80\u4ecb\uff1a<\/strong><\/p>\n

\u6e29\u5146\u94f6\uff0c<\/strong>1963\u5e747\u6708\u751f\uff0c\u76ee\u524d\u4efb\u4e0a\u6d77\u7845\u9178\u76d0\u7814\u7a76\u6240\u4e8c\u7ea7\u7814\u7a76\u5458\uff0c\u535a\u58eb\u751f\u5bfc\u5e08\u30021992\u5e749\u6708-12\u6708\u5728\u65b0\u52a0\u5761\u56fd\u5bb6\u5927\u5b66\u7269\u7406\u7cfb\u5f00\u5c55\u5408\u4f5c\u7814\u7a76\uff0c1999\u5e741\u6708-2001\u5e7411\u6708\u5728\u65e5\u672c\u4e09\u91cd\u5927\u5b66\u5ba2\u5ea7\u7814\u7a76\u5458\uff0c\u5f00\u5c55\u5168\u56fa\u6001\u9502\u7535\u6c60\u7814\u7a76\u3002\u76ee\u524d\u517c\u4efb\u4e0a\u6d77\u65e0\u673a\u80fd\u6e90\u6750\u6599\u4e0e\u5668\u4ef6\u5de5\u7a0b\u7814\u7a76\u4e2d\u5fc3\u4e3b\u4efb\u3001\u4e2d\u79d1\u9662\u80fd\u91cf\u8f6c\u6362\u6750\u6599\u91cd\u70b9\u5b9e\u9a8c\u5ba4(\u4e0e\u4e2d\u56fd\u79d1\u6280\u5927\u5b66\u8054\u5408)\u526f\u4e3b\u4efb\u7b49\u804c\u3002\u8058\u4e3a\u4e2d\u56fd\u7845\u9178\u76d0\u5b66\u4f1a\u56fa\u6001\u79bb\u5b50\u5b66\u5206\u4f1a\u7406\u4e8b\u957f\u3001\u7279\u79cd\u9676\u74f7\u5206\u4f1a\u7406\u4e8b\u3001\u4e9a\u6d32\u56fa\u6001\u79bb\u5b50\u5b66\u4f1a\u7406\u4e8b\u3001\u4e0a\u6d77\u80fd\u6e90\u7814\u7a76\u4f1a\u7406\u4e8b\u4ee5\u53ca\u300a\u7845\u9178\u76d0\u5b66\u62a5\u300b\u3001\u300a\u65e0\u673a\u6750\u6599\u5b66\u62a5\u300b\u3001\u300a\u5efa\u7b51\u6750\u6599\u5b66\u62a5\u300b\u7b49\u671f\u520a\u7684\u7f16\u59d4\u3002<\/p>\n

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