{"id":96725,"date":"2017-08-18T06:30:01","date_gmt":"2017-08-17T22:30:01","guid":{"rendered":"http:\/\/www.cailiaoniu.com\/?p=96725"},"modified":"2017-08-18T11:06:13","modified_gmt":"2017-08-18T03:06:13","slug":"%e5%88%98%e5%ae%8f%e3%80%81%e6%a1%91%e5%85%83%e5%8d%8eadv-energy-mater-%e5%85%89%e5%82%ac%e5%8c%96%e7%bb%bc%e8%bf%b0%ef%bc%9a%e5%85%a8%e5%a4%aa%e9%98%b3%e5%85%89%e8%b0%b1%e5%93%8d%e5%ba%94%e7%9a%84","status":"publish","type":"post","link":"http:\/\/www.cailiaoniu.com\/?p=96725","title":{"rendered":"\u5218\u5b8f\u3001\u6851\u5143\u534eAdv. Energy Mater.\u5149\u50ac\u5316\u7efc\u8ff0\uff1a\u5168\u592a\u9633\u5149\u8c31\u54cd\u5e94\u7684\u5149\u50ac\u5316\u5242\u7528\u4e8e\u8f6c\u5316\u592a\u9633\u80fd\u4e3a\u5316\u5b66\u80fd"},"content":{"rendered":"<p>\u73af\u5883\u548c\u80fd\u6e90\u95ee\u9898\u628a\u592a\u9633\u80fd\u7684\u5229\u7528\u63a8\u5230\u4e86\u79d1\u5b66\u4e0e\u6280\u672f\u7814\u7a76\u524d\u6cbf\uff0c\u5728\u592a\u9633\u80fd\u5229\u7528\u7684\u5404\u79cd\u65b9\u6848\u4e2d\uff0c\u5149\u50ac\u5316\u5b9e\u73b0\u592a\u9633\u5149\u80fd\u91cf\u8f6c\u5316\u4e3a\u5316\u5b66\u80fd\u7684\u8fc7\u7a0b\u662f\u4e00\u4e2a\u975e\u5e38\u91cd\u8981\u7684\u7814\u7a76\u9886\u57df\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5341\u5e74\uff0c\u7814\u7a76\u4eba\u5458\u81f4\u529b\u4e8e\u6750\u6599\u548c\u5149\u50ac\u5316\u57fa\u7840\u539f\u7406\u7814\u7a76\uff0c\u65e8\u5728\u63d0\u9ad8\u592a\u9633\u5149\u5728\u5149\u50ac\u5316\u4f53\u7cfb\u4e2d\u7684\u5229\u7528\u6548\u7387\u3002\u76ee\u524d\uff0c\u7814\u7a76\u663e\u793a\u6750\u6599\u65b9\u9762\uff0c\u5df2\u7ecf\u80fd\u591f\u901a\u8fc7\u80fd\u5e26\u8c03\u63a7\u3001\u590d\u5408\u6750\u6599\u6784\u5efa\u7b49\uff0c\u5b9e\u73b0\u5149\u50ac\u5316\u8fc7\u7a0b\u7684\u5bbd\u592a\u9633\u5149\u8c31\u54cd\u5e94\uff0c\u5728\u57fa\u7840\u539f\u7406\u65b9\u9762\uff0c\u5229\u7528\u80fd\u5e26\u8c03\u63a7\u3001\u5f02\u8d28\u7ed3\u6784\u3001\u5916\u6e90\u573a\u7b49\u63d0\u5347\u4e86\u5149\u50ac\u5316\u8fc7\u7a0b\u4e2d\u8f7d\u6d41\u5b50\u7684\u5229\u7528\u6548\u7387\uff0c\u518d\u7ed3\u5408\u50ac\u5316\u6d3b\u6027\u9762\u8c03\u63a7\u3001\u52a9\u50ac\u5316\u5242\u8f85\u52a9\u7b49\uff0c\u4f7f\u5f97\u5149\u50ac\u5316\u5728\u592a\u9633\u80fd\u8f6c\u5316\u4e3a\u5316\u5b66\u80fd\u65b9\u9762\u53d6\u5f97\u4e86\u957f\u8db3\u7684\u8fdb\u5c55\u3002\u5bf9\u8fd1\u671f\u7814\u7a76\u6210\u679c\u548c\u65b0\u65b9\u6848\u3001\u65b0\u7406\u8bba\u7684\u603b\u7ed3\u5206\u6790\uff0c\u53ef\u4ee5\u660e\u786e\u5149\u50ac\u5316\u9886\u57df\u7684\u7814\u7a76\u73b0\u72b6\uff0c\u6307\u5bfc\u5bfb\u627e\u5149\u50ac\u5316\u7814\u7a76\u65b9\u5411\u548c\u5b9e\u73b0\u91cd\u70b9\u7a81\u7834\u3002<\/p>\n<p>\u8fd1\u65e5\uff0c<strong>\u5c71\u4e1c\u5927\u5b66\u6676\u4f53\u6750\u6599\u56fd\u5bb6\u91cd\u70b9\u5b9e\u9a8c\u5ba4\u7684\u6851\u5143\u534e\u526f\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09\u548c\u5218\u5b8f\u6559\u6388\uff08\u901a\u8baf\u4f5c\u8005\uff09<\/strong>\u5728<strong>Advanced Energy Materials<\/strong>\u53d1\u8868\u9898\u4e3a<strong>\u201cFull-Spectrum Solar-Light-Activated Photocatalysts for Light\u2013Chemical Energy Conversion\u201d<\/strong>\u7684\u6587\u7ae0\u3002\u6587\u7ae0\u4ee5\u5149\u50ac\u5316\u5149\u8c31\u54cd\u5e94\u8303\u56f4\u62d3\u5c55\u4e3a\u4e3b\u7ebf\uff0c\u4ee5\u592a\u9633\u5149\u80fd\u91cf\u8f6c\u5316\u4e3a\u5316\u5b66\u80fd\u5b58\u50a8\u4e3a\u8ba8\u8bba\u7684\u8f7d\u4f53\uff0c\u5728\u5149\u89e3\u6c34\u4ea7\u6c22\u3001\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u56fa\u5b9a\u3001\u6709\u673a\u805a\u5408\u7b49\uff0c\u548c\u50ac\u5316\u53cd\u5e94\u65b9\u9762\uff0c\u603b\u7ed3\u548c\u8ba8\u8bba\u4e86\u8fd1\u671f\u5728\u5149\u50ac\u5316\u5149\u8c31\u54cd\u5e94\u8303\u56f4\u62d3\u5c55\u548c\u5149\u751f\u8f7d\u6d41\u5b50\u5229\u7528\u6548\u7387\u63d0\u5347\u65b9\u9762\u7684\u65b0\u65b9\u6cd5\u3001\u65b0\u7406\u8bba\uff0c\u5e76\u8ba8\u8bba\u4e86\u8fdb\u4e00\u6b65\u63d0\u9ad8\u5149\u50ac\u5316\u6548\u7387\u548c\u5b9e\u73b0\u5e94\u7528\u6240\u9762\u4e34\u7684\u6311\u6218\u3002<\/p>\n<p><strong>1. \u5149\u50ac\u5316\u592a\u9633\u5149\u80fd\u91cf\u8f6c\u5316\u7684\u57fa\u672c\u539f\u7406<\/strong><\/p>\n<p>\u57fa\u4e8e\u534a\u5bfc\u4f53\u6750\u6599\u7684\u5149\u50ac\u5316\u57fa\u672c\u539f\u7406\u5df2\u7ecf\u4e3a\u7814\u7a76\u8005\u6240\u719f\u77e5\uff0c\u5728\u592a\u9633\u80fd\u8f6c\u5316\u4e3a\u5316\u5b66\u80fd\u8fc7\u7a0b\u4e2d\uff0c\u534a\u5bfc\u4f53\u50ac\u5316\u5242\u4e3b\u8981\u5b9e\u73b0\u4e24\u4e2a\u4f5c\u7528\uff0c\u4e00\u662f\u5438\u6536\u7279\u5b9a\u6ce2\u957f\u7684\u5149\u5b50\uff0c\u5b9e\u73b0\u7535\u5b50\u80fd\u7ea7\u8dc3\u8fc1\uff0c\u5f62\u6210\u5149\u751f\u8f7d\u6d41\u5b50\uff08\u7535\u5b50\u548c\u7a7a\u7a74\uff09\uff1b\u4e8c\u662f\u534a\u5bfc\u4f53\u7279\u6709\u7684\u80fd\u5e26\u7279\u5f81\uff0c\u8d4b\u4e88\u5149\u751f\u7535\u5b50\u7279\u5b9a\u7684\u8fd8\u539f\u52bf\uff0c\u8d4b\u4e88\u5149\u751f\u7a7a\u7a74\u7279\u5b9a\u7684\u6c27\u5316\u52bf\u3002\u8fd9\u4e9b\u5149\u751f\u8f7d\u6d41\u5b50\u5728\u7279\u5b9a\u7684\u6c27\u5316\u548c\u8fd8\u539f\u52bf\u4e0b\uff0c\u5b8c\u6210\u5176\u5bf9\u5e94\u7684\u6c27\u5316\u53cd\u5e94\u548c\u8fd8\u539f\u53cd\u5e94\uff0c\u4ece\u800c\u5b9e\u73b0\u5149\u50ac\u5316\u53cd\u5e94\uff08\u56fe1\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96731 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/1-40.jpg\" alt=\"\" width=\"600\" height=\"480\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/1-40.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/1-40-300x240.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\"><span style=\"color: #808080;\"><strong>\u56fe1. \u5149\u6fc0\u53d1\u534a\u5bfc\u4f53\u5185\u8f7d\u6d41\u5b50\u7684\u4ea7\u751f\u53ca\u90e8\u5206\u50ac\u5316\u53cd\u5e94\u5bf9\u5e94\u7684\u6c27\u5316\u8fd8\u539f\u52bf\uff08pH=7\uff09<\/strong><\/span><\/p>\n<p>\u5149\u50ac\u5316\u53cd\u5e94\u7684\u6548\u7387\u4e0d\u4ec5\u4ec5\u53d7\u9650\u4e8e\u50ac\u5316\u5242\u6750\u6599\u5149\u80fd\u8f6c\u5316\u4e3a\u76f8\u5e94\u7684\u7535\u5b50\u7a7a\u7a74\u7684\u6c27\u5316\u8fd8\u539f\u80fd\u7684\u80fd\u529b\uff0c\u50ac\u5316\u5242\u8868\u9762\u7279\u6027\u548c\u50ac\u5316\u53cd\u5e94\u4f53\u7cfb\u4e5f\u5bf9\u5149\u751f\u7535\u5b50\u7a7a\u7a74\u7684\u5229\u7528\u6548\u7387\u4ea7\u751f\u663e\u8457\u7684\u5f71\u54cd\u3002\u4ee5\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u4e3a\u4f8b\uff08\u56fe2\uff09\uff0cDimitrijevic\u535a\u58eb\u7b49\u4eba\uff08J. Am. Chem. Soc. 2011, 133, 3964\uff09\u8ba4\u4e3aCO<sub>2<\/sub>\u8fd8\u539f\u8fc7\u7a0b\u5305\u62ec\u4e24\u4e2a\u91cd\u8981\u8fc7\u7a0b\uff1a\u7535\u5b50\u4f20\u9012\u7ed9\u8868\u9762\u5438\u9644\u7684CO<sub>2<\/sub>\u548c\u8d28\u5b50\u4e0e\u8868\u9762\u7535\u5b50\u6d3b\u5316\u7684CO<sub>2<\/sub>\u7684\u53cd\u5e94\u3002\u4e24\u4e2a\u8fc7\u7a0b\u4e2d\u90fd\u5b58\u5728\u7535\u5b50\u8f93\u8fd0\u6307\u5f81\u65b9\u5411\u7684\u7ade\u4e89\uff0c\u4ece\u800c\u5927\u91cf\u7684\u6d88\u8017\u5149\u751f\u7535\u5b50\uff0c\u9650\u5236\u4e86CO<sub>2<\/sub>\u8fd8\u539f\u6548\u7387\u7684\u63d0\u9ad8\u3002\u6211\u4eec\u8ba4\u4e3a\uff0c\u50ac\u5316\u53cd\u5e94\u6548\u7387\u5728\u8fd9\u79cd\u8f83\u4e3a\u590d\u6742\u7684\u53cd\u5e94\u4e2d\uff0c\u66f4\u5927\u7a0b\u5ea6\u4e0a\u5236\u7ea6\u4e86\u6574\u4f53\u5149\u50ac\u5316\u7684\u592a\u9633\u80fd\u8f6c\u5316\u6548\u7387\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96734 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/2-40.jpg\" alt=\"\" width=\"600\" height=\"166\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/2-40.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/2-40-300x83.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\"><span style=\"color: #808080;\"><strong>\u56fe2.\u6c34\u76f8\u4e2dTiO<sub>2<\/sub>\u5149\u50ac\u5316\u8fd8\u539fCO<sub>2<\/sub>\u7684\u8fc7\u7a0b\u793a\u610f\u56fe<\/strong><\/span><\/p>\n<p><strong>2. \u53ef\u89c1\u5149\u54cd\u5e94\u7684\u5149\u50ac\u5316<\/strong><\/p>\n<p><strong>2.1 <\/strong><strong>\u57fa\u4e8e\u534a\u5bfc\u4f53\u6750\u6599\u6676\u4f53\u7ed3\u6784\u8c03\u63a7\u7684\u80fd\u5e26\u7ed3\u6784\u8c03\u63a7<\/strong><\/p>\n<p><strong><u>\uff08<\/u><\/strong><strong><u>1<\/u><\/strong><strong><u>\uff09\u7f3a\u9677\u5f15\u5165\u5e26\u6765\u7684\u5bbd\u8c31\u5149\u5438\u6536\u4e0e\u8f7d\u6d41\u5b50\u9677\u9631\u6d53\u5ea6\u589e\u52a0\u7684\u5e73\u8861\u5bf9\u5168\u5149\u8c31\u5149\u50ac\u5316\u6548\u7387\u7684\u5f71\u54cd<\/u><\/strong><\/p>\n<p>\u5149\u8c31\u5438\u6536\u8303\u56f4\u7684\u62d3\u5c55\u65b9\u9762\uff0c\u6700\u4e3a\u719f\u77e5\u548c\u6613\u4e8e\u5b9e\u73b0\u7684\u662f\u901a\u8fc7\u5143\u7d20\u63ba\u6742\u6216\u5f15\u5165\u7ed3\u6784\u7a7a\u4f4d\uff0c\u5f62\u6210\u4e00\u5b9a\u7684\u534a\u5bfc\u4f53\u6676\u4f53\u7ed3\u6784\u7f3a\u9677\uff0c\u8fd9\u4e9b\u7f3a\u9677\u7684\u5f15\u5165\uff0c\u5fc5\u7136\u4f1a\u5f71\u54cd\u534a\u5bfc\u4f53\u80fd\u5e26\u7279\u5f81\uff0c\u901a\u5e38\u4f1a\u5b9e\u73b0\u7981\u5e26\u5bbd\u5ea6\u53d8\u7a84\uff0c\u4ece\u800c\u589e\u5f3a\u5bf9\u53ef\u89c1\u5149\u7684\u5438\u6536\u80fd\u529b\uff0c\u5f62\u6210\u66f4\u591a\u7684\u5149\u751f\u8f7d\u6d41\u5b50\u3002\u4f46\u662f\u7f3a\u9677\u7684\u5f15\u5165\u4f1a\u5f62\u6210\u66f4\u591a\u7684\u8f7d\u6d41\u5b50\u6355\u83b7\u4e2d\u5fc3\uff08\u590d\u5408\u4e2d\u5fc3\uff09\uff0c\u663e\u8457\u5f71\u54cd\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u4f20\u8f93\u548c\u5bff\u547d\uff0c\u8fdb\u800c\u9650\u5236\u4e86\u5149\u751f\u8f7d\u6d41\u5b50\u7684\u5b9e\u9645\u50ac\u5316\u6548\u7387\u3002\u5229\u7528\u9541\u8fd8\u539f\uff08\u56fe3a,Energy Environ. Sci. 2015, 8, 3539.\uff09\u53ef\u4ee5\u5b9e\u73b0\u8868\u9762\u7f3a\u9677\u5f15\u5165\uff0c\u5b9e\u73b0\u80fd\u5e26\u8c03\u63a7\u7684\u540c\u65f6\uff0c\u907f\u514d\u5149\u50ac\u5316\u5242\u5185\u90e8\u8f7d\u6d41\u5b50\u6355\u83b7\u4e2d\u5fc3\u7684\u5927\u91cf\u5f62\u6210\u3002\u5229\u7528\u5c0f\u4e8e10nm\u7684TiO<sub>2<\/sub>\u7eb3\u7c73\u9897\u7c92\u8868\u9762\u539f\u5b50\u5bb9\u6613\u5f62\u6210\u7f3a\u9677\u7684\u7279\u5f81\uff08\u56fe3b\uff0cNat. Commun. 2015, 6, 5881\uff09\uff0c\u4e5f\u5b9e\u73b0\u4e86TiO<sub>2<\/sub>\u7684\u53ef\u89c1\u5149\u54cd\u5e94\u548c\u9ad8\u6548\u5149\u50ac\u5316\u4ea7\u6c22\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96735 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/3-32.jpg\" alt=\"\" width=\"600\" height=\"267\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/3-32.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/3-32-300x134.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\"><span style=\"color: #808080;\"><strong>\u56fe3.(a)\u9541\u5904\u7406\u524d\u540eTiO<sub>2<\/sub>\u7684\u80fd\u5e26\u7ed3\u6784\u793a\u610f\u56fe\uff1b(b)\u666e\u901a\u91d1\u7ea2\u77f3TiO<sub>2<\/sub>\u548c10nm\u4ee5\u4e0b\u91d1\u7ea2\u77f3TiO<sub>2<\/sub>\u7684\u80fd\u5e26\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/strong><\/span><\/p>\n<p><strong><u>\uff08<\/u><\/strong><strong><u>2<\/u><\/strong><strong><u>\uff09\u6676\u4f53\u7ed3\u6784\u5e94\u529b\u5b9e\u73b0\u80fd\u5e26\u8c03\u63a7<\/u><\/strong><\/p>\n<p>\u6676\u4f53\u7ed3\u6784\u5728\u5e94\u529b\u4f5c\u7528\u4e0b\uff0c\u4e5f\u80fd\u591f\u5b9e\u73b0\u80fd\u5e26\u7ed3\u6784\u7684\u8c03\u63a7\uff0c\u8fd9\u79cd\u8c03\u63a7\u4e0d\u989d\u5916\u5f15\u5165\u8f7d\u6d41\u5b50\u7684\u6355\u83b7\u4e2d\u5fc3\u3002\u5982\u56fe4a\u4e2d\uff08Adv. Mater. 2015, 27, 4572.\uff09\uff0c\u901a\u8fc7\u5f62\u6210\u975e\u6676\u76f8\u7684C<sub>3<\/sub>N<sub>4<\/sub>\uff0c\u4f7f\u5f97C<sub>3<\/sub>N<sub>4<\/sub>\u7684\u7ed3\u6784\u4ece\u5e73\u9762\u7ed3\u6784\u53d8\u4e3a\u4e863D\u7ed3\u6784\uff0c\u4f7f\u5f97\u80fd\u5e26\u4ece2.82eV\u964d\u4f4e\u52301.90eV\u3002\u56fe4b\uff08ACS Nano 2015, 9, 7256.\uff09\u6240\u793a\u4e3aAg<sub>2<\/sub>WO<sub>4<\/sub>\u4e2d[WO6]\u57fa\u56e2\u626d\u66f2\u94fe\u63a5\uff0c\u5b9e\u73b0\u4e86\u80fd\u5e26\u95f4\u9699\u7684\u8fde\u7eed\u8c03\u63a7\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96736 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/4-27.jpg\" alt=\"\" width=\"600\" height=\"413\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/4-27.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/4-27-300x207.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><span style=\"color: #808080;\"><strong>\u56fe4. (a) \u5c42\u72b6g-C<sub>3<\/sub>N<sub>4<\/sub>\uff08\u5de6\uff09\u548c\u975e\u6676g-C<sub>3<\/sub>N<sub>4<\/sub>\uff08\u53f3\uff09\u7684\u7ed3\u6784\u793a\u610f\u56fe\uff1b(b) \u5c42\u72b6g-C<sub>3<\/sub>N<sub>4<\/sub>\u548c\u975e\u6676g-C<sub>3<\/sub>N<sub>4<\/sub>\u7684\u80fd\u5e26\u7ed3\u6784\u793a\u610f\u56fe\u3002(c) W\u539f\u5b50\u5728Ag<sub>2<\/sub>WO<sub>4<\/sub>\u4e2d\u6cbf\u7740c\u8f74\u504f\u79bb\u4f4d\u7f6e\u4e0e\u5e26\u9699\u5927\u5c0f\u7684\u5173\u7cfb\uff1b(d) \u53ef\u89c1\u5149\u54cd\u5e94\u5149\u50ac\u5316\u6750\u6599\u7684\u5b9e\u73b0\u53ca\u80fd\u5e26\u7ed3\u6784\u793a\u610f\u56fe\u3002<\/strong><\/span><\/p>\n<p><strong>2.2. <\/strong><strong>\u5f02\u8d28\u7ed3\u6784\u7684\u6784\u5efa\u5b9e\u73b0\u5bbd\u8c31\u5149\u5438\u6536\u548c\u9ad8\u6548\u8f7d\u6d41\u5b50\u8f93\u8fd0<\/strong><\/p>\n<p><strong><u>\uff08<\/u><\/strong><strong><u>1<\/u><\/strong><strong><u>\uff09\u53ef\u89c1\u5149\u54cd\u5e94\u50ac\u5316\u5242\u590d\u5408\u6750\u6599<\/u><\/strong><\/p>\n<p>\u5c06\u5177\u6709\u53ef\u89c1\u5149\u54cd\u5e94\u7684\u5149\u654f\u6750\u6599\u6216\u8005\u5149\u50ac\u5316\u6750\u6599\u4e0eTiO<sub>2<\/sub>\u7b49\u9ad8\u6548\u7d2b\u5916\u5149\u54cd\u5e94\u7684\u5149\u50ac\u5316\u5242\u6750\u6599\u590d\u5408\uff0c\u662f\u6700\u5bb9\u6613\u5b9e\u73b0\u7684\u5149\u50ac\u5316\u54cd\u5e94\u5149\u8c31\u62d3\u5c55\u7684\u65b9\u6848\u3002\u5982\u8fd1\u671f\u5728\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u4e0a\u5e7f\u6cdb\u4f7f\u7528\u7684\u6709\u673a\u65e0\u673a\u590d\u5408\u6750\u6599\u548c\u5149\u654f\u6750\u6599\uff08\u56fe5\uff0cAngew. Chem. Int. Ed. 2015, 54, 2406\u548cJ. Am. Chem. Soc. 2015, 137, 13679\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96737 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/5-19.jpg\" alt=\"\" width=\"600\" height=\"226\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/5-19.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/5-19-300x113.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><span style=\"color: #808080;\"><strong>\u56fe5. (a) \u5229\u7528Ru complex\/C<sub>3<\/sub>N<sub>4<\/sub>\u590d\u5408\u5149\u50ac\u5316\u5242\u5b9e\u73b0\u5149\u50ac\u5316CO<sub>2<\/sub>\u8fd8\u539f\u7684\u793a\u610f\u56fe\uff1b(b) TiO<sub>2<\/sub>\u4e0e\u5149\u654f\u6750\u6599\u548c\u50ac\u5316\u6750\u6599\u590d\u5408\u7684\u80fd\u5e26\u7ed3\u6784\u53d8\u5316\u793a\u610f\u56fe\u3002<\/strong><\/span><\/p>\n<p><strong><u>\uff08<\/u><\/strong><strong><u>2<\/u><\/strong><strong><u>\uff09\u7a7a\u7a74\u4f20\u8f93\u6750\u6599\u589e\u5f3a\u8f7d\u6d41\u5b50\u5206\u79bb<\/u><\/strong><\/p>\n<p>\u8f7d\u6d41\u5b50\u5206\u79bb\u901a\u5e38\u662f\u8003\u8651\u589e\u5f3a\u5149\u751f\u7535\u5b50\u7684\u4f20\u8f93\u548c\u5bff\u547d\uff0c\u4e3b\u8981\u5728\u5bfc\u5e26\u7279\u6027\u548c\u754c\u9762\u7279\u6027\u4e0a\u8fdb\u884c\u7814\u7a76\uff0c\u8fd1\u671f\u77f3\u58a8\u7094\u4f5c\u4e3a\u7a7a\u7a74\u4f20\u8f93\u4f53\uff0c\u5e94\u7528\u5728\u5149\u50ac\u5316\u4e0a\uff0c\u5b9e\u73b0\u4e86\u9ad8\u6548\u5149\u7535\u50ac\u5316\u4ea7\u6c22\uff08\u56fe6a, J. Am. Chem. Soc. 2016, 138, 3954.\uff09\u3002\u6b64\u5916\uff0c\u6c34\u6eb6\u6027\u5206\u5b50\u7a7a\u7a74\u6355\u83b7\u5242\uff0c\u4e09\u6c1f\u4e59\u9178\u5728\u6c34\u6eb6\u6db2\u4e2d\u53ef\u4ee5\u5438\u9644\u5728K<sub>4<\/sub>Nb<sub>6<\/sub>O<sub>17 <\/sub>\u7eb3\u7c73\u7247\u7684\u8868\u9762\uff0c\u4ece\u800c\u6d88\u8017\u5149\u751f\u7a7a\u7a74\uff0c\u8fdb\u800c\u5b9e\u73b0\u4e86\u9ad8\u6548\u50ac\u5316\u4ea7\u6c22\uff08\u56fe6b\uff0cNat. Commun. 2015, 6, 8647.\uff09<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96738 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/6-11.jpg\" alt=\"\" width=\"600\" height=\"919\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/6-11.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/6-11-196x300.jpg 196w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p><span style=\"color: #808080;\"><strong>\u56fe6. (a) CdSe QDs\/\u77f3\u58a8\u7094\u590d\u5408\u6750\u6599\u7684PEC\u4ea7\u6c22\u793a\u610f\u56fe\uff1b(b) \u4e09\u6c1f\u4e59\u9178\u5206\u5b50\u4e0eK<sub>4<\/sub>Nb<sub>6<\/sub>O<sub>17<\/sub>\u7eb3\u7c73\u7247\u4f5c\u7528\u5149\u50ac\u5316\u4ea7\u6c22\u793a\u610f\u56fe\u3002<\/strong><\/span><\/p>\n<p><strong><u>\uff08<\/u><\/strong><strong><u>3<\/u><\/strong><strong><u>\uff09\u65b0\u578b\u5f02\u8d28\u7ed3\u6784\u80fd\u5e26\u5173\u7cfb<\/u><\/strong><\/p>\n<p>\u4f20\u7edf\u7684\u5f02\u8d28\u7ed3\u6784\u80fd\u5e26\u5173\u7cfb\u591a\u662ftype II\u578b\uff0c\u8fd9\u79cd\u7c7b\u578b\u7684\u80fd\u5e26\u5339\u914d\u5bb9\u6613\u5b9e\u73b0\u8f7d\u6d41\u5b50\u7684\u6709\u6548\u5206\u79bb\uff0c\u4f46\u662f\u540c\u65f6\u4f1a\u9020\u6210\u590d\u5408\u534a\u5bfc\u4f53\u6574\u4f53\u7684\u6c27\u5316\u8fd8\u539f\u80fd\u529b\u4e0b\u964d\uff0c\u8fd1\u5e74\u6765\uff0c\u53d7\u7eff\u8272\u690d\u7269\u7684\u5149\u5408\u4f5c\u7528z-scheme\u7c7b\u578b\u7ed3\u6784\u542f\u53d1\uff0c\u7814\u7a76\u4eba\u5458\u5f00\u59cb\u5173\u6ce8z-scheme\u7c7b\u578b\u5f02\u8d28\u7ed3\u6784\u590d\u5408\u6750\u6599\uff0c\u65e2\u80fd\u5b9e\u73b0\u6709\u6548\u5149\u751f\u8f7d\u6d41\u5b50\u5206\u79bb\uff0c\u53c8\u80fd\u8d4b\u4e88\u6750\u6599\u5f88\u9ad8\u7684\u6c27\u5316\u8fd8\u539f\u80fd\u529b\u3002\u5982CdS\/WO<sub>3<\/sub>\u590d\u5408\u6750\u6599\uff08\u56fe7a, Small 2015, 11, 5262.\uff09\u548cTiO<sub>2<\/sub>\/rGO\/\u786b\u5316\u7269\u590d\u5408\u6750\u6599\uff08\u56fe7b, J. Am. Chem. Soc. 2015, 137, 604\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96739 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/7-9.jpg\" alt=\"\" width=\"553\" height=\"640\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/7-9.jpg 553w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/7-9-259x300.jpg 259w\" sizes=\"(max-width: 553px) 100vw, 553px\" \/><\/p>\n<p><span style=\"color: #808080;\"><strong>\u56fe7.(a)CdS\/WO<sub>3<\/sub>\u5f02\u8d28\u7ed3\u6784\u4e2d\u8f7d\u6d41\u5b50\u8f93\u8fd0\u548c\u5206\u79bb\u793a\u610f\u56fe\uff1b(b)TiO<sub>2<\/sub>\/rGO\/\u786b\u5316\u7269\u5f02\u8d28\u7ed3\u6784\u4e2d\u8f7d\u6d41\u5b50\u8f93\u8fd0\u548c\u5206\u79bb\u793a\u610f\u56fe\u3002<\/strong><\/span><\/p>\n<p><strong>3. \u8fd1\u7ea2\u5916\u5149\u54cd\u5e94\u7684\u5149\u50ac\u5316<\/strong><\/p>\n<p>\u7531\u4e8e\u8fd1\u7ea2\u5916\u5149\u7684\u5149\u5b50\u80fd\u91cf\u8f83\u4f4e\uff0c\u96be\u4ee5\u6fc0\u53d1\u5177\u6709\u4e00\u5b9a\u7981\u5e26\u5bbd\u5ea6\u7684\u534a\u5bfc\u4f53\u6750\u6599\uff0c\u5373\u4f7f\u6fc0\u53d1\u5e26\u9699\u5f88\u7a84\u7684\u534a\u5bfc\u4f53\u6750\u6599\uff0c\u6240\u4ea7\u751f\u7684\u6c27\u5316\u8fd8\u539f\u52bf\u4e5f\u975e\u5e38\u4f4e\uff0c\u5f88\u96be\u5b9e\u73b0\u6709\u6548\u50ac\u5316\u53cd\u5e94\uff0c\u6240\u4ee5\u5173\u6ce8\u5ea6\u8f83\u5c0f\u3002\u8fd1\u7ea2\u5916\u5149\u54cd\u5e94\u65b9\u9762\uff0c\u901a\u8fc7\u80fd\u5e26\u8c03\u63a7\uff0c\u4f7f\u5e26\u9699\u8fdb\u4e00\u6b65\u53d8\u5c0f\uff0c\u6216\u8005\u5229\u7528\u7279\u5b9a\u7684\u672c\u5f81\u7a84\u7981\u5e26\u7684\u534a\u5bfc\u4f53\u6750\u6599\uff0c\u5b9e\u73b0\u5149\u5438\u6536\u548c\u4ea7\u751f\u8f7d\u6d41\u5b50\uff0c\u518d\u5229\u7528\u9002\u5f53\u7684\u5f02\u8d28\u7ed3\u6784\uff0c\u5f62\u6210\u5177\u6709\u4e00\u5b9a\u50ac\u5316\u6d3b\u6027\u7684\u7535\u5b50\u6216\u8005\u7a7a\u7a74\uff0c\u8fd9\u79cd\u65b9\u6848\u9010\u6b65\u88ab\u7814\u7a76\u4eba\u5458\u5e7f\u6cdb\u91c7\u7528\u3002\u5149\u7269\u7406\u7684\u53d1\u5c55\uff0c\u8868\u9762\u7b49\u79bb\u6fc0\u5143\u5171\u632f\u5438\u6536\u4e5f\u5b9e\u73b0\u4e86\u8fd1\u7ea2\u5916\u5149\u4e0b\u6fc0\u53d1\u8f83\u5bbd\u7981\u5e26\u534a\u5bfc\u4f53\u6750\u6599\uff0c\u4ece\u800c\u5b9e\u73b0\u5149\u50ac\u5316\uff08\u56fe8\uff0cScience 2015, 347, 970\uff09\u3002<\/p>\n<p><img loading=\"lazy\" decoding=\"async\" class=\"size-full wp-image-96740 aligncenter\" src=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/8-5.jpg\" alt=\"\" width=\"600\" height=\"324\" srcset=\"http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/8-5.jpg 600w, http:\/\/www.cailiaoniu.com\/wp-content\/uploads\/2017\/08\/8-5-300x162.jpg 300w\" sizes=\"(max-width: 600px) 100vw, 600px\" \/><\/p>\n<p style=\"text-align: center;\"><span style=\"color: #808080;\"><strong>\u56fe8.\u8868\u9762\u7b49\u79bb\u6fc0\u5143\u5171\u632f\u5438\u6536\u5b9e\u73b0\u534a\u5bfc\u4f53\u6fc0\u53d1\u793a\u610f\u56fe<\/strong><\/span><\/p>\n<p><strong>4.<\/strong><strong>\u5149\u70ed\u50ac\u5316\u4f5c\u4e3a\u8fd1\u7ea2\u5916\u5149\u50ac\u5316\u7684\u8865\u5145<\/strong><\/p>\n<p>\u7531\u4e8e\u8fd1\u7ea2\u5916\u5149\u7684\u70ed\u6548\u7387\u8f83\u9ad8\uff0c\u4e3a\u4e86\u66f4\u9ad8\u6548\u7387\u7684\u5b9e\u73b0\u592a\u9633\u80fd\u5411\u5316\u5b66\u80fd\u7684\u8f6c\u5316\uff0c\u672c\u6587\u4e2d\u6982\u8ff0\u4e86\u8fd1\u671f\u5149\u70ed\u50ac\u5316\u5728CO<sub>2<\/sub>\u8fd8\u539f\u4e0a\u7684\u91cd\u8981\u8fdb\u5c55\u548c\u5e94\u7528\u3002<\/p>\n<p>\u6587\u7ae0\u6700\u540e\uff0c\u6211\u4eec\u6309\u7167\u5149\u50ac\u5316\u7684\u4e3b\u8981\u7528\u9014\uff0c\u8ba8\u8bba\u4e86\u592a\u9633\u80fd\u5411\u5316\u5b66\u80fd\u7684\u8f6c\u5316\u73b0\u72b6\u548c\u74f6\u9888\uff0c\u8ba4\u4e3a\u5728\u6c61\u6c34\u5904\u7406\u65b9\u9762\uff0c\u5149\u8c31\u54cd\u5e94\u8303\u56f4\u62d3\u5c55\u4e0e\u964d\u89e3\u6548\u7387\u4e4b\u95f4\u9700\u8981\u63a2\u5bfb\u4e00\u4e2a\u5e73\u8861\uff0c\u5e76\u4e14\u9488\u5bf9\u4e0d\u540c\u7c7b\u578b\u7684\u6c61\u6c34\uff0c\u5149\u50ac\u5316\u7684\u9009\u62e9\u9700\u8981\u6709\u6240\u8c03\u6574\uff1b\u7eff\u8272\u5408\u6210\u65b9\u9762\uff0c\u5149\u50ac\u5316\u5242\u4e3b\u8981\u4f5c\u4e3a\u80fd\u6e90\u63d0\u4f9b\u4ecb\u8d28\uff0c\u52a9\u50ac\u5316\u5242\u7684\u9009\u62e9\u548c\u534f\u540c\u4f5c\u7528\u66f4\u9700\u8981\u5f15\u8d77\u5173\u6ce8\uff1b\u5149\u89e3\u6c34\u4ea7\u6c22\u65b9\u9762\uff0c\u5b9e\u73b0\u771f\u6b63\u7684\u5149\u89e3\u6c34\uff0c\u907f\u514d\u727a\u7272\u5242\u7684\u4f7f\u7528\u662f\u76ee\u524d\u7684\u91cd\u70b9\uff1bCO<sub>2<\/sub>\u8fd8\u539f\u65b9\u9762\uff0c\u6548\u7387\u548c\u9009\u62e9\u6027\u662f\u9650\u5236\u5176\u53d1\u5c55\u7684\u6838\u5fc3\u56e0\u7d20\uff1b\u5149\u70ed\u50ac\u5316\u65b9\u9762\uff0c\u9700\u8981\u5173\u6ce8\u5149\u70ed\u6750\u6599\u4e0e\u50ac\u5316\u5242\u7684\u7cfb\u7edf\u4f5c\u7528\u3002<\/p>\n<p><strong>\u6587\u732e\u94fe\u63a5\uff1a<a href=\"http:\/\/onlinelibrary.wiley.com\/doi\/10.1002\/aenm.201700473\/abstract\" target=\"_blank\" rel=\"noopener\">Full-Spectrum Solar-Light-Activated Photocatalysts for Light\u2013Chemical Energy Conversion<\/a><\/strong>\uff08Adv. Energy Mater., 2017, DOI: 10.1002\/aenm.201700473\uff09<\/p>\n<p>\u6750\u6599\u725b\u7f16\u8f91\u5927\u57ce\u5c0f\u7231\u6574\u7406\u7f16\u8f91\u3002\u611f\u8c22\u5c71\u4e1c\u5927\u5b66\u6851\u5143\u534e\u526f\u6559\u6388\u3001\u5218\u5b8f\u6559\u6388\u7684\u652f\u6301\uff01<\/p>\n<p><strong>\u6295\u7a3f\u4ee5\u53ca\u5185\u5bb9\u5408\u4f5c\u53ef\u52a0\u7f16\u8f91\u5fae\u4fe1\uff1a<\/strong><strong>xiaofire-18<\/strong><strong>\uff0c\u5434\u73ab\uff0c\u6211\u4eec\u4f1a\u9080\u8bf7\u5404\u4f4d\u8001\u5e08\u52a0\u5165\u4e13\u5bb6\u7fa4\u3002<\/strong><\/p>\n<p>\u6750\u6599\u725b\u7f51\u4e13\u6ce8\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u53ca\u884c\u4e1a\u8fdb\u5c55\uff0c\u5982\u679c\u60a8\u5bf9\u4e8e\u8ddf\u8e2a\u6750\u6599\u9886\u57df\u79d1\u6280\u8fdb\u5c55\uff0c\u89e3\u8bfb\u9ad8\u6c34\u5e73\u6587\u7ae0\u6216\u662f\u8bc4\u8ff0\u884c\u4e1a\u6709\u5174\u8da3\uff0c<a href=\"http:\/\/www.cailiaoniu.com\/25127.html\">\u70b9\u6211\u52a0\u5165\u7f16\u8f91\u90e8<\/a>\u3002\u6b22\u8fce\u5927\u5bb6\u5230\u6750\u6599\u4eba\u5ba3\u4f20\u79d1\u6280\u6210\u679c\u5e76\u5bf9\u6587\u732e\u8fdb\u884c\u6df1\u5165\u89e3\u8bfb\uff0c\u6295\u7a3f\u90ae\u7bb1tougao@cailiaoren.com\u3002<\/p>\n<p><strong>\u4eea\u5668\u8bbe\u5907\u3001\u8bd5\u5242\u8017\u6750\u3001\u6750\u6599\u6d4b\u8bd5\u3001\u6570\u636e\u5206\u6790\uff0c\u627e<\/strong><a href=\"http:\/\/mai.cailiaoren.com\/\"><strong>\u6750\u6599\u4eba<\/strong><\/a><strong>\u3001\u4e0a<\/strong><a href=\"http:\/\/www.ceshigu.com\/\"><strong>\u6d4b\u8bd5\u8c37<\/strong><\/a><strong>\uff01<\/strong><\/p>\n","protected":false},"excerpt":{"rendered":"<p>\u73af\u5883\u548c\u80fd\u6e90\u95ee\u9898\u628a\u592a\u9633\u80fd\u7684\u5229\u7528\u63a8\u5230\u4e86\u79d1\u5b66\u4e0e\u6280\u672f\u7814\u7a76\u524d\u6cbf\uff0c\u5728\u592a\u9633\u80fd\u5229\u7528\u7684\u5404\u79cd\u65b9\u6848\u4e2d\uff0c\u5149\u50ac\u5316\u5b9e\u73b0\u592a\u9633\u5149\u80fd\u91cf\u8f6c\u5316\u4e3a\u5316\u5b66\u80fd\u7684\u8fc7\u7a0b\u662f\u4e00\u4e2a\u975e\u5e38\u91cd\u8981\u7684\u7814\u7a76\u9886\u57df\u3002\u5728\u8fc7\u53bb\u7684\u51e0\u5341\u5e74\uff0c&#8230;<\/p>\n","protected":false},"author":1369,"featured_media":0,"comment_status":"open","ping_status":"closed","sticky":false,"template":"","format":"standard","meta":{"footnotes":""},"categories":[533],"tags":[],"class_list":["post-96725","post","type-post","status-publish","format-standard","hentry","category-zongshu"],"_links":{"self":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/96725"}],"collection":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts"}],"about":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/types\/post"}],"author":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/users\/1369"}],"replies":[{"embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcomments&post=96725"}],"version-history":[{"count":3,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/96725\/revisions"}],"predecessor-version":[{"id":96743,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=\/wp\/v2\/posts\/96725\/revisions\/96743"}],"wp:attachment":[{"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fmedia&parent=96725"}],"wp:term":[{"taxonomy":"category","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Fcategories&post=96725"},{"taxonomy":"post_tag","embeddable":true,"href":"http:\/\/www.cailiaoniu.com\/index.php?rest_route=%2Fwp%2Fv2%2Ftags&post=96725"}],"curies":[{"name":"wp","href":"https:\/\/api.w.org\/{rel}","templated":true}]}}